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Volcanic relationship between wettability of the interface and water migration rate in solar steam generation systems

查看全文 作  者:Qiang [1]Fu;Xiaojuan [3]Li;Ning [2]Ma;Dier [1]Shi;Pohua [1]Chen;Junliang [1]Sun 高影响力作者 机构地区:[1]College of Chemistry and Molecular Engineering,Peking University,Beijing National Laboratory for Molecular Sciences(BNLMS),Beijing 100871,China;[2]Hubei Key Laboratory of Polymer Materials,Key Laboratory for the Green Preparation and Application of Functional Materials(Ministry of Education),Hubei Collaborative Innovation Center for Advanced Organic Chemical Materials,School of Materials Science and Engineering,Hubei University,Wuhan 430062,China;[3]College of Physics,Sichuan University,Chengdu 610065,China高影响力机构 出  处:《Nano Research》索引2022年第15卷第2期,共8页高影响力期刊 基  金:funding from the National Natural Science Foundation of China(Nos.21871009 and 21527803);the Youth Science Foundation of Hubei University(No.202011303000002);China Postdoctoral Science Foundation(No.2018M641064). 摘  要:Capturing solar energy as heat for water treatment has become a substantial approach to obtain freshwater.To obtain higher performance,the understanding of the mechanism of how water molecules interact with the interface is particularly fundamental,because the migration process of water molecules on the evaporation interface will directly affect the performance of the device.Herein we regulate the number of hydroxyl groups on the surface of reduced graphene oxide quantitatively,to study the effect of different wettability of interfaces on the performance of solar water generators.The water evaporation performance displays a volcanic shape as increasing wettability.Calculated by the computational chemistry method,deviation from proper wetting humidity is not conducive to the migration of water molecules from the surface.The double-edged sword effect of wettability on performances is clarified,and the surface energy density is the key to break through the limit by the finite element method. 关 键 词:solar water steam generation surface interface reaction WETTABILITY volcanic relationship computational modeling
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