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| 1 | Adsorption behavior of condensed phosphate on aluminum hydroxide显示文摘钠焦磷酸盐( pyro-P , Na4P2O7 ),钠 tripolyphosphate ( tripoly-P , Na5P3O10 ),并且钠 hexametaphosphate ( meta-P ,( NaPO3 ) 6 )作为压缩磷酸盐的 modelcompounds 被选择调查 hydroxide.The 吸附被发现进二个阶段吸热、可分的压缩磷酸盐 onaluminum 的吸附行为:( 1 )在 1 h 以内的快吸附;并且( 2 )在 1 和 24 h.The 之间的慢吸附修改了 Freundlich modelsimulated 快吸附阶段井;慢吸附阶段被 pyro-P 的thefirst顺序 kinetics.The 激活精力描述很好, tripoly-P ,并且 aluminumhydroxide 上的 meta-P 吸附决心是 20.2,22.8 和 10.9 kJ/mol P 分别地,在 fastadsorption 阶段并且到吸附了分别地, 66.3,53.5 和 72.5 kJ/mol P 在慢 adsorptionstage.The 吸附 incre | GUAN Xiao-hong CHEN Guang-hao SHANG Chii | 2007 | Journal of Environmental Sciences2007，19，3： | 9 |
| 2 | ATR-FTIR and XPS study on the structure of complexes formed upon the adsorption of simple organic acids on aluminum hydroxide显示文摘到金属( hydr )的器官的 ligands 的绑定的信息为在金属( hydr )上理解自然有机物的吸附行为有用的氧化物 surfacesis oxide.In 这研究,安息香酸盐和水杨酸盐作为器官的 ligands andaluminum 氢氧化物作为金属 hydroxide.The 稀释了的模型被采用全部的反射 Fourier transforminfrared ( ATR-FTIR )系列表明 ligands 安息香酸盐和水杨酸盐做并列 directlywith 含水的铝氢氧化物的表面,从而 | GUAN Xiao-hong CHEN Guang-hao SHANG Chii | 2007 | Journal of Environmental Sciences2007，19，4： | 8 |
| 3 | Molecular characterization of transformation and halogenation of natural organic matter during the UV/chlorine AOP using FT-ICR mass spectrometry显示文摘UV/chlorine process,as an emerging advanced oxidation process(AOP),was effective for removing micro-pollutants via various reactive radicals,but it also led to the changes of natural organic matter(NOM)and formation of disinfection byproducts(DBPs).By using negative ion electrospray ionization coupled with Fourier transform ion cyclotron resonance mass spectrometry(ESI FT-ICR MS),the transformation of Suwannee River NOM(SRNOM)and the formation of chlorinated DBPs(Cl-DBPs)in the UV/chlorine AOP and subsequent post-chlorination were tracked and compared with dark chlorination.In comparison to dark chlorination,the involvement of Cl O·,Cl·,and HO·in the UV/chlorine AOP promoted the transformation of NOM by removing the compounds owning higher aromaticity(AI mod)value and DBE(double-bond equivalence)/C ratio and causing the decrease in the proportion of aromatic compounds.Meanwhile,more compounds which contained only C,H,O,N atoms(CHON)were observed after the UV/chlorine AOP compared with dark chlorination via photolysis of organic chloramines or radical reactions.A total of 833 compounds contained C,H,O,Cl atoms(CHOCl)were observed after the UV/chlorine AOP,higher than 789 CHOCl compounds in dark chlorination,and one-chlorine-containing components were the dominant species.The different products from chlorine substitution reactions(SR)and addition reactions(AR)suggested that SR often occurred in the precursors owning higher H/C ratio and AR often occurred in the precursors owning higher aromaticity.Post-chlorination further caused the cleavages of NOM structures into small molecular weight compounds,removed CHON compounds and enhanced the formation of Cl-DBPs.The results provide information about NOM transformation and Cl-DBPs formation at molecular levels in the UV/chlorine AOP. | Xiaoxue Ruan Yingying Xiang Chii Shang Shuangshuang Cheng Jingfu Liu Zhineng Hao Xin Yang | 2021 | Journal of Environmental Sciences2021，33，4： | 5 |
| 4 | Effect of Fe(Ⅲ) on the bromate reduction by humic substances in aqueous solution显示文摘Humic substances are ubiquitous redox-active organic compounds of environment. In this study, experiments were conducted to determine the reduction capacity of humic acid in the matrix of bromate and Fe(Ⅲ) solutions and the role of Fe(Ⅲ) in this redox process. The results showed that the humic acid regenerated Fe(Ⅱ) and reduced bromate abiotically. The addition of Fe(Ⅲ) could accelerate the bromate reduction rate by forming humic acid-Fe(Ⅲ) complexes. Iron species acts as electron mediator and catalyst for the bromate reduction by humic acid, in which humic acid transfers electrons to the complexed Fe(Ⅲ) to form Fe(Ⅱ), and the regenerated Fe(Ⅱ) donate the electrons to bromate. The kinetics study on bromate reduction further indicated that bromate reduction by humic acid-Fe(Ⅲ) complexes is pH dependent. The rate decreased by 2-fold with the increase in solution pH by one unit. The reduction capacity of Aldrich humic acid was observed to be lower than that of humic acid or natural organic matter of Suwanne River, indicating that such redox process is expected to occur in the environment. | XIE Li SHANG Chii ZHOU Qi | 2008 | Journal of Environmental Sciences2008，20，3： | 4 |
| 5 | E. coli and bacteriophage MS2 disinfection by UV, ozone and the combined UV and ozone processes显示文摘低剂量的臭氧与的联合紫外(紫外) 照耀应该是一种选择把利益给消毒和还原剂缺点紫外并且臭氧消毒。然而,少些对消毒表演被知道紫外并且臭氧(UV/ozone ) coexposure 和顺序的 UV-followed-by-ozone (紫外臭氧) 并且 ozone-followed-by-UV (臭氧 -- 紫外) 暴露。在这研究, E 的 inactivation。coli 和抗菌素 MS2 由紫外,臭氧, UV/ozone coexposure,并且顺序紫外臭氧并且臭氧 -- 紫外暴露被调查并且比较。E 上的 0.50.9 木头杀死的 Synergistic 效果。包括率和效率的增加, coli inactivation 在象 0.05 mg 潩 ? 慷 ? 捡畴污祬椠据敲獡摥愠瑦牥挠汨牯湩瑡潩一样低的臭氧集中在 UV/ozone coexposure 以后被观察吗? | Jingyun FANG Huiling LIU Chii SHANG Minzhen ZENG Mengling NI Wei LIU | 2014 | Frontiers of Environmental Science & Engineering2014，8，4： | 3 |
| 6 | DBP formation from degradation of DEET and ibuprofen by UV/chlorine process and subsequent post-chlorination显示文摘The formation of disinfection by-products(DBPs) from the degradation of N,N-diethyl-3-methyl benzoyl amide(DEET) and ibuprofen(IBP) by the ultraviolet irradiation(UV)/chlorine process and subsequent post-chlorination was investigated and compared with the UV/H_2O_2 process.The pseudo first-order rate constants of the degradation of DEET and IBP by the UV/chlorine process were 2 and 3.1 times higher than those by the UV/H_2O_2 process, respectively, under the tested conditions. This was due to the significant contributions of both reactive chlorine species U(RCS) and hydroxyl radicals(HO) in the UV/chlorine process. Trichloromethane, 1,1,1-trichloro-2-propanone and dichloroacetic acid were the major known DBPs formed after 90% of both DEET and IBP that were degraded by the UV/chlorine process. Their yields increased by over 50%after subsequent 1-day post-chlorination. The detected DBPs after the degradation of DEET and IBP comprised 13.5% and 19.8% of total organic chlorine(TOCl), respectively, and the proportions increased to 19.8% and 33.9% after subsequent chlorination, respectively. In comparison to the UV/H_2O_2 process accompanied with post-chlorination, the formation of DBPs and TOCl in the UV/chlorine process together with post-chlorination was 5%–63% higher,Ulikely due to the generation of more DBP precursors from the attack of RCS, in addition to HO. | Ehsan Aghdam Yingying Xiang Jianliang Sun Chii Shang Xin Yang Jingyun Fang | 2017 | Journal of Environmental Sciences2017，29，8： | 3 |
| 7 | Factors affecting formation of haloacetonitriles, haloketones, chloropicrin and cyanogen halides during chloramination显示文摘 | Yang Xin Shang Chii Westerhoff Paul | 2007 | Water Research2007，41，6： | 1 |
| 8 | Mechanisms controlling adsorption of natural organic matter on surfactant-modified iron oxide-coated sand显示文摘 | Chunli Ding Chii Shang | 2010 | Water Research2010，，12： | 1 |
| 9 | Disinfection by-product forma- tion from chlommination clarified water after prechlorination and pmozonation 显示文摘 | Yang xin Zhao Quan Shang Chii | 2008 | Water Supply2008，8，3： | 1 |
| 10 | Formation of carbonaceous and nitrogenous disinfection by-products from the chlorination of Microcystis aeruginosa显示文摘 | Jingyun Fang Jun Ma Xin Yang Chii Shang | 2009 | Water Research2009，，6： | 1 |
| 11 | Factors affecting formation of haloacetonitriles, haloketones, chloropicrin and cyanogen halides during chloramination显示文摘 | Xin Yang Chii Shang Paul Westerhoff | 2007 | Water Research2007，，6： | 1 |
| 12 | Chlorination byproduct for- mation in the presence of humic acid, model nitroge- nous organic compounds, ammonia, and bromide 显示文摘 | Yang Xin Shang Chii | 2004 | Environmental Science and Technology2004，38，19： | 1 |
| 13 | Formation of haloacetic acids during monochloramination显示文摘 | Yinan Qi Chii Shang | 2004 | Water Research2004，38，12： | 1 |
| 14 | Re-use of water treatment works sludge to enhance particulate pollutant removal from sewage 显示文摘 | Xiao-Hong Guan Guang-Hao Chen Chii Shang | 2005 | Water Research2005，39，15： | 1 |
| 15 | Role of humic acid and quinone model compounds in bromate by zerovalent iron 显示文摘 | Xie Li Chii Shang | 2005 | Environ Sci Technol2005，39，4： | 1 |
| 16 | Formation of haloacetic acids during monochloramination显示文摘 | Qi Yinan Shang Chii Lo M | 2004 | Water Res2004，38，16： | 1 |
| 17 | Effects of copper and palladium on the reduction of bromate by Fe(0)显示文摘 | Li Xie Chii Shang | 2006 | Chemosphere2006，，6： | 1 |
| 18 | MS2 inactivation by chloride assisted electrochemical disinfection 显示文摘 | Qian Fang Chii Shang G Chen | 2006 | Journal of Environmental Engineering2006，132，1： | 1 |
| 19 | Chlorination of pire bacterial cultures in aqueous solution 显示文摘 | Shang Chii Blateh R Ernest Iii Let | 2001 | Water Research2001，35，1： | 1 |
| 20 | Re-use of water treatment works sludge to enhance particulate pollutant removal from sewage显示文摘 | Guan Xiaohong Chen Guanghao Shang Chii | | 0，，39： | 1 |
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