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| 1 | Graphitic carbon nitride/biochar composite synthesized by a facile ball-milling method for the adsorption and photocatalytic degradation of enrofloxacin显示文摘In order to enhance the removal performance of graphitic carbon nitride(g-C_(3)N_(4)) on organic pollutant, a simultaneous process of adsorption and photocatalysis was achieved via the compounding of biochar and g-C_(3)N_(4). In this study, g-C_(3)N_(4) was obtained by a condensation reaction of melamine at 550 °C. Then the g-C_(3)N_(4)/biochar composites were synthesized by ball milling biochar and g-C_(3)N_(4) together, which was considered as a simple, economical, and green strategy. The characterization of resulting g-C_(3)N_(4)/biochar suggested that biochar and g-C_(3)N_(4) achieved effective linkage. The adsorption and photocatalytic performance of the composites were evaluated with enrofloxacin(EFA) as a model pollutant. The result showed that all the g-C_(3)N_(4)/biochar composites displayed higher adsorption and photocatalytic performance to EFA than that of pure g-C_(3)N_(4). The 50% g-C_(3)N_(4)/biochar performed best and removed 45.2% and 81.1% of EFA(10 mg/L) under darkness and light with a dosage of 1 mg/mL, while g-C_(3)N_(4) were 19.0% and 27.3%, respectively. Besides, 50% g-C_(3)N_(4)/biochar showed the highest total organic carbon(TOC) removal efficiency(65.9%). Radical trapping experiments suggested that superoxide radical( ·O_(2)^(-)) and hole(h~+) were the main active species in the photocatalytic process. After 4 cycles, the composite still exhibited activity for catalytic removal of EFA. | Yao Xiao Honghong Lyu Chengliang Yang Beibei Zhao Lan Wang Jingchun Tang | 2021 | Journal of Environmental Sciences2021，33，5： | 8 |
| 2 | Size control of monodisperse nonporous silica particles by seed particle growth显示文摘Monodisperse nonporous silica particles were prepared by sol-precipitation via seed particle growth method,and the particle size,which varied from 1.0 to 4.7 m,was strictly controlled in our experiment. The formation of secondary particles,which resulted in a multimodal distribution of particle size,was suppressed by changing tetraethoxysilane(TEOS) concentration and reaction temperature. Furthermore,the effect of adding small amounts of electrolyte to the hydrolysis mixture was examined. | Beibei Zhao Caihua Tian Yan Zhang Tao Tang Fengyun Wang | 2011 | Particuology2011，9，3： | 7 |
| 3 | Preparation of high-purity monodisperse silica microspheres by the sol-gel method coupled with polymerization-induced colloid aggregation显示文摘Ultra-pure mesoporous silica microspheres with good monodispersity were synthesized in two steps:nanometer-sized silica sol was produced by the sol-gel process,then micrometer-sized silica microspheres were synthesized by polymerization-induced colloid aggregation of the silica sol.The total metal content of the microspheres was extremely low,which eliminated the tailing of chromatographic peaks by chelating reagents.The pore structure of the silica microspheres could be controlled by altering the sol-gel conditions.The silica microsphere particle size could be adjusted by using different polymerizationinduced colloid aggregation conditions. | Beibei Zhao Yan Zhang Tao Tang Fengyun Wang Tong Li Qiyu Lu | 2015 | Particuology2015，13，5： | 7 |
| 4 | Sulfonated carbon catalyzed oxidation of aldehydes to carboxylic acids by hydrogen peroxide显示文摘Sulfonated carbon as a strong and stable solid acid catalyst exhibited excellent catalytic performance in various acid-catalyzed reactions. Here, sulfonated carbon, as catalyst for oxidation reaction, was prepared via the carbonization of starch followed by sulfonation with concentrated sulfuric acid. N2 physisorption, X-ray diffraction, Fourier transform infrared spectroscopy, X-ray fluorescence and acid-base titration were used to characterize the obtained materials. The catalytic activity of sulfonated carbon was studied in the oxidation of aldehydes to carboxylic acids using 30 wt% H2O2 as oxidant. This oxidation protocol works well for various aldehydes including aromatic and aliphatic aldehydes. The sulfonated carbon can be recycled for three times without obvious loss of activity. | Lipeng Zhou Beibei Dong Si Tang Hong Ma Chen Chen Jie Xu Xiaomei Yang Jie Xu | 2013 | Journal of Energy Chemistry2013，22，4： | 4 |
| 5 | The landscape of aging显示文摘Aging is characterized by a progressive deterioration of physiological integrity,leading to impaired functional ability and ultimately increased susceptibility to death.It is a major risk factor for chronic human diseases,including cardiovascular disease,diabetes,neurological degeneration,and cancer.Therefore,the growing emphasis on “healthy aging” raises a series of important questions in life and social sciences.In recent years,there has been unprecedented progress in aging research,particularly the discovery that the rate of aging is at least partly controlled by evolutionarily conserved genetic pathways and biological processes.In an attempt to bring full-fledged understanding to both the aging process and age-associated diseases,we review the descriptive,conceptual,and interventive aspects of the landscape of aging composed of a number of layers at the cellular,tissue,organ,organ system,and organismal levels. | Yusheng Cai Wei Song Jiaming Li Ying Jing Chuqian Liang Liyuan Zhang Xia Zhang Wenhui Zhang Beibei Liu Yongpan An Jingyi Li Baixue Tang Siyu Pei Xueying Wu Yuxuan Liu Cheng-Le Zhuang Yilin Ying Xuefeng Dou Yu Chen Fu-Hui Xiao Dingfeng Li Ruici Yang Ya Zhao Yang Wang Lihui Wang Yujing Li Shuai Ma Si Wang Xiaoyuan Song Jie Ren Liang Zhang Jun Wang Weiqi Zhang Zhengwei Xie Jing Qu Jianwei Wang Yichuan Xiao Ye Tian Gelin Wang Ping Hu Jing Ye Yu Sun Zhiyong Mao Qing-Peng Kong Qiang Liu Weiguo Zou Xiao-Li Tian Zhi-Xiong Xiao Yong Liu Jun-Ping Liu Moshi Song Jing-Dong J.Han Guang-Hui Liu | 2022 | Science China(Life Sciences)2022，65，12： | 4 |
| 6 | Magnetic properties and magnetocaloric effects in amorphous and crystalline Gd_(55)Co_(35)Ni_(10) ribbons显示文摘The magnetic properties and magnetocaloric effects of amorphous and crystalline Gd55Co35Ni10 ribbons are investigated.A main phase with a Ho 12 Co 7-type monoclinic structure(space group P21/c) and a minor phase with a Ho4Co3-type hexagonal structure(space group P63/m) are obtained for crystalline ribbon after annealing.The amorphous ribbons order ferromagnetically and undergo a second-order transition at 192 K.For crystalline Gd55Co35Ni10 ribbons,two magnetic phase transitions occur at 158 and 214 K,respectively.The peak value of-△SM under a field change of 0-5 T is 6.5 J/kg K at 192 K for amorphous Gd55Co35Ni10 ribbons.A relatively large magnetic entropy change(~5.0 J/kg K) under a field change of 0-5 T for the crystalline Gd55Co35Ni10 ribbons is obtained in the temperature interval range of 154-214 K.The large platform of magnetic entropy change and the negligible thermal/magnetic hysteresis loss mean the crystalline Gd55Co35Ni10 compound can satisfy the requirement of the Ericsson-type refrigerator working in the temperature range from 154K to 214K. | ZHONG XiChun TANG PengFei GAO BeiBei MIN JiXiong LIU ZhongWu ZHENG ZhiGang ZENG DeChang YU HongYa QIU WanQi | 2013 | Science China(Physics,Mechanics & Astronomy)2013，56，6： | 3 |
| 7 | Targeting polarized phenotype of microglia via IL6/JAK2/ STAT3 signaling to reduce NSCLC brain metastasis显示文摘Tumor-associated macrophages have emerged as crucial factors for metastases.Microglia are indispensable components of the brain microenvironment and play vital roles in brain metastasis(BM).However,the underlying mechanism of how activated microglia promote brain metastasis of non-small cell lung cancer(NSCLC)remains elusive. | Yu Jin Yalin Kang Minghuan Wang Bili Wu Beibei Su Han Yin Yang Tang Qianxia Li Wenjie Wei Qi Mei Guangyuan Hu Veronika Lukacs-Kornek Jian Li Kongming Wu Xianglin Yuan Wei Wang | 2022 | Signal Transduction and Targeted Therapy2022，7，3： | 3 |
| 8 | Nafion-assisted exfoliation of MoS2 in water phase and the application in quick-response NIR light controllable multi-shape memory membrane显示文摘 | Wei Jia Beibei Tang Peiyi Wu | 2018 | Nano Research2018，11，1： | 3 |
| 9 | Convergence analysis of the formal energies of symplectic methods for Hamiltonian systems显示文摘Based on Feng's theory of formal vector fields and formal flows, we study the convergence problem of the formal energies of symplectic methods for Hamiltonian systems and give the clear growth of the coefficients in the formal energies. With the help of B-series and Bernoulli functions, we prove that in the formal energy of the mid-point rule, the coefficient sequence of the merging products of an arbitrarily given rooted tree and the bushy trees of height 1(whose subtrees are vertices), approaches 0 as the number of branches goes to ∞; in the opposite direction, the coefficient sequence of the bushy trees of height m(m ≥ 2), whose subtrees are all tall trees, approaches ∞ at large speed as the number of branches goes to +∞. The conclusion extends successfully to the modified differential equations of other Runge-Kutta methods. This disproves a conjecture given by Tang et al.(2002), and implies:(1) in the inequality of estimate given by Benettin and Giorgilli(1994) for the terms of the modified formal vector fields, the high order of the upper bound is reached in numerous cases;(2) the formal energies/formal vector fields are nonconvergent in general case. | ZHANG RuiLi TANG YiFa ZHU BeiBei TU XiongBiao ZHAO Yue | 2016 | Science China Mathematics2016，59，2： | 2 |
| 10 | Upcycling of phosphogypsum waste for efficient zinc-ion batteries显示文摘Zinc metal is a promising anode material for next-generation aqueous batteries,but its practical application is limited by the formation of zinc dendrite.To prevent zinc dendrite growth,various Zn^(2+)-conducting but water-isolating solid-electrolyte interphase(SEI)films have been developed,however,the required high-purity chemical materials are extremely expensive.In this work,phosphogypsum(PG),an industrial byproduct produced from the phosphoric acid industry,is employed as a multifunctional protective layer to navigate uniform zinc deposition.Theoretical and experimental results demonstrate that PG-derived CaSO_(4)2H_(2)O can act as an artificial SEI layer to provide fast channels for Zn^(2+)transport.Moreover,CaSO_(4)2H_(2)O could release calcium ions(Ca^(2+))due to its relatively high Kspvalue,which have a higher binding energy than that of Zn^(2+)on the Zn surface,thus preferentially adsorbing to the tips of the protuberances to force zinc ions to nucleate at inert region.As a result,the Zn@PG anode achieves a high Coulombic efficiency of 99.5%during 500 cycles and long-time stability over 1000 hours at 1 m A cm^(-2).Our findings will not only construct a low-cost artificial SEI film for practical metal batteries,but also achieve a high-value utilization of phosphogypsum waste. | Huanwen Wang Can Luo Yinyin Qian Caihong Yang Xiaojun Shi Yansheng Gong Rui Wang Beibei He Jun Jin Aidong Tang Edison Huixiang Ang Huaming Yang | 2023 | Journal of Energy Chemistry2023，，6： | 1 |
| 11 | A facile design for multifunctional AIEgen based on tetraaniline derivatives显示文摘Aniline oligomers have been widely used in many fields due to their excellent physicochemical properties. Owing to strong intermolecular interactions, their emission is always weakened or quenched when they are in high concentration or aggregated state, which greatly limits their fluorescent applications. Inspired by the concept of aggregation-induced emission(AIE), herein we introduced large steric groups onto the aniline oligomer to prevent the formation of packing structure. In particular, diphenyl vinyl group was bonded with oligomeric tetraaniline by a facile synthetic procedure with high yield. The obtained aniline oligomer derivative exhibited typical AIE features, which was also confirmed by density functional theoretical calculation. More importantly, this AIE oligomer was able to detect Fe^(3+) ions selectively and quantitatively. The fluorescence intensity decreased linearly along with the increment of Fe^(3+) concentration. Moreover, we demonstrated that this AIE oligomer could stain live bacteria, such as E. coli and S. aureus efficiently. All these results suggest that such a readily accessible and multifunctional tetraaniline derivative provides a new platform for the construction of fluorescent materials. | Beibei Liu Wei He Hao Lu Kun Wang Mingming Huang Ryan Tsz Kin Kwok Jacky Wing Yip Lam Longcheng Gao Jiping Yang Benzhong Tang | 2019 | Science China Chemistry2019，62，6： | 1 |
| 12 | A novel positively charged asymmetry membranes from poly(2,6-dimethyl-1,4-phenylene oxide) by benzyl bromination and in situ amination Part Ⅱ:Effect of charged group species on membrane performance and morphologies显示文摘 | Tang Beibei Xu Tongwen Yang Weihua | 2006 | Journal of Membrane Science2006，268，： | 1 |
| 13 | A novel of positively charged asymmetry membrane prepared from poly(2,6-dimethyl-1,4- phenylene oxide) by in situ amination Part Ⅲ:Effect of benzyl and aryl bromination degrees of polymer on membrane performance and morphologies显示文摘 | Tang Beibei Xu Tongwen Sun Peijian | 2006 | Journal of Membrane Science2006，279，： | 1 |
| 14 | Adsorption of aqueous Cu(Ⅱ) and Ag(Ⅰ) by silica anchored Schiff base decorated polyamidoamine dendrimers: Behavior and mechanism显示文摘A class of silica anchored Schiff base decorated polyamidoamine(PAMAM) dendrimers were synthesized for removing aqueous Cu(Ⅱ) and Ag(Ⅰ). The adsorption performance was investigated synthetically and the adsorption mechanism was revealed. Results indicate the adsorption capacity depends on dendrimer generation, solution p H, contact time, temperature and initial metal ion concentration.The optimum adsorption pH is 6 for both metal ion. Adsorption kinetic suggests the adsorption can achieve equilibrium at 180 and 150 min for Cu(Ⅱ) and Ag(Ⅰ). The kinetic process is found to be in good agreement with pseudo-second-order model and film diffusion is the rate-controlling step. The adsorption isotherm indicates the adsorption is proceeded by monolayer behavior with chemical mechanism. These adsorbents exhibit competitive adsorption capacity as compared with other reported adsorbents. Theoretical calculation demonstrates the participation of hydroxyl, carbonyl, and amide groups during the adsorption of Cu(Ⅱ), while hydroxyl and amide groups are mainly responsible for capturing Ag(Ⅰ). | Kaiyan Wu Bingxiang Wang Bentian Tang Liping Luan Wenlong Xu Beibei Zhang Yuzhong Niu | 2022 | Chinese Chemical Letters2022，33，5： | 1 |
| 15 | A novel pathogenesis-related protein (SsPR10) from Solanum surattense with ribonucleolytic and antimicrobial activity is stress- and pathogen-inducible显示文摘 | Xiaojun Liu Beibei Huang Juan Lin Jiong Fei Zhonghai Chen Yongzhen Pang Xiaofen Sun Kexuan Tang | 2005 | Journal of Plant Physiology2005，，5： | 1 |
| 16 | Development of novel SiO2 - GO nanohybrid/polysulfone membrane with enhanced performance显示文摘 | Huiqing Wu Beibei Tang Peiyi Wu | 2014 | Journal of Membrane Science2014，，451： | 1 |
| 17 | Effect of ischaemic brain injury on sexual function in adult mice显示文摘Objective:Priapism refers to a condition with persistent abnormal erection of the penis,which is usually caused by disease or injury in the brain or spinal cord,or obstruction to the outflow of blood through the dorsal vein at the root of the penis,without sexual desires.The effect of cerebral ischaemia on sexual function is unknown.The aim of this study is to explore whether priapism occurs in adult mice.Furthermore,we examined the relationship between priapism and the region of infarct in the brain.Design:Adult male CD-1 mice who underwent permanent middle cerebral artery occlusion(pMCAO)were closely examined from 2 hours to 14 days postoperation.Results:We found that priapism occurs in∼80%of the mice with pMCAO,which could persist up to 14 days.Further study has demonstrated that the occurrence of priapism is related to the infarct region:priapism is found only in mice with ischaemic injury extending to the hypothalamus and the hippocampus regions.Conclusion:Our result suggested priapism may be used as a deep brain injury marker for evaluating brain injury in mice after pMCAO. | Yaohui Tang Falei Yuan Beibei Cai Weiliang Xia Yongting Wang Guo-Yuan Yang | 2016 | Stroke & Vascular Neurology2016，1，3： | 0 |
| 18 | Improving the protective effects of a FGF for peripheral nerve injury repair using sulfated chitooligosaccharides显示文摘Injury to the peripheral nerves can result in temporary or life-long neuronal dysfunction and subsequent economic or social disability. Acidic fibroblast growth factor(a FGF) promotes the growth and survival of neurons and is a possible treatment for peripheral nerve injury. Yet,the actual therapeutic utility of a FGF is limited by its short half-life and instability in vivo. In the present study,we prepared sulfated chitooligosaccharides(SCOS),which have heparinlike properties,to improve the bioactivity of a FGF. We investigated the protective effects of SCOS with or without a FGF on RSC96 cells exposed to Na2 S2 O4 hypoxia/reoxygenation injury. Cell viability was measured by MTT assay and cytotoxicity induced by Na2 S2 O4 was assessed by lactate dehydrogenase(LDH) release into the culture medium. Pretreatment with a FGF and SCOS dramatically decreased LDH release after injury compared to pretreatment with a FGF or SCOS alone. We subsequently prepared an a FGF/SCOS thermo-sensitive hydrogel with poloxamer and examined its effects in vivo. Paw withdrawal thresholds and thermal withdrawal latencies were measured in rats with sciatic nerve injury. Local injection of the a FGF/SCOS hydrogels(a FGF: 40,80 μg/kg) increased the efficiency of sciatic nerve repair compared to a FGF(80 μg/kg) hydrogel alone. Especially a FGF/SCOS thermo-sensitive hydrogel decreased paw withdrawal thresholds from 117.75 ± 8.38(g,4 d) to 65.74 ± 3.39(g,10 d),but a FGF alone group were 140.58 ± 27.54(g,4 d) to 89.12 ± 5.60(g,10 d)(a FGF dose was 80 μg/kg,P < 0.05,n = 8). The thermal withdrawal latencies decreased from 11.61 ± 2.26(s,4 d) to 2.37 ±0.67(s,10 d). However,a FGF alone group were from 17.69 ± 1.47(s,4 d) to4.65 ± 1.73(s,10 d)(P < 0.05,n = 8). Furthermore,the a FGF/SCOS hydrogels also exhibited good biocompatibility in mice. In summary,SCOS improved the protective effects of a FGF in RSC96 cells injured with Na2S2O4 and increased the efficiency of nerve repair and recovery of function in rats with sciatic nerve injury. These findings pave an avenue for the development of novel prophylactic and therapeutic strategies for peripheral nerve injury. | Yanmei Liu Fenglin Yu Beibei Zhang Meng Zhou Yu Bei Yifan Zhang Jianzhong Tang Yan Yang Yadong Huang Qi Xiang Yueping Zhao Qian Liang Yang Liu | 2019 | Asian Journal of Pharmaceutical Sciences2019，14，5： | 0 |
| 19 | Synthesis and Characterization of Novel Hydrolytically Degradable Polyesters显示文摘Six novel hydrolytically degradable polyesters were synthesized from thiodipropionic acid(TDPA)and five diols by melt polycondensation,and characterized by FT-IR,1H NMR,gel permeation chromatography,differential scanning calorimetry and thermogravimetry analysis.The polystyrene-equivalent number-average(Mn)and weight-average molecular weight(Mw)of these polyesters ranged from 4900-11100 Da and 7900-20879 Da,respectively,with PDI values of 1.48-1.98.The melting point varied from 62.3-127.9℃,and the 50%mass-loss temperature ranged between 387-417℃.The degradation of these polyesters was studied in terms of relative weight loss in distilled water at different pH.Weight losses of 14%-26%were obtained at pH 7.0,26%-38%at pH 6.0,and 32%-43%at pH 8.3 over a 20-week period.The ecotoxicity study suggested that safety of the synthesized polyesters for the eisenia foetida.These results indicate that these polyesters have a combination of good thermal and degradability behaviors,which can be tailored through selection of the diol monomers used in the synthesis. | SUN Xin CHENG Zhengzai DJOUONKEP Lesly Dasilva Wandji LAN Chupeng JIA Ruyan ZENG Sheng CHENG Junpeng TANG Ran LI Yi YUAN Beibei GAUTHLLER Mario | 2023 | Journal of Wuhan University of Technology(Materials Science)2023，38，2： | 0 |
| 20 | Artificial intelligence-based non-invasive tumorsegmentation, grade stratification and prognosisprediction for clear-cell renal-cell carcinoma显示文摘Due to the complicated histopathological characteristics of clear-cell renal-cell carcinoma(ccRcC),non-invasive prognosis before operative treatment is crucial in selecting the appropriate treatment.A total of 126345 computerized tomography(cT)images from four independent patient cohorts were included for analysis in this study.We propose a V Bottieneck multi-resolution and focus-organ network(VB-MrFo-Net)using a cascade framework for deep learning analysis.The VB-MrFo-Net achieved better performance than VB-Net in tumor segmentation,with a Dice score of 0.87.The nuclear-grade prediction model performed best in the logistic regression classifier,with area under curve values from 0.782 to 0.746.Survival analysis revealed that our prediction model could significantly distinguish patients with high survival risk,with a hazard ratio(HR)of 2.49[95%confidence interval(CI):1.13-5.45,P=0.023]in the General cohort.Excellent performance had also been verified in the Cancer Genome Atlas cohort,the Clinical Proteomic Tumor Analysis Consortium cohort,and the Kidney Tumor Segmentation Challenge cohort,with HRs of 2.77(95%CI:1.58-4.84,P=0.0019),3.83(95%CI:1.22-11.96,P=0.029),and 2.80(95%CI:1.05-7.47,P=0.025),respectively.In conclusion,we propose a novel VB-MrFo-Net for the renal tumor segmentation and automatic diagnosis of ccRcc.The risk stratification model could accurately distinguish patients with high tumor grade and high survival risk based on non-invasive CT images before surgical treatments,which couid provide practical advicefordecidingtreatmentoptions. | Siteng Chen Dandan Song Lei Chen Tuanjie Guo Beibei Jiang Aie Liu Xianpan Pan Tao Wang Heting Tang Guihua Chen Zhong Xue Xiang Wang Ning Zhang Junhua Zheng | 2023 | Precision Clinical Medicine2023，6，3： | 0 |
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