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Single-atom catalysts for the electrochemical reduction of carbon dioxide into hydrocarbons and oxygenates

查看全文 作　　者：Karl Adrian [1]Gandionco;Juwon [1]Kim;Lieven [2]Bekaert;Annick [2]Hubin;Jongwoo [1]Lim 高影响力作者 机构地区：[1]Department of Chemistry,Seoul National University,Seoul,Republic of Korea;[2]Research Group Electrochemical and Surface Engineering(SURF),Department of Materials and Chemistry,Vrije Universiteit Brussel,Brussels,Belgium高影响力机构 出　　处：《Carbon Energy》索引2024年第6卷第3期,共54页高影响力期刊 基　　金：supported by the National Research Foundation of Korea(NRF)grant funded by the Korean government(MSIP)(NRF,2021R1C1C1013953,2022K1A4A7A04094394,2022K1A4A7A04095890)。 摘　　要：The electrochemical reduction of carbon dioxide offers a sound and economically viable technology for the electrification and decarbonization of the chemical and fuel industries.In this technology,an electrocatalytic material and renewable energy-generated electricity drive the conversion of carbon dioxide into high-value chemicals and carbon-neutral fuels.Over the past few years,single-atom catalysts have been intensively studied as they could provide near-unity atom utilization and unique catalytic performance.Single-atom catalysts have become one of the state-of-the-art catalyst materials for the electrochemical reduction of carbon dioxide into carbon monoxide.However,it remains a challenge for single-atom catalysts to facilitate the efficient conversion of carbon dioxide into products beyond carbon monoxide.In this review,we summarize and present important findings and critical insights from studies on the electrochemical carbon dioxide reduction reaction into hydrocarbons and oxygenates using single-atom catalysts.It is hoped that this review gives a thorough recapitulation and analysis of the science behind the catalysis of carbon dioxide into more reduced products through singleatom catalysts so that it can be a guide for future research and development on catalysts with industry-ready performance for the electrochemical reduction of carbon dioxide into high-value chemicals and carbon-neutral fuels. 关 键 词：ELECTROCATALYSIS electrochemical CO_(2)reduction hydrocarbons OXYGENATES single-atom catalysts
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