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1Boosting triplet self-trapped exciton emission in Te(IV)-doped Cs_(2)SnCl_(6) perovskite variants显示文摘Perovskite variants have attracted wide interest because of the lead-free nature and strong self-trapped exciton (STE) emission. Divalent Sn(II) in CsSnX3 perovskites is easily oxidized to tetravalent Sn(IV), and the resulted Cs2SnCl6 vacancy-ordered perovskite variant exhibits poor photoluminescence property although it has a direct band gap. Controllable doping is an effective strategy to regulate the optical properties of Cs2SnX6. Herein, combining the first principles calculation and spectral analysis, we attempted to understand the luminescence mechanism of Te4+-doped Cs2SnCl6 lead-free perovskite variants. The chemical potential and defect formation energy are calculated to confirm theoretically the feasible substitutability of tetravalent Te4+ ions in Cs2SnCl6 lattices for the Sn-site. Through analysis of the absorption, emission/excitation, and time-resolved photoluminescence (PL) spectroscopy, the intense green-yellow emission in Te4+:Cs2SnCl6 was considered to originate from the triplet Te(IV) ion 3P1→1S0 STE recombination. Temperature-dependent PL spectra demonstrated the strong electron-phonon coupling that inducing an evident lattice distortion to produce STEs. We further calculated the electronic band structure and molecular orbital levels to reveal the underlying photophysical process. These results will shed light on the doping modulated luminescence properties in stable lead-free Cs2MX6 vacancy-ordered perovskite variants and be helpful to understand the optical properties and physical processes of doped perovskite variants.Ruosheng Zeng Kun Bai Qilin Wei Tong Chang Jun Yan Bao Ke Jialuo Huang Liushun Wang Weichang Zhou Sheng Cao Jialong Zhao Bingsuo Zou 2021Nano Research2021,14,5:4
2Polymorphisms of DNA repair gene XRCC1 and hepatocellular carcinoma risk among East Asians: a meta-analysis显示文摘Jie Li Zhenzhen Li Liushun Feng Wenzhi Guo Shuijun Zhang 2013Tumor Biology2013,,1:1
3Norcantharidin enhances ABT-737-induced apoptosis in hepatocellular carcinoma cells by transcriptional repression of Mcl-1显示文摘Shuijun Zhang Gongquan Li Xiuxian Ma Yu Wang Guangzhi Liu Liushun Feng Yongfu Zhao Gong Zhang Yang Wu Xuexiang Ye Baoming Qin Jianfeng Lu 2012Cellular Signalling2012,,9:1
4Gauze:enabling communication-friendly block synchronization with cuckoo filter显示文摘Block synchronization is an essential component of blockchain systems.Traditionally,blockchain systems tend to send all the transactions from one node to another for synchronization.However,such a method may lead to an extremely high network bandwidth overhead and significant transmission latency.It is crucial to speed up such a block synchronization process and save bandwidth consumption.A feasible solution is to reduce the amount of data transmission in the block synchronization process between any pair of peers.However,existing methods based on the Bloom filter or its variants still suffer from multiple roundtrips of communications and significant synchronization delay.In this paper,we propose a novel protocol named Gauze for fast block synchronization.It utilizes the Cuckoo filter(CF)to discern the transactions in the receiver’s mempool and the block to verify,providing an efficient solution to the problem of set reconciliation in the P2P(Peer-to-Peer Network)network.By up to two rounds of exchanging and querying the CFs,the sending node can acknowledge whether the transactions in a block are contained by the receiver’s mempool or not.Based on this message,the sender only needs to transfer the missed transactions to the receiver,which speeds up the block synchronization and saves precious bandwidth resources.The evaluation results show that Gauze outperforms existing methods in terms of the average processing latency(about lower than Graphene)and the total synchronization space cost(about lower than Compact Blocks)in different scenarios.Xiaoqiang DING Liushun ZHAO Lailong LUO Junjie XIE Deke GUO Jinxi LI 2023Frontiers of Computer Science2023,17,3:0
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