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| 1 | Reduced graphene oxide@carbon sphere based metacomposites for temperature-insensitive and efficient microwave absorption显示文摘With the increasing advance of fifth generation(5G)network and the gradual expansion of digital devices,harsh working environment for electronic devices has spawned higher requirements for microwave absorbing materials(MAMs).Since both the electromagnetic response and energy conversion character vary with temperature,to achieve temperature insensitive microwave absorption behaviour in wide temperature range has become extremely challenging.In this work,structured metacomposites containing sub-wavelength reduced graphene oxide(RGO)@carbon spheres were fabricated,and the microwave absorption was further improved through structural and composition design of the RGO@carbon units.Due to the unique anti-reflection effect on microwave of the metacomposites,the temperature-insensitive electromagnetic performance at elevated temperature could be exhibited.Moreover,both the dielectric relaxation behaviour and microwave absorption proformance of the system could be further increased.As a result,the effective absorption bandwidth(reflection loss(RL)<−10 dB)of the metacomposites with only 3.0 wt.%filler content could cover the entire X-band(8.2–12.4 GHz)frequency ranging from 298 to 473K.The metacomposite proposed in this work provides a“de-correlating”strategy to break the linkage between microwave absorption behaviour and temperature,which offers an interesting plateau for fabricating efficient high-temperature microwave absorption structures with tunable and designable advantages. | Zhiyang Jiang Haoxu Si Yi Li Dan Li Huihui Chen Chunhong Gong Jingwei Zhang | 2022 | Nano Research2022，15，9： | 4 |
| 2 | Heteroatoms-doped carbon nanocages with enhanced dipolar and defective polarization toward light-weight microwave absorbers显示文摘Light-weight and exceptional microwave absorption are two vital characteristics for microwave absorbers in practical applications,but still face challenges.Herein,we employ a sacrificial template strategy to fabricate heteroatoms-doped carbon nanocages(CNs)via chemical vapor deposition,in which heteroatoms are simultaneously doped into the carbon frameworks by bubbling flowing source liquid.Compared with CNs,doped heteroatoms,accompanied with the inevitably defective arrangements in the lattice,not only decrease the electrical conductivity and balance the impedance characteristics,but also introduce structuralchemical defects and trigger dominant dipolar/defect polarization.As a result,both the minimum reflection loss(R_(L,min))and effective absorption bandwidth(EAB)greatly increase at an ultralow filler loading of 5 wt.%owing to internal hollow void and high specific surface area.The R_(L,min) values reach−53.6,−43.2,and−50.1 dB for N-CNs,S-CNs,and N,S-CNs with the corresponding EAB of 4.9,2.5,and 3.1 GHz,respectively.Furthermore,this work provides an effective strategy for the construction of heteroatoms-doped hollow carbon frameworks in large-scale production and the obtained doped carbon nanocages can be used as light-weight and high-performance microwave absorbers. | Hanxiao Xu Guozheng Zhang Yi Wang Yiruo Wang Huanlei Wang Ying Huang Panbo Liu | 2022 | Nano Research2022，15，10： | 2 |
| 3 | Enhanced electromagnetic wave absorption via optical fiber-like PMMA@Ti_(3)C_(2)T_(x)@SiO_(2) composites with improved impedance matching显示文摘Ti_(3)C_(2)T_(x) nanosheets have attracted significant attention for their potential in electromagnetic wave absorption(EWA).However,their inherent self-stacking and exorbitant electrical conductivity inevitably lead to serious impedance mismatch,restricting their EWA application.Therefore,the optimization of impedance matching becomes crucial.In this work,we developed polymethyl methacrylate(PMMA)@Ti_(3)C_(2)T_(x)@SiO_(2) composites with a sandwich-like core–shell structure by coating SiO_(2) on PMMA@Ti_(3)C_(2)T_(x).The results demonstrate that the superiority of the SiO_(2) layer in combination with PMMA@Ti_(3)C_(2)T_(x),outperforming other relative graded distribution structures and meeting the requirements of EWA equipment.The resulting PMMA@Ti_(3)C_(2)T_(x)@SiO_(2) composites achieved a minimum reflection loss of-58.08 dB with a thickness of 1.9 mm,and an effective absorption bandwidth of 2.88 GHz.Mechanism analysis revealed that the structural design of SiO_(2) layer not only optimized impedance matching,but also synergistically enhanced multiple loss mechanisms such as interfacial polarization and dipolar polarization.Therefore,this work provides valuable insights for the future preparation of high-performance electromagnetic wave absorbing Ti_(3)C_(2)T_(x)-based composites. | Huanhuan Niu Xuewen Jiang Wei Li Zhiyu Min Budi Riza Putra Wulan Tri Wahyuni Hailong Wang Rui Zhang Bingbing Fan | 2024 | Nano Research2024，17，3： | 0 |
| 4 | Cu_(x)S_(y)-MoS_(2)异质结构的介电损耗调控及其高效电磁波吸收显示文摘二硫化钼(MoS_(2))因高的比表面积和独特的电子结构在电磁波(EMW)吸收领域备受关注,但其高导电性导致EMW吸收性能较差。为了解决这个问题,本文引入Cu_(x)S_(y)纳米颗粒,构建一种独特的Cu_(x)S_(y)-MoS_(2)异质结构,以实现适当的阻抗匹配和衰减能力。通过调控Cu_(x)S_(y)纳米颗粒,达到调节介电损耗能力,以使Cu_(x)S_(y)-MoS_(2)材料在低、中、高频率下都能表现出优异的EMW吸收性能。Cu_(x)S_(y)-MoS_(2)样品在12.68 GHz的频率下,表现出高达-72.77 dB的反射损耗(RL),而材料的匹配厚度仅为1.99 mm,优于大多数金属硫化物异质结构。此外,它还具有宽的有效吸收带宽(EAB),在1.73 mm处达到5.1 GHz(12.9~18.0 GHz)。这项工作为设计具有强吸收、宽频带和薄厚度的MoS_(2)基吸波材料提供了新的策略。 | 蒋肖 李博 何邦 曾小军 | 2024 | 人工晶体学报2024，53，2： | 0 |
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