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4篇 您的检索式:作者名="Shaoying QI"
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1Elemental sulfur in northern South China Sea sediments and its significance显示文摘Elemental sulfur(ES) is one of the intermediates in the inorganic sulfur cycle and thus plays a key role in the fractionation of stable sulfur isotopes in different reservoirs and the marine environment. In this study, solid ES is discovered in sediments near the Jiulong Methane Reef in the northern South China Sea by scanning electron microscopy and Raman spectroscopy. Combining the morphology and distribution of ES, pyrite concentrations, and sulfur isotopes, we conclude that:(1) solid ES coexists with pyrite microcrystals and sulfide(oxyhydr)oxides as well as clay minerals, and they are mainly distributed on the surface of mineral aggregates;(2) ES mainly occurs within and near the sulfate-methane transition zone(SMTZ) despite little morphological diversity;(3) ES formation might be related to hydrogen sulfide oxidation and is therefore linked with fluctuations in the SMTZ. Within the SMTZ, hydrogen sulfide is produced and pyrite precipitates because of enhanced anaerobic oxidation of methane coupled with dissimilatory sulfate reduction. This enhances the efficiency of the inorganic sulfur cycle and provides favorable conditions for ES formation. The discovery of solid ES in sediments near the Jiulong Methane Reef suggests an important relationship with SMTZ fluctuations that could have implications for the evolution of methane hydrate in the South China Sea.LIN Qi WANG JiaSheng FU ShaoYing LU HongFeng BU QingTao LIN RongXiao SUN Fei 2015Science China Earth Sciences2015,58,12:6
2Modeling and verifying chlorine decay and chloroacetic acid formation in drinking water chlorination显示文摘This study presents a phenomenological model that can be used by the water professionals to quantify chlorine decay and disinfection byproduct(DBP)formation in water.The kinetic model was developed by introducing the concept of limiting chlorine demand and extending an established reactive species approach.The limiting chlorine demand,which quantifies chlorine reactive natural organic matter(NOM)on an equivalent basis,was mathematically defined by the relation between ultimate chlorine residue and initial chlorine dose.It was found experimentally that NOM in water has limiting chlorine demand that increases with chlorine dose once the ultimate residue is established.These results indicated that the complex NOM has a unique ability to adjust chemically to the change in redox condition caused by the free chlorine.It is attributed mainly to the redundant functional groups that persist in heterogeneous NOM molecules.The results also demonstrated that the effect of chlorine dose on the rate of chlorine decay can be quantitatively interpreted with the limiting chlorine demand.The kinetic model developed was validated for chlorine decay and chloroacetic acid formation in finished drinking water.Wenjun LIU Shaoying QI 2010Frontiers of Environmental Science & Engineering2010,4,1:3
3A venom protein of ectoparasitoid Pachycrepoideus vindemiae, PvG6PDH, contributes to parasitism by inhibiting host glucose-6-phosphate metabolism显示文摘To achieve successful development,female parasitoids,while laying eggs,introduce various virulence factors,mainly venoms,into host insects to manipulate their physiology.Although numerous studies have been conducted to characterize the components of venoms that regulate host immune responses,few systematic investigations have been conducted on the roles of venom proteins in host metabolic regulation.In this investigation,we characterized a novel venom protein in Pachycrepoideus vindemiae called glucose-6-phosphate dehydrogenase(PvG6PDH)and showed it has a vital role in regulating host carbohydrate metabolism.PvG6PDH encodes 510 amino acids and features a signal peptide and two conserved“G6PDH”domains.Multiple sequence alignment showed it has high amino acid identity with G6PDH from other pteromalids,and quantitative polymerase chain reaction analysis and immunofluorescent staining demonstrated a significantly higher expression of PvG6PDH in the venom apparatus compared with the carcass.We report that PvG6PDH contributes to parasitism by inhibiting the glucose-6-phosphate(G6P)metabolism of host Drosophila melanogaster,as demonstrated by PvG6PDH injection and RNA interference analysis.Further tests revealed that the accumulation of host G6P was caused by the transcriptional inhibition of G6P-metabolism-related genes.These findings greatly contribute to our understanding of venom-mediated host metabolic regulation,further laying the foundation for the development of venom proteins as biological agents for pest control.Lei Yang Liming Qiu Qi Fang Shaoying Wu Gongyin Ye 2022Insect Science2022,29,2:0
4Mathematical Advancement of General Chlorine Bulk Decay Model显示文摘An accurate chlorine bulk decay model is needed to ensure that potable water meets the microbial and the chemical safeties at the treatment plant and throughout the distribution. Among the mathematical models available,the general second-order chlorine bulk decay model( GBDM) is the most fundamentally sound.Application of the GBDM,however,has been hindered by its numerous fictive parameters and lack of an analytical solution. This theoretical work removes the two obstacles. The GBDM is solved through transformation and integration. The analytical solution provides deep insights into the GBDM and facilitates the parameterization and sensitivity analysis. The background natural organic matter( NOM) is characterized with the probabilistic distribution of functional groups. It reveals that the mean of the function group distribution is correlated with the initial chlorine decay rate coefficient( κ_0). A simple formula is developed to determine κ_0 directly from the initial chlorine decay. The theoretical treatment reduces the fictive parameters to a minimum. For the common lognormal distribution,the GBDM needs only three parameters,well defined as initial chlorine demand X_0,median rate coefficient km,and heterogeneity index σ. For more complicated scenarios,composite distributions are constructed through superposition of individual distributions. A highlighted example is to predict chlorine decay in blends of different waters. With the theoretical and mathematical advancement here,the GBDM can be applied effectively to any reactive background matter in any reaction systems.Shaoying Qi Jinfeng Lu 2017Journal of Harbin Institute of Technology(New Series)2017,24,4:0
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