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| 1 | Characterization of particulate products for aging of ethylbenzene secondary organic aerosol in the presence of ammonium sulfate seed aerosol显示文摘Aging of secondary organic aerosol(SOA) particles formed from OH– initiated oxidation of ethylbenzene in the presence of high mass(100–300 μg/m^3) concentrations of(NH_4)_2SO_4seed aerosol was investigated in a home-made smog chamber in this study.The chemical composition of aged ethylbenzene SOA particles was measured using an aerosol laser time-of-flight mass spectrometer(ALTOFMS) coupled with a Fuzzy C-Means(FCM) clustering algorithm.Experimental results showed that nitrophenol,ethyl-nitrophenol,2,4-dinitrophenol,methyl glyoxylic acid,5-ethyl-6-oxo-2,4-hexadienoic acid,2-ethyl-2,4-hexadiendioic acid,2,3-dihydroxy-5-ethyl-6-oxo-4-hexenoic acid,1H-imidazole,hydrated N-glyoxal substituted1H-imidazole,hydrated glyoxal dimer substituted imidazole,1H-imidazole-2-carbaldehyde,N-glyoxal substituted hydrated 1H-imidazole-2-carbaldehyde and high-molecular-weight(HMW) components were the predominant products in the aged particles.Compared to the previous aromatic SOA aging studies,imidazole compounds,which can absorb solar radiation effectively,were newly detected in aged ethylbenzene SOA in the presence of high concentrations of(NH_4)_2SO_4seed aerosol.These findings provide new information for discussing aromatic SOA aging mechanisms. | Mingqiang Huang Jiahui Zhang Shunyou Cai Yingmin Liao Weixiong Zhao Changjin Hu Xuejun Gu Li Fang Weijun Zhang | 2016 | Journal of Environmental Sciences2016，28，9： | 6 |
| 2 | A space power system of free piston Stirling generator based on potassium heat pipe显示文摘The power system of a free piston Stirling generator(FPSG)based on potassium heat pipes has been developed in this paper.Thanks to the advantages of long life,high reliability,and high overall thermal efficiency,the FPSG is a promising candidate for nuclear energy,especially in space exploration.In this paper,the recent progress of FPSG based on nuclear reactor for space use was briefly reviewed.A novel FPSG weighted only 4.2 kg was designed,and one dimensional thermodynamic modeling of the FPSG using Sage software was performed to estimate its performance.The experiment results indicated that this FPSG could provide 142.4 W at a thermal-to-electric efficiency of nearly 17.4%.Besides,the power system integrated with four FPSGs and potassium heat pipes was performed and the single machine failure test was conducted.The results show that this system could provide an electrical power of 300 W at an overall thermal efficiency of 7.3%.Thus,it is concluded that this power system is feasible and will have a great prospect for future applications. | Mingqiang LIN Jian MOU Chunyun CHI Guotong HONG Panhe GE Gu HU | 2020 | Frontiers in Energy2020，14，1： | 5 |
| 3 | Size distribution and chemical composition of secondary organic aerosol formed from Cl-initiated oxidation of toluene显示文摘Secondary organic aerosol (SOA) formed from Cl-initiated oxidation of toluene was investigated in a home-made smog chamber. The size distribution and chemical composition of SOA particles were measured using aerodynamic particle sizer spectrometer and the aerosol laser time-of-flight mass spectrometer (ALTOFMS), respectively. According to a large number of single aerosol diameter and mass spectra, the size distribution and chemical composition of SOA were obtained statistically. Experimental results showed that SOA particles created by Cl-initiated oxidation of toluene is predominantly in the form of fine particles, which have diameters less than 2.5 μm (i.e., PM2.5), and glyoxal, benzaldehyde, benzyl alcohol, benzoquinone, benzoic acid, benzyl hydroperoxide and benzyl methyl nitrate are the major products components in the SOA. The possible reaction mechanisms leading to these products are also proposed. | Mingqiang Huang Weijun Zhang Xuejun Gu Changjin Hu Weixiong Zhao Zhenya Wang Li Fang | 2012 | Journal of Environmental Sciences2012，24，5： | 3 |
| 4 | Phase transferring luminescent gold nanoclusters via single-stranded DNA显示文摘Atomically precise gold nanoclusters(Au NCs) are an emerging class of quantum-sized nanomaterials with discrete electronic energy levels, which has led to a range of attractive electronic and optical applications. Nevertheless, the lack of general methods to transfer Au NCs protected with hydrophobic ligands to an aqueous solution hampers their use in physiological settings. Here,we developed a single-stranded DNA-based approach that could transfer ~90% hydrophobic Au NCs into an aqueous solution.We experimentally and theoretically established that multivalent electrostatic and hydrophobic interactions between DNA strands and the hydrophobic ligand layer on Au NCs resulted in monodispersed DNA-coated Au NCs with high physical integrity in an aqueous solution. The fluorescence quantum yield of Au NCs was increased by ~13 fold, and surface-constrained DNA retained the specific recognition ability for biosensing. We further demonstrated the versatility of this phase-transfer approach, which thus holds great potential to advance biological and medical applications of Au NCs. | Yu Li Hui Lu Zhibei Qu Mingqiang Li Haoran Zheng Peilin Gu Jiye Shi Jiang Li Qian Li Lihua Wang Jing Chen Chunhai Fan Jianlei Shen | 2022 | Science China Chemistry2022，65，6： | 1 |
| 5 | Characterization of secondary organic aerosol particles using aerosol laser time-of-flight mass spectrometer coupled with FCM clustering algorithm显示文摘 | Mingqiang Huang Liqing Hao Xiaoyong Guo Changjin Hu Xuejun Gu Weixiong Zhao Zhenya Wang Li Fang Weijun Zhang | 2013 | Atmospheric Environment2013，，： | 1 |
| 6 | Layer Hall effect induced by hidden Berry curvature in antiferromagnetic insulators显示文摘The layer Hall effect describes electrons spontaneously deflected to opposite sides at different layers,which has been experimentally reported in the MnBi_(2)Te_(4) thin films under perpendicular electric fields.Here,we reveal a universal origin of the layer Hall effect in terms of the so-called hidden Berry curvature,as well as material design principles.Hence,it gives rise to zero Berry curvature in momentum space but non-zero layer-locked hidden Berry curvature in real space.We show that,compared to that of a trivial insulator,the layer Hall effect is significantly enhanced in antiferromagnetic topological insulators.Our universal picture provides a paradigm for revealing the hidden physics as a result of the interplay between the global and local symmetries,and can be generalized in various scenarios. | Rui Chen Hai-Peng Sun Mingqiang Gu Chun-Bo Hua Qihang Liu Hai-Zhou Lu X.C.Xie | 2024 | National Science Review2024，11，2： | 0 |
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