|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | In situ grown Fe_(3)O_(4)particle on stainless steel:A highly efficient electrocatalyst for nitrate reduction to ammonia显示文摘NH_(3)is an essential feedstock for fertilizer synthesis.Industry-scale NH_(3)synthesis mostly relies on the Haber-Bosch method,however,which suffers from massive CO_(2) emission and high energy consumption.Electrocatalytic NO_(3)-reduction is an attractive substitute to the Haber-Bosch method for synthesizing NH_(3)under mild conditions.As this reaction will produce a variety of products,it highly desires efficient and selective electrocatalyst for NH_(3)generation.Here,we report in situ grown Fe_(3)O_(4)particle on stainless steel(Fe_(3)O_(4)/SS)as a high-efficiency electrocatalyst for NO_(3)^(-)reduction to NH_(3).In 0.1 M NaOH with 0.1 M NaNO_(3),such Fe_(3)O_(4)/SS reaches a remarkable Faradaic efficiency of 91.5%and a high NH_(3)yield of 10,145μg·h^(-1)·cm^(-2)at-0.5 V vs.reversible hydrogen electrode(RHE).Furthermore,it owns robust structural and electrochemical stability.This work provides useful guidelines to expand the scope of metallic oxide electrocatalysts for NH_(3)synthesis.The catalytic mechanism is uncovered and discussed further by theoretical calculations. | Xiaoya Fan Lisi Xie Jie Liang Yuchun Ren Longcheng Zhang Luchao Yue Tingshuai Li Yonglan Luo Na Li Bo Tang Yang Liu Shuyan Gao Abdulmohsen Ali Alshehri Qian Liu Qingquan Kong Xuping Sun | 2022 | Nano Research2022，15，4： | 7 |
| 2 | Miniature EMP Generator Based on Marx Circuit显示文摘A monopole and a dual-polar ten-stage miniature Marx generators with avalanche transistors are designed and developed for experiments of electromagnetic pulses.These avalanche transistors,which exceed traditional gas-gap switches in stability,size and repetition rate,are used as the high-speed switches in the Marx circuit.The influences of charging resistors,capacitances and load impedances on pulse width,repetition rate of output pulses are analyzed.The monopole Marx circuit has a size of 74 mm×32 mm,and its output voltage is1.8 kV when the charging voltage is 280 V.The dual-polar Marx circuit,which is 98 mm×32 mm,can generate either positive or negative polarity pulses synchronously with an output voltage of±1.6 kV,and a repetition rate of 10 kHz.The feasibility of the presented dual-polar Marx generator is proved by further tests. | ZHOU Xing ZHAO Min FAN Lisi WANG Qingguo YANG Qingxi | 2013 | 高电压技术2013，39，10： | 3 |
| 3 | Research on the Equivalence Between Double Differential- mode Current Injection and Radiation Test Method显示文摘There are the application scope limits for single differential-mode current injection test method, so in order to carry out injection susceptibility test for two-pieces equipment interconnected with both ends of a cable simultaneously, a double differential-mode current in- jection test method (DDMCI) is proposed. The method adopted the equivalence source wave theorem and Baum-Liu-Tesche(BLT) equation as its theory foundation. The equivalent corresponding relation between injection voltage and radiation electric field intensity is derived, and the phase relation between the two injection voltage sources is confirmed. The results indicate that the amplitude and phase of the equivalent injection voltage source is closely related to the S parameter of directional coupling device, the transmission line length, and the source vector in BLT equation, but has nothing to do with the reflection coefficient between the two equipment pieces. Therefore, by choosing the right amplitude and phase of the double injection voltage sources, the DDMCI test is equivalent to the radiation test for two interconnected equipment of a system. | PAN Xiaodong WEI Guanghui FAN Lisi LU Xinfu YANG Zhe | 2013 | 高电压技术2013，39，8： | 1 |
| 4 | Frequency-time Domain Shielding Effectiveness of Materials and Their Strong Electromagnetic Field Test显示文摘To describe the shielding ability of materials accurately and comprehensively,the frequency-domain and time-domain shielding effectiveness(SE) of material is investigated.The relevance between them was analyzed based on the minimum phase method,and the time-domain SE can be derived from frequency-domain SE.The SE of an energy selective surface(ESS) made of a novel material is investigated,and the relationship between SE and radiation field intensity are analyzed.The results show that not only material,but also the intensity of radiation electric field shows influence on SE in its frequency; for some materials,the dependence of SE on radiation electric field intensity needs to be considered.Therefore,it is necessary to research on the SE of shielding material in high-intensity electromagnetic environment. | ZHANG Long WEI Guanghui FAN Lisi HU Xiaofeng ZHAO Yang ZHANG Yongqiang | 2013 | 高电压技术2013，39，10： | 1 |
| 5 | NIR-Ⅱ-absorbing conjugated polymer-based theranostic agent for NIR-Ⅱfluorescence imaging-guided photothermal therapy acting synergistically with tumor microenvironment-responsive nitric oxide therapy显示文摘Despite tremendous advances in gas therapy,there are major concerns about the inevitable concentration of toxicity and the ability to perform real-time tracking of drug delivery.Second near-infrared(NIR-Ⅱ)window absorbing nanoplatforms hold great promise for precision medicine because of their excellent tissue penetration of light and non-invasive nature.In this study,we engineered an NIR-Ⅱlaser-activated theranostic agent(named CP-bF@PEG)that was composed of amphiphilic polymers(Pluronic F127,with polyethylene glycol,PEG,moieties)coated with an NIR-Ⅱ-absorbing conjugated polymer(PTTBBT,CP)and nitric oxide(NO)donor(benzofuroxan,bF),which served as an NIR-Ⅱphotothermal inducer and NO nanogenerator.Under deep tissue penetration of NIR-Ⅱlaser irradiation,CP-bF@PEG was found to possess fluorescence imaging ability to accurately identify tumor and excellent photothermal effect.Moreover,CP-bF@PEG could generate NO via glutathione activation in the tumor microenvironment in a controllable manner.This NIR-Ⅱ-absorbing polymer for high-contrast NIR-Ⅱfluorescence imaging-guided precision photothermal therapy achieved synergistic effects with NO therapy,as evidenced by pronounced tumor therapeutic efficacy and few side effects.This nanotheranostic agent is a highly promising candidate for high-contrast NIR-Ⅱimaging-guided precision photothermal therapy combined with gas therapy against cancer. | Jie Li Lisi Xie Wei Sang Wenxi Li Guohao Wang Hao Tian Zhan Zhang Jianhua Liu Quli Fan Yunlu Dai | 2022 | ChemPhysMater2022，1，1： | 0 |
您所在的机构暂未开通此部分的功能，请联系管理员