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| 1 | Modification strategies on transition metal-based electrocatalysts for efficient water splitting显示文摘Electrocatalytic water splitting driven by electrocatalysts is recognized as a promising strategy to generate clean hydrogen fuel.Searching and constructing high-efficient and low-cost electrocatalysts is vital in the practical applications of electrocatalytic water splitting.Although transition metal-based materials have been considered as promising electrocatalysts,the satisfactory activities are usually not built on the bulk materials,but strongly relying on elaborately designing these electrocatalysts.Herein,the recent theoretical and experimental progress on modification strategies to improve the intrinsic activities is summarized,especially including element doping,phase engineering,structure cooperation,interface engineering,vacancy engineering,strain engineering and self-functionalization.Finally,the future opportunities and challenges on these modification strategies are also proposed.Overall,it is anticipated that these modification strategies offer some new understandings on rationally constructing non-noble electrocatalysts for efficient electrocatalytic water splitting. | Yaotian Yan Pengcheng Wang Jinghuang Lin Jian Cao Junlei Qi | 2021 | Journal of Energy Chemistry2021，30，7： | 4 |
| 2 | Microstructure design of C/C composites through electrochemical corrosion for brazing to Nb显示文摘Surface structure of C/C composites has been regulated through electrochemical corrosion at room temperature to modify the residual stress and improve the joining strength when brazed to Nb.The unique crevice corrosion in C/C composites is investigated to reveal the change of corrosion depth and fiber size.The interlacing zone of carbon fiber reinforced brazing alloy replaces the reaction layer in the original joint.Joining area is increased dramatically and the continuous crack will be hindered.The interlacing zone eliminates the stress concentration and relieves the residual stress through reducing the property mismatch.All advantages contribute to the joining quality of C/C–Nb.Shear strength of C/C–Nb joint with 80μm depth reached 37.7 MPa,which was 1.2 times higher than that of original joint.Surface structure design of C/C composites not only expands the application in structure component,but also exhibits the promising application in energy field. | Jin Ba Xu Ji Bin Wang Peixin Li Jinghuang Lin Jian Cao Junlei Qi | 2022 | Journal of Materials Science & Technology2022，，9： | 2 |
| 3 | Atomic-scale structural and chemical evolution of Li3V2(PO4)3 cathode cycled at high voltage window显示文摘Here,by using atomically resolved scanning transmission electron microscopy and electron energy loss spectroscopy,we investigate the structural and chemical evolution of Li3V2(PO4)3 (LVP) upon the high-voltage window (3.0-4.8 V).We find that the valence of vanadium gradually increases towards the core corresponding to the formation of electrochemically inactive Li3-xV2(PO4)3 (L3-xVP) phases.These Li-deficient phases exhibit structure distortion with superstructure stripes,likely caused by the migration of the vanadium,which can slow down the lithium ion diffusion or even block the diffusion channels.Such kinetic limitations lead to the formation of Li-deficient phase along with capacity loss.Thus,the LVP continuously losses of electrochemical activity and Li-deficient phases gradually grow from the particle core towards the surface during cycling.After 500 cycles,the thickness of active LVP layer decreases to be - 5-20 nm.Moreover,the micromorphology and chemical composition of solid electrolyte interphase (SEI) have been investigated,indicating the thick SEI film also contributes to the capacity loss.The present work reveals the structural and chemical evolution in the cycled electrode materials at an atomic scale,which is essential to understand the voltage fading and capacity decaying of LVP cathode. | Shulin Chen Jian Zou Yuehui Li Ning Li Mei Wu Jinghuang Lin Jingmin Zhang Jian Cao Jicai Feng Xiaobin Niu Jianming Bai Junlei Qi Peng Gao Liping Wang Hong Li | 2019 | Nano Research2019，12，7： | 1 |
| 4 | Mapping of wheat stripe rust resistance gene Yr041133 by BSR-Seq analysis显示文摘Puccinia striiformis Westend. f. sp. tritici(Pst) pathotype CYR34 is widely virulent and prevalent in China.Here, we report identification of a strpie rust resistance(Yr) gene, designated Yr041133, in winter wheat line 041133. This line produced a hypersensitive reaction to CYR34 and conferred resistance to 13 other pathotypes. Resistance to CYR34 in line 041133 was controlled by a single dominant gene. Bulked segregant RNA sequencing(BSR-Seq) was performed on a pair of RNA bulks generated by pooling resistant and susceptible recombinant inbred lines. Yr041133 was mapped to a 1.7 c M genetic interval on the chromosome arm 7 BL that corresponded to a 0.8 Mb physical interval(608.9–609.7 Mb) in the Chinese Spring reference genome. Based on its unique physical location Yr041133 differred from the other Yr genes on this chromosome arm. | Yahui Li Ruiming Lin Jinghuang Hu Xiaohan Shi Dan Qiu Peipei Wu Gebremedhin Habteab Goitom Siqi Wang Hongjun Zhang Li Yang Hongwei Liu Qiuhong Wu Jingzhong Xie Yang Zhou Zhiyong Liu Hongjie Li | 2022 | The Crop Journal2022，10，2： | 1 |
| 5 | Joining SiO_(2)based ceramics:recent progress and perspectives显示文摘Nowadays,SiO_(2)based material is one of the widest used materials in optical,microelectromechanical system,aerospace and some other industries.In practical application,SiO_(2)based materials are required to be joined with themselves or other heterogeneous materials to assemble products with various functions.And the joining quality directly affects the mechanical performances and functional properties of assembled products.Though many researchers studied different joining technologies,explored the microstructure of joining interface and tested after-joining properties,a review that summarizes the recent cutting-edge researches and development tendency of joining technologies for SiO_(2)based ceramics is still absent.Therefore,according to different applications and requirements,this review summarizes the widely used joining technologies and discusses corresponding joining mechanisms,current research progress and suitable applications.Due to the wide applications in specific industry,laser welding,anodic bonding and wafer bonding are discussed in detail.Further,brazing,the widest used method in SiO_(2)joining,has been elaborated deeply in its wetting mechanism,residual stress control,interfacial microstructure and mechanical performance aspects.In the end,this review proposed the future development trends of SiO_(2)ceramics joining,aiming at offering a full-view of potential improvements in SiO_(2)ceramic joining technologies. | Haohan Wang Jinghuang Lin Junlei Qi Jian Cao | 2022 | Journal of Materials Science & Technology2022，，13： | 0 |
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