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1篇 您的检索式:作者名="Tangyue Xue"
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1A shape memory scaffold for body temperature self-repairing wearable perovskite solar cells with efficiency exceeding 21%显示文摘Grain boundary cracks in flexible perovskite films can be repaired by filling with self-repairing polymers during the preparation and wearable operation.However,the self-repairing polymers are commonly active through external heating or humidification treatments,which cannot match with the human body's temperature tolerance of wearable devices.Herein,a body temperature-responsive shape memory polyurethane(SMPU)is demonstrated to achieve the real-time mechanical self-repairing of grain boundary cracks(~37°C).Furthermore,the strong intermolecular interaction between SMPU and the uncoordinated Pb2+and I−,can reduce the trap density in perovskite films.The blade-coated device achieves a power conversion efficiency(PCE)of 21.33%,which is among the best reported flexible perovskite solar cells(PSCs;0.10 cm2).Importantly,the device with SMPU can recover more than 80%of the PCE after 6000 cycles(bending radius:8 mm).Finally,the flexible PSCs are used for wearable solar power supply of a smartphone,which show great potential for self-repairing wearable electronics.Tangyue Xue Zengqi Huang Pei Zhang Meng Su Xiaotian Hu Tingqing Wu Baojin Fan Gangshu Chen Guanghui Yu Wentao Liu Xuying Liu Yiqiang Zhang Yanlin Song 2022InfoMat2022,4,12:1
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