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Metal-organic framework membranes: From synthesis to electrocatalytic applications

查看全文 作　　者：Xiaobang [1]Liu;Ting [1]Yue;Kai [1]Qi;Yubing [1]Qiu;Bao Yu [1]Xia;Xingpeng [2]Guo 高影响力作者 机构地区：[1]Key Laboratory of Material Chemistry for Energy Conversion and Storage(Ministry of Education),Hubei Key Laboratory of Material Chemistry and Service Failure,School of Chemistry and Chemical Engineering,Huazhong University of Science and Technology(HUST),Wuhan 430074,China;[2]School of Chemistry and Chemical Engineering,Guangzhou University,Guangzhou 510006,China高影响力机构 出　　处：《Chinese Chemical Letters》索引2020年第31卷第9期,共13页高影响力期刊 基　　金：financially supported by National Natural Science Foundation of China(Nos.21805103,21805104,21802048);Fundamental Research Funds for the Central Universities(Nos.2018KFYYXJJ121,2019KFYXJJS073);National 1000 Young Talents Program of China。 摘　　要：Metal-orga nic frameworks(MOFs),as an emerging family of porous inorga nic-organic crystal materials,exhibit widely applications in gas storage and separation,drug release,sensing,and catalysis,owing to easily adjustable pore sizes,uniformly distributed metal centers,high surface areas,and tunable functionalities.However,MOF crystal powders are usually difficult to be directly applied into specific devices because of their brittleness,insolubility and low compatibility.Therefore,to expand versatile MOF membranes with robustness and operational flexibility is urgent to satisfy practical applications.Although numerous reports have reviewed the synthesis and applications of MOF membranes,relatively few reports the electrocatalytic properties based on MOF membranes.Herein,this mini-review provides an overview of preparation of MOF membranes,including directed synthesis,secondary growth and electrochemical deposition method.Meanwhile,fabrication of ultrathin 2D MOF nanosheets those can be also defined as a kind of nanoscale MOF membranes is also mentioned.Electrocatalytic performance of oxygen reduction reaction(ORR),oxygen evolution reaction(OER),hydrogen evolution reaction(HER)and CO2 reduction reaction(CO2RR) for diverse MOF membranes/nanosheets and their derivatives are introduced. 关 键 词：Metal-organic frameworks Membranes NANOSHEETS DERIVATIVES SYNTHESIS ELECTROCATALYSIS
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