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| 1 | Boosting multi-hole water oxidation catalysis on hematite photoanodes under low bias显示文摘The accumulation of multiple surface holes is considered to be the key to efficient photoelectrochemical(PEC)water oxidation.Previous PEC water oxidation studies commonly apply high potentials(>1.2 VRHE)to achieve this key.But how to complete multi-hole transfer under low bias(<1.2 VRHE)remains unknown.Herein,we find that,on a typical visible-light photoanode,hematite(α-Fe_(2)O_(3)),UV excitation plays a indispensable role in driving multi-hole water oxidation under low bias.Compared with the visible-light excitation,the UV excitation promotes the formation of adjacent surface-trapped holes onα-Fe_(2)O_(3) at 0.9VRHE,thereby increasing the reaction order of surface holes from~1 to~2 and improving the PEC water oxidation activity by one order of magnitude.The UV irradiation reduces the formation probability of self-trapped excitons and results in~3 to 5-fold increase of surface holes.These advantages enable the UV excitation to contribute about 40%to the total photocurrent under 1 solar illumination,even though its energy only occupies 6%of the incident light.This mechanism is also applicable to boost selective two-hole oxidation of thioether at 0.1 VFc/Fc+and nitrite at 0.9 VRHE. | Lei Wu Daojian Tang Jing Xue Shuobo Wang Hongwei Ji Chuncheng Chen Yuchao Zhang Jincai Zhao | 2023 | Science China Chemistry2023，66，3： | 2 |
| 2 | Prospects for microbial biodiesel production显示文摘 | SHI Shuobo SIEWERS V N/ELSEN J | 2011 | Biotechnology Journal2011，6，3： | 1 |
| 3 | The Role of Dihydroresveratrol in Enhancing the Synergistic Effect of Ligilactobacillus salivarius Liol and Resveratrol in Ameliorating Colitis in Mice显示文摘Currently approved therapeutical strategies for inflammatory bowel diseases(IBD)suffer from variable efficacy and association with risk of serious side effects.Therefore,efforts have been made in searching for alternative therapeutics strategies utilizing gut microbiota manipulation.In this study,we show that the probiotic strain Ligilactobacillus salivarius Li01(Li01)and the phytochemical prebiotic resveratrol(RSV)have synergistic effect in ameliorating colitis in mice.Oral coadministration of Li01(109 CFU/d)and RSV(1.5 g/kg/d)promoted restoration of various inflammatory injuries and gut microbiota composition,exhibiting a favorable anti-inflammatory effect in DSS-induced colitis mice.The combination treatment was associated with reductions in the levels of proinflammatory cytokines IL-1βand IL-6 and increases in the levels of the anti-inflammatory cytokine IL-17A in mouse serum.Moreover,the combination treatment was found to alter the composition and metabolism of the gut microbiota,especially influencing the production of short chain fatty acids and anti-inflammatory related molecules.The mechanism underlying the improved anti-inflammatory effect from the RSV and Li01 combination treatment was found to be associated with the environmental sensor mammalian aryl hydrocarbon receptor(AHR)and tryptophan metabolism pathway.Administration of RSV in combination with Li01 in different mouse model led to enhanced conversion of RSV into metabolites,including dihydroresveratrol(DHR),resveratrol-sulfate,and resveratrol-glucuronide.DHR was found to be the dominant metabolite of RSV in conventional and colitis mice.An increased DHR/RSV ratio was confirmed to activate AHR and contribute to an enhanced anti-inflammatory effect.DHR is considered as a potential AHR ligand.The DHR/RSV ratio also affected the serotonin pathway by controlling the expression of Tph1,SERT,and 5-HT7R leading to amelioration of colitis in mice.Our data suggest that treatment with a combination of Li01 and RSV has potential as a therapeutic strategy for IBD;further investigation of this combination in clinical settings is warranted. | Yiqiu Fei Shuobo Zhang Shengyi Han Bo Qiu Yanmeng Lu Weixing Huang Fang Li Deying Chen Bjorn Berglund Hang Xiao Lanjuan Li Mingfei Yao | 2022 | Research2022，，4： | 1 |
| 4 | Functional expression and characterization of five wax ester synthases in Saccharomyces cerevisiae and their utility for biodiesel production 显示文摘 | Shuobo Shi Juan Octavio Valle Rodríguez | 2012 | Biotechnology for Biofuels2012，，5： | 1 |
| 5 | The Merrifield-Simmons index in (n,n + 1)-graphs显示文摘 | Deng Hanyuan Chen Shuobo Zhang Jie | | 0，，01： | 1 |
| 6 | Recent advances in 2D semiconductor nanomaterials for photocatalytic CO_(2)reduction显示文摘For decades,global warming and energy shortages have been two urgent problems in human society.The solar-driven photocatalytic conversion of carbon dioxide(CO_(2))into hydrocarbon fuels is expected to become a technology to solve these problems.Two-dimensional(2D)materials shine in the field of photocatalytic CO_(2)due to their layered structure,larger specific surface area,more active sites,and larger charge transfer efficiency.This article reviews the progress of CO_(2)reduction by several types of 2D materials in recent years.Generally,the reduction of CO_(2)is difficult in terms of kinetics and thermodynamics,but it is found through theoretical calculations and experiments that 2D materials have certain advantages in the reduction of CO_(2).Then the preparation methods of 2D materials are summarized and a variety of 2D materials are discussed and classified.Finally,an outlook on the development trend of 2D materials is made.This review aims to provide systematic and concise guidance for the design of 2D nanomaterials for photocatalytic CO_(2)reduction. | Tong Li Hongwei Huang Shuobo Wang Yan Mi Yihe Zhang | 2023 | Nano Research2023，16，7： | 0 |
| 7 | Opportunities of CO_(2)-based biorefineries for production of fuels and chemicals显示文摘Biorefinery production of fuels and chemicals represents an attractive route for solving current energy crisis,as well as reducing green-house gas(GHG)emissions from ships,planes,and long-haul trucks.The current biorefinery industry is under transition from the use of food(1G,1st generation),to the use of biomass(2G,2nd generation).Moreover,the use of atmospheric CO_(2)(3G,3rd generation)has caught increased attention as the possible next-generation biorefinery.Here we discuss how microorganisms can be engineered for CO_(2)-based biorefineries to produce fuels and chemicals.We start through reviewing different metabolic pathways that can be recruited for CO_(2)fixation,followed by different opportunities for CO_(2)fixation,either through co-consumption with sugars or used as the sole carbon source.Key challenges and future research directions for advancing 3rd-generation biorefineries are also be discussed. | Zihe Liu Shuobo Shi Yuchao Ji Kai Wang Tianwei Tan Jens Nielsen | 2023 | Green Carbon2023，1，1： | 0 |
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