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| 1 | Synthesis of Large-Area, Few-Layer Graphene on Iron Foil by Chemical Vapor Deposition显示文摘我们表明一个简单、可控制的方法综合大区域,由优化化学蒸汽免职(CVD ) 的铁底层上的很少层 graphene 用甲烷和氢的混合物的方法。基于 Fe-C 阶段图的分析,为 Fe 表面上的 graphene 的成功的合成的一个合适的过程被设计。适当温度和冷却过程被发现在高度水晶的很少层 graphene 的合成很重要。基于 Graphene 的地效果晶体管(联邦货物税) 设备用产生很少层 graphene 被制作,并且与 3001150 cm2/ 的提取活动性显示出好质量(V 敢椠 ?? 敤瑢吗? | Yunzhou Xue Bin Wu Yunlong Guo Liping Huang Lang Jiang Jianyi Chen Dechao Geng Yunqi Liu Wenping Hu Gui Yu | 2011 | Nano Research2011，4，12： | 7 |
| 2 | Human movement monitoring and behavior recognition for intelligent sports using customizable and flexible triboelectric nanogenerator显示文摘Effective collection,recognition,and analysis of sports information is the key to intelligent sports,which can help athletes to improve their skills and formulate scientific training plans and competition strategies.At present,wearable electronic devices used for movement monitoring still have some limitations,such as high cost and energy consumption,incompatibility of suitable flexibility and personalized spatial structure,dissatisfactory data analysis methods,etc.In this work,a novel three-dimensionalprinted thermoplastic polyurethane is introduced as the elastic shell and friction layer,and it endows the proposed customizable and flexible triboelectric nanogenerator(CF-TENG)with personalized spatial structure and robust correlation to external pressure.In practical application,it exhibits highly sensitive responses to the joint-bending motion of the finger,wrist,or elbow.Furthermore,a pressure-sensing insole and smart ski pole based on CF-TENG are manufactured to build a comprehensive sports monitoring system to transmit the athletes’motion information from feet and hands through the plantar pressure distribution and ski pole action.To recognize the movement status,the self-developed automatic peak recognition algorithm(P-Find)and machine learning algorithm(subspace K-Nearest Neighbors)were introduced to accurately distinguish the four typical motion behaviors and three primary sub-techniques of cross-country skiing,with accuracy rates of 98.2%and 100%.This work provides a novel strategy to promote the personalized applications of TENGs in intelligent sports. | YANG Yun HOU XiaoJuan GENG WenPing MU JiLiang ZHANG Le WANG XiangDong HE Jian XIONG Ji Jun CHOU XiuJian | 2022 | Science China(Technological Sciences)2022，65，4： | 6 |
| 3 | A static-dynamic energy harvester for a self-powered ocean environment monitoring application显示文摘Ocean intelligent buoy is important for ocean environment monitoring.With the increase of requisite sensors and transportable data,a long power supply has become a problem to be solved urgently.In this work,a hybrid nanogenerator integrating triboelectric,piezoelectric,electromagnetic,photovoltaic,and thermotropic units is proposed to maximize ocean ambient energy harvesting,which includes static energy(solar and thermal energy)and dynamic energy(wave energy).Compared with a device with a single energy conversion mechanism,this structural design breaks the limit of harvesting time and natural conditions during the energy harvesting process,thereby increasing the harvested energy.Static energy harvesting is realized by the thermoelectric(TG)and photovoltaic(PV)units located inside the device and the PV unit attached to the device surface.Results show that the maximum open-circuit voltage and short-circuit current are 5 V and 41 mA in the external PV and 1.33 V and 49 mA in the internal PV under 30000 Lux illumination,respectively.The open-circuit voltage and short-circuit current of the TG unit are 5 V and 15 m A,respectively.The core component of the dynamic generation unit is the gimbal used to harvest wave energy by the triboelectric nanogenerator(TENG),piezoelectric generator(PENG),and electromagnetic generator.When the frequency is 2.4 Hz,the maximum peak-to-peak power of the TENG,PENG,and EMG are 0.25,1.58,and 13.8 mW,respectively.Finally,an intelligent ocean buoy is fabricated by the integration of an energy harvester,a power management circuit,sensors,a microcontroller,and a wireless communication module.Driven by static and dynamic energy,temperature signal,humidity signal,GPS signal,and sound signal are sent to the receiving terminal wirelessly.The ocean energy harvester proposed in this work is of great significance for ocean energy harvesting and ocean wireless monitoring systems. | XUE Feng CHEN Liang LI ChunCheng REN Jing YU JunBin HOU XiaoJuan GENG WenPing MU JiLiang HE Jian CHOU XiuJian | 2022 | Science China(Technological Sciences)2022，65，4： | 2 |
| 4 | Synergistic piezoelectricity enhanced BaTiO_(3)/polyacrylonitrile elastomer-based highly sensitive pressure sensor for intelligent sensing and posture recognition applications显示文摘Designing stretchable and skin-conformal self-powered sensors for intelligent sensing and posture recognition is challenging.Here,based on a multi-force mixing and vulcanization process,as well as synergistically piezoelectricity of BaTiO_(3)and polyacrylonitrile,an all-in-one,stretchable,and self-powered elastomer-based piezo-pressure sensor(ASPS)with high sensitivity is reported.The ASPS presents excellent sensitivity(0.93 V/104 Pa of voltage and 4.92 nA/104 Pa of current at a pressure of 10-200 kPa)and high durability(over 10,000 cycles).Moreover,the ASPS exhibits a wide measurement range,good linearity,rapid response time,and stable frequency response.All components were fabricated using silicone,affording satisfactory skinconformality for sensing postures.Through cooperation with a homemade circuit and artificial intelligence algorithm,an information processing strategy was proposed to realize intelligent sensing and recognition.The home-made circuit achieves the acquisition and wireless transmission of ASPS signals(transmission distance up to 50 m),and the algorithm realizes the classification and identification of ASPS signals(accuracy up to 99.5%).This study proposes not only a novel fabrication method for developing self-powered sensors,but also a new information processing strategy for intelligent sensing and recognition,which offers significant application potential in human-machine interaction,physiological analysis,and medical research. | Junbin Yu Shuai Xian Zhenpeng Zhang Xiaojuan Hou Jian He Jiliang Mu Wenping Geng Xiaojun Qiao Le Zhang Xiujian Chou | 2023 | Nano Research2023，16，4： | 2 |
| 5 | Porous fiber paper and 3D patterned electrodes composed high-sensitivity flexible piezoresistive sensor for physiological signal monitoring显示文摘The research on flexible pressure sensors has drawn widespread attention in recent years,especially in the fields of health care and intelligent robots.In practical applications,the sensitivity of sensors directly affects the precision and integrity of weak pressure signals.Here,a pressure sensor with high sensitivity and a wide measurement range composed of porous fiber paper and 3D patterned electrodes is proposed.Multi-walled carbon nanotubes with excellent conductivity were evenly sprayed on the fiber paper to form the natural spatial conducting networks,while the copper-deposited polydimethylsiloxane films with micropyramids array were used as electrodes and flexible substrates.Increased conducting paths between electrodes and fibers can be obtained when high-density micro-pyramids fall into the porous structures of the fiber paper under external pressure,thereby promoting the pressure sensor to show an ultra-high sensitivity of 17.65 kPa^(-1)in the pressure range of 0–2 kPa,16 times that of the device without patterned electrodes.Besides,the sensor retains a high sensitivity of 2.06 kPa^(-1)in an ultra-wide measurement range of 150 kPa.Moreover,the sensor can detect various physiological signals,including pulse and voice,while attached to the human skin.This work provides a novel strategy to significantly improve the sensitivity and measurement range of flexible pressure sensors,as well as demonstrates attractive applications in physiological signal monitoring. | HOU XiaoJuan ZHONG JiXin HE Jian YANG ChangJun YU JunBin MEI LinYu MU JiLiang GENG WenPing CHOU XiuJian | 2022 | Science China(Technological Sciences)2022，65，5： | 2 |
| 6 | A high-performance, single-electrode and stretchable piezotriboelectric hybrid patch for omnidirectional biomechanical energy harvesting and motion monitoring显示文摘Triboelectric nanogenerators(TENGs)have recently drawn much attention in the field of biomechanical energy harvesting and motion monitoring.However,the electrode stretchability and contact-separation model induced complicated packed structure remain a problem that heavily affects output performance during various human movements and requires to be urgently addressed.Here,a single-electrode piezotriboelectric hybrid nanogenerator(SEP-TENG)integrated with stretchable liquid-metal metal electrodes is reported,which simultaneously achieves outstanding energy harvesting performance and skincomfort human motion monitoring.A polarized piezoelectric BaTiO_(3)/silicon rubber(SR)composites film is served as the effective negative tribomaterial,benefiting from the improved dielectric constant and piezoelectric charge transfer,the optimized SEP-TENG generates a high peak power density of 5.7 W/m^(2) while contacted with human skin.Besides,owing to the ultralow Young's modulus of the SR encapsulation layer and tribo-piezoelectric hybrid layer,the homogeneous integrated multilayer composite serves no break till a 745%elongation,promoting that the SEP-TENG could effectively harvest biomechanical energy and realize stable power supplying for wearable electronics even under large deformation state.Furthermore,the SEP-TENG could comfortably attach to the finger joints and collect bending energy.This work provides a novel design methodology for a single-electrode TENG to realize omnidirectional biomechanical energy harvesting and motion monitoring. | Xiaojuan Hou Jixin Zhong Changjun Yang Yun Yang Jian He Jiliang Mu Wenping Geng Xiujian Chou | 2022 | Journal of Materiomics2022，8，5： | 1 |
| 7 | Chemical vapor deposition for few‐layer two‐dimensional materials显示文摘Chemical vapor deposition(CVD)approach offers a controllable strategy for preparing large‐area and high‐quality few‐layer(mainly bilayer or trilayer)twisted or untwisted two‐dimensional(2D)materials,and is predicted to boost the development of 2D materials from laboratory research to industrial applications. | Qing Zhang Dechao Geng Wenping Hu | 2023 | SmartMat2023，4，3： | 1 |
| 8 | Near‐Equilibrium Chemical Vapor Deposition of High‐Quality Single‐Crystal Graphene Directly on Various Dielectric Substrates显示文摘 | Jianyi Chen Yunlong Guo Lili Jiang Zhiping Xu Liping Huang Yunzhou Xue Dechao Geng Bin Wu Wenping Hu Gui Yu Yunqi Liu | 2014 | Adv. Mater2014，，9： | 1 |
| 9 | Multi-stage anisotropic etching of two-dimensional heterostructures显示文摘Regarding the reverse process of materials growth,etching has been widely concerned to indirectly probe the growth kinetics,offering an avenue in governing the growth of two-dimensional(2D)materials.In this work,interface-driven anisotropic etching mode is demonstrated for the first time to be generally applied to 2D heterostructures.It is shown that the typical in-plane graphene and hexagonal boron nitride(h-BN)heterostructures follow a multi-stage etching behavior initiated first along the interfacial region between the two materials and then along edges of neighboring h-BN flakes and finally along central edges of hBN.By accurately tuning etching conditions in the chemical vapor deposition process,series of etched 2D heterostructure patterns are controllably produced.Furthermore,scaled formation of graphene and h-BN heterostructures arrays has been realized with full assist of as-proposed etching mechanism,offering a direct top-down method to make 2D orientated heterostructures with order and complexity.Detection of interface-driven multi-staged anisotropic etching mode will shed light on understanding growth mechanism and further expanding wide applications of 2D heterostructures. | Lin Li Jichen Dong Dechao Geng Menghan Li Wei Fu Feng Ding Wenping Hu Hui Ying Yang | 2022 | Nano Research2022，15，6： | 0 |
| 10 | A non-contact flexible pyroelectric sensor for wireless physiological monitoring system显示文摘Recently,human physiological information wireless monitoring in real-time is particularly important in health analysis.As a solution,a non-contact wireless physiological monitoring system based on pyroelectric generator(Py G),whose core part consists of a wireless circuit processing module and a polyvinylidene fluoride(PVDF)film,has been successfully designed.Owing to the temperature change under the stimulation of an external heat source,the output voltage of the Py G self-powered flexible sensor increases with the heat source temperature variation in the range of 295–355 K.Furthermore,based on the natural temperature oscillation between the living body and surrounding environment,the sensor can realize human physiological information assessment,for example,temperature monitoring of the palms,fingers,respiratory heat signals from mouth or nose or non-contact spatial heat mapping recognition of finger movement via sensor array.On this basis,a portable wireless monitoring system was designed by integrating the intelligent sensor with a signal conditioning circuit,data conversion storage module,Bluetooth module,and power module.This system can acquire real-time human oral or nasal breathing signals in the personal mobile app to evaluate the physiological state of individuals.Additionally,the wireless monitoring system can be activated within 10 m,demonstrating the application of Py G sensors in remote data transmission. | Jian HE Sen LI Xiaojuan HOU Yongjun ZHOU Hao LI Min CUI Tao GUO Xiangdong WANG Jiliang MU Wenping GENG Xiujian CHOU | 2022 | Science China(Information Sciences)2022，65，2： | 0 |
| 11 | Erratum to:Multi-stage anisotropic etching of two-dimensional heterostructures显示文摘Erratum to Nano Research 2022,15(6):4909−4915 http://gffzzd3cc09b8251d45dfskcufnqk60qov60wv.ffgz.tsg.suse.edu.cn/10.1007/s12274-022-4193-x The affiliation of the author“Feng Ding”was unfortunately mistakenly marked.This error did not affect any of the content and conclusions from the published paper.In addition,one funding was unfortunately forgotten.This error did not affect any of the content and conclusions from the published paper. | Lin Li Jichen Dong Dechao Geng Menghan Li Wei Fu Feng Ding Wenping Hu Hui Ying Yang | 2022 | Nano Research2022，15，7： | 0 |
| 12 | Wide measurement range and high sensitivity spongy MWCNT/polydimethylsiloxane pressure sensor based on a single-electrode enhanced triboelectric nanogenerator显示文摘Flexible pressure sensors have broad application prospects,such as human motion monitoring and personalized recognition.However,their applicability is limited by complex structures,low output performance,low sensitivity,and narrow measurement range.In this study,we report a single-electrode spongy triboelectric sensor(SSTS)mainly composed of spongy composite multi-walled carbon nanotubes/polydimethylsiloxane(MWCNT/PDMS)film and conductive fabric,which can simultaneously generate contact electrification and electrostatic induction coupling in a single-electrode contact-separation mode.The SSTS combines the triboelectric effect,properties of doping material,and spongy porous structure(soft sugar as a sacrificial template).An SSTS with an MWCNT content of 10 wt%and a porosity of 64%exhibits high sensitivity,a wide measurement range,and excellent linearity.It also displays two sensitivity regions(slopes):1.324 V/kPa from 1.5 to 28 kPa in the low-pressure range and 0.096 V/kPa from 28 to 316.5 kPa in the high-pressure range,with linearities of 0.980 and 0.979,respectively.Furthermore,the SSTS delivers a high-performance output and high stability,thus enhancing the monitoring of hand pressure changes,human movement,personalized spatial recognition,and other detection tasks.This new strategy for human motion monitoring shows great potential in the healthcare fields,sports rehabilitation,and human-computer interactions. | XIE Xin HOU XiaoJuan QIAN Shuo HOU JianWei ZHANG Jie BI XiaoXue GENG WenPing MU JiLiang HE Jian CHOU XiuJian | 2023 | Science China(Technological Sciences)2023，66，6： | 0 |
| 13 | Flexible multilayer MEMS coils and their application in energy harvesters显示文摘Electromagnetic vibration energy harvesters are promising for the power supply of wireless sensor nodes,small electronic devices,and wearable electronics.Conventional electromagnetic harvesters usually increase output by increasing the size of coils and magnets,limiting the improvement of energy conversion efficiency and power density.In this study,multilayer microelectromechanical system(MEMS)coils were prepared using flexible electronics,and their high integration performance in arbitrary space was utilized to greatly improve the utilization of the space magnetic field by the electromagnetic harvester.The core magnet of the generator was magnetically balanced to achieve levitation,which improved the sensitivity and reduced fatigue damage compared with traditional spring structures.The wound coils on the top and bottom of the magnet and the flexible coils on the sides worked together to improve the energy efficiency and output of the devices.The output performance of the device with different number distributions was simulated using mathematical models to obtain the optimal structural parameters.The results show that by introducing flexible multilayer MEMS coils on the side surface of the energy harvester,the open-circuit voltage of the energy generators increased from 7 to 10 V by more than 43%.Flexible multilayer MEMS coils can enhance energy conversion rates and possess compact dimensions,making them suitable for integration onto complex surfaces.After the vibration energy harvesting system testing,the maximum peak power of the harvester was 7.1 m W at an acceleration of1 g and a resonant frequency of 11 Hz with a resistor of 3.5 kΩinternal resistance.Moreover,a 470μF capacitor can be charged to 3.5 V within 10 s to drive a hygrothermograph to work for more than 80 s and can supply a light bulb continuously.This strategy shows the great potential of vibration-energy-driven electromagnetic generators for powering small electronics in limited spaces. | ZHANG Jie HOU XiaoJuan QIAN Shuo BI XiaoXue HU DongXu LIU JianJun GENG WenPing MU JiLiang HE Jian CHOU XiuJian | 2024 | Science China(Technological Sciences)2024，67，4： | 0 |
| 14 | Controlled growth of Mo2C pyramids on liquid Cu surface显示文摘Precise spatial control of 2D materials is the key capability of engineering their optical,electronic,and mechanical properties.However,growth of novel 2D Mo2C on Cu surface by chemical vapor deposition method was revealed to be seed-induced 2D growth,limiting further synthesis of complex Mo2C spatial structures.In this research,we demonstrate the controlled growth of Mo2C pyramids with numerous morphologies,which are characterized with clear terraces within the structures.The whole evolution for Mo2C pyramids in the coursed of CVD process has been detected,posing significant potential in probing growth mechanism.The formation of the Mo2C pyramids arises from the supersaturation-induced nucleation and concentration-gradient driven diffused growth of a new Mo2C layer on the edged areas of intrinsic ones,as supported by STEM imaging.This work provides a novel Mo2C-based pyramid structure and further reveals a sliding growth mechanism,which could offer impetus for the design of new 3D spatial structures of Mo2C and other 2D materials. | Yixuan Fan Le Huang Dechao Geng Wenping Hu | 2020 | Journal of Semiconductors2020，41，8： | 0 |
| 15 | Recent Advances in Growth,Properties and Applications of 2D Inorganic Molecular Crystals显示文摘Comprehensive Summary Since the concept of 2D inorganic molecular crystals(2DIMCs)was introduced,intensive attentions have been gradually devoted to this field.Herein,the very recent advances in growth,properties,and applications of 2D inorganic molecular crystals are comprehensively reviewed.Firstly,the newly emerged 2DIMCs are classified into three categories.Then the two typical production methods are present,thus leading to discrepancy in size,distribution,morphology and structures of 2DIMCs.Moreover,the unique physicochemical properties of 2DIMCs are demonstrated on the basis of the as-obtained 2DIMCs,the various applications are exhibited,demonstrating significant potential in related fields.Finally,the perspective and prospects are outlooked to offer insights in further development of 2DIMCs. | Menghan Li Yang Guo Lin Li Dechao Geng Wenping Hu | 2023 | Chinese Journal of Chemistry2023，41，15： | 0 |
| 16 | High-density stacked microcoils integrated microminiaturized electromagnetic vibration energy harvester for self-powered acceleration sensing显示文摘With the rapid development of microelectronics and flexible electronics technology,self-powered sensors have significant application prospects in human-machine interface systems and Internet of Things.However,piezoelectric-and triboelectricbased sensors have low current output and are easily affected,while electromagnetic-based sensors are difficult to miniaturize.This work proposes a high-density stacked microcoil integrated microminiaturized electromagnetic vibration energy harvester(EVEH).The double-layer high-density microcoil is fabricated on both sides of the flexible polyimide substrate interconnected via the central through-hole.Owing to reduced single coil line width,line spacing,and stacked structure,the number of turns can be substantially enhanced.Moreover,the relative position of the coils and magnet has a considerable influence on the performances;due to the huge change rate in magnetic flux when the coil is placed in the radial direction of the magnet than in the axial direction,the open-circuit voltage in the radial direction is 10 times greater.The microcoil can maintain good performance at high,low temperatures and under bending conditions.When the distance between the ends of the coil changes from 2 to 20 mm in 2 mm steps,the bending angle of the coil changes from 45°to 270°in 45°steps;furthermore,when the coil is exposed to-40and 60℃conditions,the coil resistance is maintained at approximately 447Ω.The peak open-circuit voltage of three-piece microcoils reaches 0.41 V at 4 Hz under 2g,and the output voltage and current increase with an increasing number of stacked layers.These excellent properties indicate that EVEH can be used for self-powered acceleration sensing.The sensitivity is measured to be 0.016 V/(m/s^(2))with a correlation coefficient of 0.979 over the acceleration range of 1–18 m/s^(2).Thus,the developed microminiaturized EVEH has enormous potential for self-powered sensing applications in confined spaces and harsh environments. | HOU XiaoJuan ZHANG RuoYang BI XiaoXue ZHAO HuiPeng ZHANG Jie ZHU Jie GENG WenPing HE Jian CHOU XiuJian | 2023 | Science China(Technological Sciences)2023，66，12： | 0 |
| 17 | A high-power and high-efficiency mini generator for scavenging energy from human foot movement显示文摘Harvesting energy from human movement and converting it into electricity is a promising method to address the issue of sustainable power supply for wearable electronic devices.Using traditional energy harvesters for practical applications is difficult due to their low output power.In this paper,an energy harvester with high power and efficiency is reported based on the principle of electromagnetic induction.It adopts a tiny compound mechanism comprising symmetrical lever-sector gear,which can amplify the vertical displacement of the human heel of 1.44 times without affecting the flexibility and comfort of human movement.The lever-sector gear and gear acceleration mechanism can achieve high output power from the tiny vertical movements of the heel.The results demonstrated that the average power and energy harvesting efficiency of the device are 1 W and 63%,respectively.Moreover,combining a novel controllable electric switch and energy management circuit allows the energy harvester to be worn by individuals with different weights and functions as a continuous real-time power supply for various electronic devices(mobile phones,smartwatches,etc.).Therefore,this research provides a new approach for the highly efficient harvesting of human motion energy and sustainable power supply of wearable electronics. | WU Hui QIAN Shuo HOU XiaoJuan ZHAO JuanHong ZHANG Jie SONG XiaoGuang LIU YanLi SHI ShuZheng GENG WenPing MU JiLiang HE Jian CHOU XiuJian | 2023 | Science China(Technological Sciences)2023，66，12： | 0 |
| 18 | Stretchable and skin-conformal piezo-triboelectric pressure sensor for human joint bending motion monitoring显示文摘Stretchable,skin-conformal,and self-powered wearable pressure sensors have garnered significant attention for use in human joint bending motion monitoring.Here,a piezo-triboelectric pressure sensor(P-TPS)based on triboelectric nanogenerator and piezoelectric nanogenerator is demonstrated.The P-TPS can generate an enhanced electrical output by coupling the dual-mode triboelectrification and piezoelectric effect.The P-TPS shows high sensitivity(voltage=0.3 V/kPa;current=4.3 nA/kPa;pres-sure range=0-200 kPa),high linearity,and good stability.Furthermore,it demonstrates a wide mea-surement range(0-800 kPa),table frequency response,and fast response time.Additionally,all components of the P-TPS are fabricated using flexible and stretchable materials,affording satisfactory stretchability and excellent skin conformality.Owing to their ability to self-power,they can be attached to the outside of joints to monitor human joint bending movements in real time.Hence,this study provides a novel method of using a stretchable and skin-conformal piezo-triboelectric nanogenerator with high electrical performance as a self-powered pressure sensor,which offers significant potential in personalized recognition,medical research,and human machine interface. | Junbin Yu Liang Chen Xiaojuan Hou Jiliang Mu Jian He Wenping Geng Xiaojun Qiao Xiujian Chou | 2022 | Journal of Materiomics2022，8，2： | 0 |
| 19 | Polymer: Non-fullerene acceptor heterojunction-based phototransistor for short-wave infrared photodetection显示文摘It remains full of challenge for extending short-wave infrared(SWIR)spectral response and weak-light detection in the context of broad spectral responses for phototransistor.In this work,a novel poly(2,5-bis(4-hexyldodecyl)-2,5-dihydro-3,6-di-2-thienyl-pyrrolo[3,4-c]pyrrole-1,4-dione-alt-thiophene)(PDPPT3-HDO):COTIC-4F organic bulk-heterojunction is prepared as active layer for bulk heterojunction phototransistors.PDPPT3-HDO serves as a hole transport material,while COTIC-4F enhances the absorption of SWIR light to 1020 nm.As a result,smooth and connected PDPPT3-HDO film is fabricated by blade coating method and exhibits high hole mobility up to 2.34 cm^(2)·V^(-1)·s^(-1) with a current on/off ratio of 4.72×10^(5) in organic thin film transistors.PDPPT3-HDO:COTIC-4F heterojunction phototransistors exhibit high responsivity of 2680 A·W^(-1) to 900 nm and 815 A·W^(-1) to 1020 nm,with fast response time(rise time~20 ms and fall time~100 ms).The photosensitivity of the heterojunction phototransistor improves as the mass ratio of non-fullerene acceptors increases,resulting in an approximately two orders of magnitude enhancement compared to the bare polymer phototransistor.Importantly,the phototransistor exhibits decent responsivity even under ultra-weak light power of 43μW·cm^(-2) to 1020 nm.This work represents a highly effective and general strategy for fabricating efficient and sensitive SWIR light photodetectors. | Jing Li Weigang Zhu Yang Han Yanhou Geng Wenping Hu | 2024 | Nano Research2024，17，4： | 0 |
| 20 | Large electrical strain in lead-free K_(0.5)Na_(0.5)NbO_(3)-based ceramics by heterovalent doping显示文摘Heterovalent doped(K_(0.48-0.07)xNa_(0.52-0.43)xBi_(0.5)x)(Nb_(0.95-0.95x)Sb_(0.05-0.05x)Zrx)O_(3)ceramics were fabricated using conventional solid-state reaction.Then,the phase structures,dielectric,ferroelectric,and electricstrain properties were investigated.The compositions were tuned to be located at polymorphic phase boundary with increasing heterovalent Bi3t and Zr4t doping levels.A large strain of 0.19%was obtained at relatively low electric fields of 30 kV/cm in the composition of x=0.04.The normalized large-signal d33*values were approximately 633 pm/V under a low driving electric field of 30 kV/cm,which were comparable or larger than the values reported for other lead-free families.The large strains obtained can be attributed to the formation of nanodomains and high-density domain walls,which were confirmed by the observations of domain morphology using transmission electron microscopy(TEM)technique.Excellent temperature stability of the strain properties of the x=0.04 sample could be ascribed to the sluggish behaviour for the local structural heterogeneity in heterovalent-ion doped KNN ceramic.Theoretical simulations revealed that the Zr^(4t)produce the local stress at the BO6 octahedra and Bi3t could yield off-centering of AO12 ployhedron due to the nature of Bi 6s lone pair electrons,which induced lattice expansion and local distortions in the sample.The local displacements are strongly anisotropic in heterovalent-ion doped system.It is believed that random local fields exist in these compositions owing to the eixstence of charge distribution.Such heterovalent doping of Bi^(3t)and Zr^(4t)could destory simultaneously the orthorhombic symmetry and the short-range ferroelecctric order,leading to the formation of complex nanodomains and local structral hetergenenity.Heterovalent doping may,therefore,offer a new avenve to design novel K0.5Na0.5NbO3(KNN)-based materials for their mutifunctional applications. | Xiangjian Wang Jun Wang Wenping Geng Guohua Dong Brahim Dkhil Xiaojie Lou | 2023 | Journal of Materiomics2023，9，5： | 0 |
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