|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Rapid epitaxy of 2-inch and high-quality α-Ga_(2)O_(3) films by mist-CVD method显示文摘High thickness uniformity and large-scale films of α-Ga_(2)O_(3) are crucial factors for the development of power devices.In this work, a high-quality 2-inch α-Ga_(2)O_(3) epitaxial film on c-plane sapphire substrates was prepared by the mist-CVD method.The growth rate and phase control mechanisms were systematically investigated. The growth rate of the α-Ga_(2)O_(3) films was limited by the evaporation of the microdroplets containing gallium acetylacetonate. By adjusting the substrate position(z) from 80 to 50 mm, the growth rate was increased from 307 nm/h to 1.45 μm/h when the growth temperature was fixed at 520 °C.When the growth temperature exceeded 560 °C, ε-Ga_(2)O_(3) was observed to form at the edges of 2-inch sapphire substrate.Phase control was achieved by adjusting the growth temperature. When the growth temperature was 540 °C and the substrate position was 50 mm, the full-width at half maximum(FWHM) of the rocking curves for the(0006) and(10-14) planes were 0.023° and 1.17°. The screw and edge dislocations were 2.3 × 10~6 and 3.9 × 10~(10)cm~(-2), respectively. Furthermore, the bandgaps and optical transmittance of α-Ga_(2)O_(3) films grown under different conditions were characterized utilizing UV-visible and near-IR scanning spectra. | Xiaojie Wang Wenxiang Mu Jiahui Xie Jinteng Zhang Yang Li Zhitai Jia Xutang Tao | 2023 | Journal of Semiconductors2023，44，6： | 1 |
| 2 | In situ generated layered NiFe-LDH/MOF heterostructure nanosheet arrays with abundant defects for efficient alkaline and seawater oxidation显示文摘As the main limiting step of overall water splitting,oxygen evolution reaction(OER)is urgent to be enhanced by developing efficient catalysts to promote the process of electrolytic water.Based on theoretical analysis,the Ni-metal-organic framework(Ni-MOF)and NiFe-layered double hydroxide(NiFe-LDH)(NiFe-LDH/MOF)heterostructure can optimize the energy barrier of the OER process and decrease the adsorption energy of oxygen-containing intermediates,effectively accelerating the OER kinetics.Accordingly,layered NiFe-LDH/MOF heterostructures are in situ constructed through a facile two-step reaction process,with substantial oxygen defects and lattice defects that further improve the catalytic performance.As a result,only 208 and 275 mV OER overpotentials are needed for NiFe-LDH/MOF to drive the current densities of 20 and 100 mA·cm^(-2)in 1 M KOH solutions,and even maintain catalytic stability of 100 h at 20 mA·cm^(-2).When applied to seawater oxidation,only 235 and 307 mV OER overpotentials are required to achieve the current densities of 20 and 100 mA·cm^(-2),respectively,with almost no attenuation for 100 h stability test at 20 mA·cm^(-2),all better than commercial RuO_(2).This work provides the theoretical and experimental basis and a new idea for efficiently driving fresh water and seawater cracking by heterostructure and defect coupling design toward catalysts. | Manjie Xiao Can Wu Jiawei Zhu Chengtian Zhang Yan Li Jiahui Lyu Weihao Zeng Haiwen Li Lei Chen Shichun Mu | 2023 | Nano Research2023，16，7： | 1 |
| 3 | Efficient conversion of lignin waste and self-assembly synthesis of C@MnCo_(2)O_(4)for asymmetric supercapacitors with high energy density显示文摘Lignin waste from the papermaking and biorefineries industry is a significantly promising renewable resource to prepare advanced carbon materials for diverse applications,such as the electrodes of supercapacitors;however,the improvement of their energy density remains a challenge.Here,we design a green and universal approach to prepare the composite electrode material,which is composed of lignin-phenolformaldehyde resins derived hierarchical porous carbon(LR-HPC)as conductive skeletons and the self-assembly manganese cobaltite(MnCo_(2)O_(4))nanocrystals as active sites.The synthesized C@MnCo_(2)O_(4)composite has an abundant porous structure and superior electronic conductivity,allowing for more charge/electron mass transfer channels and active sites for the redox reactions.The composite shows excellent electrochemical performance,such as the maximum specific capacitance of~726 mF cm^(-2)at 0.5 mV s^(-1),due to the significantly enhanced interactive interface between LR-HPC and MnCo_(2)O_(4)crystals.The assembled all-solid-state asymmetric supercapacitor,with the LR-HPC and C@MnCo_(2)O_(4)as cathode and anode,respectively,exhibits the highest volumetric energy density of 0.68 mWh cm^(-3)at a power density of 8.2 mW cm^(-3).Moreover,this device shows a high capacity retention ratio of~87.6%at 5 mA cm^(-2)after 5000 cycles. | Jiahui Mu Cuihuan Li Jiankang Zhang Xianliang Song Sheng Chen Feng Xu | 2023 | Green Energy & Environment2023，8，5： | 0 |
| 4 | Mechanically strong,flexible,and multi-responsive phase change films with a nacre-mimetic structure for wearable thermal management显示文摘Phase change materials(PCMs)are a highly promising candidate for thermal energy storage owing to their large latent heat and chemical stability.However,their intrinsic brittle induces poor flexibility and low mechanical strength,which limits them use for wearable thermal management.And,the electrical insulation and weak solar absorption make them lack multi-responsive capability.Herein,we report a facile strategy to synthesize mechanically strong and flexible multi-responsive phase change films by stirring an aqueous dispersion of cellulose nanofibrils(CNFs),MXene(Ti_(2)C_(3))nanosheets,and polyethylene glycol(PEG),followed by air-drying self-assembly and coating with hydrophobic fluorocarbon.The hydrogen bonds and nacre-mimetic synergistic toughening networks formed by ternary CNFs,Ti_(2)C_(3)nanosheets,and PEG endow films with high mechanical strength(16.7 MPa)and strain(10.4%),which are 18.6 and 8.7 times higher than those of pure PEG film,respectively.The films exhibit outstanding flexibility and do not crack or fracture even when bent,twisted,and folded into a complex small boat.Meanwhile,the laminar structure formed by the self-assembly Ti_(3)C_(2)nanosheets enhances electrical conductivity(3.95 S/m)and solar absorption,affording excellent electro-thermal(68.3%–81.0%)and solarthermal(85.6%–90.6%)conversion efficiency,thus achieving multi-response to external stimuli(electron/solar radiation).In addition,the as-prepared films also deliver large latent heat(136.1 J/g),outstanding cyclic and shape stability,leak-free encapsulation even under compressed at above 5000 times its weight,excellent hydrophobicity(131.4°),and self-cleaning function.This work paves the way for developing flexible,mechanically strong,and self-cleaning phase change film with multi-responsive function for wearable thermal management devices under high humidity condition. | Jiankang Zhang Jiahui Mu Sheng Chen Feng Xu | 2022 | Journal of Energy Chemistry2022，，12： | 0 |
| 5 | HDR-Net-Fusion:Real-time 3D dynamic scene reconstruction with a hierarchical deep reinforcement network显示文摘Reconstructing dynamic scenes with commodity depth cameras has many applications in computer graphics,computer vision,and robotics.However,due to the presence of noise and erroneous observations from data capturing devices and the inherently ill-posed nature of non-rigid registration with insufficient information,traditional approaches often produce low-quality geometry with holes,bumps,and misalignments.We propose a novel 3D dynamic reconstruction system,named HDR-Net-Fusion,which learns to simultaneously reconstruct and refine the geometry on the fly with a sparse embedded deformation graph of surfels,using a hierarchical deep reinforcement(HDR)network.The latter comprises two parts:a global HDR-Net which rapidly detects local regions with large geometric errors,and a local HDR-Net serving as a local patch refinement operator to promptly complete and enhance such regions.Training the global HDR-Net is formulated as a novel reinforcement learning problem to implicitly learn the region selection strategy with the goal of improving the overall reconstruction quality.The applicability and efficiency of our approach are demonstrated using a large-scale dynamic reconstruction dataset.Our method can reconstruct geometry with higher quality than traditional methods. | Hao-Xuan Song Jiahui Huang Yan-Pei Cao Tai-Jiang Mu | 2021 | Computational Visual Media2021，7，4： | 0 |
您所在的机构暂未开通此部分的功能，请联系管理员