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| 1 | An all-round AI-Chemist with a scientific mind显示文摘The realization of automated chemical experiments by robots unveiled the prelude to an artificial intelligence(AI)laboratory.Several AI-based systems or robots with specific chemical skills have been demonstrated,but conducting all-round scientific research remains challenging.Here,we present an all-round AI-Chemist equipped with scientific data intelligence that is capable of performing basic tasks generally required in chemical research.Based on a service platform,the AI-Chemist is able to automatically read the literatures from a cloud database and propose experimental plans accordingly.It can control a mobile robot in-house or online to automatically execute the complete experimental process on 14 workstations,including synthesis,characterization and performance tests.The experimental data can be simultaneously analysed by the computational brain of the AI-Chemist through machine learning and Bayesian optimization,allowing a new hypothesis for the next iteration to be proposed.The competence of the AI-Chemist has been scrutinized by three different chemical tasks.In the future,the more advanced all-round AI-Chemists equipped with scientific data intelligence may cause changes to the landscape of the chemical laboratory. | Qing Zhu Fei Zhang Yan Huang Hengyu Xiao LuYuan Zhao XuChun Zhang Tao Song XinSheng Tang Xiang Li Guo He BaoChen Chong JunYi Zhou YiHan Zhang Baicheng Zhang JiaQi Cao Man Luo Song Wang GuiLin Ye WanJun Zhang Xin Chen Shuang Cong Donglai Zhou Huirong Li Jialei Li Gang Zou WeiWei Shang Jun Jiang Yi Luo | 2022 | National Science Review2022,9,10: | 5 |
| 2 | 显示文摘 | Tang Jinsong Jing Xiabin Wang Baochen | 1998 | Synth Met1998,24,: | 1 |
| 3 | APBT-based image coding at low bit rates with down-sampling and all phase DCT interpolation 显示文摘 | Wang Chengyou Xie Songzhao Jiang Baochen | 2013 | Journal of Information and Computational Science2013,10,12: | 1 |
| 4 | In- frared spectra of soluble polyaniline 显示文摘 | TANG Jinsong JING Xiabing WANG Baochen | 1988 | Synthetic Metals1988,24,: | 1 |
| 5 | Structural design of imidazolium and its application in PP/montmorillonite nanocomposites显示文摘 | Aihua He Limei Wang Wei Yao Baochen Huang Dujin Wang Charles C. Han | 2009 | Polymer Degradation and Stability2009,,4: | 1 |
| 6 | 显示文摘 | Tang Jinsong Jing Xiabin Wang Baochen | 1998 | Synth Met1998,24,: | 1 |
| 7 | APBT-based image coding at low bit rates with down-sampling and all phase DCT interpolation显示文摘 | Wang Chengyou Xie Songzhao Jiang Baochen | 2013 | Journal of Information and Computational Science2013,10,12: | 1 |
| 8 | Deep desulfufization of diesel oil oxidized by Fe (VI) systems显示文摘 | Liu Shuzhi Wang Baohui Cui Baochen | 2008 | Fuel2008,87,: | 1 |
| 9 | Modeling of tunneling-induced ground surface movements using stochastic medium theory显示文摘 | YANG Junsheng LIU Baochen WANG Mingchun | 2004 | Tunnelling and Underground Space Technology2004,19,2: | 1 |
| 10 | Preparation of Amorphous LiZn Ferrites Hollow Microspheres by Self-reactive Quenching Technology显示文摘NaCl aqueous solution(15 wt%) was used as the quenching medium to prepare amorphous Lithium-Zinc ferrite hollow microspheres(LiZn FHMs) based on self-reactive quenching technology. Investigations by scanning electro microscope, X-ray diffraction, electron diffraction of transmission electron microscope, and differential scanning calorimetry prove that LiZn FHMs are susceptible to amorphization. It is indicated that NaCl aqueous solution(15 wt%) has ultra-fast quenching speed, and the growth rate of crystals on LiZn FHMs is so large that the formation and growth of the crystal nucleus are significantly restrained. This is the main reason for the formation of amorphous LiZn FHMs. | 蔡旭东 WANG Jianjiang LI Baochen XU Baocai WU Aihua WANG Bing | 2017 | Journal of Wuhan University of Technology(Materials Science)2017,32,4: | 1 |
| 11 | Infiared spectra of sol- uble polyaniline显示文摘 | Jinsong Tang Xiabin Jing Baochen Wang | 1988 | Synthetic Metals1988,24,: | 1 |
| 12 | Deep desulfuriza tion of diesel oil oxidized by Fe ( VI ) systems显示文摘 | Liu Shuzhi Wang Baohui Cui Baochen | 2008 | Fuel2008,87,3: | 1 |
| 13 | A novel Tb^(3+) and Eu^(3+) co-doped dual-emitting phosphate K_(3)SrBi(P_(2)O_(7))_(2) phosphor for application in FIR thermometers显示文摘Rare earth co-doped phosphor for fluorescence intensity ratio(FIR) thermometer has gained increasing attention in recent years. Herein, the novel Tb^(3+)and Eu^(3+)co-doped K_(3)SrBi(P_(2)O_(7))_(2)(KSBP) phosphate phosphors were reported. The crystal structure of the title phosphor was determined using Rietveld refinement and proved to have a three-dimensional structure. The time-resolved spectroscopy reveals that there is almost no energy transfer between Tb^(3+)and Eu^(3+). More importantly, Tb^(3+)and Eu^(3+)emissions show different thermal quenching behaviors, which claims the potential of this material for application in optical thermometer. The FIR of the typical KSBP:0.02Tb^(3+),0.04Eu^(3+)sample demonstrates a polynomial relationship as a function of temperature and the absolute and relative sensitivity are0.025 K^(-1) and 0.59%/K, respectively. In general, our study reports a novel and potential KSBP:Tb^(3+),Eu^(3+)phosphate phosphor that is promising for use in high-sensitive FIR thermometers. | Baochen Wang Shifeng Sun Zeqi Li Zongwang Li Weiwei Lin Chao Zeng Yan-gai Liu Ruiyu Mi | 2024 | Journal of Rare Earths2024,42,3: | 0 |
| 14 | A Combined Weight of Evidence and Logistic Regression Method for Susceptibility Mapping of Earthquake-induced Landslides: A Case Study of the April 20, 2013 Lushan Earthquake, China显示文摘The M_s 7.0 Lushan earthquake triggered a huge number of landslides. Landslide susceptibility mapping is of great importance. Weight of Evidence(Wo E) and Logistic Regression(LR) methods have been widely used for LSM(Landslide Susceptibility Mapping). However, limitations still exist. Wo E is capable of assessing the influence of different classes of each factor, but neglects the correlation between factors. LR is able to analyze the relationship among the factors while it is not capable of evaluating the influence of different classes. This paper proposes a combined method of LR and Wo E for LSM, taking advantage of their individual merits and overcoming their limitations. An inventory of 1289 landslides was used: 70% were random-selected for training and the remaining for validation. 11 landslide condition factors were employed in the model and the result was validated using Receiver Operating Characteristic(ROC) curve. The results showed that the LRWo E model had a better accuracy than the LR model, producing an area below the curve with values of 0.802 success and 0.791 predictive, higher than that of the LR model(0.715 success and 0.722 predictive). It is therefore concluded that the combined method of Wo E and LR can provide a promising level of accuracy for earthquake-induced landslide susceptibility mapping. | ZHOU Suhua WANG Wei CHEN Guangqi LIU Baochen FANG Ligang | 2016 | Acta Geologica Sinica(English Edition)2016,90,2: | 0 |
| 15 | Copolymerization of 1-butene and 1-hexene with supported titanium catalyst显示文摘With TiCl4/MgCl2(Ti)and Al(i-Bu)3(Al)as catalysts,the thermoplastic copolymer of 1-butene(Bt)and 1-hexene(He)was synthesized successfully.The effects of Bt/He,Ti/(He+Bt),Al/Ti,temperature and reaction time on conversion,catalyst efficiency(CE),intrinsic viscosity([g])and insoluble content were studied.The copolymer was analyzed with Fourier transform-infrared(FTIR)and nuclear magnetic resonance(1H-NMR).Results showed that the optimal polymerization conditions were:He/Bt=0.25,temperature 40℃–50℃,Al/Ti=400–500,Ti/(Bt+He)=3x10-5-4x10-5,time 4 h.Intrinsic viscosity was found to increase with increasing Ti/(Bt+He)and decreasing Al/Ti and polymerization temperature.When the molar content of He,Al/Ti and polymerization temperature increased,the insoluble content in CH2Cl2 of copolymers decreased.When Ti/(Bt+He)and reaction time increased,the insoluble con-tent in CH2Cl2 of copolymers also increased.The crystal-lization and stereoregularity of poly(1-butene)decreased with the addition of He. | ZHAO Yongxian SHAO Huafeng WANG Bo YAO Wei HUANG Baochen | 2007 | Frontiers of Chemical Science and Engineering2007,1,3: | 0 |