5篇
您的检索式：作者名="Hongwei Shou"
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| 1 | Modified affine arithmetic is wore accurate than centered interval arithmetic or affine arithmetic显示文摘 | Huahao Shou Hongwei Lin Ralph Martin Guojin Wang | 2003 | Mathematics of Surfaces2003，2768，： | 1 |
| 2 | Probing self-optimization of carbon support in oxygen evolution reaction显示文摘Despite acknowledgment of structural reconstruction of materials following oxygen evolution reaction (OER) reaction, the role of support during the reconstruction process has been ignored. Given this, we directly in situ transform the residual iron present in raw single-walled carbon nanotubes (SWCNT) into Fe_(2)O_(3) and thus build Fe_(2)O_(3)-CNT as the model system. Intriguingly, an anomalous self-optimization occurred on SWCNT and the derived components show satisfactory electrochemical performance. Soft X-ray absorption spectroscopy (sXAS) analysis and theory calculation correspondingly indicate that self-optimization yields stronger interaction between SWCNT and Fe_(2)O_(3) nanoparticles, where the electrons migrate from Fe_(2)O_(3) to optimized SWCNT. Such polarization will generate a positive charge center and thus boost the OER activity. This finding directly observes the self-optimization of support effect, providing a new perspective for OER and related electrochemical reactions. | Wenjie Xu Dengfeng Cao Oyawale Adetunji Moses Beibei Sheng Chuanqiang Wu Hongwei Shou Xiaojun Wu Shuangming Chen Li Song | 2021 | Nano Research2021，14，12： | 1 |
| 3 | Support induced phase engineering toward superior electrocatalyst显示文摘The phase transformation of catalysts has been extensively observed in heterogeneous catalytic reactions that hinder the long cycling catalysis,and it remains a big challenge to precisely control the active phase during the complex conditions in electrochemical catalysis.Here,we theoretically predict that carbon-based support could achieve the phase engineering regulation of catalysts by suppressing specific phase transformation.Taken single-walled carbon nanotube(SWCNT)as typical support,combined with calculated E-pH(Pourbaix)diagram and advanced synchrotron-based characterizations technologies prove there are two different active phases source from cobalt selenide which demonstrate that the feasibility of using support effect regulating the potential advantageous catalysts.Moreover,it is worth noting that the phase engineering derived Co_(3)O_(4)-SWCNT exhibits a low overpotential of 201 mV for delivering the current density of 10 mA/cm^(2)in electrocatalytic oxygen evolution reaction(OER).Also,it reaches a record current density of 529 mA/cm^(2)at 1.63 V(vs.RHE)in the electrocatalytic urea oxidation reaction(UOR),overwhelming most previously reported catalysts. | Beibei Sheng Dengfeng Cao Hongwei Shou Oyawale Adetunji Moses Wenjie Xu Yujian Xia Yuzhu Zhou Huijuan Wang Ping Wan Shuang Zhu Wangsheng Chu Xiaojun Wu Shuangming Chen Li Song | 2022 | Nano Research2022，15，3： | 0 |
| 4 | Persistence of charge density wave against variation of band structures in V_(x)Ti_(1−x)Se_(2)(x=0–0.1)显示文摘Charge density wave(CDW)is a phenomenon that occurs in materials,accompanied by changes in their intrinsic electronic properties.The study of CDW and its modulation in materials holds tremendous significance in materials research,as it provides a unique approach to controlling the electronic properties of materials.TiSe_(2) is a typical layered material with a CDW phase at low temperatures.Through V substitution for Ti in TiSe_(2),we tuned the carrier concentration in V_(x)Ti_(1-x)Se_(2) to study how its electronic structures evolve.Angle-resolved photoemission spectroscopy(ARPES)shows that the band-folding effect is sustained with the doping level up to 10%,indicating the persistence of the CDW phase,even though the band structure is strikingly different from that of the parent compound TiSe_(2).Though CDW can induce the band fold effect with a driving force from the perspective of electronic systems,our studies suggest that this behavior could be maintained by lattice distortion of the CDW phase,even if band structures deviate from the electron-driven CDW scenario.Our work provides a constraint for understanding the CDW mechanism in TiSe_(2),and highlights the role of lattice distortion in the band-folding effect. | Zhanfeng Liu Tongrui Li Wen Zhu Hongwei Shou Mukhtar Lawan Adam Qilong Cui Yuliang Li Sheng Wang Yunbo Wu Hongen Zhu Yi Liu Shuangming Chen Xiaojun Wu Shengtao Cui Li Song Zhe Sun | 2024 | Nano Research2024，17，3： | 0 |
| 5 | Interfacial electronic interaction enabling exposed Pt(110)facets with high specific activity in hydrogen evolution reaction显示文摘To achieve a complete industrial chain of hydrogen energy,the development of efficient electrocatalysts for hydrogen evolution reaction(HER)is of great concerns.Herein,a nickel nitride supported platinum(Pt)catalyst with highly exposed Pt(110)facets(Pt_((110))-Ni_(3)N)is obtained for catalyzing HER.Combined X-ray spectra and density functional theory studies demonstrate that the interfacial electronic interaction between Pt and Ni3N support can promote the hydrogen evolution on Pt(110)facets by weakening hydrogen adsorption.As a result,the Pt_((110))-Ni_(3)N catalyst delivers an obviously higher specific activity than commercial 20 wt.%Pt/C in acidic media.This work suggests that the suitable interface modulation may play a vital role in rationally designing advanced electrocatalysts. | Sicong Qiao Qun He Quan Zhou Yuzhu Zhou Wenjie Xu Hongwei Shou Yuyang Cao Shuangming Chen Xiaojun Wu Li Song | 2023 | Nano Research2023，16，1： | 0 |
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