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| 1 | Coking wastewater treatment for industrial reuse purpose: Combining biological processes with ultrafiltration, nanofiltration and reverse osmosis显示文摘A full-scale plant using anaerobic, anoxic and oxic processes (A1/A2/O), along with a pilot-scale membrane bioreactor (MBR), nanofiltration (NF) and reverse osmosis (RO) integrated system developed by Shanghai Baosteel Chemical Co. Ltd., was investigated to treat coking wastewater for industrial reuse over a period of one year. The removals reached 82.5% (COD), 89.6% (BOD), 99.8% (ammonium nitrogen), 99.9% (phenol), 44.6% (total cyanide (T-CN)), 99.7% (thiocyanide (SCN-)) and 8.9% (fluoride), during the A1/A2/O biological treatment stage, and all parameters were further reduced by over 96.0%, except for fluoride (86.4%), in the final discharge effluent from the currently operating plant. The pilot-scale MBR process reduced the turbidity to less than 0.65 NTU, and most of the toxic organic compounds were degraded or intercepted by the A1/A2/O followed MBR processes. In addition, parameters including COD, T-CN, total nitrogen, fluoride, chloride ion, hardness and conductivity were significantly reduced by the NF-RO system to a level suitable for industrial reuse, with a total water production ratio of 70.7%. However, the concentrates from the NF and RO units were highly polluted and should be disposed of properly or further treated before being discharged. | Xuewen Jin Enchao Li Shuguang Lu Zhaofu Qiu Qian Sui | 2013 | Journal of Environmental Sciences2013，25，8： | 38 |
| 2 | Occurrence, sources and fate of pharmaceuticals and personal care products in the groundwater: A review显示文摘The presence of pharmaceuticals and personal care products(PPCPs)in the aquatic environment may pose potential threat to the ecosystem and human health,hence PPCPs have aroused much concern over the world.The contamination of PPCPs in the groundwater,the main source of drinking water supply in many countries and regions,has been extensively studied in the last decade.This paper reviews the occurrence of frequently detected PPCPs,including antibiotics,anti-inflammatories,lipid-regulators,carbamazepine,caffeine,and N,N-diethyl-m-toluamide in groundwater,with special concern to the progress made over the past three years.Possible emission sources for PPCPs in groundwater,such as wastewater and contaminated surface water,landfills,septic systems,livestock breeding and sewer leakage,are summarized.Besides,adsorption,migration and degradation,the dominant mechanisms in the subsurface transport and fate of PPCPs,are discussed,and the insights into the future study of PPCPs in the groundwater are provided. | Qian Sui Xuqi Cao Shuguang Lu Wentao Zhao Zhaofu Qiu Gang Yu | 2015 | Emerging Contaminants2015，1，1： | 20 |
| 3 | Degradation of carbon tetrachloride in thermally activated persulfate system in the presence of formic acid显示文摘碳四氯化物(CT ) 的热地激活的 persulfate (PS ) 降级面对蚁的酸(FA ) 被调查。结果显示那 CT 降级跟随了零份订单运动模型,和公司 2- | Minhui XU Xiaogang GU Shuguang LU Zhouwei MIAO Xueke ZANG Xiaoliang WU Zhaofu QIU Qian SUI | 2016 | Frontiers of Environmental Science & Engineering2016，10，3： | 6 |
| 4 | Removal of pharmaceutical and personal care products by sequential ultraviolet and ozonation process in a full-scale wastewater treatment plant显示文摘在市政的废水处理植物(WWTP ) 的适当先进处理过程的应用程序就新兴的沾染物的消除而言成为了一个重要问题,例如药品、个人的照顾产品(PPCP ) 。在现在的学习,属于不同的治疗学的班由的 13 PPCP 的移动顺序紫外(紫外) 并且在在北京的照原尺寸的 WWTP 的 ozonation 过程在十个月的功课上被调查。大多数目标 PPCP 有效地被移开,并且单个 PPCP 的中部的移动效率,从 13% ~ 89%,依赖于他们有分子的臭氧的反应率常数。在一样的 PPCP 的移动效率的显著变化在不同采样运动被观察。不过,顺序紫外并且仍然在照原尺寸的 WWTP 成为重要贡献到大多数 PPCP 的全部的消除的 ozonation 过程,由由生物学的处理补偿 PPCP 的差或变动的移动性能处理。 | Qian SU Jun HUANG Shuguang LU Shubo DENG Bin WANG Wentao ZHAO Zhaofu QIU Gang YU | 2014 | Frontiers of Environmental Science & Engineering2014，8，1： | 6 |
| 5 | Enhanced degradation of trichloroethene by calcium peroxide activated with Fe(III) in the presence of citric acid显示文摘由 Fe (III ) 的 Trichloroethene (TCE ) 降级 - 激活的钙过氧化物(CP ) 面对在水的答案的柠檬性的酸(CA ) 被调查。结果证明 CA 的存在由增加可溶的 Fe (III ) 的集中并且支持 H 2 O 2 产生。产生惊讶并且在 CP/Fe (III ) 和 CP/Fe (III ) 的 O 2-/CA 系统与化学探针被证实。激进的清除测试的结果证明那 TCE 降级主要是到期的指导氧化由惊讶,当 O 2- 加强了产生时惊讶由支持 Fe (III ) 在 CP/Fe (III )/CA 系统的转变。酸的 pH 条件为 TCE 降级是有利的,并且 TCE 降级率与增加 pH 减少了。Cl -, HCO 3-, 和腐殖的酸的存在(哈) 禁止的 TCE 降级到为 CP/Fe (III )/CA 系统的不同程度。Cl 生产的分析建议在 CP/Fe (III )/CA 系统的那 TCE 降级通过一个 dechlorination 过程发生了。在摘要,这研究提供了详细信息因为提高 CA 的 Fe (III ) 的申请激活钙过氧化物因为对待 TCE 污染了地下水。 | Xiang ZHANG Xiaogang GU Shuguang LU Zhouwei MIAO Minhui XU Xiaori FU Muhammad DANISH Mark L. BRUSSEAU Zhaofu QIU Qian SUI | 2016 | Frontiers of Environmental Science & Engineering2016，10，3： | 5 |
| 6 | Effects of substrate temperature and annealing treatment on the microstructure and magnetic characteristics of TbDyFe films显示文摘A series of TbDyFe films were prepared by DC magnetron sputtering. The effects of substrate temperature and annealing temperature on the phase structure and the magnetic properties of the sample films were investigated. The an-nealing treatment has a significant influence on the microstructure and the magnetic properties of the sample. The results obtained by XRD indicate that the films deposited at a temperature lower than 525°C are amorphous and have an easy magnetization direction perpendicular to the film plane. An RFe2 phase is formed in the sample annealed at 550°C and the residual phases observed are Fe and rare earth oxide. The magnetic properties Hc and Mr/Ms of the film annealed at 550°C obtain the maximum values,for which the formation of the RFe2 phase is mainly responsible. An annealing treatment leads to a rotation of the sample’s easy axis from being parallel to the film surface to becoming vertical. | DU Zhaofu WANG Lei ZHAO Dongliang | 2007 | Rare Metals2007，26，5： | 4 |
| 7 | Nucleate Pool Boiling Heat Transfer of Pure Refrigerants and Binary Mixtures显示文摘Heat transfer coefficients in nucleate boiling on a smooth flat surface were measured for pure fluids of R-134a, propane, isobutane and their binary mixtures at different pressure from 0.1 to 0.6 MPa. Series of experiments with different heat flux and mixture concentrations were carried out. The influences of pressure and heat flux on the heat transfer coefficient for different pure fluids were studied. Isobutane and propane were used to make up binary mixtures. Compared to the pure components, binary mixtures show lower heat transfer coefficients. This reduction was more pronounced as the heat flux increasing. Several heat transfer correlations are obtained for different pure refrigerants and their binary mixtures. | Zhaofu SUN Maoqiong GONG Yanfeng QI Zhijian LI Jianfeng WU | 2004 | Journal of Thermal Science2004，13，3： | 3 |
| 8 | Carbonaceous matter in glacier at the headwaters of the Yangtze River:Concentration,sources and fractionation during the melting process显示文摘Carbonaceous matter has an important impact on glacial retreat in the Tibetan Plateau,further affecting the water resource supply.However,the related studies on carbonaceous matter are still scarce in Geladaindong(GLDD)region,the source of the Yangtze River.Therefore,the concentration,source and variations of carbonaceous matter at Ganglongjiama(GLJM)glacier in GLDD region were investigated during the melting period in 2017,which could deepen our understanding on carbonaceous matter contribution to glacier melting.The results showed that dissolved organic carbon(DOC)concentration of snowpit samples(283±200μg/L)was much lower than that of precipitation samples(624±361μg/L),indicating that large parts of DOC could be rapidly leached from the snowpit during the melting process.In contrast,refractory black carbon(rBC)concentration measured by Single Particle Soot Photometer of snowpit samples(4.27±3.15μg/L)was much higher than that of precipitation samples(0.97±0.49μg/L).Similarly,DOC with high mass absorption cross-section measured at 365 nm value was also likely to enrich in snowpit during the melting process.In addition,it was found that both r BC and DOC with high light-absorbing ability began to leach from the snowpit when melting process became stronger.Therefore,rBC and DOC with high light-absorbing ability exhibited similar behavior during the melting process.Based on relationship among DOC,rBC and K^+ in precipitation,the main source of carbonaceous matter in GLJM glacier was biomass burning during the study period. | Zhaofu Hu Shichang Kang Xiaobo He Fangping Yan Yulan Zhang Pengfei Chen Xiaofei Li Shaopeng Gao Chaoliu Li | 2020 | Journal of Environmental Sciences2020，32，1： | 3 |
| 9 | Enhanced reductive degradation of carbon tetrachloride by carbon dioxide radical anion-based sodium percarbonate/ Fe(ll)/formic acid system in aqueous solution显示文摘 | Wenchao Jiang Ping Tang Shuguang Lu Xiang Zhang Zhaofu Qiu Qian Sui | 2018 | Frontiers of Environmental Science & Engineering2018，12，2： | 3 |
| 10 | Seasonality of carbonaceous aerosol composition and light absorption properties in Karachi,Pakistan显示文摘Characteristics of carbonaceous aerosol(CA)and its light absorption properties are limited in Karachi,which is one of the most polluted metropolitan cities in South Asia.This study presents a comprehensive measurement of seasonality of CA compositions and mass absorption cross-section(MAC)of elemental carbon(EC)and water-soluble organic carbon(WSOC)in total suspended particles(TSP)collected from February 2015 to March 2017 in the southwest part of Karachi.The average TSP,organic carbon(OC),and EC concentrations were extremely high with values as 391.0±217.0,37.2±28.0,and 8.53±6.97μg/m3,respectively.These components showed clear seasonal variations with high concentrations occurring during fall and winter followed by spring and summer.SO42-,NO3-,K+,and NH4+showed similar variations with CA,implying the significant influence on atmospheric pollutants from anthropogenic activities.Relatively lower OC/EG ratio(4.20±2.50)compared with remote regions further indicates fossil fuel combustion as a primary source of CA.Meanwhile,sea salt and soil dust are important contribution sources for TSP.The average MAC of EC(632 nm)and WSOC(365 nm)were 6.56±2.70 and 0.97±0.37 m2/g,respectively.MACEC is comparable to that in urban areas but lower than that in remote regions,indicating the significant influence of local emissions.MACwsoc showed opposite distribution with EC,further suggesting that OC was significantly affected by local fossil fuel combustion.In addition,dust might be an important factor increasing MACwsoc particularly during spring and summer. | Pengfei Chen Shichang Kang Chaman Gul Lekhendra Tripathee Xiaoxiang Wang Zhaofu Hu Chaoliu Li Tao Pu | 2020 | Journal of Environmental Sciences2020，32，4： | 3 |
| 11 | Effect of pulsatile perfusion during cardiopulmonary bypass in terms of radial artery sphygmogram显示文摘OBJECTIVE: To investigate a quantitative method for using radial artery pulse waveforms to assess the effect of pulsatile flow during cardiopulmonary bypass(CPB).METHODS: A total of 34 adults with heart disease who underwent open-heart surgery between April2010 and January 2011 were randomized into a pulsatile perfusion group(n=17) and a non-pulsatile perfusion group(n=17). Radial arterial pulse waveforms of pulsatile and non-pulsatile perfusion patients were observed and compared before and during CPB.RESULTS: No pulse waveform could be detected at patients' radial artery in both groups when the aorta was cross-clamped. Pulse waveforms could be detected at pulsatile perfusion patients' radial artery, but could not be detected at non-pulsatile perfusion patients' radial artery during CPB. Additionally, patients' pulse waveforms during pulsatile perfusion were lower than those before the operation.CONCLUSION: Our findings indicate that radial artery sphygmogram can be used as a valid indicator to evaluate the effectiveness of pulsatile perfusion during CPB. | Zhifeng Zhang Jiatuo Xu Enyuan Zhu Qi Zhang Lu Yu Yongbing Qiu Jianguo Tang Zhaofu Fei Xin Li Liping Tu Chouping Han Ying Liu Zhen Guo Changle Zhou Meiyu Shi Yingxin Qian Yimin Bao Xinming Ji | 2014 | Journal of Traditional Chinese Medicine2014，34，6： | 2 |
| 12 | Investigation of phosphate adsorption from an aqueous solution using spent fluid catalytic cracking catalyst containing lanthanum显示文摘A spent fluid catalytic cracking (FCC)catalyst containing lanthanum (La)was used as a novel adsorbent for phosphorus (P)in simulated wastewater.The experiments were conducted in a batch system to optimize the operation variables,including pH,calcination temperature,shaking time,solidliquid ratio,and reaction temperature under three initial P-concentrations (C0=0.5,1.0,and 5.0mg/L). Orthogonal analysis was used to determine that the initial P-concentration was the most important parameter for P removal.The P-removal rate exceeded 99% and the spent FCC catalyst was more suitable for use in low P-concentration wastewater (C0<5.0mg/L).Isotherms,thermodynamics and dynamics of adsorption are used to analyze the mechanism of phosphorus removal.The results show that the adsorption is an endothennic reaction with high affinity and poor reversibility,which indicates a low risk of second releasing of phosphate.Moreover,chemical and physical adsorption coexist in this adsorption process with LAPO4 and KH2PO4formed on the spent FCC catalyst as the adsorption product.These results demonstrate that the spent FCC catalyst containing La is a potential adsorbent for P-removal from wastewater,which allows recycling of the spent FCC catalyst to improve the quality of water body. | Zhen Li Zhaofu Qiu Ji Yang Benteng Ma Shuguang Lu Chuanhui Qin | 2018 | Frontiers of Environmental Science & Engineering2018，12，6： | 2 |
| 13 | Relationship between glutathione and malonaldehyde levels in erythrocytes and the deformation index of erythrocyte in patients at various periods following acute cerebral infarction显示文摘BACKGROUND: Glutathione, as an in vivo free radical scavenger, plays an important role in the anti-oxidation defense mechanism in patients with acute cerebral infarction. OBJECTIVE: To observe the relationship between the levels of glutathione (GSH) and malonaldehyde (MDA), the metabolite of lipid peroxidation, in erythrocyte and deformation index of erythrocyte in patients at various periods following acute cerebral infarction. DESIGN: Controlled observation. SETTING: Qilu Hospital of Shandong University and Institute of Cerebrovascular Disease of Qingdao Medical College. PARTICIPANTS: We chose 98 inpatients with acute cerebral infarction from Department of Neurology, Qilu Hospital of Shandong University from January to December 2000 , serving as cerebral infarction group, including 50 male and 48 female , with mean age of (62±7)years. There were 23 cases found on the 1st day after onset; 25 cases on the 3rd day after onset; 25 cases on the 7th day after onset; 25 cases on the 14th days after onset, and they were all confirmed by craniocerebral CT or MRI. Another 30 homeochronous inpatients with neurosis, cervical syndrome, lumbar intervertebral disc herniation and motor neuron disease were chosen as control group, including 20 male and 10 female, with mean age of (52±8)years . There was no significant difference in age and gender distribution between two groups (P > 0.05). Patients in the two groups were informed of detected index. METHODS: ①Ulnar venous blood was chosen from the patients who were fasted on the 1st, 3rd, 7th and 14th days after onset. Deformation index of erythrocyte was measured with BL88-CKX laser diffraction erythrocyte deformeter and photographing was performed. GSH level in erythrocyte was measured with DTNB assay introduced by Beu-tler. MDA level in erythrocyte was measured with modified thiobarbituric acid colorimetric method. ②At each sample collecting , according to the criteria accepted by the Fourth National Conference of Cerebrovascular Disease, intergrant of neurologic impairment < 15 points was regarded as mild (n=46),15 to 30 points as moderate (n=40)and, > 30 points as severe (n=12). ③ t test was used to compare data between two groups , and linear correlation analysis was used in relationship analysis among indexes. MAIN OUTCOME MEASURES: ① Comparison of erythrocyte GSH and MDA levels and deformation index of erythrocyte at various periods between patients with acute cerebral infarction and controls. ②Correlation of erythrocyte GSH level with erythrocyte MDA level and with deformation index of erythrocyte in patients with cerebral infarction. ③ Relationship between erythrocyte GSH level and severity of disease in patients with acute cerebral infarction. RESULTS: Totally 98 patients with acute cerebral infarction and 30 controls all entered the stage of result analysis. ① Erythrocyte GSH level and deformation index of erythrocyte were lower on the 1st, 3rd, 7th and 14th days after onset in cerebral infarction group than in control group (P < 0.05-0.01), and erythrocyte MDA level was significantly higher in cerebral infarction group than in control group (P < 0.05-0.01). The three indexes changed most significantly on day 3 after onset in patients, and began to recover or decrease on day 7 after onset and inclined to be normal on day 14 after onset. ② Erythrocyte GSH level was significantly negatively correlated with erythrocyte MDA level in patients with acute cerebral infarction on the 1st, 3rd, 7th and 14th days after onset (r=-0.534, -0.713, -0.645, -0.656, respectively, P < 0.05-0.01),and significantly positively correlated with erythrocyte deformation index (r=0.502, 0.560, 0.455, 0.504, respectively, P < 0.05). ③Erythrocyte GSH level was significantly lower in moderate or severe patients with acute cerebral infarction than in mild patients[(0.215±0.088),(0.192±0.102),(0.281±0.090) g/L, P < 0.05]. CONCLUSION: ①Erythrocyte GSH and MDA levels and deformation index of erythrocyte change significantly on the 3rd day following acute cerebral infarction. Index detection results gradually tended to be normal on from the 7th day to 14th days day after onset. ② Change of erythrocyte GSH level can reflect the severity of disease of patients with acute cerebral infarction. ③Decrease of erythrocyte GSH level in patients with acute cerebral infarction is one of reasons that result in the decrease of deformation ability of erythrocyte. | Dongjun Zhang Guangrun Xu Zhaofu Chi Bingxia Shi | 2006 | Neural Regeneration Research2006，1，1： | 2 |
| 14 | Intracerebral haemorrhage: from clinical settings to animal models显示文摘Spontaneous intracerebral haemorrhage(ICH)is a devastating type of stroke with high mortality and morbidity and for which no effective treatments are available to date.Much experimental and clinical research have been performed to explore its mechanisms regard the subsequent inflammatory cascade and to seek the potential therapeutic strategies.The aim of this review is to discuss insights from clinical settings that have led to the development of numerous animal models of ICH.Some of the current and future challenges for clinicians to understand ICH are also surveyed. | Qian Bai Zhaofu Sheng Yang Liu Ruiyi Zhang Voon Wee Yong Mengzhou Xue | 2020 | Stroke & Vascular Neurology2020，5，4： | 2 |
| 15 | A density-functional-theory-based and machine-learning-accelerated hybrid method for intricate system catalysis显示文摘Being progressively applied in the design of highly active catalysts for energy devices,machine learning(ML)technology has shown attractive ability of dramatically reducing the computational cost of the traditional density functional theory(DFT)method,showing a particular advantage for the simulation of intricate system catalysis.Starting with a basic description of the whole workflow of the novel DFT-based and ML-accelerated(DFT-ML)scheme,and the common algorithms useable for machine learning,we presented in this paper our work on the development and performance test of a DFT-based ML method for catalysis program(DMCP)to implement the DFT-ML scheme.DMCP is an efficient and user-friendly program with the flexibility to accommodate the needs of performing ML calculations based on the data generated by DFT calculations or from materials database.We also employed an example of transition metal phthalocyanine double-atom catalysts as electrocatalysts for carbon reduction reaction to exhibit the general workflow of the DFT-ML hybrid scheme and our DMCP program. | Xuhao Wan Zhaofu Zhang Wei Yu Yuzheng Guo | 2021 | Materials Reports(Energy)2021，1，3： | 2 |
| 16 | Metal-organic frameworks derived from imidazolium dicarboxylates and group Ⅰ and Ⅱ salts显示文摘 | Zhaofu Fei Tilmann J Paul J | 2006 | Inorg Chem2006，45，： | 1 |
| 17 | A nearly planar water sheet sandwiched between strontium-imidazolium carboxylate coordination polymers显示文摘 | Zhaofu Fei Tilmann J Paul J Dyson | 2005 | Inorg Chem2005，44，： | 1 |
| 18 | A synthetic zwitterionic water channel:Characterization in the solid state by X-ray crystall-ography and NMR spectroscopy显示文摘 | Zhaofu Fei Paul J Dyson Sasa Antonijevic | 2005 | Angew Chem Int Ed2005，44，： | 1 |
| 19 | Evaluation of ionic liquid soluble imidazolium tetrachloropalladate pre-catalysts in Suzuki coupling reactions显示文摘 | SONG HONGBING NING YANA FEI ZHAOFU | 2012 | Catalysis Today2012，183，： | 1 |
| 20 | Clofibric acid degradation in UV254/H2 O2 process:Effect of temperature显示文摘 | Li Wenzhen Lu Shuguang Qiu Zhaofu | | 0，，1： | 1 |
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