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| 1 | Multifunctional flower-like core-shell Fe/Fe_(4)N@SiO_(2)composites for broadband and high-efficiency ultrathin electromagnetic wave absorber显示文摘The nano-iron nitride soft magnetic material has excellent magnetic properties and is expected to be a brilliant electromagnetic wave absorber.However,how to fully exploit its wave-absorbing potential re-mains a thought-provoking question.Here,we have synthesized Fe/Fe_(4)N@SiO_(2)nanomagnetic core-shell materials with different Fe/Fe_(4)N ratios by performing nitridation reactions at different temperatures.Then,the flower-like core-shell Fe/Fe_(4)N@SiO_(2)structure was obtained by the etching method.Finally,with the synergy of the excellent magnetic and dielectric losses,an outstanding absorption performance could be achieved with a minimum refection loss(RL min)of−71.31 dB at the matching thickness of 1.4 mm,and the widest effective absorption bandwidth(EAB max)of 6.1 GHz less than−10 dB was realized at 1.16 mm.Moreover,this material also shows a preeminent advance in corrosion resistance to adapt to harsh environments.Hence,this iron nitride flower-like core-shell structure exhibits great potential in microwave absorption in harsh conditions. | Wanjia Li Wangchang Li Yao Ying Jing Yu Jingwu Zheng Liang Qiao Juan Li Shenglei Che | 2023 | Journal of Materials Science & Technology2023，，1： | 2 |
| 2 | Corrosion mechanism of H_2O on Sm_2Fe_(17) and nitrogenation process of corroded Sm_2Fe_(17)显示文摘Sm_2 Fe_(17) prepared by reduction-diffusion method needs to be washed with water to remove calcium oxide. Electrochemical corrosion occurs when Sm_2 Fe_(17) powder is in contact with liquid water. Corrosion mechanism of H_2 O on Sm_2 Fe_(17) powder and nitrogenation process of corroded Sm_2 Fe_(17) were studied by analyzing the structure and morphology. It is indicated that the metallic hydroxide forms and deposits on the Sm_2 Fe_(17) powder surfaces during water corrosion. At the same time, oxygen and hydrogen enter the unit cell of Sm2 Fe_(17), causing a slight increase in Curie temperature. In the subsequent nitriding process,the hydroxide is dehydrated and hydrogen is desorbed. The resulting oxide reacts with Sm_2 Fe_(17)N_x to form a-Fe and Sm_2 O_3. Thermodynamic calculations using the HSC Chemistry 6.0 software indicate that the reaction can occur spontaneously. The effect of water corrosion on the magnetic properties of the nitride can be eliminated by hydrogen reduction prior to nitriding. | Jianwei Xu Jingwu Zheng Haibo Chen Liang Qiao Yao Ying Wei Cai Wangchang Li Jing Yu Min Lin Shenglei Che | 2019 | Journal of Rare Earths2019，37，6： | 1 |
| 3 | Enhanced maximum energy product of(SmY)FeN caused by abundant yttrium doping显示文摘Replacement of samarium(Sm) with abundant yttrium(Y) can help solve the potential shortage of Sm in the preparation of promising Sm2 Fe17 Nx magnets.In this article,phase composition,microstructure and magnetic properties of(Sm1-yYy)2 Fe17Nx(y=0,0.2,0.4,0.6,0.8,1.0) were investigated.Maximum energy product(BH)max is improved when less than 40 at% Y is doped in(Sm1-yYy)2 Fe17Nx powder.In particular,when 20 at% Y replaces Sm,(BH)max of(Sm1-yYy)2 Fe17Nx powder increases by 15.1% from 131.7 to151.6 kJ/m3.The effect of annealing temperature on the structural properties of high Y doping(Sm0.6Y0.4)2 Fe17 and the magnetic properties of the corresponding nitrides were subsequently investigated.In the RE2 Fe17 phase grain combination process,the interlaced structure of the rhombohedral Th2 Zn17-type structural phase and the hexagonal Th2 Ni17-type structural phase is formed.Due to shortrange exchange coupling,the nitride with the highest content of two interlaced RE2 Fe17 phases has the highest magnetic properties:Br=1.23 T,HcJ=443.9 kA/m and(BH)max=197.6 kJ/m3. | Jianwei Xu jingwu Zheng Haibo Chen Liang Qiao Yao Ying Wei Cai Wangchang Li Jjing Yu Min Lin Shenglei Che | 2020 | Journal of Rare Earths2020，38，10： | 1 |
| 4 | Enhancement mechanism of maximum energy product in hot-deformed Nd-Fe-B magnets by addition of ferromagnetic substances显示文摘It has been proved that the maximum magnetic energy product(BH)maxof hot-deformed Nd-Fe-B magnets can be effectively improved by adding substances with either high melting point or high saturation magnetization.In this work,we selected a ferromagnetic nano Fe_(55)Ni_(28)Co_(17) alloy powders with both high melting point and high saturation magnetization as the dopant to improve the(BH)max.By the addition of 1 wt% FeNiCo,the remanence increases by over 5%(from 1.36 to 1.44 T),resulting in a significant enhancement of(BH)maxfrom 355 to 396 kJ/m^(3)(from 44.6 to 49.7 MGOe).Microstructure observations reveal that the texture of grain alignment is improved,the concentrations of ferro magnetic elements(Fe,Ni,and Co) in the main phase and intergranular phase are increased so that the magnetization behavior of hot-deformed magnet changes(more easily shows reversible magnetization behaviors),which are the reasons why the high maximum energy product of hot-deformed magnet,is obtained. | Lian Wu Xianshuang Xia Wenzong Yin Xu Tang Jinyun Ju Yeyuan Du Renjie Chen Zhiyi Xu Shenglei Che Aru Yan | 2023 | Journal of Rare Earths2023，41，12： | 0 |
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