| 9 | Current Progress and Future Perspectives of Electrolytes for Rechargeable Aluminum-Ion Batteries显示文摘Aluminum-ion batteries(AIBs)with Al metal anode are attracting increasing research interest on account of their high safety,low cost,large volumetric energy density(≈8046 mA h cm−3),and environmental friendliness.Specifically,the reversible Al electrostripping/deposition is achieved with the rapid development of room temperature ionic liquids,and rapid progress has been made in fabricating high-performance and durable AIBs during the past decade.This review provides an integrated comprehension of the evolution of AIBs and highlights the development of various non-aqueous and aqueous electrolytes including high-temperature molten salts,room temperature ionic liquids,and gel–polymer electrolytes.The critical issues on the interplay of electrolytes are outlined in terms of the voltage window span,the effective ion species during charge storage(Al 3+or Al x Cl?y)and their underlying charge transfer(e.g.,interfacial transfer and diffusion),and the solid electrolyte interface formation and its role.Following the critical insight,future perspectives on how to practically design feasible AIBs are given. | Dongwei Ma Du Yuan Carlos Ponce de Leon Zheng Jiang Xin Xia Jiahong Pan | 2023 | Energy & Environmental Materials2023，6，1： | 0 |
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