|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Dynamical changes in hydration water accompanying lysozyme thermal denaturation显示文摘 | Francesco Mallamace Carmelo Corsaro Domenico Mallamace Nicola Cicero Sebastiano Vasi Giacomo Dugo H. Eugene Stanley | 2015 | Frontiers of physics2015，10，5： | 0 |
| 2 | The Boson peak in confined water: An experimental investigation of the liquid-liquid phase transition hypothesis显示文摘 | Francesco Mallamace Carmelo Corsaro Domenico Mallamace Zhe Wang Sow-Hsin Chen | 2015 | Frontiers of physics2015，10，5： | 0 |
| 3 | NMR investigation of degradation processes of ancient and modern paper at different hydration levels显示文摘做纤维素的材料的降级过程借助于原子磁性的回声(NMR ) 被调查光谱学,与水的角色上并且在纤维素纤丝的水和机制上的特别强调。完成这,在有不同老化历史的古老、现代的样品以内的水的结构和动力学被调查。结果主要显示了那 hydrolytic,氧化反应挑起了酸的副产品的形成。而且,降级过程被给纤维素的非结晶的区域的进步消费的水的更高的数量提高。我们为纸的降级状态的描述,以及为调查恢复处理的有效性作为一个基准建议 NMR 实验。 | Domenico Mallamace Sebastiano Vasi Mauro Missori Francesco Mallamace Carmelo Corsaro | 2018 | Frontiers of physics2018，13，1： | 0 |
| 4 | Contrasting microscopic interactions determine the properties of water/methanol solutions显示文摘此处,我们学习在不同甲醇发生在水 / 甲醇答案的不同显微镜的相互作用臼齿的部分,用 NMR spctroscopy。温度被发现决定相互作用统治哪个。因为象 hydrophobicity 和 hydrophilicity 一样的相互作用的存在,在水和甲醇之间混合是非理想的,这被发现。这些结果显示在吸水、恐水病的相互作用之间的比赛在不同热区域是不同的,并且解决方案的物理性质是,这自己由解决方案的字符决定了,它接着取决于甲醇并且在温度上的鼹鼠部分。 | Carmelo Corsaro Francesco Mallamace Sebastiano Vasi Sow-Hsin Chen H. Eugene Stanley Domenico Mallamace | 2018 | Frontiers of physics2018，13，1： | 0 |
| 5 | Experimental tests for a liquid-liquid critical point in water显示文摘Water is a fascinating material.Its composition is simple—one oxygen and two hydrogen atoms—but its chemistry and physics are extremely complex and exhibit 75 documented anomalies.Although these anomalies and their molecular origin are not completely understood,we know that hydrogen bonds play key roles in all of the phases of water.Moreover,there is experimental evidence that the polymorphism of the ice structure extends into the liquid phase and is associated with a liquid-liquid coexistence line.This is currently a topic of great interest in water research because there are indications that the end point of the coexistence line corresponds to a second critical point inside the supercooled liquid regime.We examine the recent progress in understanding water anomalies and the liquid-liquid phase transition hypothesis,including the results of recent experimental work and molecular simulations of both bulk and confined water.We examine experimental results that test whether the behavior of liquid water is consistent with the'liquid polymorphism'hypothesis that liquid water can exist in two distinct phases of differing densities.We also examine recent research on the anomalies of nanoconfined water and,in particular,on water in biological environments.We find that the concept of liquid polymorphism can also describe the properties of other liquids that have two characteristic length scales. | Domenico Mallamace Carmelo Corsaro Francesco Mallamace H.Eugene Stanley | 2020 | Science China(Physics,Mechanics & Astronomy)2020，63，12： | 0 |
| 6 | Preface to the special topic: New advances in water and water systems显示文摘Water and related systems play a central role in science and technology.Although water has unusual and anomalous behaviors,if compared with normal liquids,it is of fundamental interest in many research fields going from chemical-physics to life sciences.The first and well known example of these anomalies is the density maximum,at 277 K,intuited by Galilei[1]in 1612 and lately discovered in Florence[2]. | LiMei Xu Francesco Mallamace | 2019 | Science China(Physics,Mechanics & Astronomy)2019，62，10： | 0 |
| 7 | Hydrophilic and hydrophobic competition in water-methanol solutions显示文摘We study the thermal behavior of the longitudinal spin-lattice,T1,and the transverse spin-spin,T2,relaxation times of the macroscopic magnetization in water/methanol solutions.Our aim is to investigate the reciprocal influence of hydrophobic effects on water properties and of hydrophilicity(via hydrogen bond,HB,interactions)on the solute.Using classical Nuclear Magnetic Resonance spectroscopy,we find a single characteristic correlation time r c that reflects all local structural configurations and characterizes the thermal motion effects of the magnetic nuclei on the spin-spin interaction.We find that in the supercooled regime the correlations are stronger,with respect to ambient temperature,because the HB interactions have a lifetime long enough to sustain a stable water network.However,increasing the temperature,progressively decreases the HB interaction lifetime and destroys the water clusters with a consequent decoupling in the dynamic modes of the system.In addition,at temperatures higher than about 265 K,the hydrophobicity becomes gradually stronger and governs the physical properties of the solutions. | Domenico Mallamace Sow-Hsin Chen Carmelo Corsaro Enza Fazio Francesco Mallamace HEugene Stanley | 2019 | Science China(Physics,Mechanics & Astronomy)2019，62，10： | 0 |
| 8 | The Boson peak interpretation and evolution in confined amorphous water显示文摘We study the evolution of the Boson peak for water confined in cement paste obtained by means of Inelastic Neutron Scattering from room temperature to the deep supercooled regime.We analyze the data in terms of a universal-like model,developed for glass forming liquids in the frame of the energy landscape.In such a way it is possible to discriminate between the fragile and strong glass forming character of supercooled liquids and the dynamical crossover,fragile to strong,between them.Hence,we confirm the link between the Boson peak and the water polymorphism.In particular,the main result is represented by a crossover from a local energetic minima configuration to that characteristic of saddle points on going towards the deep supercooled regime up to the dynamical arrest. | Francesco Mallamace Carmelo Corsaro Domenico Mallamace Sow-Hsin Chen Emiliano Fratini Piero Baglioni | 2019 | Science China(Physics,Mechanics & Astronomy)2019，62，10： | 0 |
| 9 | A study of the hydrogen bonds effect on the water density and the liquid-liquid transition显示文摘We study the hydrogen bonds effect on the water density as a function of temperature and pressure from the supercritical region to the metastable supercooled and amorphous phases.We identify two important thermodynamic thresholds,that is P^*≈2 kbar and r^*≈315 K,that separate two different water behaviors in terms of hydrogen bonding capability.For T | Francesco Mallamace Carmelo Corsaro Enza Fazio Sow-Hsin Chen Domenico Mallamace | 2019 | Science China(Physics,Mechanics & Astronomy)2019，62，10： | 0 |
| 10 | The onset of the tetrabonded structure in liquid water显示文摘Water properties are dominated by the hydrogen bond interaction that gives rise in the stable liquid phase to the formation of a dynamical network.The latter drives the water thermodynamics and is at the origin of its well known anomalies.The HB structural geometry and its changes remain uncertain and still are challenging research subjects.A key question is the role and effects of the HB tetrahedral structure on the local arrangement of neighboring molecules in water.Here the hydrogen dynamics in bulk water is studied through the combined use of Neutron Compton Scattering and NMR techniques.Results are discussed in the framework of previous studies performed in a wide temperature range,in the liquid,solid,and amorphous states.For the first time this combined studies provide an experimental evidence of the onset of the water tetrahedral network at T^315 K,originally proposed in previous studies of transport coefficients and thermodynamical data;below this temperature the local order in water changes and the lifetime of local hydrogen bond network becomes long enough to gradually develop the characteristic tetrahedral network of water. | Carla Andreani Carmelo Corsaro Domenico Mallamace Giovanni Romanelli Roberto Senesi Francesco Mallamace | 2019 | Science China(Physics,Mechanics & Astronomy)2019，62，10： | 0 |
您所在的机构暂未开通此部分的功能，请联系管理员