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| 1 | Achieving over 16% efficiency for single-junction organic solar cells显示文摘To achieve high photovoltaic performance of bulk hetero-junction organic solar cells(OSCs), a range of critical factors including absorption profiles, energy level alignment, charge carrier mobility and miscibility of donor and acceptor materials should be carefully considered. For electron-donating materials, the deep highest occupied molecular orbital(HOMO) energy level that is beneficial for high open-circuit voltage is much appreciated. However, a new issue in charge transfer emerges when matching such a donor with an acceptor that has a shallower HOMO energy level. More to this point, the chemical strategies used to enhance the absorption coefficient of acceptors may lead to increased molecular crystallinity, and thus result in less controllable phase-separation of photoactive layer. Therefore, to realize balanced photovoltaic parameters, the donor-acceptor combinations should simultaneously address the absorption spectra, energy levels, and film morphologies. Here, we selected two non-fullerene acceptors, namely BTPT-4F and BTPTT-4F, to match with a wide-bandgap polymer donor P2F-EHp consisting of an imidefunctionalized benzotriazole moiety, as these materials presented complementary absorption and well-matched energy levels. By delicately optimizing the blend film morphology, we demonstrated an unprecedented power conversion efficiency of over 16% for the device based on P2F-EHp:BTPTT-4F, suggesting the great promise of materials matching toward high-performance OSCs. | Baobing Fan Difei Zhang Meijing Li Wenkai Zhong Zhaomiyi Zeng Lei Ying Fei Huang Yong Cao | 2019 | Science China Chemistry2019，62，6： | 38 |
| 2 | The Genome of Medicinal Plant Macleaya cordata Provides New Insights into Benzylisoquinoline Alkaloids Metabolism显示文摘在动物农业和药的抗菌素的 overuse 引起了一系列潜在的威胁到公共健康。Macleaya cordata 是从 Papaveraceae 家庭的药用的植物种,提供为抗菌剂的制造的一个安全资源为家畜喂添加剂。从 M. 的活跃成分 ? cordata 被知道包括 benzylisoquinoline 碱(偏爱) 象 sanguinarine (圣) 和 chelerythrine (CHE ) 那样的 ?,而是他们的新陈代谢的小径还得在这非模型植物被学习。在 M. 的圣和 CHE 的活跃生合成 ? cordata 被喂 13标记 C 的酷氨酸。为了增加,推进卓见,我们 de novo 定序 M 的整个染色体。cordata,第一从 Papaveraceae 家庭被定序。M.? 盖住 378 Mb 的 cordata 染色体与 43.5%being 编码 22,328 预言的编码蛋白质的基因 transposable 元素。作为基础 eudicot 的一个成员, M.? cordata 染色体缺乏 ? 发生在几乎所有 eudicots 的 paleohexaploidy 事件。从 genomics 数据, 16 的一个完全的集合 ? 新陈代谢 ? 为圣和 CHE 生合成的基因被检索,并且 14 项他们的生物化学的活动被验证。这些 genomics 和新陈代谢的数据在 M. 显示出保存 BIA 新陈代谢的小径 ? cordata 并且由庄稼改进或微生物引起的小径重建为圣和 CHE 的未来生产提供知识基础。 | Xiubin Liu Yisong Liu Peng Huang Yongshuo Ma Zhixing Qing Qi Tang Huifen Cao Pi Cheng Yajie Zheng Zejun Yuan Yuan Zhou Jinfeng Liu Zhaoshan Tang Yixiu Zhuo Yancong Zhang Linlan Yu Jialu Huang Peng Yang Qiong Peng dinbo Zhang Wenkai Jiang Zhonghua Zhang Kui Lin Dae-Kyun Ro Xiaoya Chen Xingyao Xiong Yi Shang Sanwen Huang Jianguo Zeng | 2017 | Molecular Plant2017，10，7： | 19 |
| 3 | An Outlook on Promoting Healthy Development of Renewable Energy显示文摘Importance of developing alternative energy● We shall take alternative energy as a foreseeable,strategic and long-range issue, and pay great attention to it from the angle of national strategy. | Zhao Xizheng: President, China Electricity Council Shi Dinghuan: Counselor, State Council, and Chairman, Chinese Renewable Energy Association Wang Zhongying: Director, Center for Renewable Energy Development, Energy Research Institute, National Development and Reform Commission Zha Aijun: Consultant, Economic Construction Department, Ministry of Finance Xu Haoxun: Global Director Partner, McKinsey & Company Zhang Wenkai | 2008 | Electricity2008，19，4： | 15 |
| 4 | Analysis of the Effects of Slope Geometry on the Dynamic Response of a Near-field Mountain from the Wenchuan Earthquake显示文摘Fourier spectra and acceleration response spectra of near-field acceleration records of the 2008 Wenchuan Earthquake have been calculated.Relative fundamental frequencies(or predominant periods) were characterized.Then,the natural frequencies of a range of slopes with different geometric characteristics,such as height,slope ratio,and pattern,were analyzed.The seismic responses of the slopes were compared,and the variability of seismic response with the above geometric elements was found.Results show that if slope height increases,and provided that other conditions are unchanged,the natural frequency of the first mode of a doublesurface slope will change as a power law.However,natural frequencies will diminish(based on a parabolic function) as the slope angle becomes large.Both the surface pattern and the number of surfaces on a slope can have a great impact on the seismic response of the slope.Moreover,within a certain range of slope heights or angles,either height or angle will also greatly influence the variability of the seismic response.The results of this research will be helpful to understanding seismic dynamic response features and explaining the ways that slope stability can be affected by earthquakes. | XIAO Shiguo FENG Wenkai ZHANG Jianjing | 2010 | Journal of Mountain Science2010，7，4： | 7 |
| 5 | Association between arterial stiffness and risk of coronary artery disease in a community-based population显示文摘 | Zhang Yun Ye Ping Luo Leiming Bai Yongyi Xu Ruyi Xiao Wenkai Liu Dejun Wu Hongmei | 2014 | Chinese Medical Journal2014，，22： | 3 |
| 6 | Growth mechanism of palladium clusters on rutile TiO_2 (110) surface显示文摘Oxide-supported transition metal systems have been the subject of enormous interest due to the improvement of catalytic properties relative to the separate metal.Thus in this paper,we embark on a systematic study for Pd n (n=1-5) clusters adsorbed on TiO2 (110) surface based on DFT-GGA calculations utilizing periodic supercell models.A single Pd adatom on the defect-free surface prefers to adsorb at a hollow site bridging a protruded oxygen and a five-fold titanium atom along the [110] direction,while Pd dimer is located on the channels with the Pd-Pd bond parallel to the surface.According to the transition states (TSs) search,the adsorbed Pd trimer tends to triangular growth mode,rather than linear mode,while the Pd4 and Pd5 clusters prefer three-dimensional (3D) models.However,the oxygen vacancy has almost no influence on the promotion of Pd n cluster nucleation.Additionally,of particular significance is that the Pd-TiO2 interaction is the main driving force at the beginning of Pd nucleation,whereas the Pd-Pd interaction gets down to control the growth process of Pd cluster as the cluster gets larger.It is hoped that our theoretical study would shed light on further designing high-performance TiO2 supported Pd-based catalysts. | Weina Zhao Huaxiang Lin Yi Li Yongfan Zhang Xin Huang Wenkai Chen | 2012 | Journal of Natural Gas Chemistry2012，21，5： | 3 |
| 7 | Large Room-Temperature Magnetoresistance in van der Waals Ferromagnet/Semiconductor Junctions显示文摘A magnetic tunnel junction(MTJ)is the core component in memory technologies,such as the magnetic random-access memory,magnetic sensors and programmable logic devices.In particular,MTJs based on twodimensional van der Waals(vd W)heterostructures offer unprecedented opportunities for low power consumption and miniaturization of spintronic devices.However,their operation at room temperature remains a challenge.Here,we report a large tunnel magnetoresistance(TMR)of up to 85%at room temperature(T=300 K)in vdW MTJs based on a thin(<10 nm)semiconductor spacer WSe_(2)layer embedded between two Fe_(3)GaTe_(2e)lectrodes with intrinsic above-room-temperature ferromagnetism.The TMR in the MTJ increases with decreasing temperature up to 164%at T=10 K.The demonstration of TMR in ultra-thin MTJs at room temperature opens a realistic and promising route for next-generation spintronic applications beyond the current state of the art. | Wenkai Zhu Shihong Xie Hailong Lin Gaojie Zhang Hao Wu Tiangui Hu Ziao Wang Xiaomin Zhang Jiahan Xu Yujing Wang Yuanhui Zheng Faguang Yan Jing Zhang Lixia Zhao Amalia Patanè Jia Zhang Haixin Chang Kaiyou Wang | 2022 | Chinese Physics Letters2022，39，12： | 2 |
| 8 | The chromosome-level reference genome of Coptis chinensis provides insights into genomic evolution and berberine biosynthesis显示文摘Coptis chinensis Franch, a perennial herb, is mainly distributed in southeastern China. The rhizome of C. chinensis hasbeen used as a traditional medicine for more than 2000 years in China and many other Asian countries. Thepharmacological activities of C. chinensis have been validated by research. Here, we present a de novo high-qualitygenome of C. chinensis with a chromosome-level genome of ~958.20 Mb, a contig N50 of 1.58 Mb, and a scaffold N50of 4.53 Mb. We found that the relatively large genome size of C. chinensis was caused by the amplification of longterminal repeat (LTR) retrotransposons. In addition, a whole-genome duplication event in ancestral Ranunculales wasdiscovered. Comparative genomic analysis revealed that the tyrosine decarboxylase (TYDC) and (S)-norcoclaurinesynthase (NCS) genes were expanded and that the aspartate aminotransferase gene (ASP5) was positively selected inthe berberine metabolic pathway. Expression level and HPLC analyses showed that the berberine content was highestin the roots of C. chinensis in the third and fourth years. The chromosome-level reference genome of C. chinensisprovides important genomic data for molecular-assisted breeding and active ingredient biosynthesis. | Da-xia Chen Yuan Pan Yu Wang Yan-Ze Cui Ying-Jun Zhang Rang-yu Mo Xiao-li Wu Jun Tan Jian Zhang Lian-an Guo Xiao Zhao Wenkai Jiang Tian-lin Sun Xiao-Di Hu Long-yun Li | 2021 | Horticulture Research2021，8，1： | 2 |
| 9 | Estimating Seismic Intensity Maps of the 2021 Mw 7.3 Madoi,Qinghai and Mw 6.1 Yangbi,Yunnan,China Earthquakes显示文摘This study focuses on rapidly determining seismic intensity maps of earthquakes because it offers fundamental information for effective emergency rescue and subsequent scientific research,and remains challenging to accurately determine seismic intensity map in regions with sparse instrumental observations.Here we applied a novel method that consisted of array technology(backprojection),ground-motion prediction equations,and site corrections,to estimate the seismic intensity maps of the 2021 Mw 7.3 Madoi,Qinghai and the Mw 6.1 Yangbi,Yunnan,China earthquakes.We used seismic data recorded at European stations to back-project the source processes of the 2021 Mw7.3 Madoi,Qinghai and the Mw 6.1 Yangbi,Yunnan,China earthquakes.The back-projected energy radiations were then used as subevents or used to define the fault geometry.Summing the contributions of each subevent or estimating the shortest distances from each site to the rupture fault,we obtained the ground motion(PGA and PGV)for each site under rock site conditions.The estimated ground motions were corrected at each site for local site amplification according to the Vs30 database.Our estimated seismic intensity maps and field reports showed high similarity,which further validated the effectiveness of the novel approach,and pushed the limit of earthquake size down to~M 6.Such efforts would substantially help in the fast and accurate evaluation of earthquake damage,and precise rescue efforts. | Wenkai Chen Dun Wang Can Zhang Qiang Yao Hongjun Si | 2022 | Journal of Earth Science2022，33，4： | 2 |
| 10 | Melon short internode(CmSi)encodes an ERECTA-like receptor kinase regulating stem elongation through auxin signaling显示文摘Plant height is one of the most important agronomic traits that directly determines plant architecture,and compact or dwarf plants can allow for increased planting density and land utilization as well as increased lodging resistance and economic yield.At least four dwarf/semidwarf genes have been identified in different melon varieties,but none of them have been cloned,and little is known about the molecular mechanisms underlying internode elongation in melon.Here,we report map-based cloning and functional characterization of the first semidwarf gene short internode(Cmsi)in melon,which encodes an ERECTA-like receptor kinase regulating internode elongation.Spatial-temporal expression analyses revealed that CmSI exhibited high expression in the vascular bundle of the main stem during internode elongation.The expression level of CmSI was positively correlated with stem length in the different melon varieties examined.Ectopic expression of CmSI in Arabidopsis and cucumber suggested CmSI as a positive regulator of internode elongation in both species.Phytohormone quantitation and transcriptome analysis showed that the auxin content and the expression levels of a number of genes involved in the auxin signaling pathway were altered in the semidwarf mutant,including several well-known auxin transporters,such as members of the ABCB family and PINFORMED genes.A melon polar auxin transport protein CmPIN2 was identified by protein–protein interaction assay as physically interacting with CmSI to modulate auxin signaling.Thus,CmSI functions in an auxin-dependent regulatory pathway to control internode elongation in melon.Our findings revealed that the ERECTA family gene CmSI regulates stem elongation in melon through auxin signaling,which can directly affect polar auxin transport. | Sen Yang Kaige Zhang Huayu Zhu Xiaojing Zhang Wenkai Yan Nana Xu Dongming Liu Jianbin Hu Yufeng Wu Yiqun Weng Luming Yang | 2020 | Horticulture Research2020，7，1： | 2 |
| 11 | Efficacy of Danggui Buxue decoction(当归补血汤)on diabetic nephropathy-induced renal fibrosis in rats and possible mechanism显示文摘OBJECTIVE:To observe the efficacy of Danggui Buxue decoction(当归补血汤,DBD) on diabetic nephropathyinduced renal fibrosis in rats,and to study the possible mechanism.METHODS:Sixty male Goto Kakizaki(GK) rats were randomly assigned to the model group,gliquidone group,astragaloside Ⅳ group,and high-,medium-and lowdoses DBD groups.After 8 weeks,changes in body weight,blood glucose,serum creatinine,serum urea nitrogen,and total cholesterol were observed.Changes in transforming growth factor-β1(TGF-β1),Smad3,and Smad5 pathways and the expression of the fibrosisrelated proteins collagen Ⅳ(col Ⅳ),α-smooth muscle actin(α-SMA),and vimentin were assessed.The degree of renal fibrosis was observed by immunohistochemistry and Mason staining.The expression of interleukin 6(IL-6),interleukin 10(IL-10),tumor necrosis factor(TNF-α),and C-reactive protein(CRP) in the kidneys was assessed using enzyme linked immunosorbent assay.RESULTS:Our experiments showed that DBD effectively reduced blood glucose,blood urea nitrogen,and creatinine levels after 8 weeks of administration,improved renal function in diabetic rats,alleviated renal fibrosis,and reduced the renal tissue levels of IL-6,IL-10,TNF-α,and CRP.Furthermore,DBD decreased the expression of TGF-β1,Smad3,col IV,α-SMA,and vimentin in renal tissues and increased the expression of Smad5.CONCLUSIONS:DBD ameliorates diabetic renal interstitial fibrosis by modulating the TGF-β1/Smads pathway. | ZHAO Ye WANG Xian GU Ling LI Zihang ZHU Jingtian WANG Wenkai ZHANG Liang XUE Mei | 2023 | Journal of Traditional Chinese Medicine2023，43，3： | 2 |
| 12 | Spectroscopic studies of dye-surfactant interactions with the co-existence of heavy metal ions for foam fractionation显示文摘The interaction between a cationic dye Methylene Blue(MB) and an anionic surfactant sodium dodecyl sulfate(SDS) with the presence of Cd2+ was investigated spectrophotometrically in a certain concentration range.The spectrophotometric measurements of dye-metal ion-surfactant system were carried out.The results indicated that the SDS concentration had a significant influence on the dye spectrum,while the addition of Cd2+ hardly caused change of the maximum value of absorbance.According to this observation,we concluded that electrostatic and hydrophobic interaction between dye and surfactant occurred up to a certain level,and the homo-ions Cd2+ almost exerted no effect on the dye-surfactant complexation,establishing a theoretical foundation for simultaneous removal of organic dye and heavy metal using foam fractionation.Meanwhile,the effects of their interaction on foam performance were investigated.The results showed that the addition of Cd2+ favored the tendency to ameliorate foam properties just contrary to MB.The feasibility of foam separation for dye and heavy metal removal from simulated wastewater was also confirmed using a continuous foam fractionator.In the simultaneous removal process,with the initial SDS concentration ranging from 0.5 to 5.0mmol/L,the maximum removal efficiencies of MB and Cd2+ were obtained as 99.69% and 99.61%,respectively.The enrichment ratios were reduced from24.34 to 7.65 for MB and from22.01 to 3.35 for Cd2+. | Dongmei Zhang Guangming Zeng Jinhui Huang Wenkai Bi Gengxin Xie | 2012 | Journal of Environmental Sciences2012，24，12： | 2 |
| 13 | Density functional theory study of CO catalytic oxidation on Co_2B_2/TiO_2(110) surface显示文摘Titanium dioxide with CoB amorphous alloys nanoparticles deposited on the surface is known to exhibit higher catalytic activity than the CoB amorphous.A study of the structure of such system is necessary to understand this effect.A quantum chemical study of Co2B2 on the TiO2(110) surface was studied using periodic slab model within the framework of density functional theory(DFT).The results of geometry optimization indicated that the most stable model of adsorption was Co2B2 cluster adsorbed on the hollow site of TiO2 .The adsorption energy calculated for Co2B2 on the hollow site was 439.3 kJ/mol.The adsorption of CO and O2 was further studied and the results indicated that CO and O2 are preferred to adsorb on the Co2 site.Co-adsorption of CO and O2 shows that Co2B2 /TiO2 is a good catalyst for the oxidation of CO to carbon dioxide in the presence of oxygen. | Qingsong Zeng Wenkai Chen Yongfan Zhang Wenxin Dai Xin Guo | 2010 | Journal of Natural Gas Chemistry2010，19，3： | 2 |
| 14 | Trace water triggers high-efficiency photocatalytic hydrogen peroxide production显示文摘Photocatalytic production of hydrogen peroxide(H_(2)O_(2))has attracted much attentions as a promising method for sustainable solar fuel.Here,we demonstrate that trace water can drastically boost highefficiency photocatalytic production of H_(2)O_(2) with a record-high concentration of 113 mmol L^(-1) using alkali-assisted C_(3)N_(4) as photocatalyst in water/alcohol mixture solvents.By electron paramagnetic resonance(EPR)measurement,the radical species generated during the photocatalytic process of H_(2)O_(2) are identified.We propose alcohol is used to provide and stabilize-OOH radicals through hydrogen bond,while trace water could trigger photocatalytic production of H_(2)O_(2) via providing and transferring indispensable free protons to completely consume OOH radicals,which breaks the reaction balance of-OOH radical generation from alcohol.Thus-OOH radicals could be supplied by alcohol continuously to serve as a reservoir for high-efficiency production of H_(2)O_(2).These results pave the way towards photocatalytic method on semiconductor catalysts as an outstanding approach for production of hydrogen peroxide. | Zaixiang Xu Yang Li Yongyong Cao Renfeng Du Zhikang Bao Shijie Zhang Fangjun Shao Wenkai Ji jun Yang Guilin Zhuang Shengwei Deng Zhongzhe Wei Zihao Yao Xing Zhong Jianguo Wang | 2022 | Journal of Energy Chemistry2022，31，1： | 1 |
| 15 | Land cover classification in a mixed forest-grassland ecosystem using LResU-net and UAV imagery显示文摘Using an unmanned aerial vehicle (UAV) paired with image semantic segmentation to classify land cover within natural vegetation can promote the development of forest and grassland field. Semantic segmentation normally excels in medical and building classification, but its usefulness in mixed forest-grassland ecosystems in semi-arid to semi-humid climates is unknown. This study proposes a new semantic segmentation network of LResU-net in which residual convolution unit (RCU) and loop convolution unit (LCU) are added to the U-net framework to classify images of different land covers generated by UAV high resolution. The selected model enhanced classification accuracy by increasing gradient mapping via RCU and modifying the size of convolution layers via LCU as well as reducing convolution kernels. To achieve this objective, a group of orthophotos were taken at an altitude of 260 m for testing in a natural forest-grassland ecosystem of Keyouqianqi, Inner Mongolia, China, and compared the results with those of three other network models (U-net, ResU-net and LU-net). The results show that both the highest kappa coefficient (0.86) and the highest overall accuracy (93.7%) resulted from LResU-net, and the value of most land covers provided by the producer’s and user’s accuracy generated in LResU-net exceeded 0.85. The pixel-area ratio approach was used to calculate the real areas of 10 different land covers where grasslands were 67.3%. The analysis of the effect of RCU and LCU on the model training performance indicates that the time of each epoch was shortened from U-net (358 s) to LResU-net (282 s). In addition, in order to classify areas that are not distinguishable, unclassified areas were defined and their impact on classification. LResU-net generated significantly more accurate results than the other three models and was regarded as the most appropriate approach to classify land cover in mixed forest-grassland ecosystems. | Chong Zhang Li Zhang Bessie Y.J.Zhang Jingqian Sun Shikui Dong Xueyan Wang Yaxin Li Jian Xu Wenkai Chu Yanwei Dong Pei Wang | 2022 | Journal of Forestry Research2022，33，3： | 1 |
| 16 | Study of usingcomplementary S matrix to enhance SNR in Hadamardspeclrometer显示文摘 | Zhang Wenkai Zhang Zhihai Gao Lingxiao | 2014 | Optik2014，125，3： | 1 |
| 17 | Deconvolutive Short-time FourierTransform Spectrogram显示文摘 | Lu Wenkai Zhang Qiang | 2009 | IEEE Signal Processing Letters2009，16，7： | 1 |
| 18 | Higher-orderstatisticsand supertrace-based coherence-estimation algorithm显示文摘 | Lu Wenkai Li Yandong Zhang Shanwen | 2005 | Geophysics2005，70，3： | 1 |
| 19 | Higher-order-statistics and supertrace-based coherence-estimation algorithm 显示文摘 | Lu Wenkai Li Yandong Zhang Shanwen | 2005 | Geophys- ics2005，70，3： | 1 |
| 20 | Prediction of thermodynamic properties of actinide and lanthanide compounds显示文摘Several relationship models for thermodynamic functions of actinide and lanthanide compounds are built. The descriptors such as the difference of atomic radii between metal atoms and nonmetal atoms and the molecular mass are used in quantitative structure-activity/property relationships. The relative errors for entropy and heat capacity are less than 20% in the majority of gaseous compounds. Similar results are obtained from solid compounds. | LU Chunhai NI Shijun SUN Ying CHEN Wenkai ZHANG Chengjiang | 2008 | Nuclear Science and Techniques2008，19，3： | 1 |
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