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| 1 | Relative Contributions of Boundary-Layer Meteorological Factors to the Explosive Growth of PM2.5 during the Red-Alert Heavy Pollution Episodes in Beijing in December 2016显示文摘Based on observations of urban mass concentration of fine particulate matter smaller than 2.5 μm in diameter(PM_(2.5)), ground meteorological data, vertical measurements of winds, temperature, and relative humidity(RH), and ECMWF reanalysis data, the major changes in the vertical structures of meteorological factors in the boundary layer(BL) during the heavy aerosol pollution episodes(HPEs) that occurred in winter 2016 in the urban Beijing area were analyzed. The HPEs are divided into two stages: the transport of pollutants under prevailing southerly winds, known as the transport stage(TS), and the PM_(2.5) explosive growth and pollution accumulation period characterized by a temperature inversion with low winds and high RH in the lower BL, known as the cumulative stage(CS). During the TS, a surface high lies south of Beijing, and pollutants are transported northwards. During the CS, a stable BL forms and is characterized by weak winds, temperature inversion, and moisture accumulation. Stable atmospheric stratification featured with light/calm winds and accumulated moisture(RH > 80%) below 250 m at the beginning of the CS is closely associated with the inversion, which is strengthened by the considerable decrease in near-surface air temperature due to the interaction between aerosols and radiation after the aerosol pollution occurs. A significant increase in the PLAM(Parameter Linking Aerosol Pollution and Meteorological Elements) index is found, which is linearly related to PM mass change. During the first 10 h of the CS, the more stable BL contributes approximately 84% of the explosive growth of PM_(2.5) mass. Additional accumulated near-surface moisture caused by the ground temperature decrease, weak turbulent diffusion, low BL height, and inhibited vertical mixing of water vapor is conducive to the secondary aerosol formation through chemical reactions, including liquid phase and heterogeneous reactions, which further increases the PM_(2.5) concentration levels. The contribution of these reaction mechanisms to the explosive growth of PM_(2.5) mass during the early CS and subsequent pollution accumulation requires further investigation. | junting zhong xiaoye zhang yaqiang wang junying sun yangmei zhang jizhi wang kaiyan tan xiaojing shen haochi che lu zhang zhouxiang zhang xuefei qi huarong zhao sanxue ren yang li | 2017 | Journal of Meteorological Research2017，31，5： | 25 |
| 2 | Characteristics and recent trends of sulfur dioxide at urban,rural,and background sites in North China:Effectiveness of control measures显示文摘SO 2 measurements made in recent years at sites in Beijing and its surrounding areas are performed to study the variations and trends of surface SO 2 at different types of sites in Northern China.The overall average concentrations of SO 2 are (16.8±13.1) ppb,(14.8±9.4) ppb,and (7.5±4.0) ppb at China Meteorological Administration (CMA,Beijing urban area),Gucheng (GCH,relatively polluted rural area,110 km to the southwest of Beijing urban area),and Shangdianzi (SDZ,clean background area,100 km to the northeast of Beijing urban area),respectively.The SO 2 levels in winter (heating season) are 4-6 folds higher than those in summer.There are highly significant correlations among the daily means of SO 2 at different sites,indicating regional characteristics of SO 2 pollution.Diurnal patterns of surface SO 2 at all sites have a common feature with a daytime peak,which is probably caused by the downward mixing and/or the advection transport of SO 2 -richer air over the North China Plain.The concentrations of SO 2 at CMA and GCH show highly significant downward trends (-4.4 ppb/yr for CMA and -2.4 ppb/yr for GCH),while a less significant trend (-0.3 ppb/yr) is identified in the data from SDZ,reflecting the character of SDZ as a regional atmospheric background site in North China.The SO 2 concentrations of all three sites show a significant decrease from period before to after the control measures for the 2008 Olympic Games,suggesting that the SO 2 pollution control has long-term effectiveness and benefits.In the post-Olympics period,the mean concentrations of SO 2 at CMA,GCH,and SDZ are (14.3±11.0) ppb,(12.1±7.7) ppb,and (7.5±4.0) ppb,respectively,with reductions of 26%,36%,and 13%,respectively,compared to the levels before.Detailed analysis shows that the differences of temperature,relative humidity,wind speed,and wind direction were not the dominant factors for the significant differences of SO 2 between the pre-Olympics and post-Olympics periods.By extracting the data being more representative of local or regional characteristics,a reduction of up to 40% for SO 2 in polluted areas and a reduction of 20% for regional SO 2 are obtained for the effect of control measures implemented for the Olympic Games. | Weili Lin Xiaobin XU Zhiqiang Ma Huarong Zhao Xiwen Liu Ying Wang | 2012 | Journal of Environmental Sciences2012，24，1： | 15 |
| 3 | Gold nanorod-photosensitizer conjugate with extracellular pH-driven tumor targeting ability for photothermal/photodynamic therapy显示文摘氯 e6-pHLIP <候补选手class=“ a-plus-plus ”> ss -AuNRs,金使nanorod具有感光性结合包含 pH (低)有给予细胞外的 pH 的一张二硫化物契约的插入肽( pHLIP )( pH <候补选手class=“ a-plus-plus ”> e )-driven 肿瘤指向能力,成功地为光力学的 bimodal 和 photothermal 治疗被开发了。在这 bimodal 治疗,氯 e6 (Ce6 ) ,第二代的 photosensitizer (PS ) ,被用于光力学的治疗(太平洋夏季时间) 。金 nanorods (AuNRs ) 作为 Ce6 的 nanocarrier 和 quencher 为 photothermal 治疗(PTT ) 并且也被用作一个过高热代理人。pHLIPss 作为一根驾驶 pHe 的指向探针被设计在低 pH 在癌症房间提高 Ce6 和 AuNRs 的累积。在 Ce6-pHLIP < 潜水艇 class= “ a-plus-plus ” > ss -AuNRs, Ce6 接近并且由 AuNRs 熄灭了,引起小太平洋夏季时间效果。当暴露了到正常生理的 pH 时 7.4, Ce6-pHLIP < 潜水艇 class= “ a-plus-plus ” > ss -AuNRs 泛泛地与房间膜联系。然而,曾经暴露了到酸的 pH 6.2, pHLIP 活跃地插入到房间膜,和 conjugates 是进房间的 translocated。当这发生时, Ce6 由于二硫化物与 AuNRs 分开细胞内部的谷胱甘肽(GSH ) 引起的契约劈开,和汗衫氧在光之上为太平洋夏季时间被生产照耀。作为单个 PTT 代理人,另外, AuNRs 能由提高的浸透和保留(EPR ) 效果在肿瘤提高 PS 的累积。因此由我们的数据显示了当暴露了到酸的 pH 时, Ce6-pHLIP < 潜水艇 class= “ a-plus-plus ” > ss -AuNRs 能为癌症治疗完成 synergistic PTT/PDT bimodality。 | Nannan Wang Zilong Zhao Yifan Lv Huanhuan Fan Huarong Bai Hongmin Meng Yuqian Long Ting Fu Xiaobing Zhang Weihong Tan | 2014 | Nano Research2014，7，9： | 11 |
| 4 | Hydrogeochemical and mineralogical characteristics related to heavy metal attenuation in a stream polluted by acid mine drainage:A case study in Dabaoshan Mine,China显示文摘Dabaoshan Mine,the largest mine in south China,has been developed since the 1970s.Acid mine drainage (AMD) discharged from the mine has caused severe environmental pollution and human health problems.In this article,chemical characteristics,mineralogy of ocher precipitations and heavy metal attenuation in the AMD are discussed based on physicochemical analysis,mineral analysis,sequential extraction experiments and hydrogeochemistry.The AMD chemical characteristics were determined from the initial water composition,water-rock interactions and dissolved sulfide minerals in the mine tailings.The waters,affected and unaffected by AMD,were Ca-SO4 and Ca-HCO3 types,respectively.The affected water had a low pH,high SO42 and high heavy metal content and oxidation as determined by the Fe2+ /Fe3+ couple.Heavy metal and SO42 contents of Hengshi River water decreased,while pH increased,downstream.Schwertmannite was the major mineral at the waste dump,while goethite and quartz were dominant at the tailings dam and streambed.Schwertmannite was transformed into goethite at the tailings dam and streambed.The sulfate ions of the secondary minerals changed from bidentate-to monodentate-complexes downstream.Fe-Mn oxide phases of Zn,Cd and Pb in sediments increased downstream.However,organic matter complexes of Cu in sediments increased further away from the tailings.Fe3+ mineral precipitates and transformations controlled the AMD water chemistry. | Huarong Zhao Beicheng Xia Jianqiao Qin Jiaying Zhang | 2012 | Journal of Environmental Sciences2012，24，6： | 8 |
| 5 | Aerosol Hygroscopicity during the Haze Red-Alert Period in December 2016 at a Rural Site of the North China Plain显示文摘A humidification system was deployed to measure aerosol hygroscopicity at a rural site of the North China Plain during the haze red-alert period 17–22 December 2016. The aerosol scattering coefficients under dry [relative humidity(RH) < 30%] and wet(RH in the range of 40%–85%) conditions were simultaneously measured at wavelengths of450, 550, and 700 nm. It is found that the aerosol scattering coefficient and backscattering coefficient increased by only 29% and 10%, respectively when RH went up from 40% to 80%, while the hemispheric backscatter fraction went down by 14%, implying that the aerosol hygroscopicity represented by the aerosol scattering enhancement factor f(RH) is relatively low and RH exerted little effects on the aerosol light scattering in this case. The scattering enhancement factors do not show significant differences at the three wavelengths, only with an approximate 2% variation, suggesting that the aerosol hygroscopicity is independent of the wavelength. Aerosol hygroscopicity is highly dependent on the aerosol chemical composition. When there is a large mass fraction of inorganics and a small mass fraction of organic matter, f(RH) reaches a high value. The fraction of NO_3^- was strongly correlated with the aerosol scattering coefficient at RH = 80%, which suggests that NO_3^- played an important role in aerosol hygroscopic growth during the heavy pollution period. | Xuefei QI Junying SUN Lu ZHANG Xiaojing SHEN Xiaoye ZHANG Yangmei ZHANG Yaqiang WANG Haochi CHE Zhouxiang ZHANG Junting ZHONG Kaiyan TAN Huarong ZHAO Sanxue REN | 2018 | Journal of Meteorological Research2018，32，1： | 7 |
| 6 | A High-Performance Composite Epoxy Coating Based on the Cooperative Enhancement of 2D Co_(2)(OH)2BDC and Electrospun PAN Nanofiber Membrane显示文摘Based on a two-dimensional(2D)Co-MOF(Co_(2)(OH)_(2)BDC)with a self-contained organic interface and low conductivity,a composite epoxy coating(2D Co_(2)(OH)_(2)BDC-PAN/EP)was constructed by a two-step preparation.First,a polyacrylonitrile(PAN)nanofiber membrane was electrospuned on the surface of Q235 steel,followed by coating using the epoxy coating(EP)containing 2D Co_(2)(OH)_(2)BDC.The 2D Co_(2)(OH)_(2)BDC-PAN/EP composite epoxy coatings showed robust mechanical performance and excellent corrosion resistance capacity. | Zhao Huarong Zhang Yueshuang Gan Shaojie Yue Qiankun Liu Zan Cheng Zhilin | 2022 | China Petroleum Processing & Petrochemical Technology2022，24，2： | 2 |
| 7 | Comparison of Submicron Particles at a Rural and an Urban Site in the North China Plain during the December 2016 Heavy Pollution Episodes显示文摘An extensive field experiment for measurement of physical and chemical properties of aerosols was conducted at an urban site in the Chinese Academy of Meteorological Sciences(CAMS) in Beijing and at a rural site in Gucheng(GC), Hebei Province in December 2016. This paper compares the number size distribution of submicron particle matter(PM1, diameter < 1 μm) between the two sites. The results show that the mean PM1 number concentration at GC was twice that at CAMS, and the mass concentration was three times the amount at CAMS. It is found that the accumulation mode(100–850 nm) particles constituted the largest fraction of PM1 at GC, which was significantly correlated with the local coal combustion, as confirmed by a significant relationship between the accumulation mode and the absorption coefficient of soot particles. The high PM1 concentration at GC prevented the occurrence of new particle formation(NPF) events, while eight such events were observed at CAMS. During the NPF events, the mass fraction of sulfate increased significantly, indicating that sulfate played an important role in NPF. The contribution of regional transport to PM1 mass concentration was approximately 50% at both sites, same as that of the local emission. However, during the red-alert period when emission control took place, the contribution of regional transport was notably higher. | Xiaojing SHEN Junying SUN Xiaoye ZHANG Yangmei ZHANG Yaqiang WANG Kaiyan TAN Peng WANG Lu ZHANG Xuefei QI Haochi CHE Zhouxiang ZHANG Junting ZHONG Huarong ZHAO Sanxue REN | 2018 | Journal of Meteorological Research2018，32，1： | 2 |
| 8 | Human health risk from soil heavy metal contamination under different land uses near Dabaoshan Mine, Southern China 显示文摘 | Huarong Zhao Beicheng Xia Chen Fan | 2012 | Science of The Total Environment2012，，417418： | 1 |
| 9 | Intrinsic stress-induced adaptive ferroelectric domain rearrangement in the monoclinic Pb(Mg1/3 Nb2/3 )O3-PbTiO3 single crystal显示文摘 | Zhao Kunyu Zeng Huarong Song Hongzhang | 2009 | Mater Lett2009，63，： | 1 |
| 10 | Immunoenhancement effect of rehmannia glutinosa polysaccharide on lymphocyte proliferation and dendritic cell显示文摘 | Yee Huang Chunmao Jiang Yuanliang Hu Xiaojuan Zhao Cheng Shi Yun Yu Cui Liu Yang Tao Huarong Pan Yibo Feng Jiaguo Liu Yi Wu Deyun Wang | 2013 | Carbohydrate Polymers2013，，2： | 1 |
| 11 | Human health risk from soil heavy metal contamination under different land uses near Dabaoshan Mine,Southern China显示文摘 | Zhao Huarong Xia Beicheng Fan Chen | 2012 | Science of the Total Environment2012，，： | 1 |
| 12 | Assessment of wetland frag-mentation in the Tarim River basin, western China显示文摘 | Zhao Ruifeng Chen Yaning Zhou Huarong | 2009 | Environmental Geology2009，57，2： | 1 |
| 13 | Ratiometrie and selective fluorescent sensor for Zn2+ as an 'Off-On- Off' switch and logic gate 显示文摘 | Li Yaping Yang Huarong Zhao Qiang | 2012 | Inorg Chem2012，51，： | 1 |
| 14 | Scaled Bipartite Consensus Controller Design for Second-Order Multi-Agent Systems with Mixed Time-Delays显示文摘The scaled bipartite consensus of second-order multi-agent systems is investigated in this paper.The internal delay and distributed delay are also considered in the dynamic model of each agent,in which the delays can be time-varying and large.The communication topology among agents is assumed to be directed and structurally balanced.On one hand,in order to guarantee scaled bipartite consensus of second-order multi-agent systems,an adaptive periodically intermittent control protocol is applied.On the other hand,some consensus criteria in the form of matrix inequalities are obtained by using Jensen inequality,Lyapunov stability theory and graph theory.Finally,a numerical simulation example is given to demonstrate the feasibility of theoretical results. | YANG Ruitian PENG Li YANG Yongqing ZHAO Huarong | 2022 | Journal of Systems Science & Complexity2022，35，3： | 1 |
| 15 | Human health risk from soil heavy metal contamination under different land uses near Dabaoshan Mine, Southern China 显示文摘 | ZHAO Huarong XlA Beicheng FAN Chen | 2012 | Sci Total Environ2012，417，： | 1 |
| 16 | Genome-wide analysis of GH3 gene family in soybean( Glycine max)显示文摘 | Wei ZHAO Xinjie SHEN Wei GUO Qingbo YOU Yanjie YAO Jianhua LU Juncheng ZHANG Lei HUANG Bingbing DUAN Huarong LV Aili BAO Yongqing JIAO | 2016 | Oil Crop Science2016，1，2： | 1 |
| 17 | Human health risk from soil heavy metal contamination under different land uses near Dabaoshan Mine, Southern China显示文摘 | Zhao Huarong Xia Beicheng Fan Chen | 2012 | Science of the Total Environment2012，，： | 1 |
| 18 | Unusual local electric field concentration in multilayer ceramic capacitors显示文摘Local electric-field around multitype pores(dielectric pore,interface pore,electrode pore)in multilayer ceramic capacitors(MLCCs)was investigated using Kelvin probe force microscopy combined with the finite element simulation to understand the effect of pores on the electric reliability of MLCCs.Electricfield is found to be concentrated significantly in the vicinity of these pores and the strength of the local electric-field is 1.5e5.0 times of the nominal strength.Unexpectedly,the concentration degree of the pores in the inner electrode is much higher than that in the dielectrics and dielectric-electrode interfaces.Meanwhile,geometry orientations are found to have a remarkable influence on the local electric field strength.The pores act as an insulation degradation precursor via local electric,thermal center,and oxygen vacancies accumulation center.Such unusual local electric field concentration of multitype pores can provide new insights into the understanding of insulation degradation evolution,processing tailoring and design optimization for MLCCs. | Wentong Du Huarong Zeng Weiwei Yang Kunyu Zhao Faqiang Zhang Guorong Li Yongxiang Li Zhifu Liu | 2023 | Journal of Materiomics2023，9，2： | 0 |
| 19 | Long-term in-vitro culture and subculture of the hemocytes of swimming crab Portunus trituberculatus显示文摘Crab cell line,especially continuous crab cell line,can provide us a useful tool for studies on the virology,immunology,and molecular biology of crabs.However,no continuous crab cell line has been available due to the lacking of suitable medium and the occurrence of mitosis-arrest.In this study,long-term in vitro culture conditions for both two-(2D)and three-dimensions(3D)were successfully developed for the circulating hemocytes of swimming crab Portunus trituberculatus,designated as PTH cells.In 2D culture,a novel crab basic medium in osmolarity of 990–1100 mOsm/kg was optimized for the first time,which is different from Leibovitz's L-15 medium in mainly the components of amino acids,containing double strengths of the contents of free amino acid mixture in the crab serum.Then an optimal crab growth medium was developed by supplementing 5%fetal bovine serum,50-g/L yeast extract powder,20-μg/L basic fibroblast growth factor and epidermal growth factor into the optimal crab basic medium,and found that it could support a long-term survival of PTH cells in a healthy monolayer up to 347 days and partially break through the mitosis-arrest of crab cells evidenced by the obvious increase of proliferating potential detected in the 10-d primarily cultured PTH cells.These 2D cultured PTH cells could be successfully sub-cultured for 11 times by physical flushing method and well cryopreserved in liquid nitrogen.In 3D culture,using the same crab growth medium,the PTH cell aggregates could be easily formed and healthily maintained on the surface of solidified Matrigel or in the ultra-low-attachment plate with a survival rate of 50%–60%on Day 103.This work largely improved the primary culture and subculture of crab cells and will facilitate the establishment of continuous crab cell line. | Liwen GUO Yaqi ZHAO Huarong GUO | 2023 | Journal of Oceanology and Limnology2023，41，5： | 0 |
| 20 | Electric field-induced photoluminescence quenching in Pr-doped BNT ceramics across the MPB region显示文摘Piezophotonics is a great interesting field of physics that has led to a number of important technologies,such as light source,smart sensors,and mechatronics.In this work,we reported Pr-doped(Bi_(0.5)Na_(0.5))TiO_(3)-based lead-free ceramics with strong red photoluminescence emission and large strain response(d_(33)^(*)=460 pm/V,S=0.32%).The PL emission can be quenched by decreasing the intensity by 93%after electrical polarization(E=50 kV/cm).The local structure and electric field-induced structural changes were systematically investigated to reveal the significant distinction in photoluminescence properties caused by electrical polarization.The results indicated that polarization treatment eliminates the structural inhomogeneities and establishes a long-range ferroelectric tetragonal and rhombohedral distortion.The crystal structure transformed irreversibly from a non-ergodic to a normal ferroelectric state.PL quenching originated from the decreased distortion of octahedral due to the transition from a non-ergodic state to a highly ordered symmetrical structure.Meanwhile,the enlarged domain structure contributed to the photoluminescence quenching effect.Our findings demonstrate that an electric field can be a robust tool for adjusting the photoluminescence property and provide insights into the rela-tionship between the structure and PL properties of BNT-based ceramics under an external stimulus. | Mingze Sun Peng Li Juan Du Weifang Han Jigong Hao Kunyu Zhao Huarong Zeng Wei Li | 2022 | Journal of Materiomics2022，8，2： | 0 |
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