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| 1 | Thiolactone copolymer donor gifts organic solar cells a 16.72% efficiency显示文摘Since 1995,bulk-heterojunction organic solar cells consisting of one or two organic donors and one or two organic acceptors have been fighting for high power conversion efficiencies(PCEs)and good stability[1].Until recent years,this next-generation photovoltaic technology starts to offer decent PCEs,shedding the light on commercialization,and attracting great attention again[2-14].Compared w让h the continuously emerging highperformance nonfullerene acceptors,high-performance donors are rare. | Ji Xiong Ke Jin Yufan Jiang Jianqiang Qin Tan Wang Jinfeng Liu Qishi Liu Haili Peng Xiongfeng Li Anxin Sun Xianyi Meng Lixiu Zhang Ling Liu Wenting Li Zhimin Fang Xue Jia Zuo Xiao Yaqing Feng Xiaotao Zhang Kuan Sun Shangfeng Yang Shengwei Shi Liming Ding | 2019 | Science Bulletin2019，64，21： | 17 |
| 2 | Phosphorite generative processes around the Precambrian-Cambrian boundary in South China: An integrated study of Mo and phosphate O isotopic compositions显示文摘Large phosphorite deposits in Central Guizhou,China,were formed around the Precambrian/Cambrian boundary(PC/C),including the Ediacaran(Doushantuo stage)and early Cambrian(Gezhongwu stage).Among them,Gezhongwu phosphorite from Zhijin are enriched in rare earth elements(REE)plus yttrium(REY),reaching 3.503 million tons.Although phosphorites have attracted great attention,the specific sources P and REY remained unclear.To determine the P and REY sources and establish a phosphogenic model of PC/C phosphorite,we present an integrated dataset of Mo and phosphate O isotopes for the first time,along with carbonate C and O isotopes,geology,petrology,and geochemistry.In all samples,d18Op,Y/Ho,and Zr/Hf decreased from the Ediacaran to the early Cambrian,indicating increased terrigenous weathering fluxes while decreased upwelling water input.Furthermore,terrigenous weathering delivery significantly elevated marine REY concentrations in the Cambrian in Zhijin.The Ceanom and d98/95Mo suggest that seawater was oxidized in the later Ediacaran and became entirely oxic in the early Cambrian.The positive feedback between oxygen levels in atmosphere and primary productivity caused progressive oxygenation in ocean-atmosphere system and enable phosphorites to be formed by different mechanisms.Results show that the Lower Doushantuo consist of abiotic intraclasts and exhibited“seawaterlike”REY types,indicating abiological and mechanical reworking phosphogenesis.The Upper Doushantuo and Gezhongwu Formation contained mainly microbial debris and abiogenic intraclasts,and exhibit “hat-shaped”REY plots,suggesting microbially mediated phosphogenesis.Based on this data set,we developed a phosphogenic model illustrating formation of these two phosphorite deposits,wherein the Lower Doushantuo phosphorite formed through the reworking of pre-existing phosphatic sediments in anoxic and abiotic ocean,whereas the Upper Doushantuo and Gezhongwu phosphorite formed via microbial metabolisms in oxic and biotic conditions.Our study has implications on the PC/C phosphorite generative processes,as well as paleoenvironmental conditions. | Haiying Yang Jiafei Xiao Yong Xia Zhuojun Xie Qinping Tan Jianbin Xu Shan He Shengwei Wu Xiqiang Liu Xingxiang Gong | 2021 | Geoscience Frontiers2021，12，5： | 5 |
| 3 | Amperometric hydrogen peroxide biosensor based on horseradish peroxidase immobilized on Fe3O4/chitosan modifiedGlassy carbon electrode显示文摘 | Tan Xuecai Zhang Jinlei Tan Shengwei | 2009 | Electroanalysis2009，21，13： | 1 |
| 4 | Spatiotemporal Changes in NDVI and Its Driving Factors in the Kherlen River Basin显示文摘Vegetation is an important factor linking the atmosphere,water,soil,and biological functions,and it plays a specific role in the climate change response and sustainable development of regional economies.However,little information is available on vegetation vulnerability and its driving mechanism.Therefore,studying temporal and spatial change characteristics of vegetation and their corresponding mechanisms is important for assessing ecosystem stability and formulating ecological policies in the Kherlen River Basin.We used Moderate-resolution Imaging Spectroradiometer(MODIS)normalized difference vegetation index(NDVI)remote sensing images from 2000 to 2020 to analyse temporal changes in NDVI with the autoregressive moving average model(ARMA)and the breaks for additive season trend(BFAST)in the basin and to assess natural,anthropogenic and topographic factors with the Geodetector model.The results show that:1)the long NDVI time series remained stable in the Kherlen River Basin from 2000 to 2020,with a certain significant mutation period from 2013 to 2017;2)the coefficient of variation(CV)in the analysis of the spatial NDVI was generally constant,mainly at the level of 0.01–0.07,and the spatial NDVI change was minimally impacted by external interference;and 3)temperature and precipitation are the key factors affecting the NDVI in the basin,and changes in local hydrothermal conditions directly affect the local NDVI.The results of this study could provide a scientific basis for the effective protection of the ecological environment and will aid in understanding the influence of vegetation change mechanisms and the corresponding factors. | MUHAMMAD Naveed HE Hongshi ZONG Shengwei DU Haibo SATTI Zulqarnain TAN Xinyuan QAZI Muhammad Yasir | 2023 | Chinese Geographical Science2023，33，2： | 1 |
| 5 | Synthesis of zinc oxide nanotetrapods by a novel fast microemulsionbased hydrothermal method显示文摘 | Jiang Junying Li Yanfen Tan Shengwei | | 0，，： | 1 |
| 6 | Enrichment characteristics and sources of the critical metal yttrium in Zhijin rare earth-containing phosphorites, Guizhou Province, China显示文摘Yttrium(Y)is a critical metallic element that is used widely in modern scientific,technological,and industrial applications.Phosphorites in the Zhijin area of Guizhou Province,China,are famous for Y enrichment,but the enrichment characteristics and sources remain unclear.Previous studies suggested that the sources of rare earth elements(REEs,La-Lu)and Y(REYs,La-Lu+Y)were related to hydrothermal deposition.However,this study presents evidence refuting that hypothesis,with major and trace elemental data collected with quadrupoleinductively coupled plasma-mass spectrometry(Q-ICPMS)analysis.These data show that Y in Zhijin REYscontaining phosphorites has a normal distribution and is particularly enriched relative to other REYs.The Y enrichment degree is different at different∑REY intervals.Specifically,the Y enrichment degree is higher at lower∑REY values and lower at higher∑REY values.The REYs-containing phosphorites show features of primary phosphorites.Both REEs and Y have good correlations with P2 O5 in the phosphorites with low REYs contents(total REYs<535 ppm),whereas at high REYs contents(total REYs>535 ppm),REEs have a good correlation with P2 O5 but Y does not.Inconsistent enrichment processes of REYs are suggestive of complex sources of Y.Thus,seafloor hydrothermal fluids were not the direct source of Y.Normal seawater mixed with terrestrial sources might have contributed to the origin of Y here.This study could lead to improvements in Y mineral resource explorations and the situation involving the global REYs supply crisis. | Xingxiang Gong Shengwei Wu Yong Xia Zhengwei Zhang Shan He Zhuojun Xie Jiafei Xiao Haiying Yang Qingping Tan Yi Huang Yuhong Yang | 2021 | Acta Geochimica2021，40，3： | 1 |
| 7 | Ultrasound-assisted extraction of bound phenolic compounds from the residue of Apocynum venetum tea and their antioxidant activities显示文摘Bound phenolic compounds from the residue of Apocynum venetum(A.venetum)tea were released by alkaline digestion with sonication,followed by extraction using ethyl acetate(EtOAc).The fragment ions of compounds in free and bound forms were identified by liquid chromatography electrospray ionization tandem mass spectrometry(LC-ESI-MS/MS)in both positive and negative modes.Further investigation of chemical constituents in the EtOAc extract led to the isolation of eleven individual compounds,and their chemical structures were identified as(−)-epicatechin(1),(−)-loliolide(2),(−)-syringaresinol-4-O-β-D-glucopyranoside(3),alloside of benzyl alcohol(4),3-[(6-O-hexopyranosylhexopyranosyl)oxy]-2-(palmitoyloxy)propyl(9Z,12Z,15Z)-9,12,15-octadecatrienoate(5),apocynoside I(6),quercetin-3-O-β-D-glucopyranoside(7),kaempferol-3-O-β-D-glucopyranoside(8),[1-acetyloxy-3-[3,4,5-trihydroxy-6-[[3,4,5-trihydroxy-6-(hydroxymethyl)oxan-2-yl]oxymethyl]oxan-2-yl]oxypropan-2-yl]hexadecanoate(9),1-stearoyl-2-palmitoyl-sn-glycerol(10),and 3-hexene-l-O-β-D-glucoside(11)using a series of spectroscopic methods.Compounds 2–5 and 9–11 were isolated for the first time from A.venetum,while antioxidant experiments showed that compounds 1,7,and 8 displayed strong DPPH and ABTS+radical scavenging activities.This study represents the first investigation of bound phenolic compounds with potential health benefits in the residue of A.venetum tea. | Shengwei Sun Yiwen Zhao Luyao Wang Yuzhi Tan Yaning Shi Rita-Cindy Aye-Ayire Sedjoah Yuting Shao Longxiang Li Mengxi Wang Jiashuai Wan Xia Fan Rong Guo Zhihong Xin | 2022 | Food Bioscience2022，47，3： | 0 |
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