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| 1 | Rational design of nitrogen doped hierarchical porous carbon for optimized zinc-ion hybrid supercapacitors显示文摘Aqueous rechargeable zinc-ion hybrid supercapacitors are considered to be a promising candidate for large-scale energy storage devices owing to their high safety,long life,and low price.In this paper,a nitrogen doped hierarchical porous carbon is evaluated as the cathode for aqueous rechargeable zinc-ion hybrid supercapacitors.Benefiting from the synergistic merits of excellent structural features of N-HPC and tiny zinc dendrite of Zn anode in ZnSO4 electrolyte,the zinc-ion hybrid supercapacitor exhibits excellent energy storage performance including high capacity of 136.8 mAh·g^−1 at 0.1·Ag^−1,high energy density of 191 Wh·kg^−1,large power density of 3,633.4 W·kg^−1,and satisfactory cycling stability of up to 5,000 cycles with a capacity retention of 90.9%.This work presents a new prospect of developing high-performance aqueous rechargeable zinc ion energy storage devices. | Penggao Liu Yang Gao Yangyang Tan Weifang Liu Yanping Huang Jun Yan Kaiyu Liu | 2019 | Nano Research2019,12,11: | 10 |
| 2 | Defects enriched hollow porous Co-N-doped carbons embedded with ultrafine CoFe/Co nanoparticles as bifunctional oxygen electrocatalyst for rechargeable flexible solid zinc-air batteries显示文摘The construction and design of highly efficient and inexpensive bifunctional oxygen electrocatalysts substitute for noble-metal-based catalysts is highly desirable for the development of rechargeable Zn-air battery(ZAB).In this work,a bifunctional oxygen electrocatalysts of based on ultrafine CoFe alloy(4-5 nm)dispersed in defects enriched hollow porous Co-N-doped carbons,made by annealing SiO2 coated zeolitic imidazolate framework-67(ZIF-67)encapsulated Fe ions.The hollow porous structure not only exposed the active sites inside ZIF-67,but also provided efficient charge and mass transfer.The strong synergetic coupling among high-density CoFe alloys and Co-N_(x) sites in Co,N-doped carbon species ensures high oxygen reduction reaction(ORR)and oxygen evolution reaction(OER)activity.First-principles simulations reveal that the synergistic promotion effect between CoFe alloy and Co-N site effectively reduced the formation energy of from O^(*)to OH^(*).The optimized CoFe-Co@PNC exhibits outstanding electrocatalytic stability and activity with the overpotential of only 320 mV for OER at 10 mA·cm^(−2) and the half-wave potential of 0.887 V for ORR,outperforming that of most recent reported bifunctional electrocatalysts.A rechargeable ZAB constructed with CoFe-Co@PNC as the air cathode displays long-term cyclability for over 200 h and high power density(152.8 mW·cm^(−2)).Flexible solid-state ZAB with our CoFe-Co@PNC as the air cathode possesses a high open circuit potential(OCP)up to 1.46 V as well as good bending flexibility.This universal structure design provides an attractive and instructive model for the application of nanomaterials derived from MOF in the field of sustainable flexible energy applications device. | Zhao Lei Yangyang Tan Zeyi Zhang Wei Wu Niancai Cheng Runzhe Chen Shichun Mu Xueliang Sun | 2021 | Nano Research2021,14,3: | 9 |
| 3 | Synthesis and Characterization of Condensed Polynuclear Aromatic Resin Derived from Ethylene Tar显示文摘As a kind of low-cost and readily available industrial byproduct, ethylene tar (ET) was for the first time utilized for the preparation of heat-resistant condensed polynuclear aromatic resin (COPNAR). The basic properties of ET and the resulted COPNAR were characterized by FT-IR, 1H-NMR, TGA and elemental analysis. The test results showed that ET with high aromatic content (>50%) was suitable for the synthesis of COPNAR with superior heat resistance. The average molecular structure of ET was obtained by means of the improved Brown-Ladner method, and the reaction mechanism was considered as an acid-catalyzed positive ion-typed polymerization. Our findings have provided a new route to develop ET into technology-added heat-resistant resins. | Wu Mingbo Shi Yangyang Li Shibin Wang Yuwei Tan Minghui Wang Ding Zheng Jingtang Tsubaki Noritatsu | 2012 | China Petroleum Processing & Petrochemical Technology2012,14,4: | 7 |
| 4 | Experimental Study on the Flow Around Two Tandem Cylinders with Unequal Diameters显示文摘In this paper, flow around two circular cylinders in tandem arrangement with unequal diameters has been investigated using the particle image velocimetry technique(PIV) in a water channel. The upstream to downstream diameter ratio was kept constant at d/D = 2/3, the centre-to-centre distance was varied from 1.2D to 5D and the Reynolds number was varied from 1200 to 4800. The flow characteristics were analyzed through ensemble-averaged patterns of velocity, vorticity, normalized Reynolds stress contours and streamlines. Based on ensemble-averaged and instantaneous flow fields, different flow patterns, including single-wakeshedding at small spacing ratio, bi-stable flow behavior(alternating behavior of reattachment and vortex shedding) at intermediate spacing ratio and co-shedding pattern at large spacing ratio were observed. The effects of Reynolds number and the centre-to-centre spacing ratio on flow patterns and turbulent characteristics were also investigated. It was found that the diameter ratio appears to have a certain effect on the flow patterns at intermediate spacing ratios, where the reattachment of shear layer depends on the lateral width of the wake flow in the lee of the upstream cylinder. Extensive discussion on the distributions of Reynolds stress and turbulent kinetic energy was presented. | GAO Yangyang ETIENNE Stephane WANG Xikun TAN Soon Keat | 2014 | Journal of Ocean University of China2014,13,5: | 3 |
| 5 | Tuning the dual-active sites of ZIF-67 derived porous nanomaterials for boosting oxygen catalysis and rechargeable Zn-air batteries显示文摘The rational control of the active site of metal-organic frameworks(MOFs)derived nanomaterials is essential to build efficient bifunctional oxygen reduction/evolution reaction(ORR/OER)catalysts.Accordingly,through designing and constructing a Co_(3)O_(4)-Co heterostructure embedded in Co,N co-doped carbon polyhedra derived(Co_(3)O_(4)-Co@NC)from the in-situ compositions of ZIF-67 and cobalt nanocrystals synthesized by the strategy of in-situ NaBH4 reduction,the dual-active site(Co_(3)O_(4)-Co and Co-N_(x))is synchronously realized in a MOFs derived nanomaterials.The formed Co_(3)O_(4)-Co@NC shows excellent bifunctional electrocatalytic activity with ultra-small potential gap(ΔE=E_(j=10)(OER)–E_(1/2)(ORR))of 0.72 V,which surpasses the commercial Pt/C and RuO_(2) catalysts.The theory calculation results reveal that the excellent bifunctional electrocatalytic activity can be attributed to the charge redistribution of Co of Co-N_(x) induced by the synergistic effects of well-tuned active sites of Co_(3)O_(4)-Co nanoparticle and Co-N_(x),thus optimizing the rate-determining step of the desorption of O_(2)^(*)intermediate in ORR and OH^(*)intermediate in OER.The rechargeable Zn-air batteries with our bifunctional catalysts exhibit superior performance as well as high cycling stability.This simple-effective optimization strategy offers prospects for tuning the active site of MOF derived bifunctional catalyst in electrochemical energy devices. | Zeyi Zhang Yangyang Tan Tang Zeng Liyue Yu Runzhe Chen Niancai Cheng Shichun Mu Xueliang Sun | 2021 | Nano Research2021,14,7: | 3 |
| 6 | On the robustness of EEG tensor completion methods显示文摘During the acquisition of electroencephalographic(EEG) signals, data may be missing or corrupted by noise and artifacts. To reconstruct the incomplete data, EEG signals are firstly converted into a three-order tensor(multi-dimensional data) of shape time × channel × trial. Then, the missing data can be efficiently recovered by applying a tensor completion method(TCM).However, there is not a unique way to organize channels and trials in a tensor, and different numbers of channels are available depending on the EEG setting used, which may affect the quality of the tensor completion results. The main goal of this paper is to evaluate the robustness of EEG completion methods with several designed parameters such as the ordering of channels and trials, the number of channels, and the amount of missing data. In this work, the results of completing missing data by several TCMs were compared. To emulate different scenarios of missing data, three different patterns of missing data were designed.Firstly, the amount of missing data on completion effects was analyzed, including the time lengths of missing data and the number of channels or trials affected by missing data. Secondly, the numerical stability of the completion methods was analyzed by shuffling the indices along channels or trials in the EEG data tensor. Finally, the way that the number of electrodes of EEG tensors influences completion effects was assessed by changing the number of channels. Among all the applied TCMs, the simultaneous tensor decomposition and completion(STDC) method achieves the best performance in providing stable results when the amount of missing data or the electrode number of EEG tensors is changed. In other words, STDC proves to be an excellent choice of TCM, since permutations of trials or channels have almost no influence on the complete results. The STDC method can efficiently complete the missing EEG signals. The designed simulations can be regarded as a procedure to validate whether or not a completion method is useful enough to complete EEG signals. | DUAN Feng JIA Hao ZHANG ZhiWen FENG Fan TAN Ying DAI YangYang CICHOCKI Andrzej YANG ZhengLu CAIAFA Cesar F. SUN Zhe SOLE-CASALS Jordi | 2021 | Science China(Technological Sciences)2021,64,9: | 2 |
| 7 | A comparativeinvestigationon structure and multiferroic properties of bismuth ferrite thin films by multielement co-doping 显示文摘 | Dong Guohua Tan Guoqiang Luo Yangyang | 2014 | Materials Research Bulletin2014,60,: | 1 |
| 8 | Do corticosteroids have a role in treating Ebola virus disease?显示文摘Dear Editor,Humans have been fighting Ebola virus disease(EVD)since its first outbreak in 1976 in Yambuku village in the Democratic Republic of the Congo(previously Zaire).EVD is part of the Filoviridae family of viruses that includes Ebola and Marburg viruses.To date,EVD,one of the most deadly communicable diseases known to humans,has had15 outbreaks in Africa.In 2014,the most severe and complicated outbreak yet swept through the West African countries of Guinea,Liberia,Nigeria,Senegal and Sierra Leone, | XU Jun TAN DingYu FU YangYang WALLINE Joseph YU XueZhong | 2015 | Science China(Life Sciences)2015,58,1: | 1 |
| 9 | Numerical Study of an Oscillating Smaller Cylinder in the Wake of an Upstream Larger Cylinder显示文摘A numerical study of flow around two tandem cylinders with unequal diameters was carried out. The upstream larger cylinder was fixed and the downstream smaller cylinder was allowed to oscillate in the transverse direction only. Comparisons of the experimental and numerical results were made to investigate the effects of the gap ratio on the maximum vibration amplitude and vortex shedding frequency. The results showed that the vibration response of the smaller cylinder was significantly affected by the presence of the upstream larger cylinder, and resulted in greatly reduced vibration amplitudes. With an increasing gap ratio, the vibration amplitude increased. However, the magnitude was lower than that corresponding to a single cylinder (with the same diameter as that of the downstream smaller cylinder) under the same flow conditions. | GAO Yangyang YU Dingyong WANG Xikun TAN Soon Keat | 2012 | Journal of Ocean University of China2012,11,2: | 0 |