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| 1 | Portosplenomesenteric vein thrombosis in patients with early-stage severe acute pancreatitis显示文摘AIM To investigate the incidence and risk factors of portosplenomesenteric vein thrombosis(PSMVT) in the early stage of severe acute pancreatitis(SAP).METHODS Patients with SAP in a tertiary care setting from January 2014 to December 2016 were retrospectively reviewed. All contrast-enhanced computed tomography(CT) studies were reassessed and reviewed. Clinical outcome measures were compared between SAP patients with and without PSMVT in the early stage of the disease. Univariate and multivariate logistic regression analyses were sequentially performed to assess potential risk factors for the development of PSMVT in SAP patients. A receiver operating characteristic(ROC) curve was generated for the qualifying independent risk factors.RESULTS Twenty-five of the one hundred and forty(17.86%) SAP patients developed PSMVT 6.19 ± 2.43 d after acute pancreatitis(AP) onset. PSMVT was confirmed by contrast-enhanced CT. Multivariate stepwise logistic regression analyses showed that Balthazar's CT severity index(CTSI) scores [odds ratio(OR): 2.742; 95% confidence interval(CI): 1.664-4.519; P = 0.000], hypoalbuminemia(serum albumin level < 25 g/L)(OR: 32.573; 95%CI: 2.711-391.353; P = 0.006) and gastrointestinal wall thickening(OR: 4.367, 95%CI: 1.218-15.658; P = 0.024) were independent risk factors for PSMVT developed in patients with SAP. The area under the ROC curve for Balthazar's CTSI scores was 0.777(P = 0.000), the sensitivity was 52%, and the specificity was 93% at a cut-off value of 5.5.CONCLUSION High Balthazar's CTSI scores, hypoalbuminemia and gastrointestinal wall thickening are independent risk factors for PSMVT developed in the early stage of SAP. | Ling Ding Feng Deng Chen Yu Wen-Hua He Liang Xia Mi Zhou Xin Huang Yu-Peng Lei Xiao-Jiang Zhou Yin Zhu Nong-Hua Lu | 2018 | World Journal of Gastroenterology2018，24，35： | 20 |
| 2 | Arabidopsis NIP3;1 Plays an Important Role in Arsenic Uptake and Root-to-Shoot Translocation under Arsenite Stress Conditions显示文摘在 Arabidopsis, nodulin 26-like 内在的蛋白质(捏) aquaporin 蛋白质的亚科由九个成员,组成哪个中的五个(NIP1; 1, NIP1; 2, NIP5; 1, NIP6; 1,并且 NIP7; 1 ) 以前被识别对亚砷酸盐可渗透。然而,角色在植物在亚砷酸盐的 root-to-shoot translocation 捏仍然保持糟糕理解。在这研究,用反向的基因策略, Arabidopsis NIP3; 1 被识别在亚砷酸盐压力条件下面在砷举起和 root-to-shoot 分发起一个重要作用。nip3; 1 loss-of-function 异种在亚砷酸盐忍耐显示了明显的改进为未葬生长和积累的更少砷在野类型的植物比那些射击,而 nip3; 1 nip1; 1 两倍异种显示出强壮的亚砷酸盐忍耐并且在亚砷酸盐压力条件下面改进了根和射击的生长。一个倡导者 -- glucuronidase 分析揭示了那 NIP3; 1 几乎专门在根被表示(与根尖端的异常) ,并且在酵母 Saccharomyces cerevisiae 的 heterologous 表示表明了那 NIP3; 1 能调停亚砷酸盐运输。一起拿,我们的结果建议那 NIP3; 1 在 Arabidopsis 涉及亚砷酸盐举起和 root-to-shoot translocation,可能作为被动、双向的亚砷酸盐 transporter。 | WenzhongXu Wentao Dai Huili Yan Sheng Li Hongling Shen Yanshan Chen Hua Xu Yangyang Sun Zhenyan He Mi Ma | 2015 | Molecular Plant2015，8，5： | 13 |
| 3 | The distribution of the oil derived from Cambrian source rocks in Lunnan area,the Tarim Basin,China显示文摘There are great differences in biomarks between Cambrian oil and Middle-Upper Ordovician oil. In this stuty, the authors analyzed 40 oils found in Lunnan area by GC-MS and calculated the content of Cambrian oil in the 40 oils according to the steroid indexes of typical oil mixture and match experiment. The results show that it is a general phenomenon in Ordovician reservoir that the oil derived from Cambrian source rock mixed with the oil derived from Middle-Upper Ordovician source rock in Lunnan area, the mixture degree of the two oils is lower in Carboniferous reservoir than in Ordovician reservoir, and the oils kept in Triassic reservoir have single source, Middle-Upper Ordovician source rock. The mixture oils mainly composed of Cambrian oil (>50%) distributed in Sangtamu fault zone, and the oils found in Lunnan fault zone are Middle-Upper Ordovician oil. This distribution of oils in Lunnan area is owing to that Lunnan fault zone is located in anticline axis part, Lunnan fault zone underwent serious erosion, and the oils from Cambrian source rock accumulated in Lunnan fault zone were degraded completely during Caledonian-Hercynian movement. But the Cambrian oil accumulated in Sangtamu fault zone was not degraded completely and some of them were left for the location of Sangtamu fault zone is lower than Lunnan fault zone. Later, the oil derived from Middle-Upper Ordovician source rock mixed with the remained Cambrian oil, and the mixture oil formed in Sangtamu fault zone. | MI JingKui ZHANG ShuiChang CHEN JianPing TANG LiPing HE ZhongHua | 2007 | Chinese Science Bulletin2007，52，A01： | 10 |
| 4 | Evidence of vacuolar compartmentalization of arsenic in the hyperaccumulator Pteris vittata显示文摘Pteris vittata can hyperaccumulate arsenic (As) to >1% of its dry weight without showing any signs of toxicity, indicating the existence of effective plant-internal detoxification mechanisms. Although vacuolar compartmentalization is known to play an important role in heavy metal detoxification and tolerance, direct evidence of arsenic compartmentalization in this hyperaccumulator was lacking. Here we report the subcellular localization of As in the callus of P. vittata. The callus induced from gametophytes of P. vittata exposed to 0.2 mmol/L arsenate for 20 days were examined by directly isolating cell walls, protoplasts and vacuoles, and determining arsenic concentrations. Of the total As in the callus, about 94% was in the protoplast, and of that, 91% was present in the vacuoles, indicating that vacuoles are a major storage site for As in P. vittata. In addition, the changes in the chemical components of vacuoles were analyzed by Fourier transform infrared spectroscopy (FTIR). | YANG XueXi CHEN Hui DAI XiaoJing XU WenZhong HE ZhenYan MA Mi | 2009 | Chinese Science Bulletin2009，54，22： | 8 |
| 5 | Integrating landscape ecological principles and land evaluation for sustainable land use显示文摘1IntroductionRisingpopulationscompetingforlimitedlandresourceshavefocusedatentionontheneedforincreasingfoodproduction,whilepr... | Fu Bo jie, Chen Li ding Research Centre for Eco Environmental Sciences, Chinese Academy of Sciences, Beijing 100085, China He Chan sheng Department of Geography, Western Michigan University, Kalamazoo, MI 49008, USA | 1999 | Journal of Environmental Sciences1999，11，2： | 8 |
| 6 | Improved hydrogen storage properties of LiBH4 confined with activated charcoal by ball milling显示文摘In order to enhance the hydrogen storage properties of LiBH4,activated charcoal (AC) was used as the scaffold to confine LiBH4 in this paper.Ball milling was used to prepare LiBH4/AC composites.Experimental results show that dehydrogenation properties of ball-milled LiBH4/AC (LiBH4/AC-BM) are greatly improved compared with that of pristine LiBH4,ball-milled LiBH4 (LiBH4-BM) and hand-milled LiBH4/AC (LiBH4/AC-HM).The onset dehydrogenation temperature of LiBH4 for LiBH4/AC-BM is around 160 ℃,which is 170 ℃ lower than that of pristine LiBH4.At around 400 ℃,LiBH4/AC-BM finishes the dehydrogenation with a hydrogen capacity of 13.6 wt%,which is approximately the theoretical dehydrogenation capacity of pure LiBH4 (13.8 wt%),while the dehydrogenation processes for LiBH4-BM and LiBH4/AC-BM do not finish even when they were heated to 600 ℃.The isothermal dehydriding measurements show that it takes only 15 min for LiBH4/AC-BM to reach a dehydrogenation capacity of 10.1 wt% at 350 ℃,whereas the pristine LiBH4 and the LiBH4/AC-HM release hydrogen less than 1 wt% under the same conditions.The dehydrogenation process and the effect of AC were discussed. | He Zhou Xin-Hua Wang Hai-Zhen Liu Shi-Chao Gao Mi Yan | 2019 | Rare Metals2019，38，4： | 7 |
| 7 | Efficacy of a Chinese herbal formula on hepatitis B e antigenpositive chronic hepatitis B patients显示文摘BACKGROUND No guideline recommends antiviral therapy for hepatitis B e antigen(HBeAg)-positive chronic hepatitis B patients with persistently normal alanine aminotransferase levels and a high hepatitis B virus(HBV)DNA viral load.AIM To evaluate the feasibility and safety of a Chinese herbal formula as a therapeutic option for chronic HBV infection.METHODS In total,395 patients(30–65 years old)with confirmed HBeAg-positive chronic hepatitis B infection and persistently normal alanine aminotransferase were randomized to receive either Chinese herbal formula or placebo for 96 wk.Endpoints to evaluate therapeutic efficacy included:(1)HBV DNA levels decreased to less than 4 log10 IU/mL at weeks 48 and 96;and(2)HBeAg clearance and seroconversion rates at weeks 48 and 96.RESULTS HBV DNA levels≤4 log10 IU/mL were 10.05%at week 48 and 18.59%at week 96 in the treatment group.The HBeAg clearance and conversion rates were 8.54%and 8.04%at week 48 and 16.08%and 14.57%at week 96,respectively.However,HBV DNA levels≤4 log10 IU/mL were 2.55%and 2.55%at weeks 48 and 96,respectively,and the HBeAg clearance rates were 3.06%and 5.61%at weeks 48 and 96,respectively,in the control group.The quantitative hepatitis B surface antigen and HBeAg levels at baseline and changes during the treatment period as well as the alanine aminotransferase elevation at weeks 12 and 24 were strong predictors of HBeAg clearance.CONCLUSION High rates of HBV DNA reduction,HBeAg clearance and seroconversion could be achieved with Chinese herbal formula treatments,and the treatments were relatively safe for HBeAg-positive chronic hepatitis B-infected patients with persistently normal alanine aminotransferase.The ability of the compound to modulate host immune function probably contributed to this effect. | Yu-Feng Xing Chun-Shan Wei Tian-Ran Zhou Dan-Ping Huang Wei-Chao Zhong Bin Chen Hua Jin Xiao-Yu Hu Zhi-Yun Yang Qing He Kai-Ping Jiang Jun-Min Jiang Zhen-Bin Hu Xin Deng Fan Yang Feng-Yi Li Gang Zhao Li-Chun Wang Yu-Qiang Mi Zuo-Jiong Gong Peng Guo Jian-Hua Wu Wei-Qun Shi Hong-Zhi Yang Da-Qiao Zhou Guang-Dong Tong | 2020 | World Journal of Gastroenterology2020，26，30： | 7 |
| 8 | Identification of quantitative trait loci affecting tolerance to low phosphorus in rice (Oryza Sativa L.)显示文摘Phosphorus (P)-deficiency in rice (Oryza. Sativa. L) may cause yield reductions. This research has been conducted to map quantitative trait loci (QTLs) for tolerance to low phosphorus stress in a doubled haploid (DH) population. By using the linkage map of this population, the OTLs for relative dry weight, relative P content and relative P utilization efficiency have been located. The results indicate that one RFLP marker located on chromosome 6 is closely associated with relative root dry weight, relative shoot dry weight and relative total dry weight, which explain 24.9%, 20.5% and 25.2% of the total phenotypic variations, respectively. Two QTLs affect relative P uptake content, which account for 20.7% of the total phenotypic variations. One micro-effect QTL has been found to be associated with relative P utilization efficiency. It is suggested that the P uptake efficiency is more associated with P efficiency. Among the secondary physiological indices of P uptake efficiency, the root dry weight is | MING Feng ZHENG Xianwu MI Guohua HE Ping ZHU Lihuang ZHANG Fusuo | 2000 | Chinese Science Bulletin2000，45，6： | 7 |
| 9 | Mechanism of catalytic hydropyrolysis of sedimentary organic matter with MoS_2显示文摘MoS2 was used as an efficient catalyst for hydropyrolysis(Hypy) of three samples of sedimentary organic matter with different maturities.Through comparison with Soxhlet extraction(SE),it was found that MoS2 catalytic Hypy can remarkably promote the yields of total chloroform extracts,saturates,aromatics,hopanes and steranes.In addition,the difference of biomarker parameters indicated that isomerization of covalently-bound biomarkers is much more difficult than their free counterparts.Meanwhile,the high conversion of total organic carbon(TOC) in MoS2 catalytic Hypy of organic matter proved that the presence of dispersed molybdenum sulfide accelerated the breaking of C-C bonds and the release of hydrocarbons.To address the catalytic mechanism,a series of control experiments based on free Hypy and catalytic Hypy were conducted.The results showed that the calculated atomic ratio of carbon conversion/hydrogen conversion for catalytic Hypy was much larger than the presumed value of 1/2,indicating that intensive hydrogenation took place and significantly influenced the distribution of liquid products.Analysis of stable hydrogen isotope data,infrared spectra and m/z 83 ion chromatograph of the saturate fraction further confirmed this hypothesis.The difference of S content changing(ΔS) between catalyst-free Hypy and catalytic Hypy,and the thermal characteristics of the catalyst,indicated that active H2S was def initely generated and it probably initiated free radical reactions in the early stage of hydropyrolysis of organic matter. | He Kun Zhang Shuichang Mi Jingkui Chen Jianping Cheng Lei | 2011 | Petroleum Science2011，8，2： | 6 |
| 10 | The pathologic relevance of metabolic criteria in patients with biopsy-proven nonalcoholic fatty liver disease and metabolic dysfunction associated fatty liver disease:A multicenter cross-sectional study in China显示文摘Background:This study aimed to assess the association between metabolic syndrome(Met S)and severity of nonalcoholic fatty liver disease(NAFLD),and to discuss the pathological relevance of the diagnostic criteria in metabolic(dysfunction)associated fatty liver disease(MAFLD).Methods:This was a multicenter,cross-sectional study.Patients with NAFLD confirmed by liver biopsy were enrolled between July 2016 and December 2018 from 14 centers across the mainland of China.Anthropometric and metabolic parameters were collected to assess the pathological relevance.Results:Of 246 enrolled patients with NAFLD,150(61.0%)had the comorbidity of Met S.With the increase of metabolic components,the proportions of nonalcoholic steatohepatitis(NASH)and significant fibrosis were notably increased.The comorbid three metabolic components significantly increased the proportion of NASH,and further increase of metabolic components did not increase the proportion of NASH.However,the increase of metabolic components was parallel to the increase of the proportion of liver fibrosis.Among the 246 patients,239(97.2%)met the diagnostic criteria of MAFLD.Although non-MAFLD patients had less NASH,they present with similar proportion of significant fibrosis and cirrhosis.In the diagnostic criteria of MAFLD,BMI≥23 kg/m2 was related to NASH(Mantel-Haenszel Common Estimate OR:2.975;95%CI:1.037–8.538;P=0.043),and T2 DM was related to significant fibrosis(Mantel-Haenszel Common Estimate OR:2.531;95%CI:1.388–4.613;P=0.002).The homeostasis model assessment of insulin resistance(HOMA-IR)≥2.5 was the most significant factor for NASH(OR:4.100;95%CI:1.772–9.487;P=0.001)and significant factor for liver fibrosis(OR:2.947;95%CI:1.398–6.210;P=0.004)after the adjustments of the BMI and diabetes.Conclusions:Metabolic dysregulations are important risk factors in NAFLD progression.The insulin resistance status may play a predominant role in the progression in MAFLD patients. | Rui-Xu Yang Zheng-Sheng Zou Bi-Hui Zhong Hong Deng Fang-Ping He Jun-Ping Shi Cai-Yan Zhao Yu-Qiang Mi Yong-Jian Zhou Fu-Sheng Di Rui-Dan Zheng Qin Du Jia Shang Branko Popovic Jin Jun Chen Jian-Gao Fan | 2021 | Hepatobiliary & Pancreatic Diseases International2021，20，5： | 5 |
| 11 | Bioactive Study on Mixtures of Epimedin C and Icariin Monomers with Invariant Molarity to Zebrafish Osteoporosis Model显示文摘Objective To evaluate the anti-osteoporosis effect of the mixtures of epimedin C and icariin monomers with invariant molarity on zebrafish osteoporosis model. Methods The zebrafishes, fertilized 4 d ago, were exposed in 11 groups of nutrient solutions with prednisolone(25 μmol/L) as well as epimedin C and icariin(15 μmol/L) of various contents. The ratio of epimedin C and icariin in the 11 groups were as follows: A(10:0), B(9:1), C(8:2), D(7:3), E(6:4), F(5:5), G(4:6), H(3:7), I(2:8), J(1:9), and K(0:10). Meanwhile, a negative control group with prednisolone(25 μmol/L) was prepare as S. The selected zebrafish fetus was put into the 24-hole culture plate, and ensure every 5 zebrafishes in 1 hole and 2 holes as a group. They were placed in incubator at 28.5 o C, and the daily changes of fluid were investigated until they were put to death on day 8and then fixed. After dyeing with alizarin red, the segmental venter of zebrafish skulls was observed and quantitative analysis of dyed area was conducted. Results Compared with the negative control group S, the integrated optical density(IOD) values of cranial dyed area in all groups increased significantly(P < 0.05); Compared with group S, the IOD value of cranial dyed area in mixtures of epimedium monomers increased significantly(P < 0.05). The mixtures of epimedium monomers were all effective in facilitating zebrafish cranial mineralization and preventing prednisolone from inducing osteoporosis. According to mixtures of A-K groups, zebrafish cranial mineralization gradually decreased with gradually reduced content of epimedin C, with significant difference among groups(P < 0.05). Conclusion The higher the content of epimedin C in mixtures with invariant molarity is, the more active the anti-osteoporosis effect of epimedin C to zebrafish osteoporosis model is. | Mi Huang Jing Feng Ping Xia Zai-xuan Zhong Shun-ping He Yu-qin Shu Jiang-yan He Ying Wang | 2017 | Chinese Herbal Medicines2017，9，1： | 5 |
| 12 | Low concentrations of NaHSO_3 enhance NAD(P)H dehydrogenasedependent cyclic photophosphorylation and alleviate the oxidative damage to improve photosynthesis in tobacco显示文摘Bisulfite at low concentrations(L-NaHSO3) increases cyclic electron transport around photosystem I(PSI) and photosynthesis.However,little is known regarding the detailed contribution of cyclic electron transport to the promoted photosynthesis by L-NaHSO3.In the present work,we used tobacco mutant defective in ndhC-ndhK-ndhJ(ndhCKJ) to investigate the role of NAD(P)H dehydrogenase(NDH)-dependent cyclic electron transport around PSI in an increase in photosynthesis by L-NaHSO3.After the treatment of tobacco leaves with L-NaHSO3(10 μmol L-1),the NDH-dependent cyclic electron transport,monitored by a transient post-illumination increase in Chl fluorescence and the amount of NDH,was notably up-regulated in wild type(WT).The NDH-dependent cyclic electron transport was severely impaired in ndhCKJ and was not significantly affected by treatment with L-NaHSO3.Accordingly,the NDH-dependent transthylakoid membrane proton gradient(pH),as reflected by the slow phase of millisecond-delayed light emission(ms-DLE),was increased by L-NaHSO3 in WT,but not in ndhCKJ;the enhancement of cyclic photophosphorylation(PSP) activity by L-NaHSO3 was more obvious in WT than ndhCKJ.The accumulation of both superoxide and hydrogen peroxide was reduced in WT when subjected to L-NaHSO3 treatment,but not in ndhCKJ.Furthermore,the increase of photosynthetic O 2 evolution rate by L-NaHSO3 was more significant in WT than in ndhCKJ.We therefore conclude that L-NaHSO3 alleviates the photo-oxidative damage by the enhancement of NDH-dependent cyclic PSP,thereby improving photosynthesis. | WU YanXia HE Wei MA WeiMin SHEN YunKang MI HuaLing | 2012 | Chinese Science Bulletin2012，57，30： | 5 |
| 13 | Development of a real-time PCR method for Thalassiosira rotula rapid detection显示文摘Gene specific primers and DNA probe were designed based on the sequence of 18S rDNA cloned from the red tide alga Thalassiosira rotula. A real-time fluorescent quantitative PCR (RFQ-PCR) method was developed for quantitative detection of T.rotula. The RFQ-PCR assay data showed that the results obtained with the RFQ-PCR quite good agreement with those with the light microscope (LM) counting method, which suggested that the RFQ-PCR could be a useful method for red tide alga detection. | HE Shanying YU Zhigang MI Tiezhu | 2007 | Acta Oceanologica Sinica2007，26，2： | 5 |
| 14 | FUNCTIONAL CHARACTERIZATION OF CADMIUM-RESPONSIVE GARLIC GENE ASMT2B: A NEW MEMBER OF METALLOTHIONEIN FAMILY显示文摘A new gene of metallothionein (MT) family was cloned from garlic (Allium sativum) seed-lings using RACE method and designated AsMT2b. The full length of AsMT2b cDNA was 520 bp encod-ing 80 amino acids. The deduced amino acids of AsMT2b showed that AsMT2b contained the char-acteristic structure of type 2 MT proteins, but the number and arrangement of the cysteine residues in the N- and C-terminal domains was different from other type 2 MT proteins. Semi-quantitative reverse transcriptase-PCR showed that transcript levels of AsMT2b were enhanced only in response to higher concentrations or longer incubation time of Cd. Such an expression pattern of AsMT2b greatly differed from that of other type 2 MT genes. Yeast cells transformed with this gene had improved resistance to Cd. AsMT2b overexpressing Arabidopsis showed stronger Cd tolerance and higher Cd accumulation compared with wild-type plants. These results sug-gest that AsMT2b should be useful in phytoremedia-tion of Cd-polluted soil in the future. | ZHANG Haiyan XUWenzhong DAI Wentao HE Zhenyan MA Mi | 2006 | Chinese Science Bulletin2006，51，4： | 5 |
| 15 | Regulation of pepc gene expression in Anabaena sp. PCC 7120 and its effects on cyclic electron flow around photosystem I and tolerances to environmental stresses显示文摘Since pepc gene encoding phosphoenolpyruvate carboxylase(PEPCase) has been cloned from Anabaena sp. PCC7120 and other cyanobacteria, the effects of pepc gene expression on photosynthesis have not been reported yet. In this study, we constructed mutants containing either upregulated(forward) or downregulated(reverse) pepc gene in Anabaena sp. PCC 7120. Results from real-time quantitative polymerase chain reaction(RT-q PCR), Western blot and enzymatic analysis showed that PEPCase activity was significantly reduced in the reverse mutant compared with the wild type, and that of the forward mutant was obviously increased.Interestingly, the net photosynthesis in both the reverse mutant and the forward mutant were higher than that of the wild type, but dark respiration was decreased only in the reverse mutant. The absorbance changes of P700 upon saturation pulse showed the photosystem I(PSI) activity was inhibited, as reflected by Y(I), and Y(NA) was elevated, and Rdark reduction of P700 t was stimulated, indicating enhanced cyclic electron flow(CEF) around PSI in the reverse mutant.Additionally, the reverse mutant photosynthesis was higher than that of the wild type in low temperature, low and high pH,and high salinity, and this implies increased tolerance in the reverse mutant through downregulated pepc gene. | Xiao-Hui Jia Peng-Peng Zhang Ding-Ji Shi Hua-Ling Mi Jia-Cheng Zhu Xi-Wen Huang Pei-Min He | 2015 | Journal of Integrative Plant Biology2015，57，5： | 4 |
| 16 | Hydrogen storage properties of Nb-compounds-catalyzed LiBH4-MgH2显示文摘In order to improve the hydrogen storage properties of LiBH_4-MgH_2 composite, two different kinds of Nb-based catalysts, NbC and NbF_5, were added to LiBH_4-MgH_2 composite by ball milling, and the effect of catalysts on hydrogen storage properties of the modified LiBH_4-MgH_2 system was investigated. The experimental results show that LiBH_4-MgH_2 composite is a two-step dehydrogenation process, and Nb-based compounds can remarkably enhance its dehydrogenation kinetics. For the composite without addition of catalysts, the starting decomposition temperature for the first dehydrogenation step is around 320℃, and there is a long period of incubation time(around 220 min) for the occurrence of the second decomposition step even at high temperature of 450℃. It needs more than 10 h to complete the decomposition process and release around 9 wt% H_2. After addition of 5 mol% NbF_5, the starting decomposition temperature for the first dehydrogenation step is around 150℃, there is no incubation time for the second decomposition step, and it takes around 40 min to complete the second step and reaches a total dehydrogenation capacity of 9.5 wt%. NbF_5 has better catalytic effect than NbC. Based on the hydrogenation/dehydrogenation behaviors and structural variation, the mechanism of catalytic effect was discussed. | He Zhou Hai-Zhen Liu Lou Xu Shi-Chao Gao Xin-Hua Wang Mi Yan | 2017 | Rare Metals2017，36，9： | 4 |
| 17 | Transparent and flame retardant cellulose/aluminum hydroxide nanocomposite aerogels显示文摘Cellulose-based nanocomposite aerogels were prepared by incorporation of aluminum hydroxide(AH) nanoparticles into cellulose gels via in-situ sol-gel synthesis and following supercritical CO_2 drying. The structure and properties of cellulose/AH nanocomposite aerogels were investigated by Fourier transform infrared spectroscopy, scanning electron microscopy,ultraviolet-visible spectrometry, N_2 adsorption, thermogravimetric analysis, and micro-scale combustion calorimetry. The results indicated that the AH nanoparticles were homogeneously distributed within matrix, and the presence of AH nanoparticles did not affect the homogeneous nanoporous structure and morphology of regenerated cellulose aerogels prepared from1-allyl-3-methylimidazolium chloride solution. The resultant nanocomposite aerogels exhibited good transparency and excellent mechanical properties. Moreover, the incorporation of AH was found to significantly decrease the flammability of cellulose aerogels. Therefore, this work provides a facile method to prepare transparent and flame retardant cellulose-based nanocomposite aerogels, which may have great potential in the application of building materials. | Bin Yuan Jinming Zhang Jian Yu Rui Song Qinyong Mi Jiasong He Jun Zhang | 2016 | Science China Chemistry2016，59，10： | 4 |
| 18 | A Multifunctional Anti-Proton Electrolyte for High-Rate and Super-Stable Aqueous Zn-Vanadium Oxide Battery显示文摘Large volumetric expansion of cathode hosts and sluggish transport kinetics in the cathode–electrolyte interface,as well as dendrite growth and hydrogen evolution at Zn anode side are considered as the system problems that cause the electrochemical failure of aqueous Zn-vanadium oxide battery.In this work,a multifunctional anti-proton electrolyte was proposed to synchronously solve all those issues.Theoretical and experimental studies confirm that PEG 400 additive can regulate the Zn^(2+) solvation structure and inhibit the ionization of free water molecules of the electrolyte.Then,smaller lattice expansion of vanadium oxide hosts and less associated by-product formation can be realized by using such electrolyte.Besides,such electrolyte is also beneficial to guide the uniform Zn deposition and suppress the side reaction of hydrogen evolution.Owing to the integrated synergetic modifica-tion,a high-rate and ultrastable aqueous Zn-V_(2)O_(3)/C battery can be constructed,which can remain a specific capacity of 222.8 m Ah g^(-1)after 6000 cycles at 5 A g^(-1),and 121.8 m Ah g^(-1) even after 18,000 cycles at 20 A g^(-1),respectively.Such“all-in-one”solution based on the electrolyte design provides a new strategy for developing high-performance aqueous Zn-ion battery. | Yangwu Chen Dingtao Ma Kefeng Ouyang Ming Yang Sicheng Shen Yanyi Wang Hongwei Mi Lingna Sun Chuanxin He Peixin Zhang | 2022 | Nano-Micro Letters2022，14，9： | 3 |
| 19 | Seasonal and spatial distribution of ammonia-oxidizing microorganism communities in surface sediments from the East China Sea显示文摘Ammonia oxidation plays a significant role in the nitrogen cycle in marine sediments. Seasonal and spatial distribution of ammonia-oxidizing archaea(AOA) and betaproteobacteria(β-AOB) in surface sediments from the East China Sea(ECS) were investigated using ammonia monooxygenase α subunit(amo A) gene. In order to characterize the community of AOA and β-AOB, real-time quantitative polymerase chain reaction(q PCR) was carried out in this study, along with environmental parameters. The abundance of β-AOB amo A gene(2.17×106–4.54×107 copy numbers per gram wet weight sediment) was always greater than that of AOA amo A gene(2.18×105–9.89×106 copy numbers per gram wet weight sediment) in all sampling stations. The q PCR results were correlated with environmental parameters. AOA amo A gene copy numbers in April were positively related to temperature and nitrite concentration(p<0.05). β-AOB amo A gene copy numbers in August correlated negatively with salinity(p<0.01), and correlated positively with ammonium concentration(p<0.05). With the increase of salinity, the amo A gene copy ratio of AOB to AOA had a tendency to decrease, which suggested β-AOB dominated in the area of high level ammonium and AOA preferred high salinity area. | HE Hui ZHEN Yu MI Tiezhu LU Xinglan YU Zhigang | 2015 | Acta Oceanologica Sinica2015，34，8： | 3 |
| 20 | Multidimensional(0D-3D)functional nanocarbon:Promising material to strengthen the photocatalytic activity of graphitic carbon nitride显示文摘As a prospective visible-light-responsive photochemical material,graphitic carbon nitride(g-C_(3)N_(4))has become a burgeoning research hot topics and aroused a wide interest as a metal-free semiconductor in the area of energy utilization and conversion,environmental protection due to its unique properties,such as facile synthesis,high physicochemical stability,excellent electronic band structure,and sustainability.However,the shortcomings of high recombination rate of charge carriers,relatively low electrical conductivity and visible light absorption impede its practical application.Various strategies,such as surface photosensitization,heteroatom deposition,semiconductor hybridization,etc.,have been applied to overcome the barriers.Among all the strategies,functional nanocarbon materials with various dimensions(0D~3D)attract much attention as modifiers of g-C_(3)N_(4)due to their unique electronic properties,optical properties,and easy functionalization.More importantly,the properties of these functional nanocarbon materials can be tuned by various dimensions and thus there will be a way to overcome the defects of g-C_(3)N_(4)by choosing different dimensional carbon materials.Distinguishing from some present reviews,this review starts with the fundamental physicochemical characteristics of g-C_(3)N_(4)materials,followed by analyzing the advantages of functional nanocarbon materials modifying gC_(3)N_(4).Then,we present a systematic introduction to various dimensional carbon materials.The design philosophy of carbon/g-C_(3)N_(4)composites and the advanced studies are exemplified in detail.Finally,a nichetargeting summary and outlook on the major challenges,opportunities for future research in high-powered carbon/g-C_(3)N_(4)composites was proposed. | Bin He Mi Feng Xinyan Chen Jian Sun | 2021 | Green Energy & Environment2021，6，6： | 3 |
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