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| 1 | Single-atom heterogeneous catalysts based on distinct carbon nitride scaffolds显示文摘Carbon nitrides integrating macroheterocycles offer unique potential as hosts for stabilizing metal atoms due to their rich electronic structure. To date, only graphitic heptazine-based polymers have been studied.Here, we demonstrate that palladium atoms can be effectively isolated on other carbon nitride scaffolds including linear melem oligomers and poly(triazine/heptazine imides). Increased metal uptake was linked to the larger cavity size and the presence of chloride ions in the polyimide structures. Changing the host structure leads to significant variation in the average oxidation state of the metal, which can be tuned by exchange of the ionic species as evidenced by X-ray photoelectron spectroscopy and supported by density functional theory. Evaluation in the semi-hydrogenation of 2-methyl-3-butyn-2-ol reveals an inverse correlation between the activity and the degree of oxidation of palladium, with oligomers exhibiting the highest activity. These findings provide new mechanistic insights into the influence of the carbon nitride structure on metal stabilization. | Zupeng Chen Evgeniya Vorobyeva Sharon Mitchell Edvin Fako Núria López Sean M.Collins Rowan K.Leary Paul A.Midgley Roland Hauert Javier Pérez-Ramírez | 2018 | National Science Review2018,5,5: | 4 |
| 2 | Efficacy of boceprevir, an NS3 protease inhibitor, in combination with peginterferon alfa-2b and ribavirin in treatment-naive patients with genotype 1 hepatitis C infection (SPRINT-1): an open-label, randomised, multicentre phase 2 trial显示文摘 | Paul Y Kwo Eric J Lawitz Jonathan McCone Eugene R Schiff John M Vierling David Pound Mitchell N Davis Joseph S Galati Stuart C Gordon Natarajan Ravendhran Lorenzo Rossaro Frank H Anderson Ira M Jacobson Raymond Rubin Kenneth Koury Lisa D Pedicone Clifford | 2010 | The Lancet2010,,9742: | 3 |
| 3 | Sofosbuvir with pegylated interferon alfa-2a and ribavirin for treatment-naive patients with hepatitis C genotype-1 infection (ATOMIC): an open-label, randomised, multicentre phase 2 trial显示文摘 | Kris V Kowdley Eric Lawitz Israel Crespo Tarek Hassanein Mitchell N Davis Michael DeMicco David E Bernstein Nezam Afdhal John M Vierling Stuart C Gordon Jane K Anderson Robert H Hyland Hadas Dvory-Sobol Di An Robert G Hindes Efsevia Albanis William T Symo | 2013 | The Lancet2013,,9883: | 3 |
| 4 | Direct characterization of a nonlinear photonic circuit’s wave function with laser light显示文摘Integrated photonics is a leading platform for quantum technologies including nonclassical state generation1–4,demonstration of quantum computational complexity5 and secure quantum communications6.As photonic circuits grow in complexity,full quantum tomography becomes impractical,and therefore an efficient method for their characterization7,8 is essential.Here we propose and demonstrate a fast,reliable method for reconstructing the two-photon state produced by an arbitrary quadratically nonlinear optical circuit.By establishing a rigorous correspondence between the generated quantum state and classical sum-frequency generation measurements from laser light,we overcome the limitations of previous approaches for lossy multimode devices9,10.We applied this protocol to a multi-channel nonlinear waveguide network and measured a 99.28±0.31%fidelity between classical and quantum characterization.This technique enables fast and precise evaluation of nonlinear quantum photonic networks,a crucial step towards complex,largescale,device production. | Francesco Lenzini Alexander N Poddubny James Titchener Paul Fisher Andreas Boes Sachin Kasture Ben Haylock Matteo Villa Arnan Mitchell Alexander S Solntsev Andrey A Sukhorukov Mirko Lobino | 2018 | Light(Science & Applications)2018,7,1: | 2 |
| 5 | Resistance exercise decreases the need for insulin in overweight women with gestational diabetes mellitus显示文摘 | Gabrielle N Brankston B.F Mitchell Edmond A Ryan Nanette B Okun | 2004 | American Journal of Obstetrics and Gynecology2004,,1: | 2 |
| 6 | 卒中介入治疗培训指南:国际多学会共识文件显示文摘1背景
缺血性卒中是全球人口死亡和残疾的首要原因。很多急性大血管闭塞(emergent large vesselocclusion,ELVO)患者都会遗留长期残疾。事实上,这些颅内大动脉闭塞经常会导致大面积脑损伤,进而造成患者死亡或严重致残。 | Lavine SD Cockroft K Hoh B Bambakidis N Khalessi AA Woo H Riina H Siddiqui A Hirsch JA Chong W Rice H Wenderoth J Mitchell P Coulthard A Signh TJ Phatorous C Khangure M Klurfan P ter Brugge K Iancu D Gunnarsson T Pongpech S Rodesch G Soderman M Taylor A Krings T Orbach D Picard L Suh DC Zheng HQ Jansen O Muto M Szikora I Pierot L Brouwer P Gralla J Renowden S Andersson T Fiehler J Turjman F White P Januel AC Spelle L Kulcsar Z Chapot R Biondi A Dima S Taschner C Szajner M Krajina A Sakai N Matsumaru Y Yoshknura S Ezura M Fujinaka T Iihara K Ishii A Higashi T Hirohata M Hyodo A Ito Y Kawanishi M Kiyosue H Kobayashi E Kobayashi S Kuwayama N Matsumoto Y Miyachi S Murayama Y Nagata I Nakahara I Nemoto S Niimi Y Oishi H Satomi J Satow T Sugiu K Tanaka M Terada T Yamagami H Diaz O Lylyk P Jayaraman MV Patsalides A Gandhi CD Lee SK Abruzzo T Albani B Ansari SA Arthur AS Baxter BW Bulsara KR Chen M Almandoz JE Fraser JF Heck DV Hetts SW Hussain MS Klucznik RP Leslie-Mawzi TM Mack WJ McTaggart RA Meyers PM Mocco J Prestigiacomo CA Pride GL Rasmussen PA Starke RM Sunenshine PJ Tarr RW Frei DF Pabo M Nogueira RG Zaidat OO Jovin T Linfante I Yavagal D Liebeskind D Novakovic R Pongpech S 许岩 孙瑞 郭芮兵 | 2017 | 国际脑血管病杂志2017,25,5: | 2 |
| 7 | Understanding SPKI/SDSI using first-order logic 显示文摘 | Li N Mitchell J | 2006 | International Journal of Information Security2006,5,1: | 1 |
| 8 | Brassins:A New Family of Plant Hormones from Rape Pollen显示文摘 | Mandava N B Worley J F | 1970 | Nature1970,225,: | 1 |
| 9 | Endovascular Stent-Graft Placement for the Treatment of Acute Aortic Dissection显示文摘 | Dake MD Kato N Mitchell RS | 1999 | N Engl J Med1999,340,20: | 1 |
| 10 | Healing of articular cartilage in intra-articular fractures in rabbits显示文摘 | Mitchell N Shepard N | | 0,,04: | 1 |
| 11 | Physical treatments for bipolar disorder:a review of electroconvulsive therapy,stereotactic surgery and other brain stimulation techniques显示文摘 | Loo C Katalinic N Mitchell PB et al | 2011 | Journal Of Affective Disorders2011,132,12: | 1 |
| 12 | Sudden cardiac death and anti- psychotics Part 2 : Monitoring and prevention 显示文摘 | Abdelmawla N Mitchell AJ | 2006 | Advances in Psychiatric Treatment2006,12,2: | 1 |
| 13 | Endovascular stent-graft placement for the treatment of acute aorticdissection显示文摘 | Dake MD Kato N Mitchell RS | 1999 | N Engl J Med1999,340,20: | 1 |
| 14 | Low density doped foams for ICF long scale length plasma experiments显示文摘 | Mitchell M A Gobby P L Ellott N E | 1995 | Fusion Technology1995,28,5: | 1 |
| 15 | Superficied mass with color flow Doppler imaging显示文摘 | Mitchell DG Laurence N Mario B | 1991 | J Clin Ultrasound1991,19,9: | 1 |
| 16 | Endovascular stent-graft placement for the treatment of acute aortic dissection显示文摘 | Dake MD Kato N Mitchell RS | 1999 | N Engl J Med1999,340,20: | 1 |
| 17 | A refined hybrid plate theory for composite laminates with piezoelectric laminate显示文摘 | Mitchell J A Reddy J N | 1996 | International Journal of Solids and Structures1996,32,16: | 1 |
| 18 | Healing of articular cartage in intra articular fracture in rabbits显示文摘 | MitchelL N | 1980 | J Bone Joint Surg(AM)1980,62,6: | 1 |
| 19 | Determination of the crystal growth rate of paracetamol as a function of solvent composition 显示文摘 | O'Ciardha C T Mitchell N A Hutton K W | 2012 | Ind Eng Chem Res2012,51,12: | 1 |
| 20 | Simple methods for measurement of bovine mucosal antibody responses in vivo 显示文摘 | MCNEILLY T N NAYLOR S W MITCHELL M C | 2007 | Vet Immunol Irnmunopathol2007,118,12: | 1 |