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| 1 | Simultaneous oxidation of NO,SO_2 and Hg^0 from flue gas by pulsed corona discharge显示文摘A process capable of simultaneously oxidizing NO,SO2,and Hg0 was proposed,using a high-voltage and short-duration positive pulsed corona discharge.By focusing on NO,SO2,and Hg0 oxidation effciencies,the influences of pulse peak voltage,pulse frequency,initial concentration,electrode number,residence time and water vapor addition were investigated.The results indicate that NO,SO2 and Hg0 oxidation effciencies depend primarily on the radicals(OH,HO2,O) and the active species(O3,H2O2,etc.) produced by the pulsed corona discharge.The NO,SO2 and Hg0 oxidation effciencies could be improved as pulse peak voltage,pulse frequency,electrode number and residence time increased,but they were reduced with increasing initial concentrations.By adding water vapor,the SO2 oxidation effciency was improved remarkably,while the NO oxidation effciency decreased slightly.In our experiments,the simultaneous NO,SO2,and Hg0 oxidation effciencies reached to 40%,98%,and 55% with the initial concentrations 479 mg/m3,1040 mg/m3,and 15.0 μg/m3,respectively. | XU Fei,LUO Zhongyang,CAO Wei,WANG Peng,WEI Bo,GAO Xiang,FANG Mengxiang,CEN Kefa State key Laboratory of Clean Energy Utilization,Zhejiang University,Hangzhou 310027,China. | 2009 | Journal of Environmental Sciences2009，21，3： | 22 |
| 2 | Research on coal staged conversion poly-generation system based on fluidized bed显示文摘A new coal staged conversion poly-generation system combined coal combustion and pyrolysis has been developed for clean and high efficient utilization of coal.Coal is the first pyrolysed in a fluidized pyrolyzer.The pyrolysis gas is then purified and used for chemical product or liquid fuel production.Tar is collected during purification and can be processed to extract high value product and to make liquid fuels by hydro-refining.Semi-coke from the pyrolysis reactor is burned in a circulating fluidized bed(CFB)combustor for heat or power generation.The system can realize coal multiproduct generation and has a great potential to increase coal utilization value.A 1 MW poly-generation system pilot plant and a 12 MW CFB gas,tar,heat and power poly-generation system was erected.The experimental study focused on the two fluidized bed operation and characterization of gas,tar and char yields and compositions.The results showed that the system could operate stable,and produce about 0.12 m^(3)/kg gas with 22 MJ/m^(3)heating value and about 10 wt%tar when using Huainan bituminous coal under pyrolysis temperature between 500 and 600℃.The produced gases were mainly H_(2),CH_(4),CO,CO_(2),C_(2)H_(4),C_(2)H_(6),C_(3)H_(6)and C_(3)H_(8).The CFB combustor can burn semi-coke steadily.The application prospect of the new system was discussed. | Mingjiang Ni Chao Li Mengxiang Fang Qinhui Wang Zhongyang Luo Kefa Cen | 2014 | International Journal of Coal Science & Technology2014，1，1： | 13 |
| 3 | A comprehensive CFD combustion model for supercritical CFB boilers显示文摘A combustion model of a large-scale supercritical circulati ng fluidized bed (CFB) boiler was developed for comprehensive computational-fluid-dynamics analysis. The model incorporates gas-solid hydrodynamics, coal combustion, heat transfer on heat exchange surfaces in the furnace, and heat transfer between fumace and working medium in the heat transfer tubes. In simulating the dense and dilute phases in the fumace, the gas-solid hydrodynamics is based on the Euler-Euler model and energy-minimization multiscale drag model. Coal combustion entails evaporation, devolatilization, char combustion, gas homoge neous reaction, and pollutant emission. The coefficient ofheat transfer between gas-solid and the waterwall is estimated using the cluster renewal model, and for radiation, the discrete ordinate model is used. Moreover, thermohydraulic processes in the membrane wall are also in eluded in the heat transfer process. The model was successfully applied in simulations of a 350-MW supercritical CFB boiler. Detailed distributions of solids concentration, oxygen, heat flux, and working medium temperature in the boiler furnace are presented. | Linjie Xu Leming Cheng JieqiangJi Qinhui Wang Mengxiang Fang | 2019 | Particuology2019，17，2： | 5 |
| 4 | Predictions of NOx/N2O emissions from an ultra-supercritical CFB boiler using a 2-D comprehensive CFD combustion model显示文摘NOx and N2O emissions from an ultra-supercritical circulating fluidized bed(CFB)boiler were predicted using a two dimensional(2-D)comprehensive computational fluid dynamics(CFD)combustion model.This model was developed from a three dimensional model for a supercritical CFB boiler previously constructed by our group.Based on an analysis of the NOx and N2O conversion processes in a CFB boiler,the primary formation and destruction reactions were introduced into the 2-D model and coupled.The resulting model was validated using data from the Baima 600 MW supercritical CFB boiler,and then applied to a 660 MW ultra-supercritical CFB boiler.The effects of excess air,the secondary air(SA)to(primary air(PA)plus SA)ratio and the SA injection height on NOx and N2O emissions were investigated.The results show that a higher excess air volume increases both NOx and N2O emissions,while increasing the SA/(PA+SA)ratio somewhat reduces both the NOx and N2O concentrations.On the basis of the results of this work,optimal locations for SA injection ports so as to lower NOx and N2O emissions are recommended. | Jieqiang Ji Leming Cheng Yangjun Wei Junfeng Wang Xinyu Gao Mengxiang Fang Qinhui Wang | 2020 | Particuology2020，18，2： | 4 |
| 5 | Effects of CO_(2)atmosphere on slow pyrolysis of high-ash lignite显示文摘Slow pyrolysis of a typical high-ash lignite in China was carried out in atmospheres of N_(2),20%CO_(2)/N_(2),40%CO_(2)/N_(2),and 60%CO_(2)/N_(2)in a fixed bed reactor.The evolution of char,tar,and gases in yield and characteristics,and the physico-chemical characteristics of chars in different atmospheres were compared.Results revealed that CO_(2)almost behaves as an inert gas in the evolution of char and CO before 600℃.The decrease in char and CO_(2)yields and the increase in CO yield at temperatures higher than 600℃are ascribed to the occurrence of char-CO_(2)gasification.The higher the CO_(2)level present in the atmosphere,the higher the severity of the gasification becomes.Introducing CO_(2)into the atmosphere raises tar and water yields but cuts down H_(2),CH_(4),and C_(2)H_(6)yields.The promotion of tar yield results from the higher phenols and aliphatics yields in the presence of CO_(2).The reduction of H_(2)yield is associated with the increase in water yield,while the decline of light hydrocarbon gases is connected with the suppression effects of CO_(2)on methyl decomposition.The role of inherent minerals was also investigated by comparing product yields from raw coal and demineralized coal.The comparison indicated that the char-CO_(2)gasification rate is sharply reduced to nearly zero without the catalytic effects of calcium,iron,and magnesium minerals.The evolution of tar and light hydrocarbon gases in the CO_(2)-containing atmosphere greatly depends on inherent minerals.Without minerals,tar yield is inhibited in the presence of CO_(2).In the absence of minerals,CO_(2)hardly has influences on CH_(4)and C_(2)H_(6)yields. | Qinhui Wang Kaikun Li Zhihang Guo Mengxiang Fang Zhongyang Luo Kefa Cen | 2018 | Carbon Resources Conversion2018，1，1： | 4 |
| 6 | Anti-wear beam effects on gas-solid hydrodynamics in a circulating fluidized bed显示文摘Anti-wear beams installed on water walls of circulating fluidized bed(CFB) boilers are one of the most effective ways to protect against water-wall erosion.Beam effects from,for example,beam size and superficial gas velocity were investigated on gas-solid hydrodynamics in a CFB test rig using CFD simulations and experimental methods.The downward flow of the wall layer solids is observed to be disrupted by the beam but is then restored some distance further downstream.When falling solids from the wall layer hit the anti-wear beam,the velocity of the falling solids decreases rapidly.A fraction of the solids accumulates on the beam.Below the beams,the falling solids have reduced velocities but upward-moving solids were observed on the wall.The effect of the beam increases with width and superficial gas velocity.Wear occurs mainly above the beam and its variation with width is different above to below the beam.There is an optimum width that,when combined with beam height,results in less erosion. | Yunfei Xia Leming Cheng Chunjiang Yu Linjie Xu Qinhui Wang Mengxiang Fang | 2015 | Particuology2015，13，2： | 3 |
| 7 | Rotation speed measurement of moving particles in a CFB riser显示文摘This paper presents a study on measuring rotation speed of moving glass beads with an average diameter of 500 m in a pilot-scale circulating fluidized bed (CFB) riser with a high-speed digital imaging system. Two methods have been developed to calculate particle rotation speed from the particle images. The first method consists of a fully automated algorithm based on cross-correlation of gray distribution of particle images for particles whose rotation axes are (nearly) perpendicular to the imaging plane, and the second method calculates the speed of particle rotation by identifying its rotation axis using two or more characteristic points on its surface. The reliability of the two methods is verified by using a small sphere with known speed and direction of rotation. The first method is shown to be capable of measuring accurately the rotation speed for the particle with a rotation axis (nearly) perpendicular to the imaging plane and filtering off other particles using an appropriate threshold of correlation coefficient. The second method is shown to be capable of yielding both the speed and direction of particle rotation, with a measurement error of less than 10%. Results of both methods on real glass beads in a CFB riser are compared against each other. | Xuecheng Wu Qinhui Wang Zhongyang Luo Mengxiang Fang Kefa Cen | 2009 | Particuology2009，7，4： | 3 |
| 8 | Experimental study on the separation of CO2 from flue gas using hollow fiber membrane contactors without wetting显示文摘 | YAN Shuiping FANG Mengxiang ZHANG Weifeng | | 0，，5： | 1 |
| 9 | Investigation of the Evolution Behavior of Light Tar During Bituminous Coal Pyrolysis in a Fluidized Bed Reactor显示文摘The evolution behavior of the light tar fraction of tar during large bituminous coal particle pyrolysis in afluidized bed reactor at 500--900 ℃ was investigated to optimize the industrial process. The coal residence time wasvaried from 30 s to 150 s. The crude tar obtained was distilled and separated into the light fraction and the heavyfraction through an evaporator under conditions of 280 ℃ and 104 Pa. The light tar was subjected to GC-MS analysis,and the 300 main species in each spectrum were determined and analyzed. The experimental results showed that theevolution behavior of the light tar fraction and the heavy tar fraction presented spectacularly different variation trendswith pyrolysis temperature and coal residence time. The molecular weight and number of rings per aromatic com-pound molecule contained in the light tar fraction increased with increasing pyrolysis temperature because of poly-merization. It was also observed that the amount of methyl substituents decreased with an increasing number of ringsper molecule of poly-aromatic ring compounds. The chain aliphatic compound evolution was suppressed and under-went heterocyclization with increasing temperature. | LI Chao FANG Mengxiang XIAO Ping SHI Zhenghai CEN Jianmeng YAN Qike WANG Qinhui LUO Zhongyang | 2016 | Chemical Research in Chinese Universities2016，32，6： | 1 |
| 10 | Development of a new external heat exchanger for a circulating fluidized bed boiler 显示文摘 | Wang Qinhui Luo Zhongyang Fang Mengxiang | 2003 | Chemical Engineering and Processing2003，42，4： | 1 |
| 11 | A multi-product cogeneration system using combined coal gasification and combustion 显示文摘 | Fang Mengxiang Luo Zhongyang Li Xuantian | 1998 | Energy1998，23，3： | 1 |
| 12 | C02 desorption from rich alkanolamine solutionby using membrane vacuum regeneration technology显示文摘 | FANG Mengxiang WANG Zhen YAN Shuiping etal | 2012 | International Journal of Greenhouse Gas Control2012，9，： | 1 |
| 13 | Regeneration of CO2 from CO2-rich alkanolamines solution by using reduced thickness and vacuum technology: regeneration feasibility and characteristic of thin-layer solvent 显示文摘 | Yan Shuiping Fang Mengxiang Luo Zhongyang | 2009 | Chemical Engineering and Processing: Process Intensification2009，48，1： | 1 |
| 14 | Regeneration of CO2 from CO2 - rich alkanolamines solution by using reduced thickness and vacuum technology: Regeneration feasibility and characteristic of thin - layer solvent 显示文摘 | Shuiping Yan Mengxiang Fang Zhongyang Luo | 2009 | Chemical Engineering and Processing2009，48，1： | 1 |
| 15 | Mild Hydrotreatment of Low Temperature Coal Tar Distillate:Product Composition显示文摘 | Tang Wei Fang Mengxiang Wang Hongyan | | 0，，01： | 1 |
| 16 | Kinetic study on pyrolysis and combustion of wood under different oxygen concentrations by using TG-FTIR analysis 显示文摘 | Fang Mengxiang Shen Dekui Li Yingxu | 2006 | Journal of Analytical and Applied Pyrolysis2006，，77： | 1 |
| 17 | A multiproduct cogeneration system using combined coal gasification and combustion显示文摘 | Fang Mengxiang Luo Zhongyang Li Xuantian | 1998 | Energy1998，23，3： | 1 |
| 18 | Mild hydrotreatment of low temperature coal tar distillate:Product composition显示文摘 | Tang Wei Fang Mengxiang Wang Hongyan | 2014 | Chem Eng J2014，236，2： | 1 |
| 19 | Experimental study on the separation of CO2 from flue gas using hollow fiber membrane contactors without wetting显示文摘 | Yan Shuiping Fang Mengxiang Zhang Weifeng Wang Shuyuan Xu Zhikang Luo Zhongyang Cen Kefa | | 0，，： | 1 |
| 20 | A multi-product cogeneration system using combined coal gasification and combustion显示文摘 | FANG Mengxiang LUO Zhongyang LI Xutian | 1998 | Energy1998，23，3： | 1 |
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