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3篇 您的检索式:作者名="Weicun Jiang"
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1Graphitizing N-doped mesoporous carbon nanospheres via facile single atom iron growth for highly efficient oxygen reduction reaction显示文摘Single atom catalyst is of great importance for the oxygen reduction reaction(ORR).However,facile preparation of single atom catalyst without using well-designed precursors or labor-intensive acid leaching remains an urgent challenge.Herein,a simple pyrolysis of Fe3+-loaded mesoporous phenolic resin(mPF)-melamine precursor is used to prepare the single atom iron-anchored N-doped mesoporous graphitic carbon nanospheres(Fe/N-MGN).Investigation of the synthesis reveals the appropriate Fe-assisted catalysis effect and mPF template effect,which not only spurs the highly graphitic porous framework of Fe/N-MGN with plentiful pyridinic N/graphitic N,but also assures the dispersed single atom Fe anchoring without elaborated procedures.As a result,the as-synthesized Fe/N-MGN demonstrates high catalytic activity,good durability and excellent methanol tolerance for ORR.This work promises a facile method to regulate the graphitic carbon growth and single atom Fe loading for the highly efficient electrocatalysis.Yunshi Xu Liping Zhu Xuexue Cui Mingyu Zhao Yaling Li Leilei Chen Weicun Jiang Ting Jiang Shuguang Yang Yi Wang 2020Nano Research2020,13,3:5
2Integrating reduced graphene oxides and PPy nanoparticles for enhanced electricity from water evaporation显示文摘Developing high-performance nanostructured materials is key to deliver the potential of hydrovoltaic technology into practical applications.As single-component materials have approached its limit in generating hydrovoltaic electricity,the development of multi-component hydrovoltaic materials has been necessary in continuously boosting the electricity output.Here,we report a hydrovoltaic material by integrating reduced graphene oxides and polypyrrole nanoparticles(rGO/PPy),where the rGO contributes improved conductivity and large specific surface area while PPy nanoparticles enable enhanced interaction with water.The device fabricated with this material generates a short-circuit current of 6μA as well as a maximum power density of over 1μW/cm3 from natural evaporation of water.And the substantial ion-PPy interaction enables robust voltage generation from evaporation of various salt solutions.Moreover,an outstanding scaling ability is demonstrated by connecting 10 devices in series that generate a sustainable voltage of up to~2.5 V,sufficing to power many commercial devices,e.g.LED bulb and LCD screen.Bingkun Tian Xiaofeng Jiang Weicun Chu Chunxiao Zheng Wanlin Guo Zhuhua Zhang 2023International Journal of Smart and Nano Materials2023,14,2:1
3Role of electrodes in study of hydrovoltaic effects显示文摘The last decade has witnessed the emergence of hydrovoltaic technology,which can harvest electricity from different forms of water movement,such as raindrops,waves,flows,moisture,and natural evaporation.In particular,the evaporation-induced hydrovoltaic effect received great attention since its discovery in 2017 due to its negative heat emission property.Nevertheless,the influence of electrode reactions in evaporation-induced power generation is not negligible due to the chemical reaction between active metal electrodes and water,which leads to“exceptional”power generation.Herein,we designed a series of experiments based on air-laid paper devices with electrodes of different activities as the top and bottom electrodes.To verify the contribution of electrodes,we compared the output performance of different electrode combinations when the device was partially-wetted and fully-wetted.The device hydrophilicity,salt concentration,and acidity or basicity of solutions were also comprehensively investigated.It is demonstrated that the chemical reaction of active metals(Zn,Cu,Ag,etc.)with different aqueous solutions can generate considerable electrical energy and significantly distort the device performance,especially for Zn electrodes with an output voltage from~1.26 to~1.52 V and current from~1.24 to~75.69μA.To promote the long-term development of hydrovoltaic technology,we recommend use of inert electrodes in hydrovoltaic studies,such as Au and Pt,especially in water and moisture environment.Chunxiao Zheng Sunmiao Fang Weicun Chu Jin Tan Bingkun Tian Xiaofeng Jiang Wanlin Guo 2023Nano Research2023,16,8:0
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