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| 1 | Malignant transformation of craniopharyngioma in an infradiaphragmatic case显示文摘Till now,13 cases of malignant craniopharyngioma (CP) have been reported around the world,including 11 cases of transformation from benign tumors and 2 cases of congenital ones.Irradiation seemed to contribute a lot to the cellular transformation.The controversies about the radical surgery or irradiation have not ceased for many decades.In this article,we report a case of infradiaphragmatic CP (Id-CP) in a child who experienced almost all current treatments.However,after multiple tumor recurrences,finally the malignant transformation occurred.The analysis of the tumor regrowth pattern and clinical characteristics provided some clues to standardize and individualize the treatment of Id-CP. | Lu Yuntao Qi Songtao Peng Junxiang Pan Jun Zhang Xi'an | 2014 | Chinese Medical Journal2014，，17： | 4 |
| 2 | Large-scale multiferroic complex oxide epitaxy with magnetically switched polarization enabled by solution processing显示文摘Complex oxides with tunable structures have many fascinating properties,though high-quality complex oxide epitaxy with precisely controlled composition is still out of reach.Here we have successfully developed solution-based single-crystalline epitaxy for multiferroic(1-x)BiTi(1-y)/2FeyMg(1-y)/2O3–(x)CaTiO3(BTFM–CTO)solid solution in large area,confirming its ferroelectricity at the atomic scale with strong spontaneous polarization.Careful compositional tuning leads to a bulk magnetization of 0.07±0.035μB/Fe at room temperature,enabling magnetically induced polarization switching exhibiting a large magnetoelectric coefficient of 2.7–3.0×10^-7 s/m.This work demonstrates the great potential of solution processing in large-scale complex oxide epitaxy and establishes novel room-temperature magnetoelectric coupling in epitaxial BTFM–CTO film,making it possible to explore a much wider space of composition,phase,and structure that can be easily scaled up for industrial applications. | Cong Liu Feng An Paria S.M.Gharavi Qinwen Lu Junkun Zha Chao Chen Liming Wang Xiaozhi Zhan Zedong Xu Yuan Zhang Ke Qu Junxiang Yao Yun Ou Zhiming Zhao Xiangli Zhong Dongwen Zhang Nagarajan Valanoor Lang Chen Tao Zhu Deyang Chen Xiaofang Zhai Peng Gao Tingting Jia Shuhong Xie Gaokuo Zhong Jiangyu Li | 2020 | National Science Review2020，7，1： | 2 |
| 3 | Light emission properties of sapphire under shock loading in the stress range of 40-120 GPa显示文摘The measurement of emissions from the window material of sapphire was performed through multi-wavelength pyrometer and spontaneous spectroscopic techniques in the pressure range of 40-120 GPa.The results showed that the spectral distribution with wavelength clearly fit well with the grey-body spectrum.We have analyzed the emissions and discovered they mostly came from the shear banding,which is a typical thermal radiation.The radiance intensity changing linearly with time revealed it was a volume effect.All of the data from pyrometer can be explained by the model of Boslough's study,especially for pressures over megabar.The color temperature of shocked sapphire changing with increased stress disagrees with the computed melt curve which is likely explained by the different phase structures of sapphire. | ZHANG NingChao LIU FuSheng PENG XiaoJuan ZHANG MingJian CHEN JunXiang | 2013 | Science China Chemistry2013，56，3： | 2 |
| 4 | Understanding the sluggish and highly variable transport kinetics of lithium ions in LiFePO_4显示文摘LiFePO_(4),one of the mainstream cathode materials of current EV batteries,exhibits experimental diffusion coefficients(D_(c))of Li^(+)which are not only several orders of magnitude lower than those predicted by the ionic hopping barriers obtained from theoretical calculations and spectroscopic measurements,but also span several orders from 10^(-14)to 10^(-18)cm^(2)s^(-1)under different states of charge(SOC)and the charging rates(C-rates).Atomic level understanding of such sluggishness and diversity of Li^(+)transport kinetics would be of significance in improving the rate performance of LiFePO_(4)through material and operation optimization but remain challenging.Herein,we show that the high sensitivity of Li^(+)hopping barriers on the local Li–Li coordination environments(numbers and configurations)plays a key role in the ion transport kinetics.This is due a neural network-based deep potential(DP)which allows accurate and efficient calculation of hopping barriers of Li^(+)in LiFePO_(4)with various Li–Li coordination environments,with which the kinetic Monte-Carlo(KMC)method was employed to determine the D_(c)values at various C-rates and SOC across a broad spectrum.Especially,an accelerated KMC simulation strategy is proposed to obtain the D_(c)values under a wide range of SOC at low C-rates,which agree well with that obtained from the galvanostatic intermittent titration technique(GITT).The present study provides accurate descriptions of Li^(+)transport kinetics at both very high and low C-rates,which remains challenging to experiments and first-principles calculations,respectively.Finally,it is revealed that the gradient distributions of Li^(+)density along the diffusion path result in great asymmetry in the barriers of the forward and backward hopping,causing very slow diffusion of Li^(+)and the diverse variation of D_(c). | Youcheng Hu Xiaoxiao Wang Peng Li Junxiang Chen Shengli Chen | 2023 | Science China Chemistry2023，66，11： | 0 |
| 5 | The Enhancement of Selectivity and Activity for Two-Electron Oxygen Reduction Reaction by Tuned Oxygen Defects on Amorphous Hydroxide Catalysts显示文摘Amorphous catalysts,thanks to their uniquely coordinated unsaturated properties and abundance of defect sites,tend to possess higher activity and selectivity than their crystalline counterparts.In this work,we report a facile and general solventcontrolled precipitation method to prepare hybrids of graphene oxide(GO)supporting amorphous metal hydroxide[A-M(OH)_(x)/GO,M=Cu,Co,and Mn],which provides us with tangible materials to study the structure–performance relationship of various amorphous oxides.The systematic investigation of A-Cu(OH)_(2)/GO by coupling ex situ/in situ characteristic techniques with electrochemical studies reveals that electrocatalytic activity and selectivity toward a two-electron oxygen reduction reaction(ORR)is highly dependent on the coordinated Cu catalytic sites and the disordered structure of A-Cu(OH)_(2).In situ X-ray absorption near-edge structure(XANES)and density functional theory(DFT)calculation verify that the degree of OH*poisoning(ΔG0 OH*)tuned by three-OH-coordinated Cu sites in amorphous structures plays a crucial role in selective catalysis of ORR for H_(2)O_(2) production.The optimized A-Cu(OH)_(2)/GO shows superior activity and high selectivity(~95%)toward H_(2)O_(2),as demonstrated by a zinc–air battery capable of on-site H_(2)O_(2) production with a rate as high as 3401.5 mmol h^(−1) g^(−1). | Junheng Huang Changle Fu Junxiang Chen Nangan Senthilkumar Xinxin Peng Zhenhai Wen | 2022 | CCS Chemistry2022，4，2： | 0 |
| 6 | Growth hormone promotes the reconstruction of injured axons in the hypothalamo-neurohypophyseal system显示文摘Previous studies have shown that growth hormone can regulate hypothalamic energy metabolism, stress, and hormone release. Therefore, growth hormone has great potential for treating hypothalamic injury. In this study, we established a specific hypothalamic axon injury model by inducing hypothalamic pituitary stalk electric lesions in male mice. We then treated mice by intraperitoneal administration of growth hormone. Our results showed that growth hormone increased the expression of insulin-like growth factor 1 and its receptors, and promoted the survival of hypothalamic neurons, axonal regeneration, and vascular reconstruction from the median eminence through the posterior pituitary. Altogether, this alleviated hypothalamic injury-caused central diabetes insipidus and anxiety. These results suggest that growth hormone can promote axonal reconstruction after hypothalamic injury by regulating the growth hormone-insulin-like growth factor 1 axis. | Kai Li Zhanpeng Feng Zhiwei Xiong Jun Pan Mingfeng Zhou Weizhao Li Yichao Ou Guangsen Wu Mengjie Che Haodong Gong Junjie Peng Xingqin Wang Songtao Qi Junxiang Peng | 2024 | Neural Regeneration Research2024，19，10： | 0 |
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