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| 1 | Hydrothermal reduction of graphene oxide by glucose for the preparation of graphene/polyester staple sponge and its applications in oil spill cleanup显示文摘Graphene/polyester staple sponge(GPSS)is a high-performance adsorbent for the cleanup of crude oil spill,but the use of hydrazine hydrate as the reducing agent for the preparation of GPSS is not friendly to the environment.Herein,we reported that graphene oxide/polyester staple composite could be hydrothermally reduced by bioresource glucose to prepare GPSS of similar performance.GPSS could be applied in the absorption of oils and organic solvents thanks to its large pore volume and hydrophobicity.The absorption capacity of the novel glucose-reduced GPSS was competitive to those of the most effective absorbents for oil spill cleanup.The used GPSS could be easily regenerated by soaking in ethanol to remove the absorbed oil.The green synthesis,high oil absorption performance and easy recycling of the glucose-reduced GPSS make it a good candidate for cleaning oil spills. | Ruihan Wu Yitong Bai Zhu Ming Linyun Chen Hua Yang Sheng-Tao Yang Jianbin Luo | 2017 | Journal of Bioresources and Bioproducts2017,2,2: | 0 |
| 2 | Two-dimensional molybdenum carbide(MXene)as an efficient nanoadditive for achieving superlubricity under ultrahigh pressure显示文摘In this study,a robust macroscale liquid superlubricity with a coefficient of friction of 0.004 was achieved by introducing molybdenum carbide(Mo_(2)CT_(x))MXene nanoparticles as lubricating additives in a lithium hexafluorophosphate-based ionic liquid at Si_(3)N_(4)-sapphire interfaces.The maximal contact pressure in the superlubricity state could reach 1.42 GPa,which far exceeds the limit of the superlubricity regime in previous studies.The results indicate that a composite tribofilm(mainly containing molybdenum oxide and phosphorus oxide)that formed at the interface by a tribochemical reaction contributed to the excellent antiwear performance.Furthermore,the extremely low shear strength of the tribofilm and the interlayers of Mo_(2)CT_(x)MXene contributed to the superlubricity.This work demonstrates the promising potential of Mo_(2)CT_(x)MXene in improving superlubricity properties,which could accelerate the application of superlubricity in mechanical systems. | Shuang YI Yitong GUO Jinjin LI Yuxin ZHANG Aiguo ZHOU Jianbin LUO | 2023 | Friction2023,11,3: | 0 |
| 3 | Short-term variations and influencing factors of suspended sediment concentrations at the Heisha Beach,Guangdong,China显示文摘Knowledge of sediment variation processes is essential to understand the evolution mechanism of beach morphology changes.Thus,a field measurement was conducted at the Heisha Beach,located on the west coast of the Zhujiang River(Pearl River)Estuary,to investigate the short-term variation in suspended sediment concentrations(SSCs)and the relationship between the SSC and turbulent kinetic energy,bottom shear stress(BSS),and relative wave height.Based on extreme event analysis results,extreme events have a greater influence on turbulent kinetic energy than SSC.Although a portion of the turbulent kinetic energy dissipates directly into the water column,it plays an important role in suspended sediment motion.Most of the time,the wave-current interaction is strong enough to drive sediment incipience and resuspension.When combined,the wave-current interaction and wave-induced BSSs have a greater influence on suspended sediment transport and SSC variation than current-induced BSS alone.The relative wave height also has a strong correlation with SSC,indicating that the combined effect of water depth and wave height significantly impacts SSC variation.Water depth is mainly controlled by the tide on the beaches;thus,the effects of tides and waves should be conjunctively considered when analyzing the factors influencing SSC. | Jintang Ou Haoyan Dong Liangwen Jia Xiangxin Luo Zixiao He Kanglin Chen Jing Liu Yitong Lin Mingdong Yu Mingen Liang | 2022 | Acta Oceanologica Sinica2022,41,5: | 0 |
| 4 | Single-Atom Ce-N_(4)-C-(OH)_(2)Nanozyme-Catalyzed Cascade Reaction to Alleviate Hyperglycemia显示文摘The enzyme-mimicking catalytic activity of single-atom nanozymes has been widely used in tumor treatment.However,research on alleviating metabolic diseases,such as hyperglycemia,has not been reported.Herein,we found that the single-atom Ce-N_(4)-C-(OH)_(2)(SACe-N_(4)-C-(OH)_(2))nanozyme promoted glucose absorption in lysosomes,resulting in increased reactive oxygen species production in HepG2 cells.Furthermore,the SACe-N_(4)-C-(OH)_(2)nanozyme initiated a cascade reaction involving superoxide dismutase-,oxidase-,catalase-,and peroxidase-like activity to overcome the limitations associated with the substrate and produce•OH,thus improving glucose intolerance and insulin resistance by increasing the phosphorylation of protein kinase B and glycogen synthase kinase 3β,and the expression of glycogen synthase,promoting glycogen synthesis to improve glucose intolerance and insulin resistance in high-fat diet-induced hyperglycemic mice.Altogether,these results demonstrated that the novel nanozyme SACeN_(4)-C-(OH)_(2)alleviated the effects of hyperglycemia without evident toxicity,demonstrating its excellent clinical application potential. | Guangchun Song Jia Xu Hong Zhong Qi Zhang Xin Wang Yitong Lin Scott PBeckman Yunbo Luo Xiaoyun He Jin-Cheng Li Kunlun Huang Nan Cheng | 2023 | Research2023,,4: | 0 |
| 5 | Fabrication of Durable Superhydrophobic Stainless Steel Mesh with Nano/Micro Flower-Like Morphologies for Self-Cleaning and Efficient Oil/Water Separation显示文摘How to fabricate durable superhydrophobic materials for cyclic oil/water separation to solve oil-induced pollutions is still a problem.Herein,we fabricated a durable Superhydrophobic Stainless Steel Mesh(SH-SSM)with nano/micro flower-like sheets by self-assembly of zinc stearate for the cyclic separation of various oil/water mixtures.The SH-SSM exhibits durable superhydrophobicity against static or dynamic treatments.In virtue of durable superhydrophobicity of the SH-SSM,the dusts on surface of SH-SSM can be removed completely by running water immediately showing excellent self-cleaning performance.Moreover,the SH-SSM can be used to perform gravity-driven separation of heavy oil/water and light oil/water mixtures by utilizing its superhydrophobicity that oil phase penetrates the mesh and water phase is restricted.Separation efficiencies of the SH-SSM can reach 99.99%.After 20 cycles of separation,the separation efficiencies for are>97.00%and>98.25%for heavy oil/water and light oil/water mixtures,respectively.Flux values of dichloromethane,hexane and petroleum ether are 2.5×10^(5) L m^(−2) h^(−1),1.7×10^(5) L m^(−2) h^(−1),and 1.8×10^(5) L m^(−2) h^(−1),respectively.This study proposes a facial approach to prepare durable superhydrophobic and self-cleaning material for cyclic and fast separation of oil/water. | Changlian Xu Yitong Luo Lu Zhou Yiwen Bi Hao Sun | 2022 | Journal of Bionic Engineering2022,19,6: | 0 |