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| 1 | Influence of urban morphological parameters on the distribution and diffusion of air pollutants: A case study in China显示文摘Air pollution has a serious fallout on human health,and the influences of the different urban morphological characteristics on air pollutants cannot be ignored.In this study,the relation-ship between urban morphology and air quality(wind speed,CO,and PM_(2.5))in residential neighborhoods at the meso-microscale was investigated.The changes in the microclimate and pollutant diffusion distribution in the neighborhood under diverse weather conditions were simulated by Computational Fluid Dynamics(CFD).This study identified five key urban morphological parameters(Building Density,Average Building Height,Standard Deviation of Building Height,Mean Building Volume,and Degree of Enclosure)which significantly im-pacted the diffusion and distribution of pollutants in the neighborhood.The findings of this study suggested that three specific strategies(e.g.volume of a single building should be re-duced,DE should be increased)and one comprehensive strategy(the width and height of the single building should be reduced while the number of single buildings should be in-creased)could be illustrated as an optimized approach of urban planning to relief the air pollution.The result of the combined effects could provide a reference for mitigating air pollution in sustainable urban environments. | Zhiwen Jiang Haomiao Cheng Peihao Zhang Tianfang Kang | 2021 | Journal of Environmental Sciences2021，33，7： | 3 |
| 2 | Catalytic oxidation of carbon monoxide, toluene, and ethyl acetate over the xPd/OMS-2 catalysts: Effect of Pd loading显示文摘在 cryptomelane 类型锰氧化物上支持的 Pd 催化剂八面的分子的筛(OMS-2 ) 被准备。在 xPd/OMS-2 上在碳一氧化物,甲苯,和乙醇醋酸盐的催化氧化上装载的 Pd 的效果被调查了。结果证明装载的 Pd 在与是的 0.5Pd/OMS-2 催化剂超过 Pd 免费的对应物的 xPd/OMS-2 催化剂的物理化学的性质上起一个重要作用最好。为 50% 变换的温度是 25, 240 和 160 迥龔鳥蚈? 蒚? ?? ? | Zhidan Fu Lisha Liu Yong Song Qing Ye Shuiyuan Cheng Tianfang Kang Hongxing Dai | 2017 | Frontiers of Chemical Science and Engineering2017，11，2： | 3 |
| 3 | Adsorption performance of CMK-3 and C-FDU-15 in NO removal at low temperature显示文摘CMK-3 and C-FDU-15 samples were synthesized using hard-templating and evaporationinduced self-assembly(EISA)methods,respectively.The pore structures of CMK-3 and CFDU-15 as well as commercial activated carbon were characterized by means of X-ray diffraction,field emission scanning electron microscopy,transmission electron microscopy,and N2 adsorption–desorption.Adsorption of NO was investigated by means of thermogravimetric analysis,temperature-programmed desorption of NO+O2,and in situ diffuse reflectance Fourier transform infrared spectroscopy.The results show that the CMK-3 and C-FDU-15 materials possessed ordered and uniform structures.The coadsorption capacity of NO and O2 decreased in the sequence CMK-3(88.6 mg/g)>C-FDU-15(71.7 mg/g)>AC(25.3 mg/g).There were two main adsorption species on CMK-3 and CFDU-15:nitrite and nitrate.Nitrite is converted to nitrate easily.However,the adsorption species were more complex on AC,with nitrite being the main species.Moreover,CMK-3 and C-FDU-15 exhibit excellent regeneration efficiency compared with AC.The excellent NO adsorption performance of CMK-3 and C-FDU-15 was associated with their ordered mesoporous structures and high surface areas.The research provides more options for NO adsorption in the future. | Runping Wu Qing Ye Kai Wu Shuiyuan Cheng Tianfang Kang Hongxing Dai | 2020 | Journal of Environmental Sciences2020，32，1： | 2 |
| 4 | Enhanced catalytic performance of Cu-and/or Mn-loaded Fe-Sep catalysts for the oxidation of CO and ethyl acetate显示文摘The Fe-modi fied sepiolite-supported Mn–Cu mixed oxide(Cux Mny/Fe-Sep) catalysts were prepared using the co-precipitation method.These materials were characterized by means of the XRD,N_2 adsorption–desorption,XPS,H_2-TPR,and O_2-TPD techniques,and their catalytic activities for CO and ethyl acetate oxidation were evaluated.The results show that catalytic activities of the Cux Mny/Fe-Sep samples were higher than those of the Cu1/Fe-Sep and Mn2/Fe-Sep samples,and the Mn/Cu molar ratio had a distinct in fluence on catalytic activity of the sample.Among the Cux Mny/Fe-Sep and Cu1Mn2/Sep samples,Cu1Mn2/Fe-Sep performed the best for CO and ethyl acetate oxidation,showing the highest reaction rate and the lowest T50 and T90 of 4.4×10^(-6) mmol·g-1·s-1,110,and 140 °C for CO oxidation,and 1.9×10^(-6) mmol·g-1·s-1,170,and210 °C for ethyl acetate oxidation,respectively.Moreover,the Cu1Mn2/Fe-Sep sample possessed the best lowtemperature reducibility and the lowest temperature of oxygen desorption as well as the highest surface Mn^(4+)/Mn^(3+) and Cu^(2+)/CuO atomic ratios.It is concluded that factors,such as the strong interaction between the Cu or Mn and the Fe-Sep support,good low-temperature reducibility,and good mobility of chemisorbed oxygen species,might account for the excellent catalytic activity of Cu1Mn2/Fe-Sep. | Lisha Liu Yong Song Zhidan Fu Qing Ye Shuiyuan Cheng Tianfang Kang Hongxing Dai | 2017 | Chinese Journal of Chemical Engineering2017，25，10： | 2 |
| 5 | Investigation of DNA damage treated with perfluorooctane sulfonate (PFOS) on ZrO 2/DDAB active nano-order film 显示文摘 | Lu Liping Xu Laihui Kang Tianfang | 2012 | Bio- sens Bioelectron2012，35，1： | 1 |
| 6 | Excellent performance of Cu-Mn/Ti-sepiolite catalysts for low-temperature CO oxidation显示文摘 | Yong Song Lisha Liu Zhidan Fu Qing Ye Shuiyuan Cheng Tianfang Kang Hongxing Dai | 2017 | Frontiers of Environmental Science & Engineering2017，11，2： | 1 |
| 7 | Immobilization of acetylcholinesterase via biocompatible interface of silk fibroin for detection of organophosphate and carbamate pesticides显示文摘 | XUE Rui KANG Tianfang LU Liping | 2012 | Applied Surface Science2012，258，16： | 1 |
| 8 | Electrochemical sensor for formaldehyde based on Pt - Pd nanoparticles and a Nafion modified glassy carbon electrode显示文摘 | ZHOU Zhongliang KANG Tianfang ZHANG Yan | 2009 | Microchim Acta2009，164，12： | 1 |
| 9 | Au-Fe(Ⅲ) nanoparticle modified glassy carbon electrode for electrochemical nitrite sensor显示文摘 | LIU Tongshen KANG Tianfang LU Liping | 2009 | J Electroanal Chem2009，632，12： | 1 |
| 10 | Electrochemical sensor based on the graphene-nafion matrix for sensitive de- termination of organophosphorus pesticides 显示文摘 | Xue Rui Kang Tianfang Lu Liping | 2012 | Analytical Letters2012，46，1： | 1 |
| 11 | Low-temperature CO oxidation over Au-doped 13X-type zeolite catalysts:preparation and catalytic activity显示文摘Au-supported 13X-type zeolite(Au/13X)was synthesized using a common deposition-precipitation(DP)method with a solution of sodium carbonate as a precipitate agent.Further testing was conducted to test for catalytic oxidation of CO.A study was conducted on the effects of different preparation conditions(i.e.,chloroauric acid concentration,solution temperature,pH of solution,and calcinations temperature)on Au/13X for CO oxidation.In respect to the catalytic activity,the relationship between different the preparation conditions and gold particles in 13X zeolite was analyzed using X-ray diffraction,TEM and XPS.The activity of Au/13X catalysts in CO oxidation was dependent on the chloroauric acid concentration.From XRD results,a higher chloroauric acid concentration induced larger gold nanoparticles,which resulted in lower catalytic activity.Results revealed that higher temperatures induced higher Au loading,homogeneous deposit,and smaller gold clusters on the support of 13X,resulting in higher CO activity.Furthermore,a pH of 5 or 6 generated greater amounts of Au loading and smaller Au particles on 13X than at a pH of 8 or 9.This may be a result of an effective exchange between Au(OH)_(2)Cl_(2)^(-)and Au(OH)_(3)Cl^(-)on specific surface sites of zeolite under the pH’s 5 and 6.The sample calcined at 300℃showed the highest activity,which may be due to the sample’s calcined at 200℃inability to decompose completely to metallic gold while the sample calcined at 400℃had larger particles of gold deposited on the support.It can be concluded from this study that Au/13X prepared from a gold solution with an initial chloroauric acid solution concentration of 1.5×10^(-3)mol·L^(-1)gold solution pH of 6,solution temperature of around 90℃,and a calcination temperature of 300℃provides optimum catalytic activity for CO oxidation. | Qing YE Donghui LI Jun ZHAO Jiansheng ZHAO Tianfang KANG Shuiyuan CHENG | 2011 | Frontiers of Environmental Science & Engineering2011，5，4： | 0 |
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