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| 1 | Evolutionary processes and sources of high-nitrate haze episodes over Beijing,Spring显示文摘Rare and consecutive high-nitrate haze pollution episodes were observed in Beijing in spring2012. We present detailed characterization of the sources and evolutionary mechanisms of this haze pollution, and focus on an episode that occurred between 15 and 26 April. Submicron aerosol species were found to be substantially elevated during haze episodes, and nitrates showed the largest increase and occupation(average: 32.2%) in non-refractory submicron particles(NR-PM_1), which did not occur in other seasons as previously reported. The haze episode(HE) was divided into three sub-episodes, HEa, HEb, and HEc. During HEa and HEc, a shallow boundary layer, stagnant meteorological conditions, and high humidity favored the formation of high-nitrate concentrations, which were mainly produced by three different processes —daytime photochemical production, gas-particle partitioning, and nighttime heterogeneous reactions — and the decline in visibility was mainly induced by NR-PM_1.However, unlike HEa and HEc, during HEb, the contribution of high nitrates was partly from the transport of haze from the southeast of Beijing — the transport pathway was observed at ~800–1000 m by aerosol Lidar —and the decline in visibility during HEb was primarily caused by PM_(2.5). Our results provide useful information for air quality improvement strategies in Beijing during Spring. | Ting Yang Yele Sun Wei Zhang Zifa Wang Xingang Liu Pingqing Fu Xiquan Wang | 2017 | Journal of Environmental Sciences2017，29，4： | 2 |
| 2 | Recent Progress in Atmospheric Chemistry Research in China: Establishing a Theoretical Framework for the “Air Pollution Complex”显示文摘Atmospheric chemistry research has been growing rapidly in China in the last 25 years since the concept of the“air pollution complex”was first proposed by Professor Xiaoyan TANG in 1997.For papers published in 2021 on air pollution(only papers included in the Web of Science Core Collection database were considered),more than 24000 papers were authored or co-authored by scientists working in China.In this paper,we review a limited number of representative and significant studies on atmospheric chemistry in China in the last few years,including studies on(1)sources and emission inventories,(2)atmospheric chemical processes,(3)interactions of air pollution with meteorology,weather and climate,(4)interactions between the biosphere and atmosphere,and(5)data assimilation.The intention was not to provide a complete review of all progress made in the last few years,but rather to serve as a starting point for learning more about atmospheric chemistry research in China.The advances reviewed in this paper have enabled a theoretical framework for the air pollution complex to be established,provided robust scientific support to highly successful air pollution control policies in China,and created great opportunities in education,training,and career development for many graduate students and young scientists.This paper further highlights that developing and low-income countries that are heavily affected by air pollution can benefit from these research advances,whilst at the same time acknowledging that many challenges and opportunities still remain in atmospheric chemistry research in China,to hopefully be addressed over the next few decades. | Tong ZHU Mingjin TANG Meng GAO Xinhui BI Junji CAO Huizheng CHE Jianmin CHEN Aijun DING Pingqing FU Jian GAO Yang GAO Maofa GE Xinlei GE Zhiwei HAN Hong HE Ru-Jin HUANG Xin HUANG Hong LIAO Cheng LIU Huan LIU Jianguo LIU Shaw Chen LIU Keding LU Qingxin MA Wei NIE Min SHAO Yu SONG Yele SUN Xiao TANG Tao WANG Tijian WANG Weigang WANG Xuemei WANG Zifa WANG Yan YIN Qiang ZHANG Weijun ZHANG Yanlin ZHANG Yunhong ZHANG Yu ZHAO Mei ZHENG Bin ZHU Jiang ZHU | 2023 | Advances in Atmospheric Sciences2023，40，8： | 2 |
| 3 | A novel method for the synthesis of carbon dots assisted by free radicals显示文摘Carbon dots(CDs)have gradually become a widely favored type of fluorescent nanomaterials with unlimited and promising applications.This work reports a means of breaking the shackle of method to develop new red and white CDs by introducing free radicals.The resulting white emissive CDs in this strategy are employed to demonstrate electroluminescent white-light-emitting diodes(WLEDs)and achieve a record-high external quantum efficiency(0.95%)of one-step-produced white CDs(WCD)-LEDs,which dramatically simplifies the whole fabrication processes of WLEDs.With additional passivation treatment,the red CDs(RCD2)with excellent properties such as N and S co-doping,bright(quantum yield=49%)and stable photoluminescence(PL),large positive zeta potential(+20.5 mV),and two-photon fluorescence are obtained.Such RCD2 are used for rapid staining(5 min)of yeast cells.The two CDs synthesized via this method have outstanding performance in different aspects,which provides new promise of CDs for further functionalization and applications. | Xinyue Zhou Kebing Yi Yeling Yang Guohua Xie Xinghu Ji Zhike He | 2022 | Nano Research2022，15，10： | 1 |
| 4 | Ultralong organic room-temperature phosphorescence of electrondonating and commercially available host and guest molecules through efficient Förster resonance energy transfer显示文摘Ultralong organic room-temperature phosphorescence(RTP)materials have attracted tremendous attention recently due to their diverse applications.Several ultralong organic RTP materials mimicking the host-guest architecture of inorganic systems have been exploited successfully.However,complicated synthesis and high expenditure are still inevitable in these studies.Herein,we develop a series of novel host-guest organic phosphorescence systems,in which all luminophores are electron-rich,commercially available and halogen-atom-free.The maximum phosphorescence efficiency and the longest lifetime could reach 23.6%and 362 ms,respectively.Experimental results and theoretical calculation indicate that the host molecules not only play a vital role in providing a rigid environment to suppress non-radiative decay of the guest,but also show a synergistic effect to the guest through Förster resonance energy transfer(FRET).The commercial availability,facile preparation and unique properties also make these new host-guest materials an excellent candidate for the anti-counterfeiting application.This work will inspire researchers to develop new RTP systems with different wavelengths from commercially available luminophores. | Yeling Ning Junfang Yang Han Si Haozhong Wu Xiaoyan Zheng Anjun Qin Ben Zhong Tang | 2021 | Science China Chemistry2021，64，5： | 1 |
| 5 | Comparison of Physical Isolation on Large Active Area Perovskite Solar Cells显示文摘To reduce the quadratic scaling of the series resistance(R)and sheet resistance(Rs)of the devices,physi-cal isolation of the large area devices into small pieces has been proven to be a reliable and cost-efficient patterning technique.In this paper,we got an interesting result that the physical isolation did not show obvious effct on the photovoltaic performance of perovskite solar cells(PSCs)when fixing the active area.Three different isolation types,unetched ITO,etched ITO,and laser etching whole devices,have been induced to investigate the physical isolation roles.The results show that the electrons and holes could be collected efficiently in active area for all the isolation types.The proposed mechanism illustrates that the nonradiative recombination and recombination of electrons and hole in inactive area do not influence the performance of devices.This work may open a new way for the commer-cialization of PSCs by reducing the complex process and the etching costs. | GAO Liguo YAN Yeling LI Yang MA Tingli | 2020 | Chemical Research in Chinese Universities2020，36，6： | 0 |
| 6 | Fluorescence Properties and Chemical Composition of Fine Particles in the Background Atmosphere of North China显示文摘To understand the aerosol characteristics in a regional background environment,fine-particle(PM_(2.5),n=228)samples were collected over a one-year period at the Shangdianzi(SDZ)station,which is a Global Atmospheric Watch regional background station in North China.The chemical and optical characteristics of PM_(2.5)were analyzed,including organic carbon,elemental carbon,water-soluble organic carbon,water-soluble inorganic ions,and fluorescent components of watersoluble organic matter.The source factors of major aerosol components are apportioned,and the sources of the fluorescent chromophores are further analyzed.The major chemical components of PM_(2.5)at SDZ were NO_(3)^(-),organic matter,SO_(4)^(2-),and NH_(4)^(+).Annually,water-soluble organic carbon contributed 48%±15%to the total organic carbon.Secondary formation(52%)and fossil fuel combustion(63%)are the largest sources of water-soluble organic matter and water-insoluble organic matter,respectively.In addition,three humic-like and one protein-like matter were identified via parallel factor analysis for excitation–emission matrices.The fluorescence intensities of the components were highest in winter and lowest in summer,indicating the main impact of burning sources.This study contributes to understanding the chemical and optical characteristics of ambient aerosols in the background atmosphere. | Ping LI Siyao YUE Xiaoyang YANG Di LIU Qiang ZHANG Wei HU Shengjie HOU Wanyu ZHAO Hong REN Gang LI Yuanguan GAO Junjun DENG Qiaorong XIE Yele SUN Zifa WANG Pingqing FU | 2023 | Advances in Atmospheric Sciences2023，40，7： | 0 |
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