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Defect Engineering of Carbons for Energy Conversion and Storage Applications

查看全文 作  者:Xianyou [1,2]Luo;Heng [2]Zheng;Wende [2]Lai;Ping [2]Yuan;Shengwei [2]Li;De [2,3]Li;Yong [1,2,3]Chen 高影响力作者 机构地区:[1]Guangdong Key Laboratory for Hydrogen Energy Technologies,School of Materials Science and Hydrogen Energy,Foshan University,Foshan 528000,China;[2]State Key Laboratory of Marine Resource Utilization in South China Sea,Hainan Provincial Key Laboratory of Research on Utilization of Si-Zr-Ti Resources,Hainan University,Haikou 570228,China;[3]Key Laboratory of Advanced Energy Materials Chemistry(Ministry of Education),Nankai University,Tianjin 300071,China高影响力机构 出  处:《Energy & Environmental Materials》索引2023年第6卷第3期,共22页高影响力期刊 基  金:the National Natural Science Foundation of China(52062012);Key Science&Technology Project of Hainan Province(ZDYF2020028);Key-Area Research and Development Program of Guangdong Province(2019B1102109003);the Innovation Team of Universities of Guangdong Province(2020KCXTD011);Guangdong Province Key Discipline Construction Project(2021ZDJS102). 摘  要:Sustainable energy conversion and storage technologies are a vital prerequisite for neutral future carbon.To this end,carbon materials with attractive features,such as tunable pore architecture,good electrical conductivity,outstanding physicochemical stability,abundant resource,and low cost,have used as promising electrode materials for energy conversion and storage.Defect engineering could modulate the structures of carbon materials,thereby affecting their electronic properties.The presence of defects on carbons may lead to asymmetric charge distribution,change in geometrical configuration,and distortion of the electronic structure that may result in unexpected electrochemical performances.In this review,recent advances in defects of carbons used for energy conversion and storage were examined in terms of types,regulation strategies,and fine characterization means of defects.The applications of such carbons in supercapacitors,rechargeable batteries,and electrocatalysis were also discussed.The perspectives toward the development of defect engineering carbons were proposed.In all,novel insights related to improvement in high-performance carbon materials for future energy conversion and storage applications were provided. 关 键 词:carbon materials defect engineering ELECTROCATALYSIS rechargeable batteries SUPERCAPACITORS
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