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| 1 | Chip-scale broadband spectroscopic chemical sensing using an integrated supercontinuum source in a chalcogenide glass waveguide显示文摘On-chip spectroscopic sensors have attracted increasing attention for portable and field-deployable chemical detection applications. So far, these sensors largely rely on benchtop tunable lasers for spectroscopic interrogation. Large footprint and mechanical fragility of the sources, however, preclude compact sensing system integration. In this paper, we address the challenge through demonstrating, for the first time to our knowledge, a supercontinuum source integrated on-chip spectroscopic sensor, where we leverage nonlinear Ge_(22)Sb_(18)Se_(60) chalcogenide glass waveguides as a unified platform for both broadband supercontinuum generation and chemical detection. A home-built, palm-sized femtosecond laser centering at 1560 nm wavelength was used as the pumping source. Sensing capability of the system was validated through quantifying the optical absorption of chloroform solutions at 1695 nm. This work represents an important step towards realizing a miniaturized spectroscopic sensing system based on photonic chips. | QINGYANG DU ZHENGQIAN LUO HUIKAI ZHONG YIFEI ZHANG YIZHONG HUANG TUANJIE DU WEI ZHANG TIAN GU JUEJUN HU | 2018 | Photonics Research2018，6，6： | 9 |
| 2 | High spatial and temporal resolution synthetic aperture phase microscopy显示文摘A new optical microscopy technique,termed high spatial and temporal resolution synthetic aperture phase microscopy(HISTR-SAPM),is proposed to improve the lateral resolution of wide-field coherent imaging.Under plane wave illumination,the resolution is increased by twofold to around 260 nm,while achieving millisecond-level temporal resolution.In HISTR-SAPM,digital micromirror devices are used to actively change the sample illumination beam angle at high speed with high stability.An off-axis interferometer is used to measure the sample scattered complex fields,which are then processed to reconstruct high-resolution phase images.Using HISTR-SAPM,we are able to map the height profiles of subwavelength photonic structures and resolve the period structures that have 198 nm linewidth and 132 nm gap(i.e.,a full pitch of 330 nm).As the reconstruction averages out laser speckle noise while maintaining high temporal resolution,HISTR-SAPM further enables imaging and quantification of nanoscale dynamics of live cells,such as red blood cell membrane fluctuations and subcellular structure dynamics within nucleated cells.We envision that HISTR-SAPM will broadly benefit research in material science and biology. | Cheng Zheng Di Jin Yanping He Hongtao Lin Juejun Hu Zahid Yaqoo Peter T.C.So Renjie Zhou | 2020 | Advanced Photonics2020，2，6： | 5 |
| 3 | All-optical computing based on convolutional neural networks显示文摘The rapid development of information technology has fueled an ever-increasing demand for ultrafast and ultralow-en-ergy-consumption computing.Existing computing instruments are pre-dominantly electronic processors,which use elec-trons as information carriers and possess von Neumann architecture featured by physical separation of storage and pro-cessing.The scaling of computing speed is limited not only by data transfer between memory and processing units,but also by RC delay associated with integrated circuits.Moreover,excessive heating due to Ohmic losses is becoming a severe bottleneck for both speed and power consumption scaling.Using photons as information carriers is a promising alternative.Owing to the weak third-order optical nonlinearity of conventional materials,building integrated photonic com-puting chips under traditional von Neumann architecture has been a challenge.Here,we report a new all-optical comput-ing framework to realize ultrafast and ultralow-energy-consumption all-optical computing based on convolutional neural networks.The device is constructed from cascaded silicon Y-shaped waveguides with side-coupled silicon waveguide segments which we termed“weight modulators”to enable complete phase and amplitude control in each waveguide branch.The generic device concept can be used for equation solving,multifunctional logic operations as well as many other mathematical operations.Multiple computing functions including transcendental equation solvers,multifarious logic gate operators,and half-adders were experimentally demonstrated to validate the all-optical computing performances.The time-of-flight of light through the network structure corresponds to an ultrafast computing time of the order of several picoseconds with an ultralow energy consumption of dozens of femtojoules per bit.Our approach can be further expan-ded to fulfill other complex computing tasks based on non-von Neumann architectures and thus paves a new way for on-chip all-optical computing. | Kun Liao Ye Chen Zhongcheng Yu Xiaoyong Hu Xingyuan Wang Cuicui Lu Hongtao Lin Qingyang Du Juejun Hu Qihuang Gong | 2021 | Opto-Electronic Advances2021，4，11： | 3 |
| 4 | Nonlinear optical properties of integrated GeSbS chalcogenide waveguides显示文摘In this paper, we report the experimental characterization of highly nonlinear Ge Sb S chalcogenide glass waveguides.We used a single-beam characterization protocol that accounts for the magnitude and sign of the real and imaginary parts of the third-order nonlinear susceptibility of integrated Ge23 Sb7 S70(GeSbS) chalcogenide glass waveguides in the near-infrared wavelength range at λ =1580 nm. We measured a waveguide nonlinear parameter of 7.0±0.7 W^(-1)· m(-1), which corresponds to a nonlinear refractive index of n_2=0.93±0.08 × 10^(-18) m^2∕W,comparable to that of silicon, but with an 80 times lower two-photon absorption coefficient βTPA=0.010± 0.003 cm∕GW, accompanied with linear propagation losses as low as 0.5 dB/cm. The outstanding linear and nonlinear properties of Ge Sb S, with a measured nonlinear figure of merit FOMTPA=6.0 ±1.4 at λ =1580 nm, ultimately make it one of the most promising integrated platforms for the realization of nonlinear functionalities. | SAMUEL SERNA HONGTAO LIN CARLOS ALONSO-RAMOS ANUPAMA YADAV XAVIER LE ROUX KATHLEEN RICHARDSON ERIC CASSAN NICOLAS DUBREUIL JUEJUN HU LAURENT VIVIEN | 2018 | Photonics Research2018，6，5： | 3 |
| 5 | Fabrication of single-crystalline silicon nanowires by scratching a silicon surface with catalytic metal particles 显示文摘 | Peng Kuiqing Hu Juejun Yah Yuniie | 2006 | Adv Funct Mater2006，16，3： | 1 |
| 6 | Metal-particle-induced,highly localized site-specific etching of Si and formation of single-crystalline Si nanowires in aqueous fluoride solution显示文摘 | Peng Kuiqing Fang Hui Hu Juejun | 2006 | CHEMISTRY-A EUROPEAN JOURNAL2006，12，30： | 1 |
| 7 | Fabrication of single-crystalline silicon nanowires by scratching a silicon surface with catalytic metal particles显示文摘 | Peng Kuiqing Hu Juejun Yan Yunjie | 2006 | Adv Funet Mater2006，16，： | 1 |
| 8 | Fabrication of Single-Crystalline Silicon Nanowires by Scratching a Silicon Surface with Catalytic Metal Particles显示文摘 | KUIQING JUEJUN HU YUNJIE YAN | 2006 | Advanced Functional Materials2006，，16： | 1 |
| 9 | Real-time,in situ probing of gamma radiation damage with packaged integrated photonic chips显示文摘Integrated photonics is poised to become a mainstream solution for high-speed data communications and sensing in harsh radiation environments,such as outer space,high-energy physics facilities,nuclear power plants,and test fusion reactors.Understanding the impact of radiation damage in optical materials and devices is thus a prerequisite to building radiation-hard photonic systems for these applications.In this paper,we report real-time,in situ analysis of radiation damage in integrated photonic devices.The devices,integrated with an optical fiber array package and a baseline-correction temperature sensor,can be remotely interrogated while exposed to ionizing radiation over a long period without compromising their structural and optical integrity.We also introduce a method to deconvolve the radiation damage responses from different constituent materials in a device.The approach was implemented to quantify gamma radiation damage and post-radiation relaxation behavior of SiO2-cladded SiC photonic devices.Our findings suggest that densification induced by Compton scattering displacement defects is the primary mechanism for the observed index change in SiC.Additionally,post-radiation relaxation in amorphous SiC does not restore the original pre-irradiated structural state of the material.Our results further point to the potential of realizing radiation-hard photonic device designs taking advantage of the opposite signs of radiation-induced index changes in SiC and SiO2. | QINGYANG DU JEROME MICHON BINGZHAO LI DEREK KITA DANHAO MA HAIJIE ZUO SHAOLIANG YU TIAN GU ANURADHA AGARWAL MO LI JUEJUN HU | 2020 | Photonics Research2020，8，2： | 1 |
| 10 | The impact of vertical π-extension on redox mechanisms of aromatic diimide dyes显示文摘Aromatic diimide dyes are an attractive class of redox-active organic molecules for lithium-ion batteries,whose battery performances(stabilities,conductivities and cyclicities) are strongly dependent on the sizes of their π-systems.However,due to the different Clar’s structures possessed,three vertically7 r-extended aromatic diimides,namely,naphthalene diimide(two one-electron reductions),perylene diimide and terrylene diimide(two one-electron reductions),exhibit different electronic redox mechanisms when served as cathode materials in organic lithium-ion batteries.Herein,we have studied carefully the different electrochemical characteristics of the three aromatic diimides through experimental and theoretical calculations.Their battery present different shape of charge/discharge curves resulting from stability of their reduction state during charge/discharge process.Terrylene diimide shows better cycle and rate capacities than those of naphthalene diimide and perylene diimide,which could be attributed to the more energies released during terrylene diimide combining with lithium ions than those of other two diimides. | Lei Li Juejun Wang Mengting Chen Yong Chen Wangchuan Xiao Dongyang Chen Meijin Lin | 2019 | Chinese Chemical Letters2019，30，12： | 0 |
| 11 | 3D integrated photonics platform with deterministic geometry control显示文摘3D photonics promises to expand the reach of photonics by enabling the extension of traditional applications to nonplanar geometries and adding novel functionalities that cannot be attained with planar devices.Available material options and device geometries are,however,limited by current fabrication methods.In this work,we pioneer a method that allows for placement of integrated photonic device arrays at arbitrary predefined locations in 3D using a fabrication process that capitalizes on the buckling of a 2D pattern.We present theoretical and experimental validation of the deterministic buckling process,thus demonstrating implementation of the technique to realize what we believe to be the first fully packaged 3D integrated photonics platform.Application of the platform for mechanical strain sensing is further demonstrated. | JEROME MICHON SARAH GEIGER LAN LI CLAUDIA GONCALVES HONGTAO LIN KATHLEEN RICHARDSON XINQIAO JIA JUEJUN HU | 2020 | Photonics Research2020，8，2： | 0 |
| 12 | Pd-Catalyzed Synthesis of a-Awl Vinylphosphonates via Suzuki Arylation of a-Phosphonovinyl Nonaflates显示文摘 | Meijuan Yuan Yewen Fang Li Zhang Xiaoping Jin Minjia Tao Qilin Ye Ruifeng Li Jinjian Li Hui Zheng Juejun Gu | 2015 | Chinese Journal of Chemistry2015，33，10： | 0 |
| 13 | Wide field-of-view metalens: a tutorial显示文摘Wide field-of-view(FOV)optics are essential components in many optical systems,with applications spanning imaging,display,sensing,and beam steering.Conventional refractive wide FOV optics often involve multiple stacked lenses,resulting in large size and weight as well as high cost.Metasurface lenses or metalenses promise a viable solution to realizing wide FOV optics without complex lens assembly.We review the various architectures of wide FOV metalenses,elucidate their fundamental operating principles and design trade-offs,and quantitatively evaluate and contrast their imaging performances.Emerging applications enabled by wide FOV metasurface optics are also discussed. | Fan Yang Mikhail YShalaginov Hung-I Lin Sensong An Anu Agarwal Hualiang Zhang Clara Rivero-Baleine Tian Gu Juejun Hu | 2023 | Advanced Photonics2023，5，3： | 0 |
| 14 | Angle-selective perfect absorption with two-dimensional materials显示文摘Two-dimensional(2D)materials have great potential in photonic and optoelectronic devices.However,the relatively weak light absorption in 2D materials hinders their application in practical devices.Here,we propose a general approach to achieve angleselective perfect light absorption in 2D materials.As a demonstration of the concept,we experimentally show giant light absorption by placing large-area single-layer graphene on a structure consisting of a chalcogenide layer atop a mirror and achieving a total absorption of 77.6%in the mid-infrared wavelength range(~13μm),where the graphene contributes a record-high 47.2%absorptivity of mid-infrared light.Construction of such an angle-selective thin optical element is important for solar and thermal energy harvesting,photo-detection and sensing applications.Our study points to a new opportunity to combine 2D materials with photonic structures to enable novel device applications. | Linxiao Zhu Fengyuan Liu Hongtao Lin Juejun Hu Zongfu Yu Xinran Wang Shanhui Fan | 2015 | Light(Science & Applications)2015，4，1： | 0 |
| 15 | 1,1’-Binaphthol annulated perylene diimides: Aggregation-induced emission enhancement and chirality inversion显示文摘Aggregation-induced emission enhancement and aggregation-induced chirality inversion are two individ-ual phenomena for the enantiomerically pure organic dyes in the aggregates.Herein we reported for the first time that these two interesting phenomena could be observed simultaneously in the aggregated states of enantiomerically pure S/R-1,1?-binaphthol annulated perylene diimides,in which two perylene diimides moieties were bridged by S/R-1,1?-binaphthol(BINOL)at the bay positions.Owing to the rotat-able C2 axes between two naphthol annulated perylene diimides moieties,both of them display intrinsic behaviors of aggregation-induced emission enhancements.At the same time,due to the steric hindrances in the imide and methoxy positions,the neighboring twoπ-systems of these two unique polycyclic aro-matic imides in poor solvents are preferable to adopt a cross-stacking mode and thus form helical X-aggregates of opposite chirality(M/P)with chirality inversion characteristics in their circular dichroism and circularly polarized luminescence spectroscopic studies. | Yang Zhang Juejun Wang Hongming Chen Meijin Lin | 2022 | Chinese Chemical Letters2022，33，5： | 0 |
| 16 | Monolithically integrated stretchable photonics显示文摘Mechanically stretchable photonics provides a new geometric degree of freedom for photonic system design and foresees applications ranging from artificial skins to soft wearable electronics.Here we describe the design and experimental realization of the first single-mode stretchable photonic devices.These devices,made of chalcogenide glass and epoxy polymer materials,are monolithically integrated on elastomer substrates.To impart mechanical stretching capability to devices built using these intrinsically brittle materials,our design strategy involves local substrate stiffening to minimize shape deformation of critical photonic components,and interconnecting optical waveguides assuming a meandering Euler spiral geometry to mitigate radiative optical loss.Devices fabricated following such design can sustain 41%nominal tensile strain and 3000 stretching cycles without measurable degradation in optical performance.In addition,we present a rigorous analytical model to quantitatively predict stressoptical coupling behavior in waveguide devices of arbitrary geometry without using a single fitting parameter. | Lan Li Hongtao Lin Shutao Qiao Yi-Zhong Huang Jun-Ying Li Jérôme Michon Tian Gu Carlos Alosno-Ramos Laurent Vivien Anupama Yadav Kathleen Richardson Nanshu Lu Juejun Hu | 2017 | Light(Science & Applications)2017，6，1： | 0 |
| 17 | Electrical programmable multilevel nonvolatile photonic random-access memory显示文摘Photonic Random-Access Memories(P-RAM)are an essential component for the on-chip non-von Neumann photonic computing by eliminating optoelectronic conversion losses in data links.Emerging Phase-Change Materials(PCMs)have been showed multilevel memory capability,but demonstrations still yield relatively high optical loss and require cumbersome WRITE-ERASE approaches increasing power consumption and system package challenges.Here we demonstrate a multistate electrically programmed low-loss nonvolatile photonic memory based on a broadband transparent phase-change material(Ge2Sb2Se5,GSSe)with ultralow absorption in the amorphous state.A zero-staticpower and electrically programmed multi-bit P-RAM is demonstrated on a silicon-on-insulator platform,featuring efficient amplitude modulation up to 0.2 dB/μm and an ultralow insertion loss of total 0.12 dB for a 4-bit memory showing a 100×improved signal to loss ratio compared to other phase-change-materials based photonic memories.We further optimize the positioning of dual microheaters validating performance tradeoffs.Experimentally we demonstrate a half-a-million cyclability test showcasing the robust approach of this material and device.Low-loss photonic retention-of-state adds a key feature for photonic functional and programmable circuits impacting many applications including neural networks,LiDAR,and sensors for example. | Jiawei Meng Yaliang Gui Behrouz Movahhed Nouri Xiaoxuan Ma Yifei Zhang Cosmin-Constantin Popescu Myungkoo Kang Mario Miscuglio Nicola Peserico Kathleen Richardson Juejun Hu Hamed Dalir Volker J.Sorger | 2023 | Light(Science & Applications)2023，12，11： | 0 |
| 18 | Detecting the single chiral molecule during the reaction显示文摘Detecting an individual molecule during the chemistry dynamics is essential for capturing accurate information about the chemical process in the time domain,which could be achieved by precisely forming single-molecule junctions between two electrodes and reading out the variation in electrical signals[1–3],but has yet to penetrate the stereochemistry study.There is a crucial pursuit of chirality chemistry to develop effective asymmetric synthesis methodologies and reveal the physicochemical mechanisms[4,5].And the key obstacle lies in achieving in situ detection of chiral intermediates in reactions[6].Chirality is a fundamental molecular property arising from the structure asymmetry,with two mirror-image forms known as enantiomers.Due to similar signals of enantiomeric isomers,it is a great challenge to distinguish chiral species and the process of their configurational transformation in single-molecule techniques.It then comes up with a question—how to detect chirality changes in stereochemistry. | Juejun Wang Zepeng Zhang Shurui Ji Yanxi Zhang Wenjing Hong | 2023 | Science China Materials2023，66，8： | 0 |
| 19 | Electric field-driven folding of single molecules显示文摘Folding of molecules is an essential process in nature,and various molecular machines achieve their chemical and mechanical function via controlled folding of molecular conformations.The electric field offers a unique strategy to drive the folding of molecular conformation and to control charge transport through single molecules but remains unexplored.The single-molecule break junction technique provides access to detect the conformational changes via the monitoring of single-molecule conductance,and the electric field between two metal electrodes with nanoscale spacing can provide an extremely strong to achieve in-situ control and detection of molecular folding at the single-molecule level.Here,we use the electric field to control the single-molecule folding using the scanning tunneling microscope break junction(STM-BJ)technique.The electric fields induced folding could lead to a∼1400%conductance change of the single-molecule junctions,and the folding/unfolding process can be in-situ switched at the scale of milliseconds.DFT calculations suggest the conformational control originates from the electric fieldinduced charge injection,and the formation of homoconjugated conformation with the overlapped orbitals.This work provides the first demonstration of electric field-driven molecular folding,which is essential for the understanding of molecular machines in nature and for the design of artificial molecular machines. | Saisai Yuan Yu Zhou Tengyang Gao Lichuan Chen Wei Xu Ping Duan Juejun Wang Zhichao Pan Chun Tang Yang Yang Ruiyun Huang Zongyuan Xiao Wenjing Hong | 2024 | Chinese Chemical Letters2024，35，1： | 0 |
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