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| 1 | 等级孔分子筛的可控合成、扩散研究及催化应用显示文摘等级孔分子筛是一类具有两种或多种以特定形式排布的孔结构的分子筛材料.多层等级的孔结构使得分子筛孔道内的分子扩散得到显著改善,进而提升了其在吸附和非均相催化等领域的应用性能.等级孔分子筛的制备策略通常有两种,即“自上而下”后处理法(如对母样分子筛进行脱铝、脱硅产生介孔)和“自下而上”合成法(如软模板、硬模板法).本文主要对近20年来等级孔分子筛的合成方法进行了梳理,并着重介绍了具有较高应用潜力的“自上而下”制备法.鉴于合成等级孔分子筛的主要目的是提高分子的晶内扩散,对近年来客体分子在等级孔分子筛内扩散的实验研究也进行了简要综述.此外,本文还综合评述了等级孔分子筛与传统分子筛在催化应用中的对比,以展示前者在提升催化性能方面(如活性、选择性等)的独特优势. | 邹润 董霄 矫义来 D'AGOSTINO Carmine 闫文付 范晓雷 | 2021 | 高等学校化学学报2021，42，1： | 3 |
| 2 | The Androgen Excess and PCOS Society Criteria for the Polycystic Ovary Syndrome: The Complete Task Force Report 显示文摘 | Azziz R Carmine E Dewailly D | 2009 | Fertil Steril2009，91，2： | 1 |
| 3 | Gupta, Operational and Financial Effectiveness of E - collaboration Tools in Supply Chain Integration 显示文摘 | Adolfo Crespo Marquez Carmine Bianchi Jatinder N D | 2004 | European Journal of Operational Research2004，159，： | 1 |
| 4 | Angiotensin II Type 2 receptors contribute to vascular responses in spontaneously hypertensive rats treated with angiotensin II Type 1 receptor antagonists 显示文摘 | Francesco C Carmine S Paola D P | 2005 | Am J Hypertens2005，18，： | 1 |
| 5 | Annunziata Soriente and Placido Neri显示文摘 | Carmine G Margherita D R Marina F | | 0，，： | 1 |
| 6 | NURR1 promoter polymorphisms:Parkinson's disease,schizophrenia,and personality traits显示文摘 | Carmine A Buervenich S Galter D | 2003 | Am J Med Genet B Neuropsychiatr Genet2003，120，1： | 1 |
| 7 | Biomechanical evalution of early fracture healing in normal and diabetic rats显示文摘 | Funk JR Hale JE Carmines D | 2000 | J Orthop Res2000，18，： | 1 |
| 8 | Tissue-and species-specific expression patterns of classⅠ,Ⅲ,and Ⅳ Adh and Aldh 1 mRNAs in rodent embryos显示文摘 | Westerlund M Galter D Carmine A Olson L | 2005 | Cell Tissue Res2005，322，2： | 1 |
| 9 | External-beam PIGE for fluorine de termination in atmospheric aerosol 显示文摘 | CALASTRINI F CARMINE P D LUCAREL- LI F et ai | 1998 | Nuclear Instruments and Methods in Physics Research B1998，，： | 1 |
| 10 | Biomechanical evaluation of early fraction healing in normal and diabetic rats显示文摘 | Funk JR Hale JE Carmines D | 2000 | J Orthop Res2000，18，： | 1 |
| 11 | ALDH1 mRNA: presence in hmnan dopamine neurons and decreases in sabstantia nigra in Parkinson's disease and in the ventral tegmental area in schizophrenia显示文摘 | Gaiter D Buervenich S Carmine A | 2003 | Neurobiol Dis2003，14，3： | 1 |
| 12 | Biomechanicalevaluation of early fraeture healing in normal and diabetie rats 显示文摘 | FUNK JR HALE JE CARMINES D | 2000 | J Orthop Res2000，118，1： | 1 |
| 13 | Biomechaincal evaluation of early facture healing in normal and diabetic rats显示文摘 | Funk JR Hale JE Carmines D | | 0，，01： | 1 |
| 14 | Operational and financial effective-ness of e-collaboration tools in supply chain integration显示文摘 | Adolfo Crespo Marquez Carmine Bianchi Jatinder Gupta N D | 2003 | European Journal of Operational Research2003，，8： | 1 |
| 15 | Biomechanical evalution of early fracture healing in normal and diabetic rats显示文摘 | Funk J R Hale J E Carmines D | 2000 | J Orthop Res2000，18，1： | 1 |
| 16 | Non-hematopoietic cells contribute to protective tolerance to Aspergillus fumigatus via a TRIF pathway converging on IDO显示文摘Innate responses combine with adaptive immunity to generate the most effective form of anti-Aspergillus immune resistance.Whereas the pivotal role of dendritic cells in determining the balance between immunopathology and protective immunity to the fungus is well established,we determined that epithelial cells(ECs)also contributes to this balance.Mechanistically,EC-mediated protection occurred through a Toll-like receptor 3/Toll/IL-1 receptor domain-containing adaptor-inducing interferon(TLR3/TRIF)-dependent pathway converging on indoleamine 2,3-dioxygenase(IDO)via non-canonical nuclear factor-kB activation.Consistent with the high susceptibility of TRIF-deficient mice to pulmonary aspergillosis,bone marrow chimeric mice with TRIF unresponsive ECs exhibited higher fungal burdens and inflammatory pathology than control mice,underexpressed the IDO-dependent T helper 1/regulatory T cell(Th1/Treg)pathway and overexpressed the Th17 pathway with massive neutrophilic inflammation in the lungs.Further studies with interferon(IFN)-c,IDO or IL-17R unresponsive cells confirmed the dependency of immune tolerance to the fungus on the IFN-c/IDO/Treg pathway and of immune resistance on the MyD88 pathway controlling the fungal growth.Thus,distinct immune pathways contribute to resistance and tolerance to the fungus,to which the hematopoietic/non-hematopoietic compartments contribute through distinct,yet complementary,roles. | Antonella de Luca Silvia Bozza Teresa Zelante Silvia Zagarella Carmen D’Angelo Katia Perruccio Carmine Vacca Agostinho Carvalho Cristina Cunha Franco Aversa Luigina Romani | 2010 | Cellular & Molecular Immunology2010，7，6： | 1 |
| 17 | Biomeehanical evaluation of early fracture healing in normal and diabetic rats 显示文摘 | Funk JR Hale JE Carmines D | 2000 | J Orthopaedic Res2000，1，： | 1 |
| 18 | Advantages of multidisciplinary management of bile duct injuries occurring during cholecystectomy显示文摘 | Gennaro Nuzzo Felice Giuliante Ivo Giovannini Marino Murazio Fabrizio D’Acapito Francesco Ardito Maria Vellone Riccardo Gauzolino Guido Costamagna Carmine Di Stasi | 2008 | The American Journal of Surgery2008，，6： | 1 |
| 19 | Reverberation time measurement by the product of two room impulse responses显示文摘 | Raffaele D Carmine L Rosario A R | 2009 | Applied Acoustics2009，70，1： | 1 |
| 20 | Biomechanical evalution of early fracture healing in normal and diabetic rats显示文摘 | Funk JR Hale JE Carmines D | 2000 | J Orthop Res2000，18，： | 1 |
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