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| 1 | Changes of soil microbial communities during decomposition of straw residues under different land uses显示文摘Monitoring soil microbial communities can lead to better understanding of the transformation processes of organic carbon in soil. The present study investigated the changes of soil microbial communities during straw decomposition in three fields, i.e., cropland, peach orchard and vineyard. Straw decomposition was monitored for 360 d using a mesh-bag method. Soil microbial metabolic activity and functional diversity were measured using the Biolog-Eco system. In all three fields, dried straws with a smaller size decomposed faster than their fresh counterparts that had a larger size. Dried corn straw decomposed slower than dried soybean straw in the early and middle stages, while the reverse trend was found in the late stage. The cropland showed the highest increase in microbial metabolic activity during the straw decomposition, whereas the peach orchard showed the lowest. There was no significant change in the species dominance or evenness of soil microbial communities during the straw decomposition. However, the species richness fluctuated significantly, with the peach orchard showing the highest richness and the cropland the lowest. With different carbon sources, the peach orchard utilised carbon the most, followed by the cropland and the vineyard. In all three fields, carbon was utilized in following decreasing order: saccharides>amino acids>polymers>polyamines>carboxylic acids>aromatic compounds. In terms of carbon-source utilization, soil microbial communities in the peach orchard were less stable than those in the cropland. The metabolic activity and species dominance of soil microbial communities were negatively correlated with the straw residual percentage. Refractory components were primarily accumulated in the late stages, thus slowing down the straw decomposition. The results showed that dried and crushed corn straw was better for application in long-term fields. The diversity of soil microbial communities was more stable in cropland than in orchards during the straw decomposition. | ZHANG Hong XU Wenxin LI Yubao LYU Jialong CAO Yingfei HE Wenxiang | 2017 | Journal of Arid Land2017，9，5： | 9 |
| 2 | A discriminative training algo- rithm for VQ-based speaker identification 显示文摘 | HE JIALONG LI LIU PALM G | 1999 | IEEE Transactions on Audio Speech and Language Processing1999，7，3： | 1 |
| 3 | Geochemistry and environmental effect of cadmium in the super-large Jinding Pb-Zn deposit,Yunnan Province, China显示文摘The Jinding Pb-Zn deposit in Yunnan Province is the representative of a Cd-enriched area and mining activities lead to the release of Cd into the hypergenic ecosystem, resulting in Cd pollution. The concentrations of Cd vary greatly from one type to another type of rocks in the mining district. In the host rock, Cd concentrations range from 50×10-6 to 650×10-6 with an average of 310×10-6. In primary ores, Cd concentrations range from 14×10-6 to 2800×10-6 with an average of 767×10-6. However, in oxidized ores, Cd concentrations are highest, varying within the range of 110×10-6 to 8200×10-6 , averaging 1661×10-6. It is shown that the oxidized ores are the main carrier and environmental source of Cd. Leaching test showed that Pb/Zn ores are easy to oxidize and thereafter release Cd and other harmful elements. These leached elements in the leachate may be precipitated rapidly in the order of Zn>Pb>Cd. As for the concentration distribution of Cd in the Bijiang River, it is estimated to be 15.7 μg/L Cd in water, 49.3 mg/L in suspended substances, and 203.7 mg/L in sediments. The average value of Cd in soil from the polluted area is 83.0 mg/kg. Natural weathering of Cd-rich rocks and minerals imposes a potential environmental risk on the aquatic ecosystem of the Bijiang catchment. | LI Hang LI Dahua XIAO Tangfu HE Libin NING Zengping SUN Jialong ZHU Changsheng SHUANG Yan | 2008 | Chinese Journal Of Geochemistry2008，27，1： | 1 |
| 4 | Autocatalytic reduction-assisted synthesis of segmented porous PtTe nanochains for enhancing methanol oxidation reaction显示文摘Morphology engineering has been developed as one of the most widely used strategies for improving the performance of electrocatalysts.However,the harsh reaction conditions and cumbersome reaction steps during the nanomaterials synthesis still limit their industrial applications.Herein,one-dimensional(1D)novel-segmented PtTe porous nanochains(PNCs)were successfully synthesized by the template methods assisted by Pt autocatalytic reduction.The PtTe PNCs consist of consecutive mesoporous architectures that provide a large electrochemical surface area(ECSA)and abundant active sites to enhance methanol oxidation reaction(MOR).Furthermore,1D nanostructure as a robust sustaining frame can maintain a high mass/charge transfer rate in a long-term durability test.After 2,000 cyclic voltammetry(CV)cycles,the ECSA value of PtTe PNCs remained as high as 44.47 m^(2)·gPt^(-1),which was much larger than that of commercial Pt/C(3.95 m^(2)·gPt^(-1)).The high catalytic activity and durability of PtTe PNCs are also supported by CO stripping test and density functional theory calculation.This autocatalytic reduction-assisted synthesis provides new insights for designing efficient low-dimensional nanocatalysts. | Qiqi Zhang Tianyu Xia He Huang Jialong Liu Mengyuan Zhu Hao Yu Weifeng Xu Yuping Huo Congli He Shipeng Shen Cong Lu Rongming Wang Shouguo Wang | 2023 | Nano Research Energy2023，2，1： | 1 |
| 5 | Small molecule interfacial cross-linker for highly efficient two-dimensional perovskite solar cells显示文摘The nonradiative recombination of charge carriers at the hole transport layer(HTL)/perovskite interface generally induces remarkable performance loss of the inverted two-dimensional perovskite solar cells(2D PSCs). Herein, a cross-linkable small molecule of 2-mercaptoimidazole(2-MI) was introduced into the nickel oxide(NiO_(x))/2D perovskite interface. Experiments have confirmed the formation of Ni-N covalent bond by N atom in the 2-MI and Ni in the NiO_(x) and the coordinating between S atom of 2-MI and under-coordinated Pb^(2+) near to the NiO_(x)/perovskite interface, which contributes to creating a crosslinking between NiO_(x)/perovskite interface to restrain charge carrier recombination and enhance the extraction of hole carriers at the interface. Besides, the 2-MI modification layer is also beneficial for promoting the crystallinity of 2D perovskite. Consequently, the inverted 2D PSCs with 2-MI modification achieved the best power conversion efficiency of 15%. This paves a route to acquire highly efficient 2D PSCs by constructing a cross-linking at the NiO_(x)HTL/2D perovskite interface. | Hongming Hou Taotao Hu Fu Zhang Rui Liu Jialong He Chang Liu Yue Yu Dong Chen Qiaofeng Wu Meng Zhang Hua Yu | 2022 | Journal of Energy Chemistry2022，31，5： | 0 |
| 6 | EFFECTS OF TENSILE STRESS AND IMPURITIES ON CREEP ACTIVATION ENERGY OF PLATINUM显示文摘The effect of tensile stress and trace amounts of impurities on the creep activation energyof platinum was studied and the creep mechanism was disscussed. | Mu,Jialong He,Huachun Institute of Precious Metal,Kunming 650221,China | 1993 | 中国有色金属学会会刊:英文版1993，3，4： | 0 |
| 7 | Effects of Long-term K Fertilizer Application on the Crop Yield and K Distribution of Soil Aggregates in a Paddy-Upland Rotation System显示文摘[Objective]A long-term paddy-upland experiment was conducted to evaluate the effects of the recommended amount of potassium( K)fertilizer on crop yield,distribution of soil aggregate,and soil available K content. It was mainly to ascertain the distribution of K in the soil aggregate components in the paddy-upland rotation system,and then to provide theoretical basis for soil structure improvement,K pool management,and reasonable application of K fertilizer. [Method]There were 2 treatments selected,namely,NP(-K) treatment and NPK( + K) treatment in this study. Then the effects of K fertilizer application on the yield,available K content,and aggregate distribution in the middle rice-winter rape rotation system were analyzed. [Result]The results showed that the output of the crop rotation was affected by the year and fertilization. Compared with NP(-K),the average yield increases of rice and winter rape after application of K fertilizer were 0.51 and 0.33 t/hm2,with the increments of 7.5%and 14. 1% respectively. The long-term application of K fertilizer( 7 a) had no significant effects on the distribution of soil aggregates but could significantly increase the water-soluble K content and available K content at depths of 20-30 and 30-40 cm,and available K content of aggregates in each particle size. In addition,the balance of available K at the 10-20 and 30-40 cm of soil layers was the most significant through calculation of surplus-deficit value of available K in agglomerates of different soil layers. [Conclusion]Compared with the initial available K content in the farmland in 2011,the current K fertilizer application could lead to that farmland K content continues to decline. Therefore,we should pay attention to straw returned and supplement of organic K fertilizer,to maintain crop rotation system's productivity and soil K balance. | Song Meifang Hu Yitao Huang Shuai He Junfeng Chen Fowen Zou Jialong Li Jifu | 2019 | Meteorological and Environmental Research2019，10，1： | 0 |
| 8 | Realizing efficient emission and triple-mode photoluminescence switching in air-stable tin(IV)-based metal halides via antimony doping and rational structural modulation显示文摘Recently,many lead-free metal halides with diverse structures and highly efficient emission have been reported.However,their poor stability and single-mode emission color severely limit their applications.Herein,three homologous Sb^(3+)-doped zero-dimensional(0D)air-stable Sn(IV)-based metal halides with different crystal structures were developed by inserting a single organic ligand into SnCl_(4)lattice,which brings different optical properties.Under photoexcitation,(C_(25)H_(22)P)SnC_(l5)@Sb⋅CH_(4O)(Sb^(3+)−1)does not emit light,(C_(25)H_(22)P)_(2)SnC_(l6)@Sb-α(Sb^(3+)−2α)shines bright yellow emission with a photoluminescence quantum yield(PLQY)of 92%,and(C_(25)H_(22)P)_(2)SnC_(l6)@Sb-β(Sb^(3+)−2β)exhibits intense red emission with a PLQY of 78%.The above three compounds show quite different optical properties should be due to their different crystal structures and the lattice distortions.Particularly,Sb^(3+)−1 can be successfully converted into Sb^(3+)−2αunder the treatment of C_(25)H_(22)PCl solution,accompanied by a transition from nonemission to efficient yellow emission,serving as a“turn-on”photoluminescence(PL)switching.Parallelly,a reversible structure conversion between Sb^(3+)−2αand Sb^(3+)−2βwas witnessed after dichloromethane or volatilization treatment,accompanied by yellow and red emission switching.Thereby,a triple-mode tunable PL switching of off-onI-onII can be constructed in Sb^(3+)-doped Sn(IV)-based compounds.Finally,we demonstrated the as-synthesized compounds in fluorescent anticounterfeiting,information encryption,and optical logic gates. | Xuefei He Hui Peng Qilin Wei Zhijie Zhou Guolun Zhang Zhentao Du Jialong Zhao Bingsuo Zou | 2024 | Aggregate2024，5，1： | 0 |
| 9 | Bioavailability of Tl in soils, uptake by crops and its environmental impact显示文摘 | Libin HE Tangfu XIAO Hang LI Jingquan PENG Zengping NING Jialong SUN Fei YANG | 2006 | Chinese Journal Of Geochemistry2006，25，B08： | 0 |
| 10 | Greenhouse area detection in Guanzhong Plain,Shaanxi,China:spatio-temporal change and suitability classification显示文摘The extensive use of greenhouses has brought soared economic benefits for farming practitioners in China and an overview of the spatio-temporal distribution of greenhouses is of great interest to agricultural practitioners and decision-makers.In this study,Landsat image based greenhouse maps in Guanzhong Plain,Shaanxi,China were made using random forest classification algorithm through visual interpretation on the Google Earth Engine.The 7-year's changes in greenhouse areas were investigated(i.e.2000,2003,2006,2010,2013,2015 and 2019)with yearly overall accuracy more than 90%.The results showed that the total area of greenhouses in Guanzhong Plain demonstrated an increasing trend,from 5.92 km2 in 2000 to 194.42 km2 in 2019 with a considerable growth between 2010 and 2015.The dominant drivers for the increase are largely attributed to the government policy as well as economic profitability.The distribution of greenhouse shifts to central and eastern regions of Guanzhong Plain.Greenhouses preferentially expand to the area near to rural roads,main rivers,and high elevation,with more than 45%greenhouses distributed within 1 km of the county rural road.The principal component analysis based suitability evaluation showed that a total of 38.44%of the area was suitable for greenhouse. | Caihong Gao Qifan Wu Miles Dyck Jialong Lv Hailong He | 2022 | International Journal of Digital Earth2022，15，1： | 0 |
| 11 | Unraveling the Effect of Cation Types on Electrochromic Properties of Titanium Dioxide Nanocrystals显示文摘Electrochromic(EC)devices have been regarded as promising candidates for energy-saving smart windows,next-generation displays,and wearable electronics.Monovalent ions such as H^(+)-and Li^(+)-based electrolytes are the benchmark insertion ions for EC devices but have serious limitations such as high cost,instability,and difficulty to handle.Seeking multivalent electrolytes is an effective alternative way to prepare high-performance EC devices;unfortunately,the related reports are currently limited to tungsten oxide EC materials.Herein,for the first time,we investigate the EC properties driven by different valence cationic(i.e.,Li^(+),Zn^(2+),and Al^(3+))electrolytes in the titanium dioxide system.It is found that the initial optical modulation ranges of TiO_(2)nanocrystal(NC)films in Li^(+),Zn^(2+),and Al^(3+)electrolytes are 76.8%,77.4%,and 77.3%,respectively.After 250 cycles,the optical contrast of these films in Zn^(2+)electrolyte decreased by only 2.3%,much lower than that in benchmark Li^(+)electrolyte of 10.1%and Al^(3+)electrolyte of 59.1%.Density functional theory calculation indicates that the potential barriers of Li^(+),Zn^(2+),and Al^(3+)in TiO_(2)are 0.59,0.55,and 0.74 eV,respectively,which makes TiO_(2)NCs show good EC properties in Zn^(2+)electrolytes.This work unravels the effect of different valence cations on the electrochromic properties of titanium dioxide NCs,which may provide some new directions for the development of excellent EC devices with long-term stability and durability. | Yi Liang Sheng Cao Yuwei Liu Lijuan He Xinxin Han Ruosheng Zeng Jialong Zhao Bingsuo Zou | 2022 | Energy Material Advances2022，，1： | 0 |
| 12 | Bifunctional polyaniline electrode tailored hybridized solar cells for energy harvesting from sun and rain显示文摘Pursuit of energy-harvesting or-storage materials to realize outstanding electricity output from nature has been regarded as a promising strategy to resolve the energy-lack issue in the future. Among them,the solar cell as a solar-to-electrical conversion device has been attracted enormous interest to improve the efficiency. However, the ability to generate electricity is highly dependent on the weather conditions,in other words, there is nearly zero power output in dark-light conditions, such as rainy, cloudy, and night, lowering the monolithic power generation capacity. Here, we present a bifunctional polyaniline film via chemical bath deposition, which can harvest energy from the rain, yielding an induced current of 2.57 μA and voltage of 65.5 μV under the stimulus of real raindrop. When incorporating the functional PANi film into the traditional dye sensitized solar cell as a counter electrode, the hybridized photovoltaic can experimentally realize the enhanced output power via harvesting energy from rainy and sunny days. The current work may show a new path for development of advanced solar cells in the future. | Jialong Duan Yanyan Duan Yuanyuan Zhao Yingli Wang Qunwei Tang Benlin He | 2018 | Journal of Energy Chemistry2018，27，3： | 0 |
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