|
|
|
题名
|
作者
|
年代
|
出处
|
被引量
|
| 1 | Room temperature phosphorescence from natural products: Crystallization matters显示文摘Efficient room temperature phosphorescence is observed in natural compounds and polymers such as starch, cellulose, bovine serum albumin (BSA), and some other carbohydrates. Whereas being practically nonluminescent in solutions and TLC plates, they emit bright phosphorescence in the crystalline states with lifetime up to microseconds, exhibiting crystallization-induced phosphorescence (CIP) characteristics. The CIP of these natural products without any conventional chromophores offers a new platform for the exploration of conceptually novel luminogens. | GONG YongYang TAN YeQiang MEI Ju ZHANG YiRen YUAN WangZhang ZHANG YongMing SUN JingZhi TANG Ben Zhong | 2013 | Science China Chemistry2013，56，9： | 8 |
| 2 | Crystallization-induced phosphorescence of benzils at room temperature显示文摘Efficient room temperature phosphorescence (RTP) is rarely observed in pure organic luminogens. However, we have newly observed that benzil and its derivatives are nonluminescent in solvents and thin layer chromatography (TLC) plates, but become highly phosphorescent in crystal state at room temperature, exhibiting typical crystallization-induced phosphorescence (CIP) characteristics. The CIP phenomenon is ascribed to the restriction of intramolecular rotations in crystals owing to effective intermolecular interactions. Such intermolecular interactions greatly rigidify the molecular conformation and significantly decrease the nonradiative deactivation channels of the triplet excitons, thus giving boosted phosphorescent emission at room temperature. | GONG YongYang TAN YeQiang LI Hong ZHANG YiRen YUAN WangZhang ZHANG YongMing SUN JingZhi TANG Ben Zhong | 2013 | Science China Chemistry2013，56，9： | 6 |
| 3 | The selection of a primary marker for the Anthropocene显示文摘Since Homo sapiens appeared,the planet has experienced continuing environmental changes[1,2].In 2000,Crutzen and Stoermer[3]systematically analysed the global changes caused by human activity over the previous 300 years and suggested that the Holocene epoch ended in the 1750s and a new geological age,the Anthropocene,began.Afterwards,the Anthropocene drew a lot of attention from both scientific community and the general public.The recognition and placement of the Anthropocene/Holocene boundary has been a subject of heated debates over the past two decades.At the 35th International Geological Congress(2016;IGC),the Anthropocene Working Group(AWG)recommended the Anthropocene to be formalised with an epoch rank,with the 1950s as its lower boundary[4]. | Tianli Wang Liangcheng Tan Hai Xu Jingjie Zang Dong Li Jianghu Lan Yongming Han Li Li | 2019 | Science Bulletin2019，64，22： | 4 |
| 4 | Performance and theoretical study on corrosion inhibition of 2 (4-pyridyl)- benzimidazole for mild steel in hydrochloric acid显示文摘 | Zhang Fan Tan Yongming Cao Ziyi | 2012 | Corro- sion Science2012，61，8： | 1 |
| 5 | High efficiency D-A structured luminogen with aggregation-induced emission and mechanochromic characteristics显示文摘A novel luminogen, CZ2TPAN, with typical D-A architecture was obtained. It shows intramolecular charge transfer and aggregation-induced emission characteristics with high solid-state efficiency of 65.3%. Moreover, it exhibits reversible mechanochromic behavior between crystalline and amorphous states with remarkable emission color change from green (504 nm) to yellow (545nm). | LU YaWei TAN YeQiang GONG YongYang LI Hong YUAN WangZhang ZHANG YongMing TANG Ben Zhong | 2013 | Chinese Science Bulletin2013，58，22： | 1 |
| 6 | A genetically engineered Escherichia coli that senses and degrades tetracycline antibiotic residue显示文摘Due to the abuse of antibiotics,antibiotic residues can be detected in both natural environment and various industrial products,posing threat to the environment and human health.Here we describe the design and implementation of an engineered Escherichia coli capable of degrading tetracycline(Tc)-one of the commonly used antibiotics once on humans and now on poultry,cattle and fisheries.A Tcdegrading enzyme,TetX,from the obligate anaerobe Bacteroides fragilis was cloned and recombinantly expressed in E.coli and fully characterized,including its Km and kcat value.We quantitatively evaluated its activity both in vitro and in vivo by UVeVis spectrometer and LC-MS.Moreover,we used a tetracycline inducible amplification circuit including T7 RNA polymerase and its specific promoter PT7 to enhance the expression level of TetX,and studied the dose-response of TetX under different inducer concentrations.Since the deployment of genetically modified organisms(GMOs)outside laboratory brings about safety concerns,it is necessary to explore the possibility of integrating a kill-switch.Toxin-Antitoxin(TA)systems were used to construct a mutually dependent host-plasmid platform and biocontainment systems in various academic and industrious situations.We selected nine TA systems from various bacteria strains and measured the toxicity of toxins(T)and the detoxifying activity of cognate antitoxins(A)to validate their potential to be used to build a kill-switch.These results prove the possibility of using engineered microorganisms to tackle antibiotic residues in environment efficiently and safely. | Zepeng Mu Zhuoning Zou Ye Yang Wenbo Wang Yue Xu Jianyi Huang Ruiling Cai Ye Liu Yajin Mo Boyi Wang Yiqun Dang Yongming Li Yushan Liu Yueren Jiang Qingyang Tan Xiaohong Liu Cheng Hu Hua Li Sha Wei Chunbo Lou Yang Yu Jiangyun Wang | 2018 | Synthetic and Systems Biotechnology2018，3，3： | 0 |
| 7 | Agronomic and Economic Evaluation for Intercropping between Chewing Cane and Peanut显示文摘[Objectives]To explore the proper intercropping pattern between chewing cane and peanut.[Methods]A field experiment was carried out to investigate the yield and economic benefit of chewing cane and peanut,as well as the changes in soil properties under different chewing cane/peanut intercropping patterns.Three chewing cane/peanut intercropping patterns were designed,in which with every row of chewing cane intercropping one row of peanut(CP_(1)),intercropping two rows of peanut(CP_(2))and chewing cane mono-cropping(MC).[Results]It had no significant effect on the agronomic characters of chewing cane and peanut in CP_(1)and CP_(2),compared with MC.The soil properties before the planting(BP)and after the harvest(AH)indicated that the chewing cane/peanut intercropping patterns significantly increased soil organic matter and soil available nitrogen contents,but decreased soil available potassium contents,and CP_(2)had better effect on soil structure than CP_(1).The total production value and economic benefit were increased significantly on the CP_(1)and CP_(2),comparing the MC,and the benefit of CP_(2)was higher significantly than that of CP_(1).The land equivalent ratios(LER)for CP_(1)and CP_(2)were 1.94 and 1.72,respectively,which was significantly higher than that of MC(0.83).Although planting cost was increased in chewing cane/peanut intercropping patterns partly,the production value and the profits were enhanced significantly.[Conclusions]CP_(2)could be significantly advantageous for the yield and benefits of chewing cane and peanut and soil properties.The favorable intercropping pattern for economic return would be one row of 120 cm width for chewing cane with two rows of peanut. | Yufeng LIU Yumo TAN Dan LIANG Yongming LAI | 2022 | Asian Agricultural Research2022，14，2： | 0 |
| 8 | Circumventing chemo-mechanical failure of Sn foil battery anode by grain refinement and elaborate porosity design显示文摘Tin (Sn) metal foil is a promising anode for next-generation high-energy–density lithium-ion batteries (LIBs) due to its high capacity and easy processibility. However, the pristine Sn foil anode suffers nonuniform alloying/dealloying reaction with lithium (Li) and huge volume variation, leading to electrode pulverization and inferior electrochemical performance. Herein, we proposed that reduced grain size and elaborate porosity design of Sn foil can circumvent the nonuniform alloy reaction and buffer the volume change during the lithiation/delithiation cycling. Experimentally, we designed a three-dimensional interconnected porous Sn (3DIP-Sn) foil by a facile chemical alloying/dealloying approach, which showed improved electrochemical performance. The enhanced structure stability of the as-fabricated 3DIP-Sn foil was verified by chemo-mechanical simulations and experimental investigation. As expected, the 3DIP-Sn foil anode revealed a long cycle lifespan of 4400 h at 0.5 mA cm^(−2) and 1 mAh cm^(−2) in Sn||Li half cells. A 3DIP-Sn||LiFePO_(4) full cell with LiFePO_(4) loading of 7.1 mg cm^(−2) exhibited stable cycling for 500 cycles with 80% capacity retention at 70 mA g^(−1). Pairing with high-loading commercial LiNi0.6Co0.2Mn0.2O_(2) (NCM622, 18.4 mg cm^(−2)) cathode, a 3DIP-Sn||NCM622 full cell delivered a high reversible capacity of 3.2 mAh cm^(−2). These results demonstrated the important role of regulating the uniform alloying/dealloying reaction and circumventing the localized strain/stress in improving the electrochemical performance of Sn foil anodes for advanced LIBs. | Shuibin Tu Xin Ai Xiancheng Wang Siwei Gui Zhao Cai Renming Zhan Yuchen Tan Weiwei Liu Hui Yang Chenhui Li Yongming Sun | 2021 | Journal of Energy Chemistry2021，30，11： | 0 |
| 9 | Stress-Regulation Design of Lithium Alloy Electrode toward Stable Battery Cycling显示文摘Metallic tin(Sn)foil is a promising candidate anode for lithium-ion batteries(LIBs)due to its metallurgical processability and high capacity.However,it suffers low initial Coulombic efficiency and inferior cycling stability due to its uneven alloying/dealloying reactions,large volume change and stress,and fast electrode structural degradation.Herein,we report an undulating LiSn electrode fabricated by a scalable two-step procedure involving mechanical lithography and chemical prelithiation of Sn foil.With the combination of experimental measurements and chemo-mechanical simulations,it was revealed the obtained undulating LiSn/Sn electrode could ensure better mechanical stability due to the pre-swelling state from Sn to Li x Sn and undulating structure of lithography in comparison with plane Sn,homogenize the electrochemical alloying/dealloying reactions due to the activated surface materials,and compensate Li loss during cycling due to the introduction of excess Li from Li_(x)Sn,thus enabling enhanced electrochemical performance.Symmetric cells consisting of undulating LiSn/Sn electrode with an active thickness of∼5 um displayed stable cycling over 1000 h at 1 mA cm^(-2) and 1 mAh cm^(-2) with a low average overpotential of<15 mV.When paired with commercial LiNi_(0.6)Co_(0.2)Mn_(0.2)O_(2)(NCM622)cathode with high mass loading of 15.8 mg cm^(-2),the full cell demonstrated a high capacity of 2.4 mAh cm^(-2) and outstanding cycling stability with 84.9% capacity retention at 0.5 C after 100 cycles.This work presents an advanced LiSn electrode with stress-regulation design toward high-performance LIBs,and sheds light on the rational electrode design and processing of other high-capacity lithium alloy anodes. | Chunhao Li Shuibin Tu Xin Ai Siwei Gui Zihe Chen Wenyu Wang Xiaoxiao Liu Yuchen Tan Hui Yang Yongming Sun | 2023 | Energy & Environmental Materials2023，6，1： | 0 |
| 10 | 6-5 Operation of HWRs for C-ADS Injector显示文摘There are two types of HWR cavities have been developed in IMP for C-ADS Injector.HWR010s have been used to accelerate proton from 2.1 MeV to 10 MeV.There are 12 HWR010s assembled in two CMs.The taper type HWR015s have been used to accelerate proton from 10MeV to 18.5 MeV.There are 5 HWRs assembled in the third CM.Proton beam has been accelerated to 26 MeV by HWR010,HWR015 and Spoke021 in June 2017.The beam has been accelerated to 18.5 MeV by HWR010 and HWR015.The CMs in the tunnel are shown in Fig.1. | Yue Weiming Zhang Shenghu Li Yongming Chang Wei Jiang Tiancai Zhang Shengxue Gao Zheng Wang Ruoxue Huang Shichun Pan Feng Chen Long Li Chunlong Song Yukun Guo Hao Xiong Pingran Cong Zhang Tan Teng Wan Yuqin Niu Xiaofei Bai Feng Hu Chuanfei Zhang Peng Liu Lubei Huang Yulu Zhao Yugang Guo Xiaohong You Zhiming Zhang Junhui Huang Guirong He Yuan | 2016 | IMP & HIRFL Annual Report2016，，1： | 0 |
| 11 | Room temperature phosphorescence from natural products: Crystallization matters显示文摘Efficient room temperature phosphorescence is observed in natural compounds and polymers such as starch,cellulose,bovine serum albumin(BSA),and some other carbohydrates.Whereas being practically nonluminescent in solutions and TLC plates,they emit bright phosphorescence in the crystalline states with lifetime up to microseconds,exhibiting crystallization-induced phosphorescence(CIP)characteristics.The CIP of these natural products without any conventional chromophores offers a new platform for the exploration of conceptually novel luminogens. | GONG YongYang TAN YeQiang MEI Ju ZHANG YiRen YUAN WangZhang ZHANG YongMing SUN JingZhi TANG BenZhong | 2013 | 中国科学:化学2013，43，9： | 0 |
| 12 | Crystallization-induced phosphorescence of benzils at room temperature显示文摘Efficient room temperature phosphorescence(RTP)is rarely observed in pure organic luminogens.However,we have newly observed that benzil and its derivatives are nonluminescent in solvents and thin layer chromatography(TLC)plates,but become highly phosphorescent in crystal state at room temperature,exhibiting typical crystallization-induced phosphorescence(CIP)characteristics.The CIP phenomenon is ascribed to the restriction of intramolecular rotations in crystals owing to effective intermolecular interactions.Such intermolecular interactions greatly rigidify the molecular conformation and significantly decrease the nonradiative deactivation channels of the triplet excitons,thus giving boosted phosphorescent emission at room temperature. | GONG YongYang TAN YeQiang LI Hong ZHANG YiRen YUAN WangZhang ZHANG YongMing SUN JingZhi TANG Ben Zhong | 2013 | 中国科学:化学2013，43，9： | 0 |
您所在的机构暂未开通此部分的功能，请联系管理员