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| 1 | Mercury Emission From Coal-fired Power Plants in China显示文摘燃煤是最大的人为汞排放源之一,燃煤电厂的汞排放控制问题也越来越为人们所关注。该文将目前公布的中国电厂的汞排放数据进行筛选汇总,得到18个电厂的汞排放数据,通过对比和分析,总结出了符合我国燃煤电厂特点的一般性汞排放规律。结果表明:与美国煤种相比,我国的燃煤具有低氯、高灰的特性,这不利于汞的排放控制;循环流化床燃烧可能会因燃尽率的不同而较煤粉炉燃烧易获得较高的Hgp;空气污染控制设备的使用能够有效地减少汞排放,选择性催化还原+静电除尘器/布袋除尘器+石灰石-石膏湿法脱硫(SCR+ESP/FF+WFGD)组合的平均脱汞率可达71.48%;SCR的大规模应用可能会将汞大量转移到飞灰和脱硫石膏中,带来二次污染的问题。 | YIN Libao ZHUO Yuqun XU Qisheng ZHU Zhenwu DU Wen AN Zhongyi | 2013 | 中国电机工程学报2013，33，29： | 29 |
| 2 | SHRIMP U-Pb Zircon Geochronology of the Xiaotongguanshan and Shatanjiao Intrusions and Its Petrological Implications in the Tongling Area, Anhui显示文摘This paper determines the crystallization ages of the Xiaotongguanshan quartz monzodiorite and Shatanjiao quartz monzonite porphyry from the Tongling area using the SHRIMP zircon U-Pb method. The crystallization age of the former is 142.8±1.8 Ma; that of the latter is 151.8±2.6 Ma. These data indicate that they were formed during the Late Jurassic (142.8 to 151.8 Ma). Zoned magma chamber was formed because of double diffusive convection. Therefore, the intrusive sequence of magma is generally from quartz monzonite through quartz monzodiorite to pyroxene monzodiorite, i.e. an inverted sequence. | DI Yongjun WU Ganguo ZHANG Da SONG Biao ZANG Wenshuan ZHANG Zhongyi LI Jinwen | 2005 | Acta Geologica Sinica(English Edition)2005，79，6： | 22 |
| 3 | Comparative profiling of genes and miRNAs expressed in the newborn, young adult, and aged human epididymides显示文摘在通过老化从出生后的开发在 epididymis 调整基因表示理解 transcriptional 因素和 miRNAs 的角色,在新生儿,年轻成年人,和年老的人表示的基因和 miRNAs 的系统的介绍 epididymides 被 cDNA 数组和 miRNA 数组分析分别地执行。新生的人的 epididymis 表示了 fewest mRNAs 但是 miRNAs 的最大的数字而成年、年老的 epididymides 表示了大多数 mRNAs 但是 fewest miRNAs,在 mRNAs 和 miRNA 之间的否定关联在老化期间。由综合分析,一套 miRNA 目标基于 miRNA 和 cDNA 数组被预言。在新生的 epididymis, 127 miRNAs 只或优先地被表示,但是仅仅 3 和 2 miRNAs 分别地在成年、年老的 epididymides 显示出一个充实年龄的表示模式。这研究在 epididymis 在基因表示的复杂规定上为进一步的研究象新卓见和基础一样提供一个基本数据库。 | Jinsong Zhang Qiang Liu Wei Zhang Jianyuan Li Zheng Li Zhongyi Tang Yixue Li Chunsheng Han Susan H. Hall Yonglian Zhang | 2010 | Acta Biochimica et Biophysica Sinica2010，42，2： | 15 |
| 4 | Novel CeO_2@TiO_2 core–shell nanostructure catalyst for selective catalytic reduction of NOx with NH_3显示文摘The CeO_2@TiO_2 core-shell nanostructure catalyst prepared by a two-step hydrothermal method was used for selective catalytic reduction(SCR) of NOx with NH_3 in this study.The catalyst presented the obvious core-shell structure,and the shell was amorphous TiO_2which could protect the active center from the SO_2 erosion.The catalyst showed high activity and stability,excellent N_2 selectivity and superior SO_2 resistance and H_2O tolerance.Characterizations such as TEM,HR-TEM,XRD,BET,XPS,NH_3-TPD,and H_2-TPR were carried out.The results indicated that the catalyst had large surface area and the active sites were well dispersed on the surface.The NH_3-TPD,H_2-TPR and XPS results implied that its increased SCR activity might be due to the enhancement of NH_3 chemisorption and the increase of active oxygen species,both of which were conductive to NH_3 activation.The excellent catalytic performance suggests that it is a promising candidate for SCR catalyst. | Bingjie Huang Danqing Yu Zhongyi Sheng Liu Yang | 2017 | Journal of Environmental Sciences2017，29，5： | 15 |
| 5 | Comparisons in subcellular and biochemical behaviors of cadmium between Iow-Cd and high-Cd accumulation cultivars of pakchoi (Brassica chinensis L.)显示文摘 | Meng XUE Yihui ZHOU Zhongyi YANG Biyun LIN Jiangang YUAN Shanshan WU | 2014 | Frontiers of Environmental Science & Engineering2014，8，2： | 14 |
| 6 | Study on the Nanosized Amorphous Ru-Fe-B/ZrO_2 Alloy Catalyst for Benzene Selective Hydrogenation to Cyclohexene显示文摘新奇 nanosized 为到环己烯的苯选择加氢的非结晶的 Ru-Fe-B/ZrO2 合金催化剂被调查。这催化剂的优异性质被归因于 nanosize 和非结晶的特性的联合以及到它的组织上特性。另外,锌离子,在泥浆的 ZrO2 的内容,和催化剂的预告的处理的集中被发现在改进这项活动和催化剂的选择有效。给词调音:Ru-Fe-B/ZrO2 非结晶的催化剂;苯选择加氢; | Shouchang Liu Zhongyi Liu Shuhui Zhao Yongmei Wu Zheng Wang Peng Yuan | 2006 | Journal of Natural Gas Chemistry2006，15，4： | 14 |
| 7 | Facile synthesis of yolk-shell Ni@void@SnO2(Ni3Sn2) ternary composites via galvanic replacement/Kirkendall effect and their enhanced microwave absorption properties显示文摘蛋黄壳第三的 composites 一个 Ni 范围核心和 SnO 2(Ni3 Sn 2) 壳被一个灵巧的二拍子的圆舞方法成功地准备。产生 composites 的尺寸,形态学,微观结构,和阶段纯净被扫描电子显微镜学描绘,精力散 X 光检查光谱学,传播电子显微镜学(TEM ) ,高分辨率的 TEM,精选区域的电子衍射,和粉末 X 光检查衍射。蛋黄壳结构的核心尺寸,空隙的空体积,和成分由改变反应时间变化了。机制为蛋黄壳结构的形成基于时间依赖者实验被建议。蛋黄壳结构被蚀刻的反应,流电的代替反应,和 Kirkendall 效果的 synergistic 联合形成。蛋黄壳第三的 SnO 2(Ni 3 Sn 2)@Ni composites 在 15 h 的一反应时间综合了显示出的优秀微波吸收性质。思考损失被发现作为在 6.1 GHz 的低 as-43 dB。提高的微波吸收性质可以被归因于好阻抗火柴,多重思考,由于在核心和壳之间的虚空散布,并且在电介质之间的有效补充损失和磁性的损失。因此,蛋黄壳第三的 composites 被期望为微波吸收应用,锂离子电池,和光催化正在答应候选人。 | Biao Zhao Xiaoqin Guo Wanyu Zhao Jiushuai Deng Bingbing Fan Gang Shao Zhongyi Bai Rui Zhang | 2017 | Nano Research2017，10，1： | 14 |
| 8 | The Qitai radio telescope显示文摘This study presents a general outline of the Qitai radio telescope(QTT)project.Qitai,the site of the telescope,is a county of Xinjiang Uygur Autonomous Region of China,located in the east Tianshan Mountains at an elevation of about 1800 m.The QTT is a fully steerable,Gregorian-type telescope with a standard parabolic main reflector of 110 m diameter.The QTT has adopted an umbrella support,homology-symmetric lightweight design.The main reflector is active so that the deformation caused by gravity can be corrected.The structural design aims to ultimately allow high-sensitivity observations from 150 MHz up to115 GHz.To satisfy the requirements for early scientific goals,the QTTwill be equipped with ultra-wideband receivers and large field-of-view multi-beam receivers.A multi-function signal-processing system based on RFSo C and GPU processor chips will be developed.These will enable the QTT to operate in pulsar,spectral line,continuum and Very Long Baseline Interferometer(VLBI)observing modes.Electromagnetic compatibility(EMC)and radio frequency interference(RFI)control techniques are adopted throughout the system design.The QTT will form a world-class observational platform for the detection of lowfrequency(nano Hertz)gravitational waves through pulsar timing array(PTA)techniques,pulsar surveys,the discovery of binary black-hole systems,and exploring dark matter and the origin of life in the universe.The QTT will also play an important role in improving the Chinese and international VLBI networks,allowing high-sensitivity and high-resolution observations of the nuclei of distant galaxies and gravitational lensing systems.Deep astrometric observations will also contribute to improving the accuracy of the celestial reference frame.Potentially,the QTT will be able to support future space activities such as planetary exploration in the solar system and to contribute to the search for extraterrestrial intelligence. | Na Wang Qian Xu Jun Ma Zhiyong Liu Qi Liu Hailong Zhang Xin Pei Maozheng Chen Richard N.Manchester Kejia Lee Xingwu Zheng Hans J.Kärcher Wulin Zhao Hongwei Li Dongwei Li Martin Süss Matthias Reichert Zhongyi Zhu Congsi Wang Mingshuai Li Rui Li Ning Li Guljaina Kazezkhan Wenming Yan Gang Wu Lang Cui Ming Zhang Haitao Li | 2023 | Science China(Physics,Mechanics & Astronomy)2023，66，8： | 14 |
| 9 | Estimation of ammonia nitrogen load from nonpoint sources in the Xitiao River catchment, China显示文摘Ammonia nitrogen (NH4+-N) is one of the three main forms of total nitrogen (TN). Most studies have estimated the load of TN from nonpoint sources instead of one specific form. The relationship between land use and concentrations of NH4+-N in runoff was analyzed using the hydraulic analysis functions of a Geographic Information Systems (GIS), and the annual loads of NH4+-N in the Xitiao River catchment were estimated according to model results. The results suggested that the calculated annual loads of NH4+-N agreed well with the observed ones, which was a good example demonstrating that it was possible to estimate the pollutant loads from nonpoint sources without enough monitoring data. Results also showed that the concentrations of NH4+-N in river waters of forest and arable land in the study area were 0.16 and 0.39 mg/L, respectively. The total nonpoint source load of NH4+-N from 1995 to 2001 (except 1998 and 2000) varied between 2,098 and 7,992 tons/year in the Xitiao River catchment. | Tao LIANG Zhongyi CHONG | 2008 | Journal of Environmental Sciences2008，20，10： | 13 |
| 10 | Research progress on electrical signals in higher plants显示文摘This review introduces the characteristics of electrical signals in higher plants and their corresponding physiological significance, and describes in detail the impact of environmental factors (e.g. light and temperature) on the electrical potential of the plants. Also, we evaluate the measurement techniques used for electrical signals in plants, including intracellular measurement, extracellular measurement, measurement of the ion channel based on the patch-clamp technique and on the non-invasive microelectrode vibrating probe technique. We also give a brief review of the applications of these methods for investigating electrical signals in plants. The ionic mechanism of electrical activity in plants is then discussed in terms of environmental response in higher plants, and this is used to provide a theoretical basis for quantitative description of the electrical signals in plants. A model for interpretation of the electrical signal mechanisms in higher plants is discussed, but further experiments are required for the verification of this model. | Xiaofei Yana, Zhongyi Wang a, Lan Huang a, Cheng Wang b, Ruifeng Hou b, Zhilong Xu b, Xiaojun Qiao b a College of Information and Electrical Engineering, China Agricultural University, Beijing 100083, China b National Engineering Research Center for Information Technology in Agriculture, Beijing 100097, China | 2009 | Progress in Natural Science:Materials International2009，19，5： | 13 |
| 11 | Residual lifetime prediction model of nonlinear accelerated degradation data with measurement error显示文摘For the product degradation process with random effect(RE), measurement error(ME) and nonlinearity in step-stress accelerated degradation test(SSADT), the nonlinear Wiener based degradation model with RE and ME is built. An analytical approximation to the probability density function(PDF) of the product's lifetime is derived in a closed form. The process and data of SSADT are analyzed to obtain the relation model of the observed data under each accelerated stress. The likelihood function for the population-based observed data is constructed. The populationbased model parameters and its random coefficient prior values are estimated. According to the newly observed data of the target product in SSADT, an analytical approximation to the PDF of its residual lifetime(RL) is derived in accordance with its individual degradation characteristics. The parameter updating method based on Bayesian inference is applied to obtain the posterior value of random coefficient of the RL model. A numerical example by simulation is analyzed to verify the accuracy and advantage of the proposed model. | Zhongyi Cai Yunxiang Chen Qiang Zhang Huachun Xiang | 2017 | Journal of Systems Engineering and Electronics2017，28，5： | 12 |
| 12 | SHRIMP zircon U-Pb dating of the intrusives in the Tongling metallogenic cluster and its dynamic setting显示文摘This paper selected five typical Mesozoic intrusives from the Tongling metallogenic cluster (Xiaotongguanshan, Fenghuangshan, Xinqiao, Dongguashan, and Shatanjiao plutons), and made a systemic SHRIMP zircon U-Pb dating for the five plutons, which produced an age range of 151.8±2.6- 142.8±1.8 Ma. This work put an accurate constraint on the formation age of the intrusives in the Tongling metallogenic cluster. These age data indicate that magmatic activity reached a peak during Late Jurassic. The intrusive sequence of magma is generally from quartz monzonite (porphyry) through monzonite to granodiorite to quartz monzodiorite to pyroxene monzodiorite to gabbro-diabase. The intrusives of different lithology differed in crystallization age, probably implying the intrusives in the Tongling area underwent an evolutional process of magma, which was closely related to geodynamical setting in the depths of the area. A dynamic model was presented for the origin of the igneous rocks in the study area as follows. The assembly between the Yangtze craton and the North China craton fini- shed at the end of T3, and then the stage of another compressional orogeny began in the Tongling area, i.e., Pacific dynamic system. Along with the subduction of the Izanagi plate underneath the Eurasian plate at J2-J3, NW-trending compression toward the East China continent was produced, and compres- sional deformation also took place, forming NE-trending fold and resulting in thickening of the crust in the Tongling area. High-density eclogite-facies rocks were produced in the low part of the crust, re- sulting in the delamination of mantle lithosphere and lower crust, and upwelling of materials in as- thenosphere. Decompression melting produced basaltic magma, and the materials in lower crust were heated by the underplating of the basaltic magma. Thus, melting of lower crust yielded granitic magma, which intruded along deep and large faults through various geological processes (J3-K1). The SHRIMP U-Pb zircon age of 151.8±2.6-142.8±1.8 Ma for intrusives in the Tongling area suggests that the de- lamination of lithosphere mantle and lower crust at least began at middle-late stage of Late Jurassic, resulting in sharp thinning of lithosphere and intense extension of middle-upper crust. Thus, a lot of decollements were produced between cover and cover, basement and cover, and middle and lower crust. This was structural layering or detachment of lithosphere in the Tongling area. Three concordant ages for old inherited cores of magmatic origin (747-823 Ma) indicated that there were obvious mag- matism in the Tongling area during Neoproterozoic, and a little more of the Neoproterozoic igneous source rocks participated in the formation of Mesozoic intrusives. | GanGuo Wu Da Zhang YongJun Di WenShuan Zang XiangXin Zhang Biao Song ZhongYi Zhang | 2008 | Science China Earth Sciences2008，51，7： | 11 |
| 13 | High cadmium pollution risk on vegetable amaranth and a selection for pollution-safe cultivars to lower the risk显示文摘一个壶实验被种蔬菜苋的 29 不同遗传型(Amaranthus spp ) 在下面执行低 --(0.12 mg 椠 ?? 牧潯敶吗? | YihuiZHOU Meng XUE Zhongyi YANG Yulian GONG Jiangang YUAN Chunyan ZHOU Baifei HUANG | 2013 | Frontiers of Environmental Science & Engineering2013，7，2： | 10 |
| 14 | Storage reliability assessment model based on competition failure of multi-components in missile显示文摘The degradation data of multi-components in missile is derived by periodical testing. How to use these data to assess the storage reliability(SR) of the whole missile is a difficult problem in current research. An SR assessment model based on competition failure of multi-components in missile is proposed. By analyzing the missile life profile and its storage failure feature, the key components in missile are obtained and the characteristics voltage is assumed to be its key performance parameter. When the voltage testing data of key components in missile are available, a state space model(SSM) is applied to obtain the whole missile degradation state, which is defined as the missile degradation degree(DD). A Wiener process with the time-scale model(TSM) is applied to build the degradation failure model with individual variability and nonlinearity. The Weibull distribution and proportional risk model are applied to build an outburst failure model with performance degradation effect. Furthermore, a competition failure model with the correlation between degradation failure and outburst failure is proposed. A numerical example with a set of missiles in storage is analyzed to demonstrate the accuracy and superiority of the proposed model. | Yunxiang Chen Qiang Zhang Zhongyi Cai Lili Wang | 2017 | Journal of Systems Engineering and Electronics2017，28，3： | 9 |
| 15 | An intracellular toxic protein (Xin) isolated from Xenorhabdus nematophilus strain BJ显示文摘An intracellular toxic protein, designated Xin and with remarkable inhibitory effect on growth of Helicoverpa armigera, was isolated from X. Nematophilus strain BJ by ion exchange chromatography and hydrophobic interaction chromatography. After placing neonates on the artificial diet containing Xin at concentration of 0 or 3.48μg/g for 7 days, the average weight of insects was 23.50mg and 0.55mg, respectively. The activity of Xin was lost by heating, freeze-drying, digestion with proteases or urea. The Xin molecular weight, over kD, was determined by gel filtration on Superose 12, and there were six component proteins analyzed by SDS-PAGE. The results show that Xin is a high molecular protein complex inhibiting growth of insect pest. | PAN Yinghong , JIAN Heng , ZHANG Jie , LIU Zheng, CHEN Zhongyi , YANG Xiufen, YANG Huaiwen and HUANG Dafang( State Key Laboratory for Biology of Plant Diseases and Insect Pests, Institute of Plant Protection, Chinese Academy of Agricultural Sciences, Beijing 100094, China Institute of Biocontrol Research, Chinese Academy of Agricultural Sciences, Beijing 100081, China Institute of Biotechnology Research, Chinese Academy of Agricultural Sciences, Beijing 100081, China.) | 2002 | Progress in Natural Science:Materials International2002，12，4： | 9 |
| 16 | Principle and theoretical analysis of continuous roll forming for three-dimensional surface parts显示文摘Continuous roll forming(CRF) is a novel forming process for three-dimensional surface parts,in which a pair of bendable forming rolls is used as sheet metal forming tool.By controlling the gap between the upper and lower forming rolls,sheet metal is non-uniformly extended in the longitudinal direction while it is bent in the transverse direction during the rolling process.As a result,longitudinal bending is gained and a doubly curved surface is formed.With the rotations of the forming rolls,the sheet metal is deformed consecutively,and a three-dimensional surface part is shaped continuously.In this paper,the mechanism of the three-dimensional surface formation in CRF is set forth.Through theoretical analysis of the CRF process,the governing equations for the bending deformation in rolling process are presented.Based on the simplification on the deformation and material model,the formulation to calculate the longitudinal bending deformation is derived,and the methods to design the compression ratio and the roll gap are given,the effects of compression ratio of rolling and the width of blank sheet on the longitudinal bending curvature are analyzed.The forming experiments on typical surface parts and measured results show that forming results with good precision can be obtained by CRF process. | CAI ZhongYi LI MingZhe | 2013 | Science China(Technological Sciences)2013，56，2： | 9 |
| 17 | Genotype variations in accumulation of cadmium and lead in celery (Apium graveolens L.) and screening for low Cd and Pb accumulative cultivars显示文摘To help reduce risks of heavy metal pollution, two pot experiments were conducted to investigate the variations, transfer potential, and stability of Cadmium (Cd) and Lead (Pb) accumulations in celery (Apium graveolens L.) and to screen for low Cd and Pb accumulative cultivars. The maximum differences in shoot Cd concentration were 4.7-fold under low-Cd exposure and 3.3-fold under high-Cd exposure. These genotype variations in Cd accumulation are sufficiently large to help reduce Cd contamination risk in soil by using the Low-Cd-Accumulative genotypes. Cd accumulation of the Low-Cd-Accumulative genotypes is significantly positive correlated with Pb accumulation. Evidence obtained proves that Cd and Pb accumulations in celery are stable and genotype-dependent at the cultivar level. The presence of high-Pb contamination in soil promoted Cd accumulation in shoots of celery. Celery is considered a species with high risks in Cd pollution and low risks in Pb pollution. Among the tested cultivars, cv. Shuanggang- kangbing (SGKB) had the lowest shoot Cd and Pb accumulating abilities, and thus is the most important material for breeding of pollution-safe cultivars (PSCs) to minimize Cd and Pb accumulations in celery. | Kun ZHANG Jianbing WANG Zhongyi YANG Guorong XIN Jiangang YUAN Junliang XIN Charlie HUANG | 2013 | Frontiers of Environmental Science & Engineering2013，7，1： | 9 |
| 18 | Cloning and expression of two sterol C-24 methyltransferase genes from upland cotton(Gossypium hirsuturm L.)显示文摘Brassinosteroids (BRs) are an important class of plant steroidal hormones that are essential in a wide variety of physiological proc-esses. Two kinds of intermediates,sitosterol and campesterol,play a crucial role in cell elongation,cellulose biosynthesis,and accumula-tion. To illuminate the effects of sitosterol and campesterol on the development of cotton (Gossypium hirsuturm L.) fibers through screening cotton fiber EST database and contigging the candidate ESTs,two key genes GhSMT2-1 and GhSMT2-2 controlling the sitos-terol biosynthesis were cloned from developing fibers of upland cotton cv. Xuzhou 142. The full length of GhSMT2-1 was 1,151 bp,in-cluding an 8 bp 5′-untranslated region (UTR),a 1,086 bp open reading frame (ORF),and a 57 bp 3′-UTR. GhSMT2-1 gene encoded a polypeptide of 361 amino acid residues with a predicted molecular mass of 40 kDa. The full length of GhSMT2-2 was 1,166 bp,including an 18 bp 5′-UTR,a 1,086 bp ORF,and a 62 bp 3′-UTR. GhSMT2-2 gene encoded a polypeptide of 361 amino acid residues with a pre-dicted molecular mass of 40 kDa. The two deduced amino acid sequences had high homology with the SMT2 from Arabidopsis thaliana and Nicotiana tabacum. Furthermore,the typical conserved structures characterized by the sterol C-24 methyltransferase,such as region I (LDVGCGVGGPMRAI),region Ⅱ (IEATCHAP),and region Ⅲ (YEWGWGQSFHF),were present in both deduced proteins. Southern blotting analysis indicated that GhSMT2-1 or GhSMT2-2 was a single copy in upland cotton genome. Quantitative real-time RT-PCR analysis revealed that the highest expression levels of both genes were detected in 10 DPA (day post anthesis) fibers,while the lowest levels were observed in cotyledon and leaves. The expression level of GhSMT2-1 was 10 times higher than that of GhSMT2-2 in all the organs and tissues detected. These results indicate that the homologue of sterol C-24 methyltransferase gene was cloned from upland cotton and both GhSMT2 genes play a crucial role in fiber elongation. The role of GhSMT2-1 may be more important than that of GhSMT2-2. | Ming Luo,Kunling Tan,Zhongyi Xiao,Mingyu Hu,Peng Liao,Kuijun Chen Key Laboratory of Biotechnology and Crop Quality Improvement,Ministry of Agriculture Biotechnology Research Center,Southwest University,Chongqing 400716,China | 2008 | Journal of Genetics and Genomics2008，35，6： | 8 |
| 19 | SnS_2@C Hollow Nanospheres with Robust Structural Stability as High?Performance Anodes for Sodium Ion Batteries显示文摘Constructing unique and highly stable structures with plenty of electroactive sites in sodium storage materials is a key factor for achieving improved electrochemical properties through favorable sodium ion di usion kinetics. An SnS_2@carbon hollow nanospheres(SnS_2@C) has been designed and fabricated via a facile solvothermal route, followed by an annealing treatment. The SnS_2@C hybrid possesses an ideal hollow structure, rich active sites, a large electrode/electrolyte interface, a shortened ion transport pathway, and, importantly, a bu er space for volume change, generated from the repeated insertion/extraction of sodium ions. These merits lead to the significant reinforcement of structural integrity during electrochemical reactions and the improvement in sodium storage properties, with a high specific reversible capacity of 626.8 mAh g^(-1) after 200 cycles at a current density of 0.2 A g^(-1) and superior high-rate performance(304.4 mAh g^(-1) at 5 A g^(-1)). | Shuaihui Li Zhipeng Zhao Chuanqi Li Zhongyi Liu Dan Li | 2019 | Nano-Micro Letters2019，11，1： | 8 |
| 20 | Kilogram-scale synthesis of carbon quantum dots for hydrogen evolution, sensing and bioimaging显示文摘The development of large-scale synthetic methods for high quality carbon quantum dots(CQDs) is fundamental to their applications.However,the macroscopic preparation and scale up synthetic of CQDs is still in its infancy.Here,we report a facile,green,kilogram-scale synthesis of high quality fluorescent CQDs derived from poplar leaves via a one-step hydrothermal method.Notably,the throughput of CQDs can reach a level up to as high as 1.4975 kg in one pot.The structure and properties of the as-prepared CQDs were assessed through TEM,XRD,XPS and various spectroscopic methods.The obtained high quality CQD s with a photoluminescent quantum yield of 10.64% showed remarkable stability in aqueous media,rich functional groups,high photostability,consistent photoluminescence within biological pH range and low cytotoxicity.On account of these good properties,we demonstrated the multifunctional application to electrocatalytic water splitting,Fe^3+ sensing and bioimaging.It showed remarkable electrocatalytic activity,Fe^3+ sensitivity and good biocompatibility.This study provides a green,facile,inexpensive and large-scale method for producing high quality CQDs,which provides application value for large-scale production of CQDs. | Weidong Li Yuan Liu Boyang Wang Haoqiang Song Zhongyi Liu Siyu Lu Bai Yang | 2019 | Chinese Chemical Letters2019，30，12： | 7 |
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