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| 1 | Further Information of the Associated Li Deposits in the No.6 Coal Seam at Jungar Coalfield, Inner Mongolia, Northern China显示文摘Total 138 coal samples and 14 parting samples were taken from the No. 6 Seam of the Jungar Coalfield, Inner Mongolia. These samples were analysed by optical microscopy, sequential chemical extraction procedure (SCEP), inductively coupled plasma mass spectrometry (ICP-MS), X-ray powder diffraction (XRD), and scanning electron microscope in conjunction with an energy-dispersive X-ray spectrometer (SEM-EDX) analysis. The results indicate that the Li contents have reached the industrial grade of the coal associated Li deposit, and the total Li reserves have reached 2406600 tons, that is, 5157000 tons Li2O in the No. 6 seam in the Jungar Coalfield. The sequential chemical extraction procedure results suggest that the Li concentration is mainly related to inorganic matter. The minerals in the coals consist of kaolinite, boehmite, chlorite-group mineral, quartz, calcite, pyrite, siderite and amorphous clay material. Some Li could be absorbed by clay minerals in the Li-bearing coal seam. The chlorite phase?could be?most likely the host for a part of Li. The Yinshan Oldland should be the most possible source of Li of the coal. | SUN Yuzhuang ZHAO Cunliang LI Yanheng WANG Jinxi ZHANG Jianya JIN Zhe LIN Mingyue Wolfgang KALKREUTH | 2013 | Acta Geologica Sinica(English Edition)2013，87，4： | 33 |
| 2 | Pollution of organic compounds and heavy metals in a coal gangue dump of the Gequan Coal Mine, China显示文摘Samples around a coal gangue dump of the Gequan Coal Mine were collected in April 2009. GC (gas chromatography) and GC/MS (gas chromatography/mass spectrometry) were employed to analyze the composition of organic matter in the samples. ICP-MS (inductively coupled plasma mass spectrometry) was used to determine the concentrations of heavy metals. The contents of organic extracts are within the range of 140-750 mg/kg. Alkand aro-ratios are relatively high. Compared to those of the background sample (GQ13 ), the contents of saturated hydrocarbon compounds in all the samples are relatively high. The contents of polycyclic aromatic hydrocarbons (PAHs) are relatively high with the distance getting closer to the coal gangue dump. These indicate that organic matter in the samples is from coal particles of the coal gangue dump. The distributions of heavy metals are very similar: the contents decrease with distance from the dump, which indicates that the harmful heavy metals from the coal gangue dump have polluted as thick as at least 500 m. | FAN Jingsen SUN Yuzhuang LI Xinyu ZHAO Cunliang TIAN Duanxin SHAO Longyi WANG Jinxi | 2013 | Chinese Journal Of Geochemistry2013，32，3： | 18 |
| 3 | Anomalous Concentrations of Rare Metal Elements, Rare-scattered(Dispersed) Elements and Rare Earth Elements in the Coal from Iqe Coalfield, Qinghai Province, China显示文摘Total of 23 bench samples were taken from the No. 7 Coal of Iqe Coalfield, Qinghai Province, China, following Chinese Standard Method GB/T 482-2008(2008). These samples were analyzed by powder X-ray diffraction(XRD), inductively coupled plasma mass spectrometry(ICPMS) and X-ray fluorescence(XRF). The results indicate that the No. 7 Coal belongs to a low rank(Ro,ran =0.659%) and high-ash coal(40.54%). Compared to common Chinese and world low-rank coals, the Iqe coal contains anomalous concentrations of rare metal elements, rare-scattered(dispersed) elements and rare earth elements. The highest contents of Rb, Cs, Ga and REY reach to 180, 26, 37, and 397 ppm, respectively. Their average contents of these elements are 10.9, 15, 4.8 and 3.5 times higher than those of world coals, respectively. Minerals in the coal include kaolinite, quartz, muscovite, siderite, and traces of rutile, and brookite. Kaolinite could be main host minerals of Rb, Cs, Ga and REY. The anomalous rare element Rb and Cs accumulation in the Iqe coal is related to both organic and inorganic matter. The REY concentrations may be related to circulation of thermal solutions, contained or sorbed by clayey particles, and organic matter as well. | SUN Yuzhuang ZHAO Cunliang LI Yanheng WANG Jinxi | 2015 | Acta Geologica Sinica(English Edition)2015，89，1： | 12 |
| 4 | Soil Microbial Population Dynamics along a Chronosequence of Moist Evergreen Broad-leaved Forest Succession in Southwestern China显示文摘Little is known about whether soil microbial population dynamics are correlated with forest succession.To test the hypotheses that(1) soil microbial composition changes over successional stages,and(2) soil microbial diversity is positively correlated with plant species diversity,we determined the soil microbial populations,community composition,and microflora diversity in evergreen broad-leaved forests along a chronosequence of vegetation succession from 5 to 300 years in southwestern China.The soil microbial community was mainly composed of bacteria(87.1-98.7% of the total microorganisms and 10 genera identified),fungi(0.3-4.0%,7 genera),and actinomycetes(2.1-9.1%,8 species and 1 genus).There were significant differences in soil microbial populations among different successional stages and within the four seasons.The seasonal variations of the soil microbial community may be associated with the seasonal changes in environmental conditions.The changes in soil microbial diversity(Shannon-Wiener index) with successional time followed one-humped,convex curves peaked at-100 years since restoration,which is identical with the trends of the aboveground plant diversity.Higher plant diversity resulting in enhanced nutrient flow and root exudation may contribute to positive relationships between the soil microbial diversity and plant diversity.Hence,decreases in soil microbial diversity in the late-successional stages appear to be related to the net loss in species richness that occurs after 100 years since restoration.Our findings confirm the intermediate disturbance hypothesis that suggests diversity peaks at midsuccessional stages. | ZHU Wanze CAI Xiaohu LIU Xingliang WANG Jinxi CHENG Song ZHANG Xiuyan LI Dengyu LI Maihe | 2010 | Journal of Mountain Science2010，7，4： | 8 |
| 5 | Whole genome sequencing of 10K patients with acute ischaemic stroke or transient ischaemic attack: design, methods and baseline patient characteristics显示文摘Background and purpose Stroke is the second leading cause of death worldwide and the leading cause of mortality and long-term disability in China,but its underlying risk genes and pathways are far from being comprehensively understood.We here describe the design and methods of whole genome sequencing(WGS)for 10914 patients with acute ischaemic stroke or transient ischaemic attack from the Third China National Stroke Registry(CNSR-III).Methods Baseline clinical characteristics of the included patients in this study were reported.DNA was extracted from white blood cells of participants.Libraries are constructed using qualified DNA,and WGS is conducted on BGISEQ-500 platform.The average depth is intended to be greater than 30×for each subject.Afterwards,Sentieon software is applied to process the sequencing data under the Genome Analysis Toolkit best practice guidance to call genotypes of single nucleotide variants(SNVs)and insertion-deletions.For each included subject,21 fingerprint SNVs are genotyped by MassARRAY assays to verify that DNA sample and sequencing data originate from the same individual.The copy number variations and structural variations are also called for each patient.All of the genetic variants are annotated and predicted by bioinformatics software or by reviewing public databases.Results The average age of the included 10914 patients was 62.2±11.3 years,and 31.4%patients were women.Most of the baseline clinical characteristics of the 10914 and the excluded patients were balanced.Conclusions The WGS data together with abundant clinical and imaging data of CNSR-III could provide opportunity to elucidate the molecular mechanisms and discover novel therapeutic targets for stroke. | Si Cheng Zhe Xu Yang Liu Jinxi Lin Yong Jiang Yilong Wang Xia Meng Anxin Wang Xinying Huang Zhimin Wang Guohua Chen Songdi Wu Zhengchang Jia Yongming Chen Xuerong Qiu Jun Wu Binbin Song Weizhong Ji Zhongping An Wenjun Xue Lili Zhao Yu Geng Hongyan Li Hao Li Yongjun Wang | 2021 | Stroke & Vascular Neurology2021，6，2： | 8 |
| 6 | Low serum albumin levels predict poor outcome in patients with acute ischaemic stroke or transient ischaemic attack显示文摘Background To examine the relationship of serum albumin with poor functional outcome and mortality in patients with acute ischaemic stroke(AIS)or transient ischaemic attack(TIA),and perform a meta-analysis to summarise the association.Methods We analysed data from the Third China National Stroke Registry(CNSR-Ⅲ).Patients were divided into four groups based on serum albumin levels at admission.The outcomes included poor functional outcome(modified Rankin Scale(mRS)score of 3 to 6)and mortality at 3 months and 1 year.Multiple logistic regression models and Cox regression models were used to evaluate the association,respectively.We used a fixed-effect model to calculate the risk ratio for poor functional outcome and a random-effect model for mortality in the meta-analysis.Results A total of 13618 patients were enrolled.During the 3-month follow-up period,compared with 40 to 44.9 g/L group,patients in<35 g/L group had an increased risk of poor functional outcome and mortality(adjusted OR 1.37(95%CI 1.12 to 1.67);adjusted HR 2.13(95%CI 1.41 to 3.23)).The relationship in per 10 g/L decreased serum albumin with prognosis was consistently inversed(adjusted OR 1.17(95%CI 1.01 to 1.35);adjusted HR 1.86(95%CI 1.30 to 2.64)).Also,low serum albumin levels were independently correlated with clinical outcomes at 1 year.In the meta-analysis,the OR for poor functional outcome pooled 3 studies per 1 g/L decrease was 1.03(95%CI 1.02 to 1.05),and the HR for mortality pooled 5 studies was 1.07(95%CI 1.03 to 1.11).Conclusions Low serum albumin levels predict poor functional outcome and mortality in patients with AIS or TIA. | Hongyu Zhou Anxin Wang Xia Meng Jinxi Lin Yong Jiang Jing Jing Yingting Zuo Yilong Wang Xingquan Zhao Hao Li Yongjun Wang | 2021 | Stroke & Vascular Neurology2021，6，3： | 7 |
| 7 | Changes in major factors affecting the ecosystem health of the Weihe River in Shaanxi Province, China显示文摘一条河的生态系统健康的维护为本地持续开发是很重要的。根据质并且 Weihe 河的生态系统功能上的自然变化和人的活动的影响的定量分析,在影响它的生态系统健康的主要因素的变化被决定,它包括:1 ) 环境的缺乏流动:自从 1960 年代,到来的溪流流动显示出一个明显的减少趋势。甚至在低流动时期,在溪流的 80% 水被水坝在 Baoji 区域为农业灌溉扣押。作为结果,为环境使用在溪流维持的水流动是很有限的。2 ) 水质量的恶化:典型污染物质的集中喜欢化学的氧需求(货到付款) 和 NH < 潜水艇 class= “ a-plus-plus ” > 3 -N 比他们中国环境质量的最大的价值高标准。很少的鱼种类能在河里幸存。3 ) 水隧道的变丑:连续隧道沉积为洪水分泌物在能力在溪流坡度,河床的收缩和衰落导致了减少。4 ) 河边的植被的损失:最河边的土地被城市的构造活动占据了,它引起了河边的植被和生物多样性和进一步的削弱的洪水控制和水纯化函数的损失。 | Qi LI Jinxi SONG Anlei WEI Bo ZHANG | 2013 | Frontiers of Environmental Science & Engineering2013，7，6： | 7 |
| 8 | Drought tolerance evaluation of tobacco plants transformed with different set of genes under laboratory and field conditions显示文摘尽管广泛的研究证明了许多干旱应答的基因授与干旱忍耐到植物,能力在各种各样的自然条件下面由不同基因授与的干旱忍耐的比较很少有报导。我们评估了并且比较 transgenes,干旱应答的基因(AtDREB1B 和 AtCBL1 ) 和根的二个集合的效果调整建筑学的基因(iaaM 和 AtCKX ) ,在在 Nicotiana tabacum 的干旱忍耐上,植物使遭到了到不同条件。根特定的倡导者 PYK10 驾驶的 AtCKX3 的表示(此后指定了为 P10;P10 : AtCKX3 ) , 35S:AtCKX3,或 P10:iaaM 支持了根生长和开发。比作怀有 P10 的植物: 展出的 AtCKX3, 35S:AtCKX3, P10:iaaM,或空向量,那些带的 35S:AtDREB1B, 35S:AtCBL1,或 35S:iaaM 在控制实验室的条件下面增加了干旱忍耐。相反地,在地里,条件,与 35S:AtDREB1 转变的植物, 35S:AtCBL1,或 35S:iaaM 对干旱应力敏感。在地条件下面,干旱应力戏剧性地减少了生长和而它在带 P10 的植物上有小效果,怀有 35S:AtDREB1B, 35S:AtCBL1, 35S:iaaM,或空向量的植物的种子生产: AtCKX3, 35S:AtCKX3,或 P10:iaaM。这研究证明到有环境条件的干旱压力变化的植物忍耐,和我们的结果显示操作控制根建筑学的基因的表示可能为处于自然条件与改进干旱忍耐设计植物是重要的。 | Yuanhua Wang Ruihong Dang Jinxi Li Yu Han Ning Ding Xingliang Li Meiru Jia Ziqiang Li Lingzhi Wei Jinzhu Jiang Yijuan Fan Bingbing Li Wensuo Jia | 2015 | Science Bulletin2015，60，6： | 3 |
| 9 | Paleostress Reconstruction of Micangshan Anticlinorium on the Southern Margin of the Qinling Orogenic Belts,China显示文摘Brittle structures in rock of different ages can be used to establish the tectonic evolution of an orogenic belt through paleostress calculations. Micangshan is located at the southern margin of the Qinling orogenic belt,between the SE-trending Longmenshan fold-and-thrust belt and the arcuate Dabashan thrust-and-fold belt. Structural observations revealed that the dominant structures are reverse and strike-slip faults and folds with E–W and NE–SE trends. To increase knowledge of the tectonic evolution of the Micangshan anticlinorium,faults,joints,veins,and folds were measured at more than eighty sites. On the basis of structural analysis,it emerged that the multiphase paleostress fields became established after the oblique collision between the North and South China plates. The earliest stress field with N–S compression was established during the Micangshan uplift associated with the E–W trending faults and folds. Subsequently,a N–S extension occurred when the Qinling orogenic belt collapsed. Then NW–SE compression developed,with NE trending faults and folds forming in relation to Longmenshan thrusting toward southwest on the eastern margin of the Tibetan plateau. With the development of the arcuate Dabashan orogenic belt,the compression stress orientation of the Micangshan anticlinorium altered from NE–SW to E–W. | LI Jinxi LI Zhiwu LIU Shugen SUN Dong DENG Bin | 2015 | Acta Geologica Sinica(English Edition)2015，89，2： | 2 |
| 10 | Characteristics of dental morphology in the Xinjiang Uyghurs and correlation with the EDARV370A variant显示文摘Teeth are one of the most important materials for anthropological studies because they are likely to be preserved in ancient remains.While the frequencies of dental characteristics can provide clues to the phylogeny of populations,genetic studies at the individual level can further reveal the biological mechanisms and evolutionary context of dental characteristics.In this study,by analyzing 38 dental characteristics of 242 Xinjiang Uyghur individuals,we found that(i)the dental characteristics of the Uyghurs showed evidence of admixture between European and East Asian populations.The admixture proportions were in line with those previously reported in population genetic studies;(ii)the Xinjiang Uyghur dental characteristics formed three clusters in pairwise correlation analysis.One of the main clusters consisted of characteristics including incisor shoveling,double shoveling and mesial ridge;and(iii)all the characteristics in this cluster were significantly correlated with the genetic variant EDARV370A.The extracted composite phenotypic factor was also significantly associated with EDARV370A,which explained 18%of the total phenotypic variance.This indicated a pleiotropic effect,i.e.,the same genetic factor affects a number of dental characteristics at the same time.Our results confirmed that EDARV370A,a genetic variant that first originated in East Asia about 30000 years ago,played an important role in incisor shoveling in East Asia.This finding suggested that incisor shoveling in modern humans in East Asia is likely to have appeared after the late Pleistocene. | TAN JingZe PENG QianQian LI JinXi GUAN YaQun ZHANG LiPing JIAO Yi YANG YaJun WANG SiJia JIN Li | 2014 | Science China(Life Sciences)2014，57，5： | 2 |
| 11 | Concentrations of Lithium in Chinese Coals显示文摘 | Yuzhuang Sun Yanheng Li Cunliang Zhao Mingyue Lin Jinxi Wang Shenjun Qin | 2010 | Energy Exploration & Exploitation2010，，2： | 2 |
| 12 | LDL-C levels,lipid-lowering treatment and recurrent stroke in minor ischaemic stroke or TIA显示文摘Background and purpose Dyslipidaemia is a major risk factor for ischaemic stroke and transient ischaemic attack(TIA).This study aimed to investigate the association between baseline low-density lipoprotein cholesterol(LDL-C)level,lipid-lowering treatment and short-term risk of new stroke in patients with a minor ischaemic stroke or TIA.Methods We derived data from the Clopidogrel in High-risk patients with Acute Non-disabling Cerebrovascular Events trial.Patients with a minor stroke or TIA were categorised by LDL-C level at baseline(<2.6 or≥2.6 mmol/L(100 mg/dL))and with or without lipid-lowering treatment after symptom onset.The primary outcome was a new ischaemic stroke at 3 months.The association of baseline LDL-C level,lowering treatment and outcomes were assessed.Results Among 3027 patients,2154(71.2%)patients had an initial LDL-C≥2.6 mmol/L,of which 1267(41.9%)received lipid-lowering treatment.Elevated LDL-C level was associated with a higher risk of new ischaemic stroke at 3 months in patients without lipid-lowering treatment(adj.HR=1.35,95%CI:1.19 to 1.53),but not in those with lipid-lowering treatment(adj.HR=0.99,95%CI:0.82 to 1.19)(p for interaction=0.007).Patients with LDL-C≥2.6 mmol/L had a numerically higher risk of ischaemic stroke(11.8%vs 8.0%,adj.HR=1.37,95%CI:0.96 to 1.96)in those without lipid-lowering treatment.For patients with LDL-C≥2.6 mmol/L,lipid-lowering treatment was associated with reduced risk of ischaemic stroke at 3 months(7.9%vs 11.8%;adj.HR=0.54,95%CI:0.39 to 0.75).Conclusions Elevated untreated baseline LDL-C level was associated with an increased short-term risk of ischaemic stroke among patients presenting with minor ischaemic stroke or TIA.There was potential benefit of lipid-lowering treatment in minor stroke or TIA patients with LDL-C≥2.6 mmol/L.Trial registration number NCT00979589. | Yuesong Pan Runqi Wangqin Hao Li Aoming Jin Jiejie Li Jinxi Lin Xia Meng Ying Xian Daniel T Laskowitz Yongjun Wang | 2022 | Stroke & Vascular Neurology2022，7，4： | 2 |
| 13 | Li distribution and mode of occurrences in Li-bearing coal seam # 6 from the Guanbanwusu Mine, Inner Mongolia, northern China显示文摘 | Yuzhuang Sun Cunliang Zhao Yanheng Li Jinxi Wang Shiming Liu | 2012 | Energy Exploration & Exploitation2012，，1： | 1 |
| 14 | Concentrations of Lithium in Chinese Coals显示文摘 | Yuzhuang Sun Yanheng Li Cunliang Zhao Mingyue Lin Jinxi Wang Shenjun Qin | 2010 | Energy Exploration & Exploitation2010，，2： | 1 |
| 15 | Li distribution and mode of occurrences in Li-bearing coal seam # 6 from the Guanbanwusu Mine, Inner Mongolia, northern China显示文摘 | Yuzhuang Sun Cunliang Zhao Yanheng Li Jinxi Wang Shiming Liu | 2012 | Energy Exploration & Exploitation2012，，1： | 1 |
| 16 | PolyvasculaR Evaluation for Cognitive Impairment and vaScular Events (PRECISE)-a population-based prospective cohort study: rationale, design and baseline participant characteristics显示文摘Background and purpose Cardiovascular diseases and dementia are two major diseases in the elderly.Atherosclerosis is associated with future vascular events and cognitive impairment.The PolyvasculaR Evaluation for Cognitive Impairment and vaScular Events(PRECISE)study is a population-based prospective cohort study with comprehensive evaluation of multiterritorial artery stenosis and plaque using advanced vascular imaging techniques and prospective collection of vascular events and cognitive assessments.Methods Between May 2017 and September 2019,the PRECISE study enrolled 3067 community-dwelling adults with ages between 50 and 75 years cluster sampled from six villages and four communities of Lishui city in China.Data are collected in face-to face interviews at baseline,2-year and 4-year follow-up visits.Brain MRI including high-resolution sequences for intracranial and carotidal arteries and CT angiography for thoracoabdominal arteries were performed at baseline and will be rescanned after 4 years.Cardiovascular/cerebrovascular events and cognitive assessment will be prospectively collected after the enrollment.Blood and urine samples were collected and biomarkers were tested at baseline.Results A total of 3067 subjects were enrolled,among which 53.5%were female with an average age of 61.2±6.7 years.Among them,2.8%,8.1%,43.1%and 21.6%had a history of stroke,coronary heart diseases,hypertension and diabetes mellitus,respectively.Conclusions The PRECISE study is a population-based prospective cohort study with comprehensive evaluation of atherosclerotic stenosis and plaque using advanced vascular imaging techniques.Data from this cohort provide us an opportunity to precisely evaluate polyvascular atherosclerosis and its association with future vascular events and cognitive impairment. | Yuesong Pan Jing Jing Xueli Cai Yilong Wang Suying Wang Xia Meng Chunlai Zeng Jiong Shi Jiansong Ji Jinxi Lin Lingchun Lyu Zhe Zhang Lerong Mei Shiping Li Shan Li Wanlin Zhu Hao Li Tiemin Wei Yongjun Wang | 2021 | Stroke & Vascular Neurology2021，6，1： | 1 |
| 17 | Palmprint Phenotype Feature Extraction and Classification Based on Deep Learning显示文摘Palmprints are of long practical and cultural interest.Palmprint principal lines,also called primary palmar lines,are one of the most dominant palmprint features and do not change over the lifespan.The existing methods utilize filters and edge detection operators to get the principal lines from the palm region of interest(ROI),but can not distinguish the principal lines from fine wrinkles.This paper proposes a novel deep-learning architecture to extract palmprint principal lines,which could greatly reduce the influence of fine wrinkles,and classify palmprint phenotypes further from 2D palmprint images.This architecture includes three modules,ROI extraction module(REM)using pre-trained hand key point location model,principal line extraction module(PLEM)using deep edge detection model,and phenotype classifier(PC)based on ResNet34 network.Compared with the current ROI extraction method,our extraction is competitive with a success rate of 95.2%.For principal line extraction,the similarity score between our extracted lines and ground truth palmprint lines achieves 0.813.And the proposed architecture achieves a phenotype classification accuracy of 95.7%based on our self-built palmprint dataset CAS_Palm. | Fan Jinxi Li Shaoying Song Haiguo Zhang Sijia Wang Guangtao Zhai | 2022 | Phenomics2022，2，4： | 1 |
| 18 | lncRNA ELFN1-AS1 upregulates TRIM29 by suppressing miR-211-3p to promote gastric cancer progression显示文摘Long noncoding RNA(lncRNA)extracellular leucine rich repeat and fibronectin type III domain containing 1-antisense RNA 1(ELFN1-AS1)has been found to be upregulated in various tumors.However,the biological functions of ELFN1-AS1 in gastric cancer(GC)are not entirely understood.In the present study,the expression levels of ELFN1-AS1,miR-211-3p,and TRIM29 are determined using reverse transcription-quantitative PCR.Subsequently,CCK8,EdU,and colony formation assays are performed to determine GC cell vitality.The migratory and invasive capabilities of GC cells are further evaluated using transwell invasion and cell scratch assays.Western blot analysis is performed to quantify the levels of proteins associated with GC cell apoptosis and epithelialmesenchymal transition(EMT).The competing endogenous RNA(ceRNA)activity of ELFN1-AS1 on TRIM29 through miR-211-3p is confirmed by pull-down,RIP,and luciferase reporter assays.Our study proves that ELFN1-AS1 and TRIM29 are highly expressed in GC tissues.ELFN1-AS1 silencing inhibits GC cell proliferation,migration,invasion and EMT,and induces cell apoptosis.Rescue experiments reveal that the oncogenicity of ELFN1-AS1 is modulated by acting as a sponge for miR-211-3p,thereby increasing the expression of the target gene of miR-211-3p,TRIM29.In summary,ELFN1-AS1 maintains GC cell tumorigenicity via the ELFN1-AS1/miR-211-3p/TRIM29 axis,indicating that this axis can be directed for GC treatment in the future. | Jinxi Huang Weiwei Yuan Beibei Chen Gaofeng Li Xiaobing Chen | 2023 | Acta Biochimica et Biophysica Sinica2023，55，3： | 1 |
| 19 | Rapid and Efficient Adsorption Removal of Reactive Blue 4 from Aqueous Solution by Cross-Linked Microcrystalline Cellulose–Epichlorohydrin Polymers: Isothermal, Kinetic, and Thermodynamic Study显示文摘In this study, we modified microcrystalline cellulose by cross-linking it with epichlorohydrin to obtain a rapid and efficient adsorbent for the removal of Reactive Blue 4 dye from aqueous solution. Evidences of the cross-linking of the microcrystalline cellulose were obtained by Fourier transform infrared spectroscopy, X-ray diff raction, Brunauer–Emmett–Teller analysis, thermogravimetric analysis, and scanning electron microscopy. We investigated the eff ects of adsorbent dosage, p H, initial dye concentration, temperature, and contact time on the dye adsorption capacity. The results showed that the adsorption equilibrium time was just 20 min and the maximum adsorption capacity was 69.79 mg/g. The adsorption isotherm data fitted the Langmuir isotherm model well, and the adsorption kinetics data followed the pseudo-second-order kinetic model. The results of the thermodynamic analysis suggest that the adsorption process was spontaneous and exothermic. Recyclability experiments demonstrated the good reusability of this adsorbent. Electrostatic interaction was found to dominate the adsorption process. | Yuanyuan Zhai Hongmei Qu Zhongxuan Li Bo Zhang Jinxi Cheng Jiaji Zhang | 2021 | Transactions of Tianjin University2021，27，1： | 1 |
| 20 | Regulating Li transport in Li-magnesium alloy for dendrite free Li metal anode显示文摘Li metal has become a strong candidate for anode due to its high theoretical specific capacity and lowest electrochemical potential.However,the poor reversibility caused by continuous chemical and electrochemical degradation hinders the practical application of Li metal.Solid-solution-based metal alloy phases have been proposed as hosts for regulating the non-dendrite electrodeposition,but the fundamental understanding remains unclear due to the drastically different deposition behaviors of Li on them.Here we found the difference in the diffusion coefficient of Li atoms on solid-solution-based metal alloy phases(Li-Mg and Li-Ag alloys)was a major contributor to the different deposition behaviors.The low Li atom diffusion coefficient of Li-Mg alloy showed a preferential Li accumulation on the upper surface rather than the inward-growth plating of Li atoms into alloy foil in Li-Ag alloy.By the process of secondary recrystallization,we improved the diffusion coefficient of Li atoms in Li-Mg alloy that facilitates the inward transfer rather than surface plating of Li atoms.In this case,the recrystallized Li-Mg alloy underwent a solidsolution phase change in the delithiation-lithiation cycles which yielded a high Coulombic efficiency of 99.3%with a reversible gravimetric capacity of 2,874 mAh·g−1 and superior cycling stability over 5,000 h without dendrite growth. | Jinxi Wang Yadong Ye Hongmin Zhou Wei Zhang Zhaowei Sun Jiawen Zhu Hongchang Jin Huanyu Xie Haoliang Huang Yi Cui Rong Huang Zezhong Li Song Jin Hengxing Ji | 2023 | Nano Research2023，16，6： | 0 |
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