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| 1 | Modeling of degradation kinetics of Salvianolic acid B at different temperatures and pH values显示文摘In this work,the effects of degradation time,temperature,and pH value on the degradation of Salvianolic acid B in aqueous solution were determined.Higher pH values,higher extraction temperature,and longer extraction time led to more degradation of Salvianolic acid B.Danshensu concentration increased as Salvianolic acid B degraded.A mechanism model was developed considering the degradation of Salvianolic acid E and lithospermic acid,which were two degradation products of Salvianolic acid B.The reverse reactions of Salvianolic acid B degradation were also considered.Degradation kinetic constants were calibrated.The degradation kinetics of Salvianolic acid B,lithospermic acid,and Danshensu in a Salvia miltiorrhiza extract aqueous solution were predicted using the mechanism model.The predicted concentrations agreed well with the experimental results.This model was developed using degradation data obtained from simple composition systems,but it can be applied in a complex botanical mixture with high prediction accuracy. | Xingchu Gong Shichao Huang Jianyang Pan Haibin Qu | 2017 | Chinese Journal of Chemical Engineering2017，25，1： | 16 |
| 2 | Enhancing both selectivity and coking-resistance of a single-atom Pd1/C3N4 catalyst for acetylene hydrogenation显示文摘选择加氢是在化学升级的一个重要工业催化过程,在因为他们的高加氢活动,基于 Pd 的催化剂广泛地被使用的地方。然而,因为重焦炭形成,差的选择和短催化剂一生是主要担心。在这个工作,原子地驱散 Pd 原子成功地在 graphitic 碳氮化物上被综合(g-C 3 用原子层免职的 N 4) 。没有 Pd nanoparticle (NP ) ,改正错误的高角度的环形的黑暗地的扫描传播电子显微镜学(HAADF 茎) 证实了孤立的 Pd 原子的主导的存在形成。在在过量乙烯的乙炔的选择加氢期间, g-C 3 N 4-supported Pd NP 催化剂比常规 Pd/Al 2 O 3 和 Pd/SiO 2 催化剂。在原处, X 光检查光致核裂变光谱学表明可观的费用从 Pd NP 转到 g-C 3 N 4 多半在催化表演改进起一个重要作用。更给人深刻印象地,单个原子的 Pd 1/C3 N 4 催化剂展出了两种更高的乙烯选择和更高的 coking 抵抗。我们的工作证明单个原子的 Pd 催化剂是在加氢反应改进选择和焦炭抵抗的一个有希望的候选人。 | Xiaohui Huang Yujia Xia Yuanjie Cao Xusheng Zheng Haibin Pan Junfa Zhu Chao Ma Hengwei Wang Junjie Li Rui You Shiqiang Wei Weixin Huang Junling Lu | 2017 | Nano Research2017，10，4： | 16 |
| 3 | Electronic structure of ZnO and its defects显示文摘 | Xu Pengshou Sun Yuming Shi Chaoshu Xu Faqiang Pan Haibin | 2001 | Science in China Series A: Mathematics2001，，9： | 1 |
| 4 | Using sediment seed banks and historical vegetation change data to develop restoration criteria for a eutrophic lake in China显示文摘 | Jing Lu Haibin Wang Min Pan Jing Xia Wei Xing Guihua Liu | 2011 | Ecological Engineering2011，，： | 1 |
| 5 | Theoretical calculations on the atomic and electronic structure of β-SiC(110) surface显示文摘We present a theoretical calculation of the atomic and electronic structure of β-SiC and its non-polar (110) surface using the full potential linear augmented plane wave (FPLAPW) approach. The calculated lattice constant and bulk modulus of p-SiC crystal are in excellent agreement with experimental data. The atomic and electronic structure of β-SiC(110) surface has been calculated by employing the slab and supercell model. It is found that the surface is characterized by a top-layer bond-length-contracting rotation relaxation in which the Si-surface atom moves closer towards the substrate while the C-surface atom moves outward. This relaxation is analogous to that of Ⅲ-Ⅴ semiconductor surface. The driving mechanism for this atomic rearrangement is that the Si atom tends to a planar sp2-like bonding situation with its three N neighbors and the N atom tends to a p3-like bonding with its three Si neighbors. Furthermore, surface relaxation induces the change from metallic to semiconducting | Changkun Xie Pengshou Xu Faqiang Xu Haibin Pan | 2002 | Chinese Science Bulletin2002，47，10： | 1 |
| 6 | Electronic structure of ZnO and its defects显示文摘 | Xu Pengshou Sun Yuming Shi Chaoshu Xu Faqiang Pan Haibin | 2001 | Science in China Series A: Mathematics2001，，9： | 1 |
| 7 | Science with the 2.5-meter Wide Field Survey Telescope(WFST)显示文摘The Wide Field Survey Telescope(WFST) is a dedicated photometric surveying facility being built jointly by University of Science and Technology of China(USTC) and the Purple Mountain Observatory(PMO). It is equipped with a 2.5-meter diameter primary mirror, an active optics system, and a mosaic CCD camera with 0.73 gigapixels on the primary focal plane for highquality image capture over a 6.5-square-degree field of view. The installation of WFST near the summit of Saishiteng mountain in the Lenghu region is scheduled in summer of 2023, and the operation is planned to start three months later. WFST will scan the northern sky in four optical bands(u, g, r and i) at cadences from hourly/daily in the deep high-cadence survey(DHS) program, to semi-weekly in the wide field survey(WFS) program. During a photometric night, a nominal 30 s exposure in the WFS program will reach a depth of 22.27, 23.32, 22.84, and 22.31(AB magnitudes) in these four bands, respectively, allowing for the detection of a tremendous amount of transients in the low-z universe and a systematic investigation of the variability of Galactic and extragalactic objects. In the DHS program, intranight 90 s exposures as deep as 23(u) and 24 mag(g), in combination with target of opportunity follow-ups, will provide a unique opportunity to explore energetic transients in demand for high sensitivities, including the electromagnetic counterparts of gravitational wave events, supernovae within a few hours of their explosions,tidal disruption events and fast, luminous optical transients even beyond redshift of unity. In addition, the final 6-year co-added images, anticipated to reach g■25.8 mag in WFS or 1.5 mags deeper in DHS, will be of fundamental importance to general Galactic and extragalactic science. The highly uniform legacy surveys of WFST will serve as an indispensable complement to those of the Vera C. Rubin Observatory's Legacy Survey of Space and Time(LSST) that monitors the southern sky. | Tinggui Wang Guilin Liu Zhenyi Cai Jinjun Geng Min Fang Haoning He Ji-an Jiang Ning Jiang Xu Kong Bin Li Ye Li Wentao Luo Zhizheng Pan Xuefeng Wu Ji Yang Jiming Yu Xianzhong Zheng Qingfeng Zhu Yi-Fu Cai Yuanyuan Chen Zhiwei Chen Zigao Dai Lulu Fan Yizhong Fan Wenjuan Fang Zhicheng He Lei Hu Maokai Hu Zhiping Jin Zhibo Jiang Guoliang Li Fan Li Xuzhi Li Runduo Liang Zheyu Lin Qingzhong Liu Wenhao Liu Zhengyan Liu Wei Liu Yao Liu Zheng Lou Han Qu Zhenfeng Sheng Jianchun Shi Yiping Shu Zhenbo Su Tianrui Sun Hongchi Wang Huiyuan Wang Jian Wang Junxian Wang Daming Wei Junjie Wei Yongquan Xue Jingzhi Yan Chao Yang Ye Yuan Yefei Yuan Hongxin Zhang Miaomiao Zhang Haibin Zhao Wen Zhao | 2023 | Science China(Physics,Mechanics & Astronomy)2023，66，10： | 1 |
| 8 | Electronic structure of ZnO and its defects显示文摘 | Pengshou Xu Yuming Sun Chaoshu Shi Faqiang Xu Haibin Pan | | 0，，： | 1 |
| 9 | An experimental method to obtain the hard alpha anomaly distribution for titanium alloy aeroengine disks显示文摘A probability-based damage tolerance methodology has been proposed to improve the recognition of material anomalies, especially hard alpha(TiN) anomalies for aeroengine rotor disks. A key input to this method is hard alpha anomaly distribution, which reflects the occurrence rate and size of anomalies present in the finished part material of titanium rotors. Since anomalies rarely occur naturally, an experimental method is proposed to obtain the anomaly distribution for titanium alloy aeroengine disks to reflect and equivalently replace the manufacturing development in titanium industry. In general, the anomaly distribution information can be divided into two parts: the Probability of Detection(POD) curve and the detected anomaly distribution, which contains the size and frequency data of the detected anomalies. The distribution can be established based on several appropriate assumptions and derivation steps with different confidence levels of POD curves and detected anomaly distributions. In this case, the distribution can be obtained in a relatively short time as a key input to the probability-based damage tolerance methodology. Then the Probability of Failure(POF) can be calculated, and the value is found to vary with different confidence levels. On this basis, the conservative estimated POF can be obtained in conjunction with confidence levels. | Shuiting DING Huimin ZHOU Bochao PAN Haibin JI Xiaojun GUO Guo LI | 2021 | Chinese Journal of Aeronautics2021，34，4： | 1 |
| 10 | Bipartite consensus problem on matrix-valued weighted directed networks显示文摘Dear editor,Consensus turns out to be an important paradigm in coordination of multi-agent systems [1]. Previous studies largely concentrate on consensus problem over networks where the weights on edges are scalars, which cannot completely characterize the correlation of different dimensions corresponding to the state of an agent in the network. | Lulu PAN Haibin SHAO Yugeng XI Dewei LI | 2021 | Science China(Information Sciences)2021，64，4： | 1 |
| 11 | Development and Validation of a Column-Switching LC–ESI–MS Assay for Determination of Huperzine?A in Rat Plasma and Cerebrospinal Fluid显示文摘 | Jianyang Pan Qiao Wang Qing Shao Yiyu Cheng Haibin Qu | 2009 | Chromatographia (-)2009，，5： | 1 |
| 12 | Oxygen modified CoP2 supported palladium nanoparticles as highly efficient catalyst for hydrolysis of ammonia borane显示文摘Ammonia borane(AB)is regarded as a promising chemical hydrogen-storage material due to its high hydrogen content,nontoxicity,and long-term stability under ambient temperature.However,constructing advanced catalysts to further promote the hydrogen production still remains a challenge for the hydrolysis of AB.Herein,we report a novel oxygen modified CoP_(2)(O-CoP_(2))material with dispersed palladium nanoparticles(Pd NPs)as a highly efficient and sustainable catalyst for AB hydrolysis.The modification of oxygen could optimize the catalytic synergy effect between CoP_(2)and Pd NPs,achieving enhanced catalytic activity with a turnover frequency(TOF)number of 532 min^(-1)and an activation energy(E_(a))value of 16.79 kJ·mol^(-1).Meanwhile,reaction kinetic experiments prove that the activation of water is the rate-determining step(RDS).The water activation mechanism is revealed by quasi in-situ X-ray photoelectron spectroscopy(XPS)and in-situ X-ray absorption fine structure(XAFS)measurements.The activation of water leads to the production of-H and-OH groups,which are further adsorbed on the oxygen atoms in P-O bond and Pd atoms,respectively.In addition,density functional theory(DFT)calculations indicate that the introduced oxygen facilitates the adsorption and activation of water molecules.This novel modulation strategy successfully sheds new light on the development of advanced catalysts for hydrolysis of AB and beyond. | Leijie Zhang Jian Ye Yi Tu Qingyu Wang Haibin Pan Lihui Wu Xusheng Zheng Junfa Zhu | 2022 | Nano Research2022，15，4： | 1 |
| 13 | Generating oxygen adatoms on Au(997) by thermal decomposition of NO_2显示文摘We report our investigation of the interaction of NO2 with the Au(997)vicinal surface by high-resolution photoelectron spectroscopy using synchrotron radiation as the excitation source.At 170 K,both core-level and valence-band photoemission results illustrate the decomposition of NO2 on the Au(997)surface at low NO2 exposures,forming coadsorbed NO(a)and O(a)species.After annealing at 300 K,NO(a)desorbs from Au(997)whereas O(a)remains on the surface.Upon annealing at 750 K,we observe no signal for adsorbed oxygen on Au(997).These results clearly demonstrate that thermal decomposition of NO2 is an effective method to generate oxygen adatoms on Au(997)under ultrahigh-vacuum conditions. | ZHANG YuLin WU ZongFang CHEN BoHao XU LingShun PAN HaiBin MA YunSheng JIANG ZhiQuan ZHU JunFa HUANG WeiXin | 2010 | Chinese Science Bulletin2010，55，34： | 0 |
| 14 | A likely autotetraploidization event shaped the Chinese mahogany(Toona sinensis)genome显示文摘Chinese mahogany(Toona sinensis) is of considerable medical and economic importance, and its genome has been deciphered. However, the process underlying its polyploidy is unclear, and the chromosomal evolutionary trajectory is poorly understood. Here, by reanalysing the T.sinensis genome, we found evidence of a tetraploidization event(T. sinensis special tetraploidization, TST) that occurred approximately 15-17 million years ago(MYA) after the core eudicot-common hexaploidization(ECH or gamma) event. We characterized the synonymous nucleotide substitution rates(Ks values) of collinear genes and found that T. sinensis genes affected by the TST evolve at a slower rate than Acer yangbiense genes. Furthermore, we identified homologous genes related to polyploidization and speciation and constructed multiple alignments with different reference genomes. Notably, the significant balance of gene retention and loss characterized in the two TST-derived subgenomes suggests an autopolyploid nature of the TST. Moreover, we deduced the chromosomal karyotypes of the two subgenomes and identified 7chromosomal fusions that have shaped the T. sinensis genome;more information is available on a newly constructed karyotype platform(http://gffzze84c5b42976d4cd7h9kck5x9fn0oq69vn.ffgz.tsg.suse.edu.cn/Toona_sinensis/index.html). The T. sinensis genome preserves the ancestral chromosome structure of dicotyledons well and could serve as a good reference for understanding genomic changes in other Meliaceae and Sapindales plants. In addition, we verified that tandem duplication and the ECH have promoted the expansion of terpene synthase(TPS) genes;conversely, the TST seems to have inhibited expansion of these genes. This present effort has clarified the polyploidy events of the T. sinensis genome, filled gaps in the history of karyotype evolution, and laid a solid foundation for further genomic studies in the Meliaceae research community and beyond. | Jianyu Wang Ziyi Yang Tianyu Lei Yan Zhang Qimeng Xiao Zijian Yu Jiaqi Zhang Sangrong Sun Qiang Xu Shaoqi Shen Zimo Yan Mengnan Fang Yue Ding Zihan Liu Qianwen Zhu Ke Ren Yuxin Pan Haibin Liu Jinpeng Wang | 2023 | Horticultural Plant Journal2023，9，2： | 0 |
| 15 | Low-coordination environment design of single Co atoms for efficient CO_(2) photoreduction显示文摘Photocatalytic carbon dioxide(CO_(2))to carbon monoxide(CO)offers a promising way for both alleviating the greenhouse effect and meeting the industrial demand.Herein,we constructed a Co single-atom catalyst with intentional low-coordination environment design on porous ZnO(denoted as Co1/ZnO).Impressively,Co1/ZnO exhibited a remarkable activity with a CO yield rate of 22.25 mmol·g^(-1)·h^(-1) and a selectivity of 80.2%for CO_(2) photoreduction reactions under visible light.The incorporation of single Co atoms provided an additional photo-generated electron transfer channel,which suppressed the carrier recombination of photocatalysts.Moreover,the unsaturated Co active sites were capable to adsorb CO_(2) molecule spontaneously,thus facilitating the activation of CO_(2) molecule during CO_(2) reduction course. | Zhentao Ma Qingyu Wang Limin Liu Rong-Ao Zhang Qichen Liu Peigen Liu Lihui Wu Chengyuan Liu Yu Bai Yida Zhang Haibin Pan Xusheng Zheng | 2024 | Nano Research2024，17，5： | 0 |
| 16 | Typical Application Scenarios and Economic Benefit Evaluation Methods of Battery Energy Storage System显示文摘Energy storage system is an important means to improve the flexibility and safety of traditional power system,but it has the problem of high cost and unclear value recovery path.In this paper,the typical application scenarios of energy storage system are summarized and analyzed from the perspectives of user side,power grid side and power generation side.Based on the typical application scenarios,the economic benefit assessment framework of energy storage system including value,time and efficiency indicators is proposed.Typical battery energy storage projects are selected for economic benefit calculation according to different scenarios,and key factors are selected for sensitivity analysis.Finally,the key factors affecting economic benefit of the energy storage system are analyzed. | Ming Zeng Haibin Cao Ting Pan Pinduan Hu Shi Tian Lijun Zhong Zhi Ling | 2022 | Energy Engineering2022，119，4： | 0 |
| 17 | Grain boundaries modulating active sites in RhCo porous nanospheres for efficient CO2 hydrogenation显示文摘 | Xusheng Zheng Yue Lin Haibin Pan Lihui Wu Wei Zhang Linlin Cao Jing Zhang Lirong Zheng Tao Yao | 2018 | Nano Research2018，11，5： | 0 |
| 18 | The residues 4 to 6 at the N-terminus in particular modulate fibril propagation of β_(2)-microglobulin显示文摘The ΔN6 truncation is the main posttranslational modification of β_(2)-microglobulin( β_(2)M)found in dialysis-related amyloid.Investigation of the interaction of wild-type(WT) β_(2)M with N-terminally truncated variants is therefore of medical relevance.However,it is unclear which residues among the six residues at the N-terminus are crucial to the interactions and the modulation of amyloid fibril propagation of β_(2)M.We herein analyzed homo-and heterotypic seeding of amyloid fibrils of WT human β_(2)M and its N-terminally-truncated variantsΔN1 toΔN6,lacking up to six residues at the N-terminus.At acidic pH 2.5,we produced amyloid fibrils in vitro from recombinant,WT β_(2)M and its six truncated variants,and found thatΔN6 β_(2)M fibrils exhibit a significantly lower conformational stability than WT β_(2)M fibrils.Importantly,under more physiological conditions(pH 6.2),we assembled amyloid fibrils in vitro only from recombinant,ΔN4,ΔN5,andΔN6 β_(2)M but not from WT β_(2)M and its three truncated variantsΔN1 toΔN3.Notably,the removal of the six,five or four residues at the N-terminus leads to enhanced fibril formation,and homoand heterotypic seeding ofΔN6 fibrils strongly promotes amyloid fibril formation of WT β_(2)M and its six truncated variants,including at more physiological pH 6.2.Collectively,these results demonstrated that the residues 4 to 6 at the N-terminus particularly modulate amyloid fibril propagation of β_(2)M and the interactions of WT β_(2)M with Nterminally truncated variants,potentially indicating the direct relevance to the involvement of the protein’s aggregation in dialysis-related amyloidosis. | Haibin Dang Zhixian Chen Wang Chen Xudong Luo Pan Liu Liqiang Wang Jie Chen Xuhai Tang Zhengzhi Wang Yi Liang | 2022 | Acta Biochimica et Biophysica Sinica2022，54，2： | 0 |
| 19 | Unraveling the advantages of Pd/CeO_(2)single-atom catalysts in the NO+CO reaction by model catalysts显示文摘Selective catalytic reduction of NO by CO is challenging in environmental catalysis but attractive owing to the advantage of simultaneous elimination of NO and CO.Here,model catalysts consisting of Pd nanoparticles(NPs)and single-atom Pd supported on a CeO_(2)(111)film grown on Cu(111)(denoted as Pd NPs/CeO_(2)and Pd_(1)/CeO_(2),respectively)were successfully prepared and characterized by synchrotron radiation photoemission spectroscopy(SRPES)and infrared reflection absorption spectroscopy(IRAS).The NO+CO adsorption/reaction on the Pd_(1)/CeO_(2)and Pd NPs/CeO_(2)catalysts were carefully investigated using SRPES,temperature-programmed desorption(TPD),and IRAS.It is found that the reaction products on both model catalysts are in good agreement with those on real catalysts,demonstrating the good reliability of using these model catalysts to study the reaction mechanism of the NO+CO reaction.On the Pd NPs/CeO_(2)surface,N_(2)is formed by the combination of atomic N coming from the dissociation of NO on Pd NPs at higher temperatures.N_(2)O formation occurs probably via chemisorbed NO combined with atomic N on the surface.While on the single-atom Pd_(1)/CeO_(2)surface,no N_(2)O is detected.The 100%N_(2)selectivity may stem from the formation of O-N-N-O^(*)intermediate on the surface.Through this study,direct experimental evidence for the reaction mechanisms of the NO+CO reaction is provided,which supports the previous density functional theory(DFT)calculations. | Qian Xu Xingwang Cheng Ningqiang Zhang Yi Tu Lihui Wu Haibin Pan Jun Hu Honghe Ding Junfa Zhu Yadong Li | 2023 | Nano Research2023，16，7： | 0 |
| 20 | Protein O-GlcNAcylation homeostasis regulates facultative heterochromatin to fine-tune sog-Dpp signaling during Drosophila early embryogenesis显示文摘Protein O-GlcNAcylation is a monosaccharide post-translational modification maintained by two evolutionarily conserved enzymes, O-GlcNAc transferase (OGT) and O-GlcNAcase (OGA). Mutations in human OGT have recently been associated with neurodevelopmental disorders, although the mechanisms linking O-GlcNAc homeostasis to neurodevelopment are not understood. Here, we investigate the effects of perturbing protein O-GlcNAcylation using transgenic Drosophila lines that overexpress a highly active OGA. We reveal that temporal reduction of protein O-GlcNAcylation in early embryos leads to reduced brain size and olfactory learning in adult Drosophila. Downregulation of O-GlcNAcylation induced by the exogenous OGA activity promotes nuclear foci formation of Polycomb-group protein Polyhomeotic and the accumulation of excess K27 trimethylation of histone H3 (H3K27me3) at the mid-blastula transition. These changes interfere with the zygotic expression of several neurodevelopmental genes, particularly short gastrulation (sog), a component of an evolutionarily conserved sog-Decapentaplegic (Dpp) signaling system required for neuroectoderm specification. Our findings highlight the importance of early embryonic O-GlcNAcylation homeostasis for the fidelity of facultative heterochromatin redeployment and initial cell fate commitment of neuronal lineages, suggesting a possible mechanism underpinning OGT-associated intellectual disability. | Yaowen Zhang Haibin Yu Dandan Wang Xiaoyun Lei Yang Meng Na Zhang Fang Chen Lu Lv Qian Pan Hongtao Qin Zhuohua Zhang Daan M.F.van Aalten Kai Yuan | 2023 | Journal of Genetics and Genomics2023，50，12： | 0 |
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