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25篇 您的检索式:作者名="ZHANG Ruixuan"
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1A vicinal effect for promoting catalysis of Pd1/TiO2:supports of atomically dispersed catalysts play more roles than simply serving as ligands显示文摘Atomically dispersing metal atoms on supports has been emerging as an effective strategy to maximize the atom utilization of metals for catalysis. However, due to the lack of effective tools to characterize the detailed structure of metal-support interface, the chemical functions of supports in atomically dispersed metal catalysts are hardly elucidated at the molecular level. In this work, an atomically dispersed Pd_1/TiO_2 catalyst with Ti(Ⅲ) vicinal to Pd is prepared and used to demonstrate the direct involvement of metal atoms on support in the catalysis of dispersed metal atoms. Systematic studies reveal that the Ti(Ⅲ)-O-Pd interface facilitates the activation of O_2 into superoxide(O_2^-), thus promoting the catalytic oxidation. The catalyst exhibits the highest CO turn-over frequency among ever-reported Pd-based catalysts,and enhanced catalysis in the combustion of harmful volatile organic compound(i.e., toluene) and greenhouse gas(i.e., methane). The demonstrated direct involvement of metal atoms on oxide support suggests that the real active sites of atomically dispersed metal catalysts can be far beyond isolated metal atoms themselves. Metal atoms on oxide supports in the vicinity serve as another vector to promote the catalysis of atomically dispersed metal catalysts.Pengxin Liu Yun Zhao Ruixuan Qin Lin Gu Peng Zhang Gang Fu Nanfeng Zheng 2018Science Bulletin2018,63,11:13
2Triboelectric–Electromagnetic Hybrid Generator for Harvesting Blue Energy显示文摘Progress has been developed in harvesting lowfrequency and irregular blue energy using a triboelectric–electromagnetic hybrid generator in recent years. However,the design of the high-efficiency, mechanically durable hybrid structure is still challenging. In this study, we report a fully packaged triboelectric–electromagnetic hybrid generator(TEHG), in which magnets were utilized as the trigger to drive contact–separation-mode triboelectric nanogenerators(CS-TENGs) and coupled with copper coils to operate rotary freestanding-mode electromagnetic generators(RF-EMGs). The magnet pairs that produce attraction were used to transfer the external mechanical energy to the CS-TENGs, and packaging of the CS-TENGpart was achieved to protect it from the ambient environment. Under a rotatory speed of 100 rpm, the CS-TENGs enabled the TEHG to deliver an output voltage, current,and average power of 315.8 V, 44.6 μA, and ~ 90.7 μW,and the output of the RF-EMGs was 0.59 V, 1.78 m A, and 79.6 μW, respectively. The cylinder-like structure made the TEHG more easily driven by water flow and demonstrated to work as a practical power source to charge commercial capacitors. It can charge a 33μF capacitor from 0 to 2.1 V in 84 s, and the stored energy in the capacitor can drive an electronic thermometer and form a self-powered water-temperature sensing system.Huiyun Shao Ping Cheng Ruixuan Chen Lingjie Xie Na Sun Qingqing Shen Xiaoping Chen Qianqian Zhu Yi Zhang Yina Liu Zhen Wen Xuhui Sun 2018Nano-Micro Letters2018,10,3:9
3One-Dimensional Magnetic FeCoNi Alloy Toward Low-Frequency Electromagnetic Wave Absorption显示文摘Rational designing of one-dimensional(1D)magnetic alloy to facilitate electromagnetic(EM)wave attenuation capability in low-frequency(2-6 GHz)microwave absorption field is highly desired but remains a significant challenge.In this study,a composite EM wave absorber made of a FeCoNi medium-entropy alloy embedded in a 1D carbon matrix framework is rationally designed through an improved electrospinning method.The 1D-shaped FeCoNi alloy embedded composite demonstrates the high-density and continuous magnetic network using off-axis electronic holography technique,indicating the excellent magnetic loss ability under an external EM field.Then,the in-depth analysis shows that many factors,including 1D anisotropy and intrinsic physical features of the magnetic medium-entropy alloy,primarily contribute to the enhanced EM wave absorption performance.Therefore,the fabricated EM wave absorber shows an increasing effective absorption band of 1.3 GHz in the low-frequency electromagnetic field at an ultrathin thickness of 2 mm.Thus,this study opens up a new method for the design and preparation of high-performance 1D magnetic EM absorbers.Bintong Yang Jiefeng Fang Chunyang Xu Hui Cao Ruixuan Zhang Biao Zhao Mengqiu Huang Xiangyu Wang Hualiang Lv Renchao Che 2022Nano-Micro Letters2022,14,10:4
4Effects of Si Addition on Microstructure,Properties and Serration Behaviors of Lightweight Al-Mg-Zn-Cu Medium-entropy Alloys显示文摘A series of as-cast lightweight multicomponent alloys Al(86-x)Mg10Zn2Cu2Six(x=0,0.3,0.6,0.9,1.2 at.%)were prepared by a vacuum induction furnace with a steel die.With the addition of Si,the reticular white Al-Cu phase deposited were gradually replaced by the gray eutectic Mg-Si phase,while the compressive strength of the alloys increases first and then decreases slowly.It is particularly noteworthy that the compression plasticity also exhibits this trend.When the Si content is 0.9 at.%,the compressive strength reaches its maximum at 779.11 MPa and the compressive plasticity reaches 20.91%.The effect of the addition of Si on the serration behavior of alloy was also studied;we found that the addition of Si introduces a new MgSi phase,and with the change of Si is significantly affects the morphology of the precipitated phase,which affects the serration behavior of the alloys.The comprehensive mechanical properties of the alloy are optimal at the critical point where the serration behavior disappears.In this work,we have provided a method and a composition for the preparation of a low-cost,high-strength,lightweight medium-entropy alloys.Yasong Li Ruixuan Li Yong Zhang 2019Research and Application of Materials Science2019,1,1:3
5Vortex tuning magnetization configurations in porous Fe_(3)O_(4) nanotube with wide microwave absorption frequency显示文摘The design and optimization of one-dimension(1D)magnetic material are of great importance for the energy conversion,storage and spin electron devices,which remain a huge challenge.Herein,1D porous Fe_(3)O_(4) nanotubes(NTs)have been fabricated via a combined process of electrospinning and calcination.In the electrospinning precursors,by regulating the content ratio between two types of polyvinyl pyrrolidone with different molecular weight,porous Fe_(3)O_(4) NTs with vortex-domain configuration have been fabricated.Based on the unique 1D nanotube structure encapsulated with multi-domains,the composite Fe_(3)O_(4) NTs exhibit high complex permeability(μʹ,μʺ)values,and hold both strong magnetic storage and dissipation capacity.Our Fe_(3)O_(4) NTs exhibit excellent microwave absorption(MA)performance with the maximum reflection loss value of−57.1 dB and the efficient absorption bandwidth of 12.0 GHz.The generated magnetic vortices make the crucial contribution to the spin-wave resonance which improves the MA dissipation under high-frequency.Related magnetic flux line distribution and magnetic domain moment were confirmed by the electron holography and micro-magnetic simulation,respectively,providing the deep insight to the microwave absorption mechanism.Ruixuan Zhang Lei Wang Chunyang Xu Chongyun Liang Xianhu Liu Xuefeng Zhang Renchao Che 2022Nano Research2022,15,7:2
6A HEA/MG composite breaks the strength-ductility trade-off by using ultrasonic technology显示文摘Metallic glasses(MGs)have aroused wide concern for their high strength,large elastic-strain limit and excellent wearresistance,while their applications as the structural materials are severely limited by their room-temperature brittleness.The crystalline in MGs have been used as dendrite/MG composite to improve the plasticity,and nowadays the high entropy alloys(HEAs)emerge from the crystalline alloys with more and more attention for their novel design principles and special properties[1,2].ZHANG Yong LI RuiXuan 2020Science China(Technological Sciences)2020,63,10:1
7Improvement of biodegradability of UV-curable adhesives modified by a novel polyurethane acrylate显示文摘Jiajian Huang Jinyuan Sun Ruoyu Zhang Ruixuan Zou Xiaoping Liu Zhuohong Yang Teng Yuan 2016Progress in Organic Coatings2016,,:1
8Cu_(2)O-SupportedAtomicallyDispersed Pd Catalysts for Semihydrogenation of Terminal Alkynes: Critical Role of Oxide Supports显示文摘Atomically dispersed catalysts have demonstrated superior catalytic performance in many chemical transformations.However,limited success has been achieved in applying oxide-supported atomically dis-persed catalysts to semihydrogenation of alkynes under mild conditions.Kunlong Liu Ruixuan Qin Lingyun Zhou Pengxin Liu Qinghua Zhang Wentong Jing Pengpeng Ruan Lin Gu Gang Fu Nanfeng Zheng 2019CCS Chemistry2019,1,2:1
9Classification of human movements with and without spinal orthosis based on surface electromyogram signals显示文摘Spinal orthoses were designed to correct poor posture;however,they may restrict trunk movements at all times,making daily activities difficult.Detecting trunk movements can provide instructions for adjusting the stiffness of the spinal orthosis.This study evaluated the feasibility of identifying movements based on surface electromyography(sEMG)signals.Ten participants were tested for different movements with two different modalities:motion without the spinal orthosis(Normal)and with the spinal orthosis(Spinal orthosis).The sEMG signals were collected from eight muscles using surface electrodes during four movements[flexion-extension,lateral bending,axial rotation,and stand to sit to stand].Four time domain features were extracted,with a total of 32 feature vectors.The principal component analysis(PCA)method was adopted to feature selection,and it was found that eight feature dimensions can make cumulative explained variance exceed 95%.The results showed that machine learning algorithms could not only identify Normal and Spinal orthosis movement modalities,but also distinguish four daily movements.Moreover,the classification performance of Random Forest(RF),k-Nearest Neighbor(kNN),and Support Vector Machine(SVM)algorithms were also compared.The results showed that all three machine algorithms have high classification accuracy.The machine learning methods can accurately identify movement patterns by considering sEMG signals,which may provide instructions for adjusting the stiffness of the spinal orthosis.In the future,the spinal orthosis with adjustable stiffness controlled by sEMG signals could help correct poor posture,and permit the wearer to achieve free movement when needed.Chenyan Wang Xiaona Li Yuan Guo Ruixuan Zhang Weiyi Chen 2022Medicine in Novel Technology and Devices2022,,4:0
10Quantized anomalous Hall resistivity achieved in molecular beam epitaxy-grown MnBi_(2)Te_(4)thin films显示文摘The intrinsic magnetic topological insulator MnBi_(2)Te_(4)provides a feasible pathway to the high-temperature quantum anomalous Hall(QAH)effect as well as various novel topological quantum phases.Although quantized transport properties have been observed in exfoliated MnBi_(2)Te_(4)thin flakes,it remains a big challenge to achieve molecular beam epitaxy(MBE)-grown MnBi_(2)Te_(4)thin films even close to the quantized regime.In this work,we report the realization of quantized anomalous Hall resistivity in MBE-grown MnBi_(2)Te_(4)thin films with the chemical potential tuned by both controlled in situ oxygen exposure and top gating.We find that elongated post-annealing obviously elevates the temperature to achieve quantization of the Hall resistivity,but also increases the residual longitudinal resistivity,indicating a picture of high-quality QAH puddles weakly coupled by tunnel barriers.These results help to clarify the puzzles in previous experimental studies on MnBi_(2)Te_(4)and to find a way out of the big difficulty in obtaining MnBi_(2)Te_(4)samples showing quantized transport properties.Yunhe Bai Yuanzhao Li Jianli Luan Ruixuan Liu Wenyu Song Yang Chen Peng-Fei Ji Qinghua Zhang Fanqi Meng Bingbing Tong Lin Li Yuying Jiang Zongwei Gao Lin Gu Jinsong Zhang Yayu Wang Qi-Kun Xue Ke He Yang Feng Xiao Feng 2024National Science Review2024,11,2:0
11Research on UAV cloud control system based on ant colony algorithm显示文摘In the cloud era, the control objects are becoming larger and the information processing is more complex, and it is difficult for traditional control systems to process massive data in a timely manner. In view of the difficulty of data processing in the cloud era, it is extremely important to perform massive data operations through cloud servers. Unmanned aeriel vehicle(UAV) control is the representative of the intelligent field. Based on the ant colony algorithm and incorporating the potential field method, an improved potential field ant colony algorithm is designed. To deal with the path planning problem of UAVs, the potential field ant colony algorithm shortens the optimal path distance by 6.7%, increases the algorithm running time by39.3%, and increases the maximum distance by 24.1% compared with the previous improvement. The cloud server is used to process the path problem of the UAV and feedback the calculation results in real time. Simulation experiments verify the effectiveness of the new algorithm in the cloud environment.ZHANG Lanyong ZHANG Ruixuan 2022Journal of Systems Engineering and Electronics2022,33,4:0
12化工产品系统评价显示文摘运用系统工程学的多目标决策分析方法,对中国化工产品的国际竞争力问题进行了较为深刻的研究,并提出了相应的策略。Zhang Liangquan,Yan Ruixuan (China National Econo technological Development Centre,Beijing 100723) 1999现代化工1999,19,2:0
13Tailoring electron vortex beams with customizable intensity patterns by electron diffraction holography显示文摘An electron vortex beam(EVB)carrying orbital angular momentum(OAM)plays a key role in a series of fundamental sci-entific researches,such as chiral energy-loss spectroscopy and magnetic dichroism spectroscopy.So far,almost all the experimentally created EVBs manifest isotropic doughnut intensity patterns.Here,based on the correlation between loc-al divergence angle of electron beam and phase gradient along azimuthal direction,we show that free electrons can be tailored to EVBs with customizable intensity patterns independent of the carried OAM.As proof-of-concept,by using computer generated hologram and designing phase masks to shape the incident free electrons in the transmission elec-tron microscope,three structured EVBs carrying identical OAM are tailored to exhibit completely different intensity pat-terns.Furthermore,through the modal decomposition,we quantitatively investigate their OAM spectral distributions and reveal that structured EVBs present a superposition of a series of different eigenstates induced by the locally varied geo-metries.These results not only generalize the concept of EVB,but also demonstrate an extra highly controllable degree of freedom for electron beam manipulation in addition to OAM.Pengcheng Huo Ruixuan Yu Mingze Liu Hui Zhang Yan-qing Lu Ting Xu 2024Opto-Electronic Advances2024,7,2:0
14Spinosin protects Neuro-2a/APP695 cells from oxidative stress damage by inactivating p38显示文摘OBJECTIVE:To explore the protective mechanism of spinosin(SPI)on Alzheimer's disease(AD)model cells,Neuro-2a/APP695(N2a/APP695),against H_(2)O_(2)-induced oxidative stress damage,to reflect the influence of oxidative stress on the development of AD,and to provide a valuable basis for the research and development of therapeutic drug for AD.METHODS:N2a/APP695 cells were exposed to H2O2 and then treated with spinosin.Firstly,the secretion level of amyloidβ(Aβ)1-42 and the production of malondialdehyde(MDA)and lactate dehydrogenase(LDH)were detected by enzyme linked immunosorbent assay kits.Secondly,the oligomerization degree of Aβ1-42 was performed by Thioflavin T staining.Thirdly,the expression levels of p-Tau(Ser199/202/396),synaptophysin(SYP),postsynaptic density protein 95(PSD95),and mitogen-activated protein kinase(MAPK)family-related proteins were detected by Western blot analysis.In addition,FITC-labeled phalloidin was used in cytoskeleton staining to reflect synaptic function.RESULTS:This study showed that H2O2 stimulated N2a/APP695 cells to produce excessive MDA and LDH and secrete a large amount of Aβ,promoted the aggregation of Aβ,induced Tau protein hyperphosphorylation,and led to synaptic dysfunction.Spinosin reversed these changes caused by H2O2 by inactivating p38,which was verified by treatment with the p38 inhibitor BIRB796.CONCLUSION:Spinosin protects N2a/APP695 cells from oxidative stress damage caused by H2O2 through inactivating p38.ZHANG Xiaoying WANG Ruixuan WANG Yiqing XU Fanxing YAN Tingxu WU Bo ZHANG Ming JIA Ying 2023Journal of Traditional Chinese Medicine2023,43,5:0
15Interfacial oxidized Pd species dominate catalytic hydrogenation of polar unsaturated bonds显示文摘The determination of catalytically active sites is crucial for the design of efficient and stable catalysts toward desired reactions.However,the complexity of supported noble metal catalysts has led to controversy over the locations of catalytically active sites(e.g.,metal,support,and metal/support interface).Here we develop a structurally controllable catalyst system(Pd/SBA-15)to reveal the catalytic active sites for the selective hydrogenation of ketones to alcohol using acetophenone hydrogenation as model reaction.Systematic investigations demonstrated that unsupported Pd nanocrystals have no catalytic activity for acetophenone hydrogenation.However,oxidized Pd species were catalytically highly active for acetophenone hydrogenation.The catalytic activity decreased with the decreased oxidation state of Pd.This work provides insights into the hydrogenation mechanism of ketones but also other unsaturated compounds containing polar bonds,e.g.,nitrobenzene,N-benzylidene-benzylamine,and carbon dioxide.Pengyao You Shaoqi Zhan Pengpeng Ruan Ruixuan Qin Shiguang Mo Yazhou Zhang Kunlong Liu Lansun Zheng Nanfeng Zheng 2024Nano Research2024,17,1:0
16Submilliwatt, widely tunable coherent microcomb generation with feedback-free operation显示文摘Microcombs are revolutionizing optoelectronics by providing parallel, mutually coherent wavelengthchannels for time-frequency metrology and information processing. To implement this essential function inintegrated photonic systems, it is desirable to drive microcombs directly with an on-chip laser in a simpleand flexible way. However, two major difficulties have prevented this goal: (1) generating mode-lockedcomb states usually requires a significant amount of pump power and (2) the requirement to align laser andresonator frequency significantly complicates operation and limits the tunability of the comb lines. Here, weaddress these problems by using microresonators on an AlGaAs on-insulator platform to generate dark-pulsemicrocombs. This highly nonlinear platform dramatically relaxes fabrication requirements and leads to arecord-low pump power of <1 mW for coherent comb generation. Dark-pulse microcombs facilitated bythermally controlled avoided mode crossings are accessed by direct distributed feedback laser pumping.Without any feedback or control circuitries, the comb shows good coherence and stability. With around150 mW on-chip power, this approach also leads to an unprecedentedly wide tuning range of over one freespectral range (97.5 GHz). Our work provides a route to realize power-efficient, simple, and reconfigurablemicrocombs that can be seamlessly integrated with a wide range of photonic systems.Haowen Shu Lin Chang Chenghao Lao Bitao Shen Weiqiang Xie Xuguang Zhang Ming Jin Yuansheng Tao Ruixuan Chen Zihan Tao Huajin Chang Shaohua Yu Qifan Yang Xingjun Wang John E.Bowers 2023Advanced Photonics2023,5,3:0
17Erratum to:Efficient flexible perovskite solar cells and modules using a stable SnO_(2)-nanocrystal isopropanol dispersion显示文摘Erratum to Nano Research,2024,17(4):2704-2711 http://gffzzd3cc09b8251d45dfs0xnvq5fwnvwn6ncf.ffgz.tsg.suse.edu.cn/10.1007/s12274-023-6115-y(1)In the article,the table of contents(TOC)image was unfortunately mispresented.Zhiwei Su Jing Li Ruixuan Jiang Shujie Zhang Chengkai Jin Feng Ye Bingcan Ke Mengjun Zhou Jinhui Tong Hyesung Park Fuzhi Huang Yi-Bing Cheng Tongle Bu 2024Nano Research2024,17,5:0
18Identification and fine mapping of a fertility restorer gene for wild abortive cytoplasmic male sterility in the elite indica rice non-restorer line 9311显示文摘The wild abortive(WA)-type cytoplasmic male sterility(CMS)derived from the wild rice species Oryza rufipogon Griff.is used widely in three-line indica hybrids.The identification and mapping of restorer of fertility(Rf)genes aided in the development of WA-type hybrids.Here we report that testcross F1 plants from the WA-type CMS line and 9311 exhibited stainable pollen grains with no seed set,indicating that 9311 carries minor-effect Rfs for WA-type CMS.We developed an advanced backcross population consisting of plants harboring small regions of donor chromosomal segments from 9311 in the WATianfeng A genetic background with moderate seed setting rates.Genetic analysis showed that the pollen fertility levels of the backcross individuals are governed by a single gene from 9311 that we named Rf19(t).By use of the RICE 40 K gene chip,three introduced segments were identified in the fertile lines,and a candidate region spanning 4.37–8.29 Mb on chromosome 1 was identified for Rf19(t).Finally,Rf19(t)was fine-mapped to a region of 90 kb between the DNA marker loci STS1-163 and STS1-183,in which eight ORFs were predicted.Also,using relative expression analyses,comparative sequence analyses and functional domain analyses,we identified LOC_Os01g10530 as the most likely candidate gene for Rf19(t).Furthermore,Rf19(t)was found to function in fertility restoration,most probably by regulating the degradation of m RNA transcribed from the mitochondrial gene WA352.These results increase our knowledge of fertility restoration in WA-type CMS lines and will facilitate the development of high-quality pairs of WAtype CMS and maintainer lines.Zuopeng Xu Yuanyue Du Xixu Li Ruixuan Wang Zhi'ai Chen Xiangqiang Zhao Qiaoquan Liu Shuzhu Tang Honggen Zhang 2023The Crop Journal2023,11,3:0
19Extraction and Structure Elucidation of Phenols from Dendrobium thyrsiflorum显示文摘[Objective] This study aimed to investigate the chemical constituents of Dendrobium thyrsiflorum and determine its bioactive compounds. [Method] The compounds were extracted by 95% alcohol and isolated by column chromatography on silica gel and Sephadex LH-20. Their structures were identified by spectroscopic analysis(1H NMR and13 C NMR). [Result] Seven compounds were obtained and identified as 4, 7-dihydroxy-2-methoxy-9, 10-dihydrophenan-threne(1), syringaldehyde(2),moscatin(3), gigantol(4), batatasin III(5), tristin(6) and stigmasterol(7). [Conclusion] Compounds 1 and 2 were isolated from this medicinal plant for the first time.Ruixuan WENG Yupeng LI Shuang LI Guihua ZHANG Ying WANG Xiaoling WEN Jun ZHANG Rong HUANG 2015Agricultural Science & Technology2015,16,10:0
20Highly efficient and aberration-free off-plane grating spectrometer and monochromator for EUV—soft X-ray applications显示文摘We demonstrate a novel flat-field,dual-optic imaging EUV—soft X-ray spectrometer and monochromator that attains an unprecedented throughput efficiency exceeding 60%by design,along with a superb spectral resolution ofλ/Δλ>200 accomplished without employing variable line spacing gratings.Exploiting the benefits of the conical diffraction geometry,the optical system is globally optimized in multidimensional parameter space to guarantee optimal imaging performance over a broad spectral range while maintaining circular and elliptical polarization states at the first,second,and third diffraction orders.Moreover,our analysis indicates minimal temporal dispersion,with pulse broadening confined within 80 fs tail-to-tail and an FWHM value of 29 fs,which enables ultrafast spectroscopic and pump-probe studies with femtosecond accuracy.Furthermore,the spectrometer can be effortlessly transformed into a monochromator spanning the EUV—soft X-ray spectral region using a single grating with an aberration-free spatial profile.Such capability allows coherent diffractive imaging applications to be conducted with highly monochromatic light in a broad spectral range and extended to the soft X-ray region with minimal photon loss,thus facilitating state-of-the-art imaging of intricate nano-and bio-systems,with a significantly enhanced spatiotemporal resolution,down to the nanometer–femtosecond level.Jie Li Kui Li Xiaoshi Zhang Dimitar Popmintchev Hao Xu Yutong Wang Ruixuan Li Guangyin Zhang Jiyue Tang Jin Niu Yongjun Ma Runyu Meng Changjun Ke Jisi Qiu Yunfeng Ma Tenio Popmintchev Zhongwei Fan 2024Light(Science & Applications)2024,13,1:0
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