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| 1 | Facile metagrating holograms with broadband and extreme angle tolerance显示文摘The emerging meta-holograms rely on arrays of intractable meta-atoms with various geometries and sizes for customized phase profiles that can precisely modulate the phase of a wavefront at an optimal incident angle for given wavelengths.The stringent and band-limited angle tolerance remains a fundamental obstacle for their practical application,in addition to high fabrication precision demands.Utilizing a different design principle,we determined that facile metagrating holograms based on extraordinary optical diffraction can allow the molding of arbitrary wavefronts with extreme angle tolerances(near-grazing incidence)in the visible–near-infrared regime.By modulating the displacements between uniformly sized meta-atoms rather than the geometrical parameters,the metagratings produce a robust detour phase profile that is irrespective of the wavelength or incident angle.The demonstration of high-fidelity meta-holograms and in-site polarization multiplexing significantly simplifies the metasurface design and lowers the fabrication demand,thereby opening new routes for flat optics with high performances and improved practicality. | Zi-Lan Deng Junhong Deng Xin Zhuang Shuai Wang Tan Shi Guo Ping Wang Yao Wang Jian Xu Yaoyu Cao Xiaolei Wang Xing Cheng Guixin Li Xiangping Li | 2018 | Light(Science & Applications)2018，7，1： | 17 |
| 2 | Arbitrary polarization conversion dichroism metasurfaces for all-in-one full Poincare sphere polarizers显示文摘The control of polarization,an essential property of light,is of broad scientific and technological interest.Polarizers are indispensable optical elements for direct polarization generation.However,arbitrary polarization generation,except that of common linear and circular polarization,relies heavily on bulky optical components such as cascading linear polarizers and waveplates.Here,we present an effective strategy for designing all-in-one full Poincare sphere polarizers based on perfect arbitrary polarization conversion dichroism and implement it in a monolayer all-dielectric metasurface.This strategy allows preferential transmission and conversion of one polarization state located at an arbitrary position on the Poincare sphere to its handedness-flipped state while completely blocking its orthogonal state.In contrast to previous methods that were limited to only linear or circular polarization,our method manifests perfect dichroism of nearly 100%in theory and greater than 90%experimentally for arbitrary polarization states.By leveraging this attractive dichroism,our demonstration of the generation of polarization beams located at an arbitrary position on a Poincare sphere directly from unpolarized light can substantially extend the scope of meta-optics and dramatically promote state-of-the-art nanophotonic devices. | Shuai Wang Zi-Lan Deng Yujie Wang Qingbin Zhou Xiaolei Wang Yaoyu Cao Bai-Ou Guan Shumin Xiao Xiangping Li | 2021 | Light(Science & Applications)2021，10，2： | 6 |
| 3 | CO_2 absorption with ionic liquids at elevated temperatures显示文摘CO_2 capture with ionic liquids(ILs) has attracted many attentions, and most works focused on absorption ability at ambient temperatures, while seldom research was concerned at elevated temperatures.This not only limits the CO_2 absorption application at elevated temperature, but also the determination of the operation condition of the CO_2 desorption generally occurring at higher temperature. This work mainly reported CO_2 solubilities in ILs at elevated temperatures and related properties were also provided. 1-alkyl-3-methylimidazolium bis(trifluoromethylsulfonyl)imide([CnMIm][Tf_2N]) ILs were selected as physical absorbents for CO_2 capture in this work due to their relative higher CO_2 absorption capacities and good thermal stabilities. The long-term stability tests showed that [CnMIm][Tf_2N] is thermally stable at 393.15 K for long time. CO_2 solubilities in [CnMIm][Tf_2N] were systematically determined at temperatures from 353.15 K to 393.15 K. It demonstrated that CO_2 solubility obviously increases with the increase of pressure while slightly decreases with increase of temperature. As the length of alkyl chain on the cation increases, CO_2 solubility in ILs increases. Additionally, the thermodynamic properties including the Gibbs free energy, enthalpy, and entropy of CO_2 were also calculated. | Lu Bai Dawei Shang Mengdie Li Zhongde Dai Liyuan Deng Xiangping Zhang | 2017 | Journal of Energy Chemistry2017，26，5： | 5 |
| 4 | Multifunctional metasurface:from extraordinary optical transmission to extraordinary optical diffraction in a single structure显示文摘We show that a metasurface composed of a subwavelength metallic slit array embedded in an asymmetric dielectric environment can exhibit either extraordinary optical transmission(EOT) or extraordinary optical diffraction(EOD). The cascaded refractive indices of the dielectrics can leverage multiple decaying passages into variant subsections with different diffraction order combinations according to the diffraction order chart in the k-vector space, providing a flexible mean to tailor resonance decaying pathways of the metallic slit cavity mode by changing the wavevector of the incident light. As a result, either the zeroth transmission or-1 st reflection efficiencies can be enhanced to near unity by the excitation of the localized slit cavity mode, leading to either EOT or EOD in a single structure, depending on the illumination angle. Based on this appealing feature, a multifunctional metasurface that can switch its functionality between transmission filter, mirror, and off-axis lens is demonstrated. Our findings provide a convenient way to construct multifunctional miniaturized optical components on a single planar device. | ZILAN DENG YAOYU CAO XIANGPING LI GUOPING WANG | 2018 | Photonics Research2018，6，5： | 5 |
| 5 | Multifunctional metasurface: from extraordinary optical transmission to extraordinary optical diffraction in a single structure: publisher's note显示文摘This publisher's note reports the revision of authors' name spelling in Photon. Res. 6, 443 (2018). | ZI-LAN DENG YAOYU CAO XIANGPING LI GUO PING WANG | 2018 | Photonics Research2018，6，7： | 2 |
| 6 | Pebax/TSIL blend thin film composite membranes for CO_2 separation显示文摘In this study a thin film composite(TFC) membrane with a Pebax/Task-specific ionic liquid(TSIL) blend selective layer was prepared. Defect-free Pebax/TSIL layers were coated successfully on a polysulfone ultrafiltration porous support with a polydimethylsiloxane(PDMS) gutter layer. Different parameters in the membrane preparation(e.g. concentration, coating time) were investigated and optimized. The morphology of the membranes was studied by scanning electron microscopy(SEM), while the thermal properties and chemical structures of the membrane materials were investigated by thermo-gravimetric analyzer(TGA), differential scanning calorimetry(DSC) and Fourier transform infrared spectroscopy(FTIR). The CO_2 separation performance of the membrane was evaluated using a mixed gas permeation test. Experimental results show that the incorporation of TSIL into the Pebax matrix can significantly increase both CO_2 permeance and CO_2/N_2 selectivity. With the presence of water vapor, the membrane exhibits the best CO_2/N_2 selectivity at a relative humidity of around 75%, where a CO_2 permeance of around 500 GPU and a CO_2/N_2 selectivity of 46 were documented. A further increase in the relative humidity resulted in higher CO_2 permeance but decreased CO_2/N_2 selectivity. Experiments also show that CO_2 permeance decreases with a CO_2 partial pressure increase, which is considered a characteristic in facilitated transport membranes. | Zhongde Dai Lu Bai Karoline Navik Hval Xiangping Zhang Suojiang Zhang Liyuan Deng | 2016 | Science China Chemistry2016，59，5： | 1 |
| 7 | Discovery of novel covalent selective estrogen receptor degraders against endocrine-resistant breast cancer显示文摘Endocrine-resistance remains a major challenge in estrogen receptorαpositive(ERα^(+))breast cancer(BC)treatment and constitutively active somatic mutations in ERαare a common mechanism.There is an urgent need to develop novel drugs with new mode of mechanism to fight endocrineresistance.Given aberrant ERαactivity,we herein report the identification of novel covalent selective estrogen receptor degraders(cSERDs)possessing the advantages of both covalent and degradation strategies.A highly potent cSERD 29c was identified with superior anti-proliferative activity than fulvestrant against a panel of ERa+breast cancer cell lines including mutant ERα.Crystal structure of ERα-29c complex alongside intact mass spectrometry revealed that 29c disrupted ERa protein homeostasis through covalent targeting C530 and strong hydrophobic interaction collied on H11,thus enforcing a unique antagonist conformation and driving the ERαdegradation.These significant effects of the cSERD on ERαhomeostasis,unlike typical ERαdegraders that occur directly via long side chains perturbing the morphology of H12,demonstrating a distinct mechanism of action(MoA).In vivo,29c showed potent antitumor activity in MCF-7 tumor xenograft models and low toxicity.This proof-of-principle study verifies that novel cSERDs offering new opportunities for the development of innovative therapies for endocrine-resistant BC. | Yubo Wang Jian Min Xiangping Deng Tian Feng Hebing Hu Xinyi Guo Yan Cheng Baohua Xie Yu Yang Chun-Chi Chen Rey-Ting Guo Chune Dong Hai-Bing Zhou | 2023 | Acta Pharmaceutica Sinica B2023，13，12： | 0 |
| 8 | Simulation and assessment of manufacturing ethylene carbonate from ethylene oxide in multiple process routes显示文摘Ethylene oxide(EO)is an important raw material for producing ethylene carbonate(EC).However,the traditional method for the separation of EO from mixture gas by water in the refining process is high energy consumption.In this paper,two processes of manufacturing EC from EO mixture gas were studied by process simulation.Two processes for producing EC from EO mixture as raw materials without EO purification,called the OSAC process and the Modified OSAC process,were developed and assessed systematically.Both processes use EC as the absorbent to capture EO,avoiding the separation process of EO from solution.For comparisons,the EC producing process containing EO absorption by water,EO refinement and carbonylation process were also modeled,which was called the ERC process.Three schemes were designed for the EO absorber using EC as absorbent.Compared with the initial absorber scheme,the optimal liquid–vapor ratio is reduced from 1.66 to 1.45(mass).Moreover,the mass distribution analysis for the three processes were carried out in the form of the material chain.It was found that,compared with the ERC process,the energy consumption of the OSAC and the Modified OSAC process is reduced by 56.89%and 30.03%,respectively.This work will provide helpful information for the industrialization of the OSAC process. | Xincheng Gu Xiaochun Zhang Xiangping Zhang Chun Deng | 2021 | Chinese Journal of Chemical Engineering2021，34，3： | 0 |
| 9 | Plant above-ground biomass and litter quality drive soil microbial metabolic limitations during vegetation restoration of subtropical forests显示文摘Changes in litter quality(carbon:nitrogen,C:N)and above-ground biomass(AGB)following vegetation restoration significantly impact soil physicochemical properties,yet their effects on soil microbial metabolic limitations remain unclear.We measured litter quality,AGB,soil physicochemical properties,and extracellular enzyme activity(EEA)along a vegetation restoration gradient(7,14,49,70 years,and nearly climax evergreen broadleaved forests)in southern China.We also evaluated soil microbial metabolic limitations by a vector analysis of the EEA.Results revealed the soil microbial metabolisms were co-limited by C and phosphorus(P).The microbial C limitation initially decreased(before 14 years)and then increased,while the microbial P limitation initially increased(before 49 years)and then decreased.Partial least squares path modeling(PLS-PM)showed that the microbial C limitation was mainly attributed to microbial C use efficiency induced by litter quality,suggesting that microorganisms may transfer cellular energy between microbial growth and Cacquiring enzyme production.The microbial P limitation was primarily correlated with AGB-driven change in soil elements and their stoichiometry,highlighting the importance of nutrient stoichiometry and balance in microbial metabolism.The shifts between microbial C and P limitations and the strong connections of plant–soil-microbe processes during vegetation restoration revealed here will provide us with helpful information for optimal management to achieve forest restoration success. | Shuo Zhang Ying-Ping Wang Xi Fang Jinlei Chen Nannan Cao Pingping Xu Mengxiao Yu Xin Xiong Xiangping Tan Qi Deng Junhua Yan | 2023 | Soil Ecology Letters2023，5，2： | 0 |
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