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| 1 | Controlling the gelation temperature of biomimetic polyisocyanides显示文摘Thermosensitive polymers show an entropy-driven transition from a well-solvated to a poorly solvated polymer chain, resulting in a more compact globular conformation. The transition at the lower critical solution temperature(LCST) is often sharp, which allows for a wide range of smart material applications.At the LCST, oligo(ethylene glycol)-substituted polyisocyanides(PICs) form soft hydrogels, composed of polymer bundles similar to biological gels, such as actin, fibrin and intermediate filaments. Here, we show that the LCST of PICs strongly depends linearly on the length of the ethylene glycol(EG) tails; every EG group increases the LCSTand thus the gelation temperature by nearly 30 ℃. Using a copolymerisation approach, we demonstrate that we can precisely tailor the gelation temperature between 10 ℃ and 60 ℃and, consequently, tune the mechanical properties of the PIC gels. | Paul H.J. Kouwer Paula de Almeida Onno ven den Boomen Zaskia H. Eksteen-Akeroyd Roel Hammink Maarten Jaspers Stijn Kragt Mathijs F.J. Mabesoone RoelandJ.M. Nolte Alan E. Rowan Martin G.T.A. Rutten Vincent A.A. Le Sage Daniel C. Schoenmakers Chengfen Xing Jialiang xu | 2018 | Chinese Chemical Letters2018，29，2： | 2 |
| 2 | Biomechanical comparison of kypboplasty with different bone cements显示文摘 | Molloy S Jasper LE | 2004 | Spine2004，29，11： | 1 |
| 3 | An ex vivo biomechanieal evaluation of a hydroxyapatite cement for use with vertebroplasty显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 4 | The biomechanies of vertebroplasty:the effect of cement volume on mechanical behavior显示文摘 | Belkoff SM Mathis JM Jasper LE | | 0，，： | 1 |
| 5 | Biomechanical comparison of kyphoplasty with different bone cements显示文摘 | Tomita S Molloy S Jasper LE | 2004 | Spine2004，29，11： | 1 |
| 6 | Biomechanical comparison of kyphoplasty with different bone cements 显示文摘 | Tomita S Molloy S Jasper LE | 2004 | Spine2004，29，： | 1 |
| 7 | The effect of oblique femoral tunnel placement on rotational constraint of the knee reconstructed using patellar tendon autografts 显示文摘 | ScoppJM Jasper LE Belkoff SM | 2004 | Arthroseopy2004，20，3： | 1 |
| 8 | The biomechan-ics of vertebroplasty:the effect of cement volume on me-chanical behavior显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 9 | Ex vivo biomechanical comparison of hydroxyapaptite andpolymethymethacrylate cements for use with vertebroplasty显示文摘 | Belkoff SM Mathis JM Jasper LE | 2002 | AJNR2002，23，： | 1 |
| 10 | An ex vivo biomechanical evaluation of a hydroxyapatite cement for use with vertebroplasty显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 11 | The biomechanica of Vente- broplasty, The effect of cement volume on hiomechnical behavior显示文摘 | Belkoff SM Mthis JM Jasper LE el al | 2001 | Spine2001，26，： | 1 |
| 12 | Biomechanical comparison of Kyphoplasty with different bone cements显示文摘 | Molloy S Jasper LE | 2004 | Spine2004，29，： | 1 |
| 13 | The biomechanics of vertebroplasty:the effect of cement volume on mechanical behavior显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 14 | The biomechanics of vertebroplasty,the effect of cement volume on mechanical behavior显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 15 | An ex vivo biomechanical evaluation of a hydroxyapatite cement for use with vertebroplasty显示文摘 | Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 16 | The biomechanics of vertebroplasty: the effect of cement vol ume on mechanical behavior显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 17 | The biomechanics of vertebroplasty: the effect of cement volume on mechanical behav- ior显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 18 | An ex vivo biomechanical evaluation of a hydroxylapatite cement for use with vertebroplasty显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 19 | The biomechanics of ver-tebroplasty: the effect of cement volume on mechanical behavior显示文摘 | Belkoff SM Mathis JM Jasper LE | 2001 | Spine2001，26，14： | 1 |
| 20 | Biomechanical comparison of kyphoplasty with different bone cements显示文摘 | Tomita S Molloy S Jasper LE | 2004 | Spine2004，29，11： | 1 |
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