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1篇 您的检索式：作者名="Jiewei Lil"

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		题名	作者	年代	出处	被引量
	1	Photoexcitation dynamics and energy engineering in supramolecular doping of organic conjugated molecules显示文摘Doping and blending strategies are crucial means to precisely control the excited states and energy level in conjugated molecular systems.However,effective models and platforms are rarely proposed to systematically explore the effects of the formation of trapped doped centers on heterogeneous structures,energy level and ultrafast photophysical process.Herein,for deeply understanding the impact of molecular doping in film energy levels and photoexcitation dynamics,we set a supramolecular N-B coordination composed by the conjugated molecules of pyridine functionalized diarylfluorene(host material),named as ODPF-Phpy and ODPF-(Phpy)2,and the molecule of tris(perfluorophenyl)borane(BCF)(guest material).The generation of the molecular-level coordination bond increased the binding energy of N atoms and tuned the band-gap,leading to a new fluorescent emission center with longer excitation wavelength and emission wavelength.The intermolecular Forster resonance energy transfer(FRET)in blending flms make it present inconsistent fluorescent behaviors compared to that in solution.The charge transfer(CT)state of N-B coordinated compounds and the changed dielectric constant of blending films resulted in a large PL spectra red-shift with the increased dopant ratio,causing a wide-tunable fluorescent color.The excited state behaviors of two compounds in blending system was further investigated by the transient absorption(TA)spectroscopy.Finally,we found supramolecular coordination blending can effectively improve the films'photoluminescence quantum yield(PLQY)and conductivity.We believe this exploration in the internal coordination mechanisms would deepen the insights about doped semiconductors and is helpful in developing novel high-efficient fluorescent systems.	Xiang An Chuanxin Wei Lubing Bai Jun Zhou Le Wang Yamin Han Lili Sun Jinyi Lin Heyuan Liu Jiewei Lil Man Xu Haifeng Ling Linghai Xie Wei Huang	2023	Light(Science & Applications)2023，12，2：	0

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