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| 1 | Key Technologies of Ultra-high Voltage Hybrid LCC-VSC MTDC Systems显示文摘The key technologies of ultra-high voltage hybrid LCC-VSC MTDC systems are investigated,focusing on the design of system configurations,converter topologies and the control and protection system.A double converter per pole of VSC connection is proposed along with the design of a 5000 MW VSC valve to develop a±800 kV/5000 MW large-capacity power transmission.The hybrid MMC topology capable of clearing the DC faults and the control strategy are developed to effectively improve the reliability in case of overhead line faults.The control and protection system of the LCC-VSC MTDC system is introduced to offer flexible operations under both normal and abnormal conditions,which includes voltage/current margin-based coordination,converter switch-in and switch-out,re-connection and drop-off of a third station.Simulations of an LCC-VSC MTDC system based on the LCC-VSC MTDC project are performed. | Hong Rao Yuebin Zhou Shukai Xu Xipeng Cai Wanyu Cao Yiliang Xu Chenglin Ren | 2019 | CSEE Journal of Power and Energy Systems2019,5,3: | 14 |
| 2 | Quantitative determination of mitiglinide in human plasma by ultra-performance liquid chromatography/electrospray ionization tandem mass spectrometry 显示文摘 | Shuang Cai Taoguang Huo Wanyu Feng | 2008 | Journal of Chromatography B2008,868,12: | 1 |
| 3 | Construction of Ru/WO3 with hetero-interface structure for efficient hydrogen evolution reaction显示文摘Water electrolysis is considered as one most promising technique for hydrogen production.The high efficiency electrocatalyst is the key to accelerating the sluggish kinetics of the hydrogen evolution reaction(HER) in alkaline media.In this work,an efficient HER electrocatalyst with hetero-interfacial metal-metal oxide structure was constructed through a redox solid phase reaction(SPR) strategy.During the annealing process under Ar atmosphere,RuO_(2) and WS_(2)in RuO_(2)/WS_(2)precursor were converted to Ru nanoparticles(NPs) and WO3in situ,where tiny Ru NPs and oxygen vacancies were uniformly distributed onto the newly formed WO3nanosheets.Different characterization techniques were adopted to confirm the successful formation of Ru/WO_(3)electrocatalyst(RWOC).The optimized RWOC sample annealed at 400℃ exhibited the low overpotential value of 13 mV at a current density of 10 mA cm^(-2)and strong durability under the alkaline condition.Density functional theoretical calculations further revealed that the promoted adsorption/desorption rate of reaction intermediates and the accelerated kinetics of HER process were deduced to the synergistic effect between Ru and WO_(3)in electrocatalyst.This work provides a feasible method to fabricate highly efficient HER electrocatalysts. | Xin Xie Yunxiao Fan Wanyu Tian Meng Zhang Jialin Cai Xingang Zhang Jie Ding Yushan Liu Siyu Lu | 2023 | Journal of Energy Chemistry2023,,8: | 0 |
| 4 | Synthesis of highly-branched Au@AgPd core/shell nanoflowers for in situ SERS monitoring of catalytic reactions显示文摘Alloy and small size nanostructure s are favorable to catalytical performance,but not to surface-enhanced Raman spectroscopy(SERS) applications.Integrating SERS and catalytic activity into the nanocrystals with both alloy and small size structures is of great interest in fabrication of SERS platform to in situ monitor catalytical reaction.Herein,we report a facile method to synthesize Au@AgPd trimetallic nanoflowers(Au@AgPd NFs) with both SERS and catalytic activities,through simultaneous selective growth of Ag and Pd on Au core to form highly-branched alloy shell.These nanocrystals have the properties of small sizes,defects abundance,and highly-dispersed alloy shell which offer superior catalytic activity,while the merits of monodisperse,excellent stability,and highly-branched shell and core/alloy-shell structure promise the enhanced SERS activity.We further studied their growth mechanisms,and found that the ratio of Ag to Pd,sizes of Au core,and surfactant cetyltrimethylammonium bromide together determine this special structure.Using this as-synthesized nanocrystals,a monolayer bifunctional platform with both SERS and catalytical activity was fabricated through selfassembly at air/water interface,and applied to in situ SERS monitoring the reaction process of Pdcatalyzed hydrogenation of 4-nitrothiophenol to 4-aminothio p henol. | Yujian Lai Lijie Dong Rui Liu Shaoyu Lu Zuoliang He Wanyu Shan Fanglan Geng Yaqi Cai Jingfu Liu | 2020 | Chinese Chemical Letters2020,31,9: | 0 |
| 5 | Personalized query suggestion diversification in information retrieval显示文摘Query suggestions help users refine their queries after they input an initial query.Previous work on query suggestion has mainly concentrated on approaches that are similarity-based or context-based,developing models that either focus on adapting to a specific user(personalization)or on diversifying query aspects in order to maximize the probability of the user being satisfied(diversification).We consider the task of generating query suggestions that are both personalized and diversified.We propose a personalized query suggestion diversification(PQSD)model,where a user's long-term search behavior is injected into a basic greedy query suggestion diversification model that considers a user's search context in their current session.Query aspects are identified through clicked documents based on the open directory project(ODP)with a latent dirichlet allocation(LDA)topic model.We quantify the improvement of our proposed PQSD model against a state-of-the-art baseline using the public america online(AOL)query log and show that it beats the baseline in terms of metrics used in query suggestion ranking and diversification.The experimental results show that PQSD achieves its best performance when only queries with clicked documents are taken as search context rather than all queries,especially when more query suggestions are returned in the list. | Wanyu CHEN Fei CAI Honghui CHEN Maarten DE RIJKE | 2020 | Frontiers of Computer Science2020,14,3: | 0 |
| 6 | Carbon Doping Triggered Efficient Electrochemical Hydrogen Evolution of Cross-Linked Porous Ru-MoO_(2) Via Solid-Phase Reaction Strategy显示文摘The defect-free structure of Mo-based materials is a“double-edged sword”,which endows the material with excellent stability,but limits its chemical versatility and application in electrochemical hydrogen evolution reaction(HER).Carbon doping engineering is an attractive strategy to effectively improve the performance of Mo-based catalyst and maintain their stability.Herein,we report a cross-linked porous carbon-doped MoO_(2)(C–MoO_(2))-based catalyst Ru/C–MoO_(2) for electrochemical HER,which is prepared by the convenient redox solid-phase reaction(SPR)of porous RuO_(2)/Mo_(2)C composite precursor.Theoretical studies reveal that due to the presence of carbon atoms,the electronic structure of C–MoO_(2) has been properly adjusted,and the loaded small Ru nanoparticles provide a fast water dissociation rate and moderate H adsorption strength.In electrochemical studies under a pH-universal environment,Ru/C–MoO_(2) electrocatalyst exhibits a low overpotential at a current density of 10 mA cm^(-2) and has a low Tafel slope.Meanwhile,Ru/C-MoO_(2) has excellent stability for more than 100 h at an initial current density of 100 mA cm^(-2). | Jialin Cai Jianye Yang Xin Xie Jie Ding Leyan Liu Wanyu Tian Yushan Liu Zhiyong Tang Baozhong Liu Siyu Lu | 2023 | Energy & Environmental Materials2023,6,1: | 0 |
| 7 | CPAL, as a New Mediator of Cardiomyocyte Metabolic Alterations and Pyroptosis, Regulates Myocardial Infarction Injury in Mice显示文摘Myocardial infarction (MI), the most serious of the ischemic heart diseases, is accompanied by myocardial metabolic disorders and the loss of cardiomyocytes. Increasing evidence has shown that long noncoding RNAs (lncRNAs) are involved in various pathological conditions such as cancer and cardiovascular diseases (CVDs), and are emerging as a novel biomarker for these disorders. This study aims to investigate the regulatory role and mechanisms of lncRNAs in myocardial remodeling in the setting of MI. We find that post-infarcted hearts exhibit a reduction of adenosine triphosphate (ATP) and an alteration of the glucose and lipid metabolism genes cluster of differentiation 36 (CD36), hexokinase 1 (HK1), and clucose transporter 4 (GLUT4), accompanied by cardiomyocyte pyroptosis. We then identify a previously unknown conserved lncRNA, AK009126 (cardiomyocyte pyroptosis-associated lncRNA, CPAL), which is remarkably upregulated in the myocardial border zone of MI mice. Importantly, the adeno-associated virus 9 (AAV9)-mediated silencing of endogenous CPAL by its short hairpin RNA (shRNA) partially abrogates myocardial metabolic alterations and cardiomyocyte pyroptosis during MI in mice. Mechanistically, CPAL is shown to bind directly to nuclear factor kappa B (NFκB) and to act as an activator of NFκB to induce NFκB phosphorylation in cardiomyocytes. We also find that CPAL upregulates caspase-1 expression at the transcriptional level and consequently promotes the release of interleukin (IL)-18 and IL-1β from cardiomyocytes. Collectively, our findings reveal the conserved lncRNA CPAL as a new regulator of cardiac metabolic abnormalities and cardiomyocyte pyroptosis in the setting of MI and suggest CPAL as a new therapeutic target to protect cardiomyocytes against ischemic injury in infarcted hearts. | Jiamin Li Hongru Xue Ning Xu Liling Gong Ming Li Sijia Li Di Huang Qingwei Zhang Pengyu Li Qingsui Li Hang Yu Yining Liu Yadong Xue Haixin Chen Jiali Liu Wanyu Zhang Mingbin Liu Siyu Chang Xianzhi Lang Xingmiao Zhao Weijie Du Benzhi Cai Ning Wang Baofeng Yang | 2023 | Engineering2023,,1: | 0 |
| 8 | Accelerated ion/electron transport kinetics and increased active sites via local internal electric fields in heterostructured VO_(2)–carbon cloth for enhanced zinc-ion storage显示文摘Although the performance of the self-standing electrode has been enhanced for aqueous zinc-ion batteries(AZIBs),it is necessary to explore and analyse the deep modification mechanism(especially interface effects).Herein,density functional theory(DFT)calculations are applied to investigate the high-performance cathode based on the VO_(2)/carbon cloth composites with heterostructures interface(H-VO_(2)@CC).The adsorption energy comparisons and electron structure analyses verify that HVO_(2)@CC has extra activated sites at the interface,enhanced electrical conductivity,and structural stability for achieving highperformance AZIBs due to the presence of built-in electric field at the interfaces.Accordingly,the designed self-standing HVO_(2)@CC cathode delivers higher rate capacity,longer-life cyclability,and faster electronic/ion transmission kinetics benefiting from the synergistic effects.The risks of active material shedding and dissolution during the dis/charge process of two cathodes were evaluated via ex-situ ultraviolet–visible(UV–vis)spectrum and inductively coupled plasma-atomic emission spectroscopy(ICP-AES)technique.Finally,this investigation also explores the charge storage mechanism of H-VO_(2)@CC through various exsitu and in-situ characterization techniques.This finding can shed light on the significant potential of heterostructures interface engineering in practical applications and provide a valuable direction for the development of cathode materials for AZIBs and other metal-ion batteries. | Ping Luo Wenwei Zhang Wanyue Cai Zhen Huang Gangyuan Liu Chang Liu Shiyu Wang Feng Chen Lixue Xia Yan Zhao Shijie Dong Lu Xia | 2023 | Nano Research2023,16,1: | 0 |