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| 1 | Enhanced photocatalytic activity of quantum-dot-sensitized one-dimensionally-ordered ZnO nanorod photocatalyst显示文摘An efcient photocatalyst was fabricated by assembling quantum dots(QDs) onto one-dimensionally-ordered ZnO nanorods, and the photocatalytic properties for Methyl Orange degradation were investigated by scanning electron microscopy, transmission electron microscopy, X-ray difraction, UV-Vis-NIR absorption spectroscopy and photoluminescence. The results indicate that the catalyst with assembled QDs is more favorable for the degradation than the pristine ZnO nanorods. The QDs with core-shell structure lower the photocatalytic ability due to the higher carrier transport barrier of the ZnS shell layer. Besides its degradation efciency, the photocatalyst has several advantages given that the one-dimensionally-ordered ZnO nanorods have been grown directly on indium tin oxide substrates. The article provides a new method to design an efective and easily recyclable photocatalyst. | Jinzhao Huang Song Liu Lei Kuang Yongdan Zhao Tao Jiang Shiyou Liu Xijin Xu | 2013 | Journal of Environmental Sciences2013，25，12： | 5 |
| 2 | Preparation and Tribological Study of a Peptide-Containing Alkylsiloxane Monolayer on Silicon显示文摘 | Song Shiyou Ren Sili Yang Jinqing | 2006 | Langmuir2006，22，14： | 1 |
| 3 | Mechanism of high-concentration electrolyte inhibiting the destructive effect of Mn(Ⅱ)on the performance of lithium-ion batteries显示文摘By optimizing electrolyte formulation to inhibit the deposition of transition metal ions(TMIs) on the surface of the graphite anode is an effective way to improve the electrochemical performance of lithium-ion batteries.At present,it is generally believed the formation of an effective interfacial film on the surface of the anode electrode is the leading factor in reducing the dissolution of TMIs and prevent TMIs from being embedded in the electrode.It ignores the influence of the solvation structures in the electrolyte system with different composition,and is not conducive to the design of the electrolyte formulation from the perspective of changing the concentration and the preferred solvent to inhibit the degradation of battery performance caused by TMIs deposition.In this work,by analyzing the special solvation structures of the high-concentra tion electrolyte,we study the main reason why high-concentration electrolyte inhibits the destructive effect of Mn(Ⅱ) on the electrochemical performance of LIBs.By combining the potentialresolved in-situ electrochemical impedance spectroscopy technology(PRIs-EIS) and density functional theory(DFT) calculation,we find that Mn(Ⅱ) mainly exists in the form of contact ions pairs(CIPs) and aggregates(AGGs) in high-concentration electrolyte.These solvation structures can reduce the destructive effect of Mn(Ⅱ) on battery performance from two aspects:on the one hand,it can rise the lowest unoccupied orbital(LUMO) value of the solvation structures of Mn(Ⅱ),thereby reducing the chance of its reduction;on the other hand,the decrease of Mn2+ions reduction can reduce the deposition of metallic manganese in the solid electrolyte interphase(SEI),thereby avoiding the continuous growth of the SEI.This study can be provided inspiration for the design of electrolytes to inhibit the destructive effect of TMls on LIBs. | Xiaoling Cui Jinlong Sun Dongni Zhao Jingjing Zhang Jie Wang Hong Dong Peng Wang Junwei Zhang Shumin Wu Linhu Song Ningshuang Zhang Chunlei Li Shiyou Li | 2023 | Journal of Energy Chemistry2023，，3： | 1 |
| 4 | Selecting nitride host for Yb^(3+) toward near-infrared emission with low-energy charge transfer band显示文摘Yb^(3+)-doped phosphors have characteristic near-infrared(NIR)emissions,but their applications in phosphor-converted light-emitting-diodes(pc-LEDs)and Si solar cells are limited due to their mismatching excitation spectra.Here,we selected nitride La3 Si6 N11(LSN)as host material to achieve Yb^(3+)NIR emission upon low-energy charge transfer(CT)excitation.The obtained phosphor LSN:Yb^(3+)has a broad CT excitation band ranging from 250 to 500 nm and narrowband NIR emissions ranging from 950 to 1100 nm centered at 983 nm.On the basis of spectral data,the vacuum referred binding energies(VRBE)schemes are constructed to locate energy levels of all lanthanide ions in LSN.We also fabricated NIR pc-LED device using 395 nm LED chip to demonstrate the potential applications of LSN:Yb^(3+)phosphors. | Shiyou Zhang Zhen Song Fangyi Zhao Shengqiang Liu Hao Cai Shuxin Wang Quanlin Liu | 2021 | Journal of Rare Earths2021，39，12： | 0 |
| 5 | Synchronous post-acceleration of laser-driven protons in helical coil targets by controlling the current dispersion显示文摘Post-acceleration of protons in helical coil targets driven by intense,ultrashort laser pulses can enhance ion energy by utilizing the transient current from the targets’self-discharge.The acceleration length of protons can exceed a few millimeters,and the acceleration gradient is of the order of GeV/m.How to ensure the synchronization between the accelerating electric field and the protons is a crucial problem for efficient post-acceleration.In this paper,we study how the electric field mismatch induced by current dispersion affects the synchronous acceleration of protons.We propose a scheme using a two-stage helical coil to control the current dispersion.With optimized parameters,the energy gain of protons is increased by four times.Proton energy is expected to reach 45 MeV using a hundreds-of-terawatts laser,or more than 100 MeV using a petawatt laser,by controlling the current dispersion. | Zhipeng Liu Zhusong Mei Defeng Kong Zhuo Pan Shirui Xu Ying Gao Yinren Shou Pengjie Wang Zhengxuan Cao Yulan Liang Ziyang Peng Jiarui Zhao Shiyou Chen Tan Song Xun Chen Tianqi Xu Xueqing Yan Wenjun Ma | 2023 | High Power Laser Science and Engineering2023，11，4： | 0 |
| 6 | Comparative DNA-methylome and transcriptome analysis reveals heterosis-and polyploidy-associated epigenetic changes in rice显示文摘Heterosis and polyploidy have an overwhelming influence on plant evolution.Recently,polyploid rice hybrids have been used to breed new rice varieties because they combine the advantages of both heterosis and polyploidy.In this study,we generated six rice lines:autotetraploid rice hybrids and their autotetraploid parents,diploid donors,and hybrids of the diploid donors.To investigate the molecular mechanism controlling the effects of both hybridization and polyploidization,we performed bisulfite and RNA sequencing on young panicles at the pollen meiosis stage to compare the DNA metabolomes and transcriptomes among the six rice lines.The hybrids lines were hypermethylated compared to their corresponding parents and the autotetraploid lines showed globally increased DNA methylation of their transposable elements compared to the diploid donors.The alteration in DNA methylation level corresponded to the differential gene expressions among the rice genotypes,suggesting that methylation changes induced by polyploidization and hybridization may affect gene expression.Groups of gene candidates were identified that may be associated with heterosis and polyploidy.Our results provide DNA information that can be used to investigate epigenetic modification during heterosis and polyploidy in rice. | Xiaolan Rao Jun Ren Wei Wang Rongrong Chen Qian Xie Yanqing Xu Dongmei Li Zhaojian Song Yuchi He Detian Cai Pingfang Yang Shiyou Lyu Li Li Wei Liu Xianhua Zhang | 2023 | The Crop Journal2023，11，2： | 0 |
| 7 | Design and performance improvement of SiNPs@graphene@C composite with a popcorn structure显示文摘Silicon anodes are considered to be the most promising alternatives owing to their theoretical specific capacity,which is almost 10 times higher than that of graphite anodes.However,huge volume changes during charging and discharging affect their interface stability,which strongly limits their application in commercial batteries.Herein,a popcorn-structured silicon-carbon composite(SiNPs@graphene@C),composed of silicon nanoparticles(SiNPs),graphene spheres and pitch-based carbon,is prepared by spraydrying followed by a wet process.The resulting SiNPs@graphene@C composite has good flexibility and elastic-strain capacity due to the graphene substrate,and it possesses macrostructural integrity and mechanical stability during cycling due to the rigid carbon–carbon chemical bonds.As a result,it shows a discharge-specific capacity of 481.3 mAh g^(-1)and a capacity retention of 82.9%after 500 cycles at 1 A g^(-1).Besides,the initial coulomb efficiency is increased from 65.7%to 86.5%by pre-lithiation,which improves the feasibility of commercialising the SiNPs@graphene@C composite. | Hong Dong Feifei Zong Jie Wang Hao Ding Peng Wang Ru Song Ningshuang Zhang Xuchun Cui Shiyou Li | 2022 | Journal of Energy Chemistry2022，31，9： | 0 |
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