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| 1 | Multiple Alleles Encoding Atypical NLRs with Unique Central Tandem Repeats in Rice Confer Resistance to Xanthomonas oryzae pv. oryzae显示文摘Plants have developed various mechanisms for avoiding pathogen invasion,including resistance(R)genes.Most R genes encode nucleotide-binding domain and leucine-rich repeat containing proteins(NLRs).Here,we report the isolation of three new bacterial blight R genes in rice,Xa1-2,Xa14,and Xa31(t),which were allelic to Xa1 and encoded atypical NLRs with unique central tandem repeats(CTRs).We also found that Xa31(t)was the same gene as Xa1-2.Although Xa1-2 and Xa14 conferred different resistance spectra,their performance could be attenuated by iTALEs,as has previously been reported for Xa1.XA1,XA1-2,XA14,and non-resistant RGAF differed mainly in the substructure of the leucine-rich repeat domain.They all contained unique CTRs and belonged to the CTR-NLRs,which existed only in Gramineae.We also found that interactions among these genes led to differing resistance performance.In conclusion,our results uncover a unique locus in rice consisting of at least three multiple alleles(Xa1,Xa1-2,and Xa14)that encode CTRNLRs and confer resistance to Xanthomonas oryzae pv.oryzae(Xoo). | Biaoming Zhang Haitao Zhang Fang Li Yidan Ouyang Meng Yuan Xianghua Li Jinghua Xiao Shiping Wang | 2020 | Plant Communications2020,1,4: | 8 |
| 2 | The RING E3 ligase CLG1 targets GS3 for degradation via the endosome pathway to determine grain size in rice显示文摘G-protein signaling and ubiquitin-dependent degradation are both involved in grain development in rice,but how these pathways are coordinated in regulating this process is unknown.Here,we show that Chang Li Geng 1(CLG1),which encodes an E3 ligase,regulates grain size by targeting the Gγprotein GS3,a negative regulator of grain length,for degradation.Overexpression of CLG1 led to increased grain length,while overexpression of mutated CLG1 with changes in three conserved amino acids decreased grain length.We found that CLG1 physically interacts with and ubiquitinats GS3which is subsequently degraded through the endosome degradation pathway,leading to increased grain size.Furthermore,we identified a critical SNP in the exon 3 of CLG1 that is significantly associated with grain size variation in a core collection of cultivated rice.This SNP results in an amino acid substitution from Arg to Ser at position 163 of CLG1 that enhances the E3 ligase activity of CLG1 and thus increases rice grain size.Both the expression level of CLG1 and the SNP CLG1163S may be useful variations for manipulating grain size in rice. | Wensi Yang Kun Wu Bo Wang Huanhuan Liu Siyi Guo Xiaoyu Guo Wei Luo Shengyuan Sun Yidan Ouyang Xiangdong Fu Kang Chong Qifa Zhang Yunyuan Xu | 2021 | Molecular Plant2021,14,10: | 6 |
| 3 | Artificial Selection in Domestication and Breeding Prevents Speciation in Rice显示文摘Speciation has long been regarded as an irreversible process once the reproductive barriers had been established.However,unlike in natural populations,artificial selection might either accelerate or prevent speciation processes in domesticated species.Asian cultivated rice is a target crop for both domestication and artificial breeding;it contains two subspecies of indica and japonica,which usually produce sterile inter-subspecific hybrids due to reproductive barriers.In this study,we constructed the evolutionary trajectory of a reproductive isolation system S5,which regulates fertility in indica-japonica hybrids via three adjacent genes,based on the data of 606 accessions including two cultivated and 11 wild rice species.Although hybrid sterility haplotypes at S5 lead to establishment of a killer-protector reproductive barrier,origin of wide-compatibility haplotypes by complex hybridization and recombination provides an opposing force to reproductive isolation and thus prevents speciation during domestication.Analysis in a diallel set of 209 crosses involving 21 parents showed that the wide-compatibility genotypes largely rescued fertility of indica-japonica hybrids,indicating that the wide-compatibility gene would enable gene flow to maintain species coherence.This counteracting system indicates that combined effects of natural evolution and artificial selection may result in reversible processes of speciation in rice,which may also have implications for genetic improvement of rice. | Jiaming Mi Guangwei Li Conghao Xu Jiangyi Yang Huihui Yu Gongwei Wang Xianghua Li Jinghua Xiao Huazhi Song Qifa Zhang Yidan Ouyang | 2020 | Molecular Plant2020,13,4: | 6 |
| 4 | Recent progress in stability of perovskite solar cells显示文摘Perovskite solar cells have attracted significant attention in just the past few years in solar cell research fields,where the power conversion efficiency was beyond 22.1%.Now,the most important challenge for perovskite solar cells in practical applications is the stability issue.In this mini-review,we will summarize the degradation mechanism of perovskite solar cells,including the perovskite material itself and also the interfaces.While we also provide our opinion on improving the stability of perovskite solar cells. | Xiaojun Qin Zhiguo Zhao Yidan Wang Junbo Wu Qi Jiang Jingbi You | 2017 | Journal of Semiconductors2017,38,1: | 4 |
| 5 | Genome-wide dissection of segregation distortion using multiple inter-subspecific crosses in rice显示文摘Mendelian inheritance can ensure equal segregation of alleles from parents to offspring, which provides fundamental basis for genetics and molecular biology. Segregation distortion(SD) leads to preferential transmission of certain alleles from generation to generation. Such violation of Mendelian genetic principle is often accompanied by reproductive isolation and eventually speciation. Although SD is observed in a wide range of species from plants to animals, genome-wide dissection of such biased transmission of gametes is rare. Using nine inter-subspecific rice crosses, a genome-wide screen for SD loci is performed, which reveals 61 single-locus quantitative trait loci and 194 digenic interactions showing distorted transmission ratio, among which 24 new SD loci are identified. Biased transmission of alleles is observed in all nine crosses, suggesting that SD exists extensively in rice populations. 72.13% distorted regions are repeatedly detected in multiple populations, and the most prevalent SD hotspot that observed in eight populations is mapped to chromosome 3. Xian alleles are transmitted at higher frequencies than geng alleles in inter-subspecific crosses, which change the genetic composition of the rice populations. Epistatic interaction contributes significantly to the deviation of Mendelian segregation at the whole-genome level in rice, which is distinct from that in animals. These results provide an extensive archive for investigating the genetic basis of SD in rice, which have significant implications in understanding the reproductive isolation and formation of inter-subspecific barriers during the evolution. | Guangwei Li Jiye Jin Yan Zhou Xufeng Bai Donghai Mao Cong Tan Gongwei Wang Yidan Ouyang | 2019 | Science China(Life Sciences)2019,62,4: | 4 |
| 6 | Facile Approach to Synthesize Gold Nanorod@Polyacrylic Acid/Calcium Phosphate Yolk–Shell Nanoparticles for Dual-Mode Imaging and pH/NIR-Responsive Drug Delivery显示文摘A facile strategy to fabricate gold nanorod@polyacrylic acid/calcium phosphate(Au NR@-PAA/Ca P) yolk–shell nanoparticles(NPs) composed with a PAA/Ca P shell and an Au NR yolk is reported. The asobtained Au NR@PAA/Ca P yolk–shell NPs possess ultrahigh doxorubicin(DOX) loading capability(1 mg DOX/mg NPs), superior photothermal conversion property(26%)and p H/near-infrared(NIR) dual-responsive drug delivery performance. The released DOX continuously increased due to the damage of the Ca P shell at low p H values. When the DOX-loaded Au NR@PAA/Ca P yolk–shell NPs wereexposed to NIR irradiation, a burst-like drug release occurs owing to the heat produced by the Au NRs. Furthermore,Au NR@PAA/Ca P yolk–shell NPs are successfully employed for synergic dual-mode X-ray computed tomography/photoacoustic imaging and chemo-photothermal cancer therapy. Therefore, this work brings new insights for the synthesis of multifunctional nanomaterials and extends theranostic applications. | Guilan Li Yidan Chen Lingyu Zhang Manjie Zhang Shengnan Li Lu Li Tingting Wang Chungang Wang | 2018 | Nano-Micro Letters2018,10,1: | 3 |
| 7 | Bract suppression regulated by the miR156/529-SPLs-NL1-PLA1 module is required for the transition from vegetative to reproductive branching in rice显示文摘Reproductive transition of grasses is characterized by switching the pattern of lateral branches,featuring the suppression of outgrowth of the subtending leaves(bracts)and rapid formation of higher-order branches in the inflorescence(panicle).However,the molecular mechanisms underlying such changes remain largely unknown.Here,we show that bract suppression is required for the reproductive branching in rice.We identified a pathway involving the intrinsic time ruler microRNAI56/529,their targets SQUAMOSA PROMOTER BINDING PROTEIN LIKE(SPL)genes,NECK LEAF1(NL1),and PLASTOCHRON1(PLA1),which regulates the bract outgrowth and thus affects the pattern switch between vegetative and reproductive branching.Suppression of the bract results in global reprogramming of transcriptome and chromatin accessibility following the reproductive transition,while these processes are largely dysregu-lated in the mutants of these genes.These discoveries contribute to our understanding of the dynamic plant architecture and provide novel insights for improving crop yields. | Lei Wang Luchang Ming Keyan Liao Chunjiao Xia Shengyuan Sun Yu Chang Hongkai Wang Debao Fu Conghao Xu Zhengji Wang Xu Li Weibo Xie Yidan Ouyang Qinglu Zhang Xianghua Li Qinghua Zhang Jinghua Xiao Qifa Zhang | 2021 | Molecular Plant2021,14,7: | 2 |
| 8 | Validation and Spatiotemporal Distribution of GEOS-5-Based Planetary Boundary Layer Height and Relative Humidity in China显示文摘Few studies have specifically focused on the validation and spatiotemporal distribution of planetary boundary layer height(PBLH) and relative humidity(RH) data in China. In this analysis, continuous PBLH and surface-level RH data simulated from GEOS-5 between 2004 and 2012, were validated against ground-based observations. Overall, the simulated RH was consistent with the statistical data from meteorological stations, with a correlation coefficient of 0.78 and a slope of 0.9. However, the simulated PBLH was underestimated compared to LIDAR data by a factor of approximately two,which was primarily because of poor simulation in late summer and early autumn. We further examined the spatiotemporal distribution characteristics of two factors in four regions—North China, South China, Northwest China, and the Tibetan Plateau. The results showed that the annual PBLH trends in all regions were fairly moderate but sensitive to solar radiation and precipitation, which explains why the PBLH values were ranked in order from largest to smallest as follows: Tibetan Plateau, Northwest China, North China, and South China. Strong seasonal variation of the PBLH exhibited high values in summer and low values in winter, which was also consistent with the turbulent vertical exchange. Not surprisingly, the highest RH in South China and the lowest RH in desert areas of Northwest China(less than 30%). Seasonally, South China exhibited little variation, whereas Northwest China exhibited its highest humidity in winter and lowest humidity in spring,the maximum values in the other regions were obtained from July to September. | Yidan SI Shenshen LI Liangfu CHEN Chao YU Zifeng WANG Yang WANG Hongmei WANG | 2018 | Advances in Atmospheric Sciences2018,35,4: | 2 |
| 9 | Degradable Hybrid CuS Nanoparticles for Imaging-Guided Synergistic Cancer Therapy via Low-Power NIR-II Light Excitation显示文摘Near-infrared(NIR)-II light-excitable photonic agents capable of generating tumor hyperthermia and cytotoxic free radicals are promising for synergistic phototherapy of tumors.However,the lack of NIR-II excitable agents makes it challenging to achieve combinational tumor phototherapy.Here,the authors have reported on a tumor-targeting and degradable hybrid copper sulfide(CuS)nanoparticle(AIBA@CuS-FA)via loading a hydrophilic Azo initiator(AIBA)into an amphiphilic lipid-encapsulating CuS nanoparticle.AIBA@CuS-FA shows high photothermal conversion efficiency(PCE≈47.5%)at 1064 nm,enabling heat production to trigger tumor hyperthermia and thermal decomposition of AIBA into cytotoxic free alkyl radicals upon irradiation with a 1064-nm laser under low-power density(0.5 W/cm2).Moreover,alkyl radicals can drive degradation of AIBA@CuS-FA and embedded CuS nanodisks,releasing Cu^(2+)ions that can catalyze a Fenton-like reaction for hydroxyl radical(•OH)production to promote tumor therapy.Findings demonstrate promise for combinational photothermal therapy(PTT),oxygen-independent alkyl radical therapy,and chemodynamic therapy(CDT)of tumors. | Yidan Sun Hua Shi Xiaoyang Cheng Luyan Wu Yuqi Wang Zhengyang Zhou Jian He Hong-Yuan Chen Deju Ye | 2021 | CCS Chemistry2021,3,5: | 2 |
| 10 | NUPR1 promotes the proliferation and metastasis of oral squamous cell carcinoma cells by activating TFE3-dependent autophagy显示文摘Oral squamous cell carcinoma(OSCC)is the most common type of oral malignancy,and metastasis accounts for the poor prognosis of OSCC.Autophagy is considered to facilitate OSCC development by mitigating various cellular stresses;nevertheless,the mechanisms of autophagy in OSCC cell proliferation and metastasis remain unknown.In our study,high-sensitivity label-free quantitative proteomics analysis revealed nuclear protein 1(NUPR1)as the most significantly upregulated protein in formalin-fixed paraffin-embedded tumour samples derived from OSCC patients with or without lymphatic metastasis. | Tengfei Fan Xiaoning Wang Sheng Zhang Ping Deng Yi Jiang Yidan Liang Sheng Jie Qing Wang Chuwen Li Guocai Tian Zhen Zhang Zhenhu Ren Bo Li Yanrong Chen Zhijing He Yan Luo Mingliang Chen Hanjiang Wu Zhengping Yu Huifeng Pi Zhou Zhou Zhiyuan Zhang | 2022 | Signal Transduction and Targeted Therapy2022,7,5: | 2 |
| 11 | Factors determining soil water heterogeneity on the Chinese Loess Plateau as based on an empirical mode decomposition method显示文摘Soil water is a critical resource,and as such is the focus of considerable physical research.Characterization of the distribution and spatial variability of soil water content(SWC)offers important agronomic and environmental information.Estimation of non-stationary and non-linear SWC distribution at different scales is a research challenge.Based on this context,we performed a case study on the Chinese Loess Plateau,with objectives of investigating spatial variability of SWC and soil properties(i.e.,soil particle composition,organic matter and bulk density),and determining multi-scale correlations between SWC and soil properties.A total of 86 in situ sampling sites were selected and 516 soil samples(0–60 cm depth with an interval of 10 cm)were collected in May and June of 2019 along the Yangling-Wugong-Qianxian transect,with a length of 25.5 km,in a typical wheat-corn rotation region of the Chinese Loess Plateau.Classical statistics and empirical mode decomposition(EMD)method were applied to evaluate characteristics of the overall and scale-specific spatial variation of SWC,and to explore scale-specific correlations between SWC and soil properties.Results showed that the spatial variability of SWC along the Yangling-Wugong-Qianxian transect was medium to weak,with a variability coefficient range of 0.06–0.18,and it was gradually decreased as scale increased.We categorized the overall SWC for each soil layer under an intrinsic mode function(IMF)number based on the scale of occurrence,and found that the component IMF1 exhibited the largest contribution rates of 36.45%–56.70%.Additionally,by using EMD method,we categorized the general variation of SWC under different numbers of IMFs according to occurrence scale,and the results showed that the calculated scales among SWC for each soil layer increased in correspondence with higher IMF numbers.Approximately 78.00%of the total variance of SWC was extracted in IMF1 and IMF2.Generally,soil texture was the dominant control on SWC,and the influence of the three types of soil properties(soil particle composition,organic matter and bulk density)was more prominent at larger scales along the sampling transect.The influential factors of soil water spatial distribution can be identified and ranked on the basis of the decomposed signal from the current approach,thereby providing critical information for other researchers and natural resource managers. | GONG Yidan XING Xuguang WANG Weihua | 2020 | Journal of Arid Land2020,12,3: | 2 |
| 12 | Transition of autophagy and apoptosis in fibroblasts depends on dominant expression of HIF-1αor p53显示文摘It has been revealed that hypoxia is dynamic in hypertrophic scars;therefore,we considered that it may have different effects on hypoxia-inducible factor-1α(HIF-1α)and p53 expression.Herein,we aimed to confirm the presence of a teeterboard-like conversion between HIF-1αand p53,which is correlated with scar formation and regression.Thus,we obtained samples of normal skin and hypertrophic scars to identify the differences in HIF-1αand autophagy using immunohistochemistry and transmission electron microscopy.In addition,we used moderate hypoxia in vitro to simulate the proliferative scar,and silenced HIF-1αor p53 gene expression or triggered overexpression to investigate the changes of HIF-1αand p53 expression,autophagy,apoptosis,and cell proliferation under this condition.HIF-1α,p53,and autophagy-related proteins were assayed using western blotting and immunofluorescence,whereas apoptosis was detected using flow cytometry analysis,and cell proliferation was detected using cell counting kit-8(CCK-8)and 5-bromo-2′-deoxyuridine(BrdU)staining.Furthermore,immunoprecipitation was performed to verify the binding of HIF-1αand p53 to transcription cofactor p300.Our results demonstrated that,in scar tissue,HIF-1αexpression increased in parallel with autophagosome formation.Under hypoxia,HIF-1αexpression and autophagy were upregulated,whereas p53 expression and apoptosis were downregulated in vitro.HIF-1αknockdown downregulated autophagy,proliferation,and p300-bound HIF-1α,and upregulated p53 expression,apoptosis,and p300-bound p53.Meanwhile,p53 knockdown induced the opposite effects and enhanced HIF-1α,whereas p53 overexpression resulted in the same effects and reduced HIF-1α.Our results suggest a teeterboard-like conversion between HIF-1αand p53,which is linked with scar hyperplasia and regression. | Min LI Yidan SU Xiaoyuan GAO Jiarong YU Zhiyong WANG Xiqiao WANG | 2022 | Journal of Zhejiang University-Science B(Biomedicine & Biotechnology)2022,23,3: | 2 |
| 13 | Immune-adjuvant loaded Bi2Se3 nanocage for photothermal-improved PD-L1 checkpoint blockade immune-tumor metastasis therapy显示文摘Checkpoint blockade based immune therapy has shown to be effective but benefit only the minority of patients whose tumors have been pre-infiltrated by T cells. To overcome this obstacles, a PEG-modified Bi2Se3 nanocage (NC) loaded with imiquimod (R848), which could efficiently destroy the tumors thus producing enough tumor-associated antigens (TAA) and with the existence of R848, a toll-like-receptor-7 agonist, could generate strong anti-cancer immune responses is reported in this study. Moreover, immunogenic Bi2Se3 NC-PEG/R848 mediated photothermal therapy (PTT) sensitizes tumors to checkpoint inhibition mediated by a PD-L1 antibody, not only ablating cancer cells upon NIR laser but also causing strong anti-cancer immunity to suppress distant tumor growth post PTT. Both in vitro and in vivo experiments demonstrate that the Bi2Se3 NC-PEG/R848 could effectively activate a PTT-induced immune response as well as silence immune resistance based on PD-L1 checkpoint blockade to ablate the primary tumor and further inhibit the tumor metastasis. Bi2Se3 NC reported here exhibits high photothermal conversion efficiency and stability, as well as competent drug loading capacity with large hollow structures and high surface area. Our study not only provides a facial way to synthesize Bi2Se3 NC, but also offers an alternative strategy for tumor metastasis. | Yilin Song Yidan Wang Siyu Wang Yu Cheng Qianglan Lu Lifang Yang Fengping Tan Nan Li | 2019 | Nano Research2019,12,8: | 2 |
| 14 | Spontaneous movement of a retrotransposon generated genic dominant male sterility providing a useful tool for rice breeding显示文摘Male sterility in plants provides valuable breeding tools in germplasm innovation and hybrid crop production.However,genetic resources for dominant genic male sterility,which hold great promise to facilitate breeding processes,are extremely rare in natural germplasm.Here we characterized the Sanming Dominant Genic Male Sterility in rice and identified the gene SDGMS using a map-based cloning approach.We found that spontaneous movement of a 1978-bp long terminal repeat(LTR)retrotransposon into the promoter region of the SDGMS gene activates its expression in anther tapetum,which causes abnormal programmed cell death of tapetal cells resulting in dominant male sterility.SDGMS encodes a ribosome inactivating protein showing N-glycosidase activity.The activation of SDGMS triggers transcription reprogramming of genes responsive to biotic stress leading to a hypersensitive response which causes sterility.The results demonstrate that an ectopic gene activation by transposon movement can give birth to a novel trait which enriches phenotypic diversity with practical utility. | Conghao Xu Yifeng Xu Zhengji Wang Xiaoyu Zhang Yuying Wu Xinyan Lu Hongwei Sun Lei Wang Qinglu Zhang Qinghua Zhang Xianghua Li Jinghua Xiao Xu Li Mingfu Zhao Yidan Ouyang Xianbo Huang Qifa Zhang | 2023 | National Science Review2023,10,9: | 1 |
| 15 | Local mild hypothermia with thrombolysis for acute ischemic stroke within a 6-h window显示文摘 | Min Bi Qilin Ma Shiyang Zhang Jianpeng Li Yidan Zhang Longting Lin Suijun Tong Desheng Wang | 2011 | Clinical Neurology and Neurosurgery2011,,: | 1 |
| 16 | Prevalence and molecular characterization of Pentatrichomonas hominis in Siberian tigers(Panthera tigris altaica)in northeast China显示文摘INTRODUCTION Pentatrichomonas hominis,an anaerobic flagellated protozoan that inhabits the large intestines of mammals and belongs to the Trichomonadidae family(Wenrich 1944;Kim et al.2010;Li et al.2014b,2016,2018a,2020;Maritz et al.2014;Zhang et al.2019),is mainly transmitted through the fecal-oral route.It was originally presumed to be a commensal protozoan(Tolbert et al.2012)but was found to cause gastrointestinal symptoms. | Hongbo ZHANG Nan ZHANG Pengtao GONG Shuqin CHENG Xiaocen WANG Xin LI Zhijun HOU Chang LIU Tianqi BI Bobo WANG Yidan CHENG Jianhua LI Xichen ZHANG | 2022 | Integrative Zoology2022,17,4: | 1 |
| 17 | trans-2-Enoyl-CoA Reductase Tecr-Driven Lipid Metabolism in Endothelial Cells Protects against Transcytosis to Maintain Blood-Brain Barrier Homeostasis显示文摘The transport and metabolism of lipids in cerebrovascular endothelial cells(ECs)have been hypothesized to regulate blood-brain barrier(BBB)maturation and homeostasis.Long-chain polyunsaturated fatty acids(LCPUFAs)as the important lipids components of cell membranes are essential for the development and function of BBB,but the direct links of lipid metabolism and ECs barrier function remain to be established.Here,we comprehensively characterize the transcriptomic phenotype of developmental cerebrovascular ECs in single-cell resolution and firstly find that trans-2-enoyl-CoA reductase(Tecr),a verylong-chain fatty acid synthesis,is highly expressed during barriergenesis and decreased after BBB maturation.EC-specific knockout of Tecr compromises angiogenesis due to delayed vascular sprouting.Importantly,EC-specific deletion of Tecr loss restrictive quality of vascular permeability from neonatal stages to adulthood,with high levels of transcytosis,but maintains the vascular tight junctions.Moreover,lipidomic analysis shows that the expression of Tecr in ECs is associated with the containing of omega-3 fatty acids,which directly suppresses caveolae vesicles formation.These results reveal a protective role for Tecr in BBB integrity and suggest that Tecr as a novel therapeutic target in the central nervous system(CNS)diseases associated with BBB dysfunction. | Jinxuan Wang Jianxiong Xu Guangchao Zang Tao Zhang Qi Wu Hongping Zhang Yidan Chen Yi Wang Weixi Qin Shuang Zhao Erdai Qin Juhui Qiu Xiaojuan Zhang Lin Wen Yeqi Wang Guixue Wang | 2022 | Research2022,,3: | 1 |
| 18 | Phosphorus-induced electronic structure reformation of hollow NiCo_(2)Se_(4) nanoneedle arrays enabling highly efficient and durable hydrogen evolution in all-pH media显示文摘With practical electrocatalytic hydrogen production frequently involving the splitting of water in various pH media,there is an urgent need but still a technical challenge to develop low-cost,highly active,and stable electrocatalysts for pH-universal hydrogen evolution reaction(HER).We report herein the adoption of a hydrothermal reaction combined with a post gas-phase doping strategy to fabricate P-doped NiCo_(2)Se_(4) hollow nanoneedle arrays on carbon fiber paper(i.e.,P-NiCo_(2)Se_(4)/CFP).Notably,the optimal arrays(P8.71-NiCo_(2)Se_(4)/CFP)can afford an outstanding pH-universal HER performance,with an overpotential as low as 33,57,and 69 mV at 10 mA·cm^(−2) and corresponding Tafel slopes down to 52,61,and 72 mV·dec^(−1) in acidic,alkaline,and neutral media,respectively,outperforming most state-of-the-art nonprecious catalysts and even the commercial Pt/C catalyst in both neutral and alkaline media at large current densities.Impressively,P_(8.71-)NiCo_(2)Se_(4)/CFP also displays good durability toward long-time stability testing in harsh acidic and alkaline electrolytes.Experimental and theoretical studies further reveal that the doping of P atoms into NiCo_(2)Se_(4) can simultaneously optimize its H*adsorption/desorption energy,water adsorption energy,and water dissociation energy by adjusting the local electronic states of various active sites,thus accelerating the rate-determining step of HER in different pH media to endow P-NiCo_(2)Se_(4) with an outstanding pH-universal HER performance.This work provides atomic-level insights into the roles of active sites in various electrolysis environments,thereby shedding new light on the rational design of highly efficient pH-universal nonprecious catalysts for HER and beyond. | Guojing Wang Yuzhuo Sun Yidan Zhao Yang Zhang Xiaohong Li Louzhen Fan Yunchao Li | 2022 | Nano Research2022,15,10: | 1 |
| 19 | HASILT:An intelligent software platform for HAZOP,LOPA,SRS and SIL verification显示文摘 | Cui Lin Shu Yidan Wang Zhaohui | | 0,,: | 1 |
| 20 | As- partic proteases gene family in rice: gene structure and expression, predicted protein features and phylo- genetic relation 显示文摘 | Chen Jiongjiong Ouyang Yidan Wang Lei | 2009 | Gene2009,442,12: | 1 |