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| 1 | Complement C3a activates osteoclasts by regulating the PI3K/PDK1/SGK3 pathway in patients with multiple myeloma显示文摘Objective:Myeloma bone disease(MBD)is the most common complication of multiple myeloma(MM).Our previous study showed that the serum levels of C3/C4 in MM patients were significantly positively correlated with the severity of bone disease.However,the mechanism of C3 a/C4 a in osteoclasts MM patients remains unclear.Methods:The formation and function of osteoclasts were analyzed after adding C3 a/C4 a in vitro.RNA-seq analysis was used to screen the potential pathways affecting osteoclasts,and the results were verified by Western blot,q RT-PCR,and pathway inhibitors.Results:The osteoclast area per view induced by 1μg/m L(mean±SD:50.828±12.984%)and 10μg/m L(53.663±12.685%)of C3 a was significantly increased compared to the control group(0μg/m L)(34.635±8.916%)(P<0.001 and P<0.001,respectively).The relative m RNA expressions of genes,OSCAR/TRAP/RANKL/cathepsin K,induced by 1μg/m L(median:5.041,3.726,1.638,and 4.752,respectively)and 10μg/m L(median:5.140,3.702,2.250,and 5.172,respectively)of C3 a was significantly increased compared to the control group(median:3.137,2.004,0.573,and 2.257,respectively)(1μg/m L P=0.001,P=0.003,P<0.001,and P=0.008,respectively;10μg/m L:P<0.001,P=0.019,P<0.001,and P=0.002,respectively).The absorption areas of the osteoclast resorption pits per view induced by 1μg/m L(mean±SD:51.464±11.983%)and 10μg/m L(50.219±12.067%)of C3 a was also significantly increased(33.845±8.331%)(P<0.001 and P<0.001,respectively)compared to the control.There was no difference between the C4 a and control groups.RNA-seq analysis showed that C3 a promoted the proliferation of osteoclasts using the phosphoinositide 3-kinase(PI3 K)signaling pathway.The relative expressions of PIK3 CA/phosphoinositide dependent kinase-1(PDK1)/serum and glucocorticoid inducible protein kinases(SGK3)genes and PI3 K/PDK1/p-SGK3 protein in the C3 a group were significantly higher than in the control group.The activation role of C3 a in osteoclasts of MM patients was reduced by the SGK inhibitor(EMD638683).Conclusions:C3 a activated osteoclasts by regulating the PI3 K/PDK1/SGK3 pathways in MM patients,which was reduced using a SGK inhibitor.Overall,our results identified potential therapeutic targets and strategies for MBD patients。 | Fengjuan Jiang Hui Liu Fengping Peng Zhaoyun Liu Kai Ding Jia Song Lijuan Li Jin Chen Qing Shao Siyang Yan Kim De Veirman Karin Vanderkerken Rong Fu | 2021 | Cancer Biology & Medicine2021，18，3： | 3 |
| 2 | Small GTPases:Structure,biological function and its interaction with nanoparticles显示文摘Small GTPase is a kind of GTP-binding protein commonly found in eukaryotic cells.It plays an important role in cytoskeletal reorganization,cell polarity,cell cycle progression,gene expression and many other significant events in cells,such as the interaction with foreign particles.Therefore,it is of great scientific significance to understand the biological properties of small GTPases as well as the GTPase-nano interplay,since more and more nanomedicine are supposed to be used in biomedical field.However,there is no review in this aspect.This review summarizes the small GTPases in terms of the structure,biological function and its interaction with nanoparticles.We briefly introduced the various nanoparticles such as gold/silver nanoparticles,SWCNT,polymeric micelles and other nano delivery systems that interacted with different GTPases.These current nanoparticles exhibited different pharmacological effect modes and various target design concepts in the small GTPases study.This will help to elucidate the conclusion that the therapeutic strategy targeting small GTPases might be a new research direction.It is believed that the in-depth study on the functional mechanism of GTPases can provide insights for the design and study of nanomedicines. | Siyang Song Wenshu Cong Shurong Zhou Yujie Shi Wenbing Dai Hua Zhang Xueqing Wang Bing He Qiang Zhang | 2019 | Asian Journal of Pharmaceutical Sciences2019，14，1： | 3 |
| 3 | Energy-Efficient Resource Allocation for Heterogeneous Network with Grouping D2D显示文摘In this paper,a new communication model is built named grouping D2D(GD2D).Different from the traditional D2D coordination,we proposed GD2D communication in licensed and unlicensed spectrum simultaneously.We formulate a resource allocation problem,which aims at maximizing the energy efficiency(EE)of the system while guaranteeing the quality-of-service(Qos)of users.To efficiently solve this problem,the non-convex optimization problem is first transformed into a convex optimization problem.By transforming the fractional-form problem into an equivalent subtractive-form problem,an iterative power allocation algorithm is proposed to maximize the system EE.Moreover,the optimal closedform power allocation expressions are derived by the Lagrangian approach.Simulation results show that our algorithm achieves higher EE performance than the traditional D2D communication scheme. | Jing Cao Xin Song Siyang Xu Zhigang Xie Yanbo Xue | 2021 | China Communications2021，18，3： | 2 |
| 4 | High and ultra-stable energy storage from all-carbon sodium-ion capacitor with 3D framework carbon as cathode and carbon nanosheet as anode显示文摘Sodium-ion capacitors(SICs)are extremely promising due to the combined merits of high energy-power characteristics and considerable price advantage.However,it is still difficult to achieve high energypower outputs and cycle stability in a typical configuration of the metal-based battery-type anode and activated carbon capacitor-type cathode due to the kinetic mismatching.In this work,a carbon nanosheet(PSCS-600)with large interlayer spacing of 0.41 nm derived from the bio-waste pine cone shell was prepared.Besides,the covalent triazine framework derived carbon(OPDN-CTF-A)was obtained through ionothermal synthesis strategy,exhibiting beneficial hierarchical pores(0.5-6 nm)and high heteroatoms(5.6 at%N,6.6 at%O).On this basis,the all-carbon SICs were fabricated by the integration of PSCS-600 anode and OPDN-CTF-A cathode.The device delivered high energy density 111 Wh kg^(-1),high power output of 14,200 W kg^(-1) and ultra-stable cycling life(~90.7%capacitance retention after 10,000 cycles).This work provides new ideas in fabricating carbon-carbon architectural SICs with high energy storage for practical application. | Fangyuan Hu Siyang Liu Shengming Li Cheng Liu Guipeng Yu Ce Song Wenlong Shao Tianpeng Zhang Xigao Jian | 2021 | Journal of Energy Chemistry2021，30，4： | 2 |
| 5 | A Novel Strategy of In Situ Trimerization of Cyano Groups Between the Ti3C2Tx(MXene) Interlayers for High-Energy and High-Power Sodium-Ion Capacitors显示文摘2D MXenes are attractive for energy storage applications because of their high electronic conductivity.However,it is still highly challenging for improving the sluggish sodium(Na)-ion transport kinetics within the MXenes interlayers.Herein,a novel nitrogen-doped Ti3C2Tx MXene was synthesized by introducing the in situ polymeric sodium dicyanamide(Na-dca)to tune the complex terminations and then utilized as intercalation-type pseudocapacitive anode of Na-ion capacitors(NICs).The Na-dca can intercalate into the interlayers of Ti3C2 Tx nanosheets and simultaneously form sodium tricyanomelaminate(Na3TCM)by the catalyst-free trimerization.The as-prepared Ti3C2Tx/Na3TCM exhibits a high N-doping of 5.6 at.%in the form of strong Ti-N bonding and stabilized triazine ring structure.Consequently,coupling Ti3C2Tx/Na3 TCM anode with different mass of activated carbon cathodes,the asymmetric MXene//carbon NICs are assembled.It is able to deliver high energy density(97.6 Wh kg-1),high power output(16.5 kW kg-1),and excellent cycling stability(≈82.6%capacitance retention after 8000 cycles). | Siyang Liu Fangyuan Hu Wenlong Shao Wenshu Zhang Tianpeng Zhang Ce Song Man Yao Hao Huang Xigao Jian | 2020 | Nano-Micro Letters2020，12，10： | 2 |
| 6 | Superior resistance to alkali metal potassium of vanadium-based NH_(3)-SCR catalyst promoted by the solid superacid SO_(4)^(2-)-TiO_(2)显示文摘The significant decrease of acid sites caused by alkali metal poisoning is the major factor in the deactivation of commercial V_(2)O_(5)-WO_(3)/TiO_(2)NH_(3)-SCR catalysts.In this work,the solid superacid SO_(4)^(2-)-TiO_(2) modified by sulfate radicals,was selected as the catalyst support,which showed superior potassium resistance.The physicochemical properties and K-poisoning resistance of the V_(2)O_(5)-WO_(3)/SO_(4)^(2-)-TiO_(2)(VWSTi) catalyst were carried out by XRD,BET,H2-TPR,NH3-TPD,XPS,in situ DRIFTS and TG.The results pointed out that the introduction of SO_(4)^(2-)significantly increased the NH3-SCR catalytic activity at high temperatures,with an exceptionally high NO_(x) conversion over 90% between 275℃ and 500℃.When 0.5%(mass) K_(2)O was doped on the catalysts,the catalytic performance of the traditional V_(2)O_(5)-WO_(3)/TiO_(2)(VWTi) catalyst decreased significantly,while the VWSTi catalyst could still maintain a NOxconversion over 90%in the range of 300–500℃.The characterizations suggested that the support of SO_(4)^(2-)-TiO_(2) greatly increased the number of acidic sites,thereby enhancing the adsorption capacity of the reactant NH_(3).The results above demonstrated a potential approach to achieve superior potassium resistance for NH3-SCR catalysts using solid superacid. | Yaoyao Peng Lei Song Siru Lu Ziyu Su Kui Ma Siyang Tang Shan Zhong Hairong Yue Bin Liang | 2023 | Chinese Journal of Chemical Engineering2023，55，3： | 1 |
| 7 | Replacing“Alkyl”with“Aryl”for inducing accessible channels to closed pores as plateau-dominated sodium-ion battery anode显示文摘Hard carbons are promising anodes for sodium-ion batteries.However,there is still considerable controversy regarding the sodium storage behaviors in hard carbons,which are mainly attributed to the varied precursors,confused pyrolysis mechanism,and different characterization methods.Herein,benefiting from the flexible molecular structure of polymers,a series of hard carbons with carefully tunedmicrostructures are fabricated by adjusting the ratio of aryl and alkyl groups in the epoxy resins.The results of dynamic mechanical analysis,insitu Fourier transform infrared spectra,and synchronous thermal gravimetricinfrared spectrum-gas chromatography/mass spectrometry reveal that replacing the alkyl with aryl groups in the resin can enhance the crosslink density,inhibit the degradation and rearrangement process,and further lead to a more disordered microstructure.In addition,it is suggested that accessible channels provided by sufficiently wide interlayer spacing are necessary for closed pore filling.The optimized anode delivers a high capacity of 375 mAh/g in half cell with an initial Coulombic efficiency of 80.61%,and an energy density of 252 Wh/kg is attained in full cell.Finally,a reliable relationship among precursor-pyrolysis mechanism-structure-performance is established,and the sodium storagemechanism of“adsorption-insertion-pore filling”iswell proved. | Wenlong Shao Qi Cao Siyang Liu Tianpeng Zhang Zihui Song Ce Song Zhihuan Weng Xigao Jian Fangyuan Hu | 2022 | SusMat2022，2，3： | 1 |
| 8 | A flexible design strategy to modify Ti3C2Tx MXene surface terminations via nucleophilic substitution for long-life Li-S batteries显示文摘MXene-based materials have gained considerable attention for lithium-sulfur(Li-S)batteries cathode materials due to their superior electric conductivity and high affinitive to polysulfides.However,there are still challenges in modifying the surface functional groups of MXene to further improve the electrochemical performance and increase the structure variety for MXene-based sulfur host.Herein,we report an efficient and flexible nucleophilic substitution(S_(N))strategy to modify the Ti_(3)C_(2)T_(x) surface terminations and purposefully designed Magnolol-modified Ti_(3)C_(2)T_(x)(M-Ti_(3)C_(2)T_(x))as powerful cathode host materials.Benefiting from more C-Ti-O bonds forming and diallyl groups terminations reducing after the dehalogenation and nucleophilic addition reactions,the given M-Ti_(3)C_(2)T_(x) electrode could effectively suppress the lithium polysulfides shuttling via chemisorption and C—S covalent bond formation.Besides,the Magnolol-modified Ti_(3)C_(2)T_(x) significantly accelerates polysulfide redox reaction and reduces the activation energy of Li_(2) S decomposition.As a result,the as-prepared M-Ti_(3)C_(2)T_(x) electrode displays an excellent rate capability and a high reversible capacity of 7.68 mAh cm^(-2)even under 7.2 mg cm^(-2)S-loaded with a low decay rate of 0.07%(from 2 nd cycle).This flexible surface-modified strategy for MXene terminations is expected to be extended to other diverse MXene applications. | Tianpeng Zhang Wenlong Shao Siyang Liu Zihui Song Runyue Mao Xin Jin Xigao Jian Fangyuan Hu | 2022 | Journal of Energy Chemistry2022，31，11： | 1 |
| 9 | Co‑packaged optics(CPO):status,challenges,and solutions显示文摘Due to the rise of 5G,IoT,AI,and high-performance computing applications,datacenter trafc has grown at a compound annual growth rate of nearly 30%.Furthermore,nearly three-fourths of the datacenter trafc resides within datacenters.The conventional pluggable optics increases at a much slower rate than that of datacenter trafc.The gap between application requirements and the capability of conventional pluggable optics keeps increasing,a trend that is unsustainable.Copackaged optics(CPO)is a disruptive approach to increasing the interconnecting bandwidth density and energy efciency by dramatically shortening the electrical link length through advanced packaging and co-optimization of electronics and photonics.CPO is widely regarded as a promising solution for future datacenter interconnections,and silicon platform is the most promising platform for large-scale integration.Leading international companies(e.g.,Intel,Broadcom and IBM)have heavily investigated in CPO technology,an inter-disciplinary research feld that involves photonic devices,integrated circuits design,packaging,photonic device modeling,electronic-photonic co-simulation,applications,and standardization.This review aims to provide the readers a comprehensive overview of the state-of-the-art progress of CPO in silicon platform,identify the key challenges,and point out the potential solutions,hoping to encourage collaboration between diferent research felds to accelerate the development of CPO technology. | Min Tan Jiang Xu Siyang Liu Junbo Feng Hua Zhang Chaonan Yao Shixi Chen Hangyu Guo Gengshi Han Zhanhao Wen Bao Chen Yu He Xuqiang Zheng Da Ming Yaowen Tu Qiang Fu Nan Qi Dan Li Li Geng Song Wen Fenghe Yang Huimin He Fengman Liu Haiyun Xue Yuhang Wang Ciyuan Qiu Guangcan Mi Yanbo Li Tianhai Chang Mingche Lai Luo Zhang Qinfen Hao Mengyuan Qin | 2023 | Frontiers of Optoelectronics2023，16，1： | 1 |
| 10 | The quasi-activity coefficients of non-electrolytes in aqueous solution with organic ions and its application on the phase splitting behaviors prediction for CO_(2) absorption显示文摘CO_(2)capture with a low energy consumption is of important application significance for reducing CO_(2)emission.The phase-change absorbent developed in recent years shows its potential for low-energy CO_(2)capture.The unclear phase-splitting rule hinders the efficient development of CO_(2)phase-change absorbents.To predict phase-splitting behaviors of mono/poly-amine-organic solvent-water system with various concentrations,a quasi-activity coefficient was developed based on Debye&Mc Aulay equation and some Density function theory descriptors.Six models based on Debye&Mc Aulay equation were developed with different ion radius,descriptors or poly-amine-CO_(2)products.The phase-splitting boundary was drawn on the model with the best predictability.This quasi-activity coefficient would provide guidance for the phase-splitting systems development,especially for polyamines. | Xiaomeng Zhao Xingyu Li Changjun Liu Shan Zhong Houfang Lu Hairong Yue Kui Ma Lei Song Siyang Tang Bin Liang | 2022 | Chinese Journal of Chemical Engineering2022，35，3： | 1 |
| 11 | Carbon spheres with rational designed surface and secondary particle-piled structures for fast and stable sodium storage显示文摘The electrochemical performance of hard carbon in sodium storage is still limited by its poor cycling stability and rate capability because of the sluggish kinetics process.In this study,we use a simple and effective method to accelerate the kinetics process by engineering the structure of the electrode to promote its surface and near-surface reactions.This goal is realized by the use of slightly aggregated ultra-small carbon spheres.The large specific surface area formed by the small spheres can provide abundant active sites for electrochemical reactions.The abundant mesopores and macropores derived from the secondary particle piled structure of the carbon spheres could facilitate the transport of electrolytes,shorten the diffusion distance of Na^(+)and accommodate the volume expansion during cycling.Benefiting from these unique structure features,PG700-3(carbon spheres with the diameters of 40-60 nm carbonized at 700℃)exhibits high performance for sodium storage.A high reversible capacity of 163 mAh g^(-1) could be delivered at a current density of 1.0 A g^(-1) after 100 cycles.Interestingly,at a current density of 10.0 A g^(-1),the specific capacity of PG700-3 gradually increases to 140 mAh g^(-1) after 10000 cycles,corresponding to a capacity retention of 112%.Given the enhanced kinetics of SIBs reactions,PG700-3 exhibits an excellent rate capability,i.e.,230 and 138 mAh g^(-1) at 0.1 and 5.0 A g^(-1),respectively.This study provides a facile method to attain high performance anode materials for SIBs.The design strategy and improvement mechanism could be extended to other materials for high rate applications. | Wenlong Shao Fangyuan Hu Siyang Liu Tianpeng Zhang Ce Song Zhihuan Weng Jinyan Wang Xigao Jian | 2021 | Journal of Energy Chemistry2021，30，3： | 1 |
| 12 | Measurements of the effective mass transfer areas for the gas–liquid rotating packed bed显示文摘Rotating packed bed(RPB) is one of the most effective gas–liquid mass transfer enhancement reactors, its effective specific mass transfer area(ae) is critical to understand the mass transfer process. By using the NaOH–CO_(2) chemical absorption method, the aevalues of three RPB reactors with different rotor sizes were measured under different operation conditions. The results showed that the high gravity factor and liquid flow rate were major affecting factors, while the gas flow rate exhibited minor influence.The radius of packing is the dominant equipment factor to affect aevalue. The results indicated that the contact area depends on the dispersion of the liquid phase, thus the centrifugal force of rotating packed bed greatly influenced the aevalue. Moreover, the measured ae/ap(effective specific mass transfer area/specific surface area of packing) values were fitted with dimensionless correlation formulas. The unified correlation formula with dimensionless bed size parameter can well predict the experimental data and the prediction errors were within 15%. | Wen Tian Junyi Ji Hongjiao Li Changjun Liu Lei Song Kui Ma Siyang Tang Shan Zhong Hairong Yue Bin Liang | 2023 | Chinese Journal of Chemical Engineering2023，55，3： | 0 |
| 13 | Secrecy-Enhancing Design for Two-Way Energy Harvesting Cooperative Networks with Full-Duplex Relay Jamming显示文摘To guarantee secure information transmission within two sources,a full-duplex(FD)relay jamming scheme for two-way energy harvesting(EH)cooperative networks is proposed,in which the relay can achieve simultaneous information reception and jamming transmission.The EH relay node scavenges energy from two source signals,and then,uses the harvested energy for information relaying and jamming transmission by the power splitting(PS)protocol.Considering multiple eavesdroppers,the nonconvex optimization for maximizing the smaller bidirectional secrecy rates is formulated by jointly optimizing the power allocation and PS factor.Furthermore,an iterative algorithm based on successive convex approximation and alternate search method is proposed to solve this non-convexity.Simulation results verify the proposed iterative algorithm and show that the proposed jamming scheme can achieve substantial performance gain than other conventional schemes. | Siyang Xu Xin Song Yiming Gao Suyuan Li Jing Cao Zhigang Xie | 2021 | China Communications2021，18，5： | 0 |
| 14 | Green rapid synthesis of Cu_(2)O/Ag heterojunctions exerting synergistic antibiosis显示文摘Semiconductor-noble metal composite has become a research focus due to its superior performance compared with its respective component.Although various methods have been developed to synthesize semiconductor-noble metal heterostructures,most of them are relatively complex multistep and use toxic reactants of high cost and risk.In this work,a series of Cu_(2)O/Ag heterojunctions were quickly prepared in one step via simple microwave-assisted green route.XRD,SEM,TEM,EDS,XPS,etc.were used to characterize obtained products,and the results indicate a Cu_(2)O/Ag metal-semiconductor heterojunction in micro-nano size was fabricated successfully.In addition,antibacterial behavior of Cu_(2)O/Ag heterojunctions against E.coli and S.aureus were investigated.Owing to the synergistic effect of Cu_(2)O and Ag,the heterojunction exhibits much better antibacterial performance than the pristine Cu_(2)O does.This work provides new insights into the green design and fabrication of surface-modified Cu_(2)O hybrid multifunctional materials for antibacterial applications. | Feiyue Hu Bo Song Xiaohan Wang Shen Bao Siyang Shang Shupei Lv Bingbing Fan Rui Zhang Jingguo Li | 2022 | Chinese Chemical Letters2022，33，1： | 0 |
| 15 | MXenes for metal-ion and metal-sulfur batteries:Synthesis,properties,and electrochemistry显示文摘In 2011,a new class of 2D materials was discovered;after 2012,they began to be concerned;in 2017,the“gold rush”of the materials was triggered,and they are exactly MXenes.2D MXenes,a new class of transition metal carbides,carbonitrides and nitrides,have become the star and cutting-edge research materials in the field of emerging batteries systems due to their unique 2D structure,abundant surface chemistry,and excellent physical and electrochemical properties.This review focuses on the MXene materials and summarizes the recent advancements in the synthesis techniques and properties,in addition to a detailed discussion on the electrochemical energy storage applications,including alkali-ion(Li^(+),Na^(+),K^(+))storage,lithium-sulfur(Li–S)batteries,sodiumsulfur(Na–S)batteries,and metal anode protection.Special attentions are given to the elaborate design of nano-micro structures of MXenes for the various roles as electrodes,multifunctional components,S hosts,modified separators,and metal anode protective layers.The paper ends with a prospective summary of the promising research directions in terms of synthesis,structure,properties,analysis,and production on MXene materials. | Siyang Liu Zihui Song Xin Jin Runyue Mao Tianpeng Zhang Fangyuan Hu | 2022 | Materials Reports(Energy)2022，2，1： | 0 |
| 16 | Molecular Docking and Spectroscopic Methods to Probe the Interaction of Acetylgliotoxin and HSA显示文摘The interaction between acetylgliotoxin and human serum albumin(HSA) has been studied by spectroscopic method.Acetylgliotoxin quenches the intrinsic fluorescence of HSA in a static quenching procedure.The binding of acetylgliotoxin to HSA causes a slight conformational change of HSA.The binding constants at different temperatures as well as enthalpy change and entropy change,are calculated according to relevant fluorescent data and Van't Hoff equation.The hydrogen bond is a predominant intermolecular force for stabilizing the complex,which is in conformity with the results of molecular modeling study. | ZHANG Lianru,CHEN Junjie,SONG Siyang,ZHENG Zhonghui,HUANG Yaojian School of Life Sciences,Xiamen University,Xiamen 361005,Fujian,China | 2010 | Wuhan University Journal of Natural Sciences2010，15，5： | 0 |
| 17 | Hybrid solid electrolyte interphases formed in conventional carbonate electrolyte enable high-voltage and ultra-stable magnesium metal batteries显示文摘Magnesium metal batteries are considered as viable alternatives of lithium-ion batteries for their low cost and high capacity of magnesium.Nevertheless,the practical application of magnesium metal batteries is extremely challenging due to a lack of suitable electrolyte that can stabilize magnesium metal anode and high-voltage cathode simultaneously.Herein,we found that in-situ formed lithium/magnesium hybrid electrolyte interphases in conventional LiPF6-containing carbonate-based electrolyte can not only prevent the production of passivation layer on the magnesium metal anode,but also inhibit the oxidation of the electrolyte under high voltage.The symmetric magnesium‖magnesium battery can achieve reversible stripping/plating for 1600 and 600 h at 0.02 and 0.1 mA cm^(-2),respectively.In addition,when coupled with a carbon fiber cathode,the magnesium metal battery exhibited a capacity retention rate of 96.3% for 1000 cycles at a current density of 500 mA g^(-1)and presented a working voltage of ~3.1 V.This research paves a new and promising path to the commercialization process of rechargeable magnesium metal batteries. | Yong Xie Huawei Song Siyang Ye Fei Tian Junjie Xie Danni Lei Chengxin Wang | 2023 | Journal of Energy Chemistry2023，，3： | 0 |
| 18 | Sulfur polymerization strategy based on the intrinsic properties of polymers for advanced binder-free and high-sulfur-content Li–S batteries显示文摘Lithium-sulfur(Li-S)batteries are the promising next-generation secondary energy storage systems,because of their advantages of high energy density and environmental friendliness.Among numerous cathode materials,organosulfur polymer materials have received extensive attentions because of their controllable structure and uniform sulfur distribution.However,the sulfur content of most organosulfur polymer cathodes is limited(S content<60%)due to the addition of large amounts of conductive agents and binders,which adversely affects the energy density of Li-S batteries.Herein,a hyperbranched sulfur-rich polymer based on modified polyethyleneimine(Ath-PEI)named carbon nanotubeentangled poly(allyl-terminated hyperbranched ethyleneimine-random-sulfur)(CNT/Ath-PEI@S)was prepared by sulfur polymerization and used as a Li-S battery cathode.The high intrinsic viscosity of Ath-PEI provided considerable adhesion and avoided the addition of PVDF binder,thereby increasing the sulfur content of cathodes to 75%.Moreover,considering the uniform distribution of elemental sulfur by the polymer,the utilization of sulfur was successfully improved,thus improving the rate capability and discharge capacity of the battery.The binder-free,sulfur-rich polymer cathode exhibited ultra-high initial discharge capacity(1520.7 mAh g^(−1) at 0.1 C),and high rate capability(804 mAh g^(−1) at 2.0 C).And cell-level calculations show that the electrode exhibits an initial capacity of 942.3 mAh g^(−1) electrode,which is much higher than those of conventional sulfur-polymer electrodes reported in the literature. | Zihui Song Tianpeng Zhang Siyang Liu Wenlong Shao Wanyuan Jiang Runyue Mao Xigao Jian Fangyuan Hu | 2023 | SusMat2023，3，1： | 0 |
| 19 | Heat shock protein 90 mediates the apoptosis and autophage in nicotinic-mycoepoxydienetreated HeLa cells显示文摘(Hsp90 ) 热吃惊蛋白质 90 由于它在与房间增长和规定联系的多重发信号的小径的十字路口的重要角色是为癌症治疗的一个迷人的目标。Hsp90 禁止者有潜力被发展进反癌症药。这里,我们识别了 nicotinic-mycoepoxydiene (NMD ) ,是的在结构上小说混合物执行反肿瘤活动的 Hsp90 禁止者。混合物有选择地跳了到 Hsp90 N 终端领域,并且降级 Hsp90 顾客蛋白质 Akt。在 non-phosphorylation 形式坏的耽搁的 Akt 的降级。联系 NMD 的 apoptosis 被碎裂的原子核的形成描绘,(自动数据处理核糖) poly,聚合酶劈开,细胞色素 c 版本, caspase-3 激活,和 sub-G1 的增加的比例分阶段执行房间。有趣地, apoptosis 伴有 autophagy,由展出 LC-3 的增加的表达式和 lysosome pH 价值的减少。我们的调查结果提供 Hsp90 禁止者在 vitro 由调整房间 apoptosis 和 autophagy 的新奇细胞的机制,建议那 NMD 不仅有一个潜力被发展进新奇反肿瘤药品,而且在经由 Hsp90 抑制调整癌症房间 apoptosis 和 autophagy 展出新机制。 | Yifei Sun Shuyan Xiao Junjie Chen Miaomiao Wang Zhonghui Zheng Siyang Song Lianru Zhang | 2015 | Acta Biochimica et Biophysica Sinica2015，47，6： | 0 |
| 20 | Resource allocation optimization for SWIPT full-duplex relaying networks with practical energy harvester显示文摘In this paper,the resource allocation optimization for the simultaneous wireless information and power transfer(SWIPT)full-duplex(FD)relaying networks is investigated,in which the power-constrained relay scavenges energy from the source signal and assists information transmission by FD operation.Taking into account non-linear energy harvesting(EH)hardware circuit characteristics of the relay,the information rate maximization problem is developed by jointly optimizing the time-switching(TS)factor and transmission powers of the source in two different phases.However,the formulated optimization is highly non-convex and difficult to solve.To cope with this problem,the primary problem is decomposed into two sub-problems with respect to the TS factor and transmission powers.After solving these two sub-problems,the final sub-optimal solutions can be obtained by alternating search.Simulation results prove that the optimization of both TS factor and transmission powers can effectively enhance the information rate for the considered networks. | Xu Siyang Song Xin Zhu Jiahui | 2023 | The Journal of China Universities of Posts and Telecommunications2023，30，1： | 0 |
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