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1篇 您的检索式:作者名="TThu Ha Do"
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1Efficient up-conversion photoluminescence in all-inorganic lead halide perovskite nanocrystals显示文摘Up-conversion photoluminescence(UCPL)refers to the elementary process where low-energy photons are converted into high-energy ones via consecutive interactions inside a medium.When additional energy is provided by intermnal thermal energy in the form of lttice vibrations(phonons),the process is called phonon-assisted UCPL.Here,we report the exceptionally large phonon-assisted energy gain of up to^8kgT(kg is Boltzmann constant,T is temperature)on all-inorganic lead halide perovskite semiconductor colloidal nanocrystals that goes beyond the maximum capabilty of only harvesting optical phonon modes.By systematic optical study in combination with a statistical probability model,we explained the nontrivial phonon-assisted UCPL process in perovskites nanocrystals,where in addition to the strong electron-phonon(light-matter)coupling,other nonlinear processes such as phonon-phonon(matter-matter)interaction also effectively boost the up-conversion efficiency.Andres Granados del Aguila TThu Ha Do Jun Xing Wen Jie Jee Jacob B.Khurgin Qihua Xiong 2020Nano Research2020,13,7:5
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